arXiv subjects

H. Mutschke

Publications and source records attributed to H. Mutschke.

At least 19 recordsLinked to original sources

arXiv2020

Interstellar oxygen along the line of sight of Cygnus X-2

Interstellar dust permeates our Galaxy and plays an important role in many physical processes in the diffuse and dense regions of the interstellar medium. High-resolution X-ray spectroscopy, coupled with modelling based on laboratory dust measurements, provides a unique probe to investigate the interstellar dust properties along our line of sight towards Galactic X-ray sources. Here, we focus on the oxygen content of the interstellar medium through its absorption features in the X-ray spectra. To model the dust features, we perform a laboratory experiment using the electron microscope facility located at the University of Cadiz in Spain, where we acquire new laboratory data in the oxygen K-edge. We study 18 dust samples of silicates and oxides with different chemical compositions. The laboratory measurements are adopted for our astronomical data analysis. We carry out a case study on the X-ray spectrum of the bright low-mass X-ray binary Cygnus X-2, observed by XMM-Newton. We determine different temperature phases of the ISM, and parameterize oxygen in both gas (neutral and ionised) and dust form. We find Solar abundances of oxygen along the line of sight towards the source. Due to both the relatively low depletion of oxygen into dust form and the shape of the oxygen cross section profiles, it is challenging to determine the precise chemistry of interstellar dust. However, silicates provide an acceptable fit. Finally, we discuss the systematic discrepancies in the atomic (gaseous phase) data of the oxygen edge spectral region using different X-ray atomic databases, and also consider future prospects for studying the ISM with the Arcus concept mission.

astro-ph.HE↗

arXiv2019

Interstellar dust along the line of sight of GX 3+1

Studying absorption and scattering of X-ray radiation by interstellar dust grains allows us to access the physical and chemical properties of cosmic grains even in the densest regions of the Galaxy. We aim at characterising the dust silicate population which presents clear absorption features in the energy band covered by the Chandra X-ray Observatory. Through these absorption features, in principle, it is possible to infer the size distribution, composition, and structure of silicate in the interstellar medium. In particular, in this work, we investigate the magnesium and silicon K-edges. By using newly acquired synchrotron measurements, we build X-ray extinction models for fifteen dust candidates. These models, adapted for astrophysical analysis, and implemented in the Spex spectral fitting program, are used to reproduce the dust absorption features observed in the spectrum of the bright low mass X-ray binary GX 3+1 which is used as a background source. With the simultaneous analysis of the two edges we test two different size distributions of dust: one corresponding to the standard Mathis-Rumpl-Nordsieck model and one considering larger grains ($n(a) \propto a_i^{-3.5}$ with $0.005<a_1<0.25$ and $0.05<a_2<0.5$, respectively, with $a$ the grain size). These distributions may be representative of the complex Galactic region towards this source. We find that up to $70\%$ of dust is constituted by amorphous olivine. We discuss the crystallinity of the cosmic dust found along this line of sight. Both magnesium and silicon are highly depleted into dust ($δ_{Z} = 0.89\ \rm{and}\ 0.94$, respectively) while their total abundance does not depart from solar values.

astro-ph.GA↗

arXiv2019

Dust absorption and scattering in the silicon K-edge

The composition and properties of interstellar silicate dust are not well understood. In X-rays, interstellar dust can be studied in detail by making use of the fine structure features in the Si K-edge. The features in the Si K-edge offer a range of possibilities to study silicon-bearing dust, such as investigating the crystallinity, abundance, and the chemical composition along a given line of sight. We present newly acquired laboratory measurements of the silicon K-edge of several silicate-compounds that complement our measurements from our earlier pilot study. The resulting dust extinction profiles serve as templates for the interstellar extinction that we observe. The extinction profiles were used to model the interstellar dust in the dense environments of the Galaxy. The laboratory measurements, taken at the Soleil synchrotron facility in Paris, were adapted for astrophysical data analysis and implemented in the SPEX spectral fitting program. The models were used to fit the spectra of nine low-mass X-ray binaries located in the Galactic center neighborhood in order to determine the dust properties along those lines of sight. Most lines of sight can be fit well by amorphous olivine. We also established upper limits on the amount of crystalline material that the modeling allows. We obtained values of the total silicon abundance, silicon dust abundance, and depletion along each of the sightlines. We find a possible gradient of $0.06\pm0.02$ dex/kpc for the total silicon abundance versus the Galactocentric distance. We do not find a relation between the depletion and the extinction along the line of sight.

astro-ph.GA↗

arXiv2017

Investigating the interstellar dust through the Fe K-edge

The chemical and physical properties of interstellar dust in the densest regions of the Galaxy are still not well understood. X-rays provide a powerful probe since they can penetrate gas and dust over a wide range of column densities (up to $10^{24}\ \rm{cm}^{-2}$). The interaction (scattering and absorption) with the medium imprints spectral signatures that reflect the individual atoms which constitute the gas, molecule, or solid. In this work we investigate the ability of high resolution X-ray spectroscopy to probe the properties of cosmic grains containing iron. Although iron is heavily depleted into interstellar dust, the nature of the Fe-bearing grains is still largely uncertain. In our analysis we use iron K-edge synchrotron data of minerals likely present in the ISM dust taken at the European Synchrotron Radiation Facility. We explore the prospects of determining the chemical composition and the size of astrophysical dust in the Galactic centre and in molecular clouds with future X-ray missions. The energy resolution and the effective area of the present X-ray telescopes are not sufficient to detect and study the Fe K-edge, even for bright X-ray sources. From the analysis of the extinction cross sections of our dust models implemented in the spectral fitting program SPEX, the Fe K-edge is promising for investigating both the chemistry and the size distribution of the interstellar dust. We find that the chemical composition regulates the X-ray absorption fine structures in the post edge region, whereas the scattering feature in the pre-edge is sensitive to the mean grain size. Finally, we note that the Fe K-edge is insensitive to other dust properties, such as the porosity and the geometry of the dust.

astro-ph.HE↗

arXiv2016

Absorption and scattering by interstellar dust in the silicon K-edge of GX 5-1

We study the absorption and scattering of X-ray radiation by interstellar dust particles, which allows us to access the physical and chemical properties of dust. The interstellar dust composition is not well understood, especially on the densest sight lines of the Galactic Plane. X-rays provide a powerful tool in this study. We present newly acquired laboratory measurements of silicate compounds taken at the Soleil synchrotron facility in Paris using the Lucia beamline. The dust absorption profiles resulting from this campaign were used in this pilot study to model the absorption by interstellar dust along the line of sight of the low-mass X-ray binary (LMXB) GX 5-1. The measured laboratory cross-sections were adapted for astrophysical data analysis and the resulting extinction profiles of the Si K-edge were implemented in the SPEX spectral fitting program. We derive the properties of the interstellar dust along the line of sight by fitting the Si K-edge seen in absorption in the spectrum of GX 5-1. We measured the hydrogen column density towards GX 5-1 to be $3.40\pm0.1\times10^{22} \rm cm^{-2}$. The best fit of the silicon edge in the spectrum of GX 5-1 is obtained by a mixture of olivine and pyroxene. In this study, our modeling is limited to Si absorption by silicates with different Mg:Fe ratios. We obtained an abundance of silicon in dust of $4.0\pm0.3\times10^{-5}$ per H atom and a lower limit for total abundance, considering both gas and dust, of $>4.4\times10^{-5}$ per H atom, which leads to a gas to dust ratio of >0.22. Furthermore, an enhanced scattering feature in the Si K-edge may suggest the presence of large particles along the line of sight.

astro-ph.GA↗

arXiv2013

Herschel's "Cold Debris Disks": Background Galaxies or Quiescent Rims of Planetary Systems?

(abridged) Infrared excesses associated with debris disk host stars detected so far peak at wavelengths around ~100μm or shorter. However, six out of 31 excess sources in the Herschel OTKP DUNES have been seen to show significant - and in some cases extended - excess emission at 160μm, which is larger than the 100μm excess. This excess emission has been suggested to stem from debris disks colder than those known previously. Using several methods, we re-consider whether some or even all of the candidates may be associated with unrelated galactic or extragalactic emission and conclude that it is highly unlikely that none of the candidates represents a true circumstellar disk. For true disks, both the dust temperatures inferred from the SEDs and the disk radii estimated from the images suggest that the dust is nearly as cold as a blackbody. This requires the grains to be larger than ~100μm, regardless of their material composition. To explain the dearth of small grains, we explore several conceivable scenarios: transport-dominated disks, disks of low dynamical excitation, and disks of unstirred primordial macroscopic grains. Our qualitative analysis and collisional simulations rule out the first two of these scenarios, but show the feasibility of the third one. We show that such disks can survive for gigayears, largely preserving the primordial size distribution. They should be composed of macroscopic solids larger than millimeters, but smaller than kilometers in size. Thus planetesimal formation, at least in the outer regions of the systems, has stopped before "cometary" or "asteroidal" sizes were reached.

astro-ph.EP↗

arXiv2013

DUst Around NEarby Stars. The survey observational results

Debris discs are a consequence of the planet formation process and constitute the fingerprints of planetesimal systems. Their solar system's counterparts are the asteroid and Edgeworth-Kuiper belts. The DUNES survey aims at detecting extra-solar analogues to the Edgeworth-Kuiper belt around solar-type stars, putting in this way the solar system into context. The survey allows us to address some questions related to the prevalence and properties of planetesimal systems. We used {\it Herschel}/PACS to observe a sample of nearby FGK stars. Data at 100 and 160 $μ$m were obtained, complemented in some cases with observations at 70 $μ$m, and at 250, 350 and 500 $μ$m using SPIRE. The observing strategy was to integrate as deep as possible at 100 $μ$m to detect the stellar photosphere. Debris discs have been detected at a fractional luminosity level down to several times that of the Edgeworth-Kuiper belt. The incidence rate of discs around the DUNES stars is increased from a rate of $\sim$ 12.1% $\pm$ 5% before \emph{Herschel} to $\sim$ 20.2% $\pm$ 2%. A significant fraction ($\sim$ 52%) of the discs are resolved, which represents an enormous step ahead from the previously known resolved discs. Some stars are associated with faint far-IR excesses attributed to a new class of cold discs. Although it cannot be excluded that these excesses are produced by coincidental alignment of background galaxies, statistical arguments suggest that at least some of them are true debris discs. Some discs display peculiar SEDs with spectral indexes in the 70-160$μ$m range steeper than the Rayleigh-Jeans one. An analysis of the debris disc parameters suggests that a decrease might exist of the mean black body radius from the F-type to the K-type stars. In addition, a weak trend is suggested for a correlation of disc sizes and an anticorrelation of disc temperatures with the stellar age.

astro-ph.SR↗

arXiv2012

Observational evidence for composite grains in an AGB outflow: MgS in the extreme carbon star LL Peg

The broad 30 μm feature in carbon stars is commonly attributed to MgS dust particles. However, reproducing the 30 μm feature with homogeneous MgS grains would require much more sulfur relative to the solar abundance. Direct gas-phase condensation of MgS occurs at a low efficiency. Precipitation of MgS on SiC precursor grains provides a more efficient formation mechanism, such that the assumption of homogeneous MgS grains may not be correct. Using a Monte Carlo-based radiative transfer code, we aim to model the 30 μm feature of the extreme carbon star LL Peg with MgS dust particles. We find that for LL Peg this modeling is insensitive to the unknown MgS optical properties at λ< 10 μm. When MgS is allowed to be in thermal contact with amorphous carbon and SiC, the amount of MgS required to reproduce the strength of 30 μm feature agrees with the solar abundance of sulfur, thereby resolving the reported MgS mass problem. We conclude that MgS is a valid candidate to be the carrier of the 30 μm feature when it is part of a composite grain population that has optical properties representative of an ensemble of particle shapes.

astro-ph.SR↗

arXiv2010

Cold dust around nearby stars (DUNES). First results: A resolved exo-Kuiper belt around the solar-like star zeta^2 Ret

We present the first far-IR observations of the solar-type stars delta Pav, HR 8501, 51 Peg and zeta^2 Ret, taken within the context of the DUNES Herschel Open Time Key Programme (OTKP). This project uses the PACS and SPIRE instruments with the objective of studying infrared excesses due to exo-Kuiper belts around nearby solar-type stars. The observed 100 um fluxes from delta Pav, HR 8501, and 51 Peg agree with the predicted photospheric fluxes, excluding debris disks brighter than Ldust/Lstar ~ 5 x 10^-7 (1 sigma level) around those stars. A flattened, disk-like structure with a semi-major axis of ~ 100 AU in size is detected around zeta^2 Ret. The resolved structure suggests the presence of an eccentric dust ring, which we interpret as an exo-Kuiper belt with Ldust/Lstar ~ 10^-5.

astro-ph.SR↗

arXiv2010

Electronic spectroscopy of medium-sized polycyclic aromatic hydrocarbons: Implications for the carriers of the 2175 Å UV bump

Mixtures of polycylic aromatic hydrocarbons (PAHs) have been produced by means of laser pyrolysis. The main fraction of the extracted PAHs were primarily medium-sized, up to a maximum size of 38 carbon atoms per molecule. The use of different extraction solvents and subsequent chromatographic fractionation provided mixtures of different size distributions. UV-VIS absorption spectra have been measured at low temperature by matrix isolation spectroscopy and at room temperature with PAHs as film-like deposits on transparent substrates. In accordance with semi-empirical calculations, our findings suggest that large PAHs with sizes around 50 to 60 carbon atoms per molecule could be responsible for the interstellar UV bump at 217.5 nm.

astro-ph.IM↗

arXiv2009

Laboratory-based grain-shape models for simulating dust infrared spectra

Analysis of thermal dust emission spectra for dust mineralogy and physical grain properties depends on laboratory-measured or calculated comparison spectra. Often, the agreement between these two kinds of spectra is not satisfactory because of the strong influence of the grain morphology on the spectra. We investigate the ability of the statistical light-scattering model with a distribution of form factors (DFF model) to reproduce experimentally measured infrared extinction spectra for particles that are small compared to the wavelength. We take advantage of new experimental spectra measured for free particles dispersed in air with accompanying information on the grain morphology. For the calculations, we used DFFs that were derived for aggregates of spherical grains, as well as for compact grain shapes corresponding to Gaussian random spheres. Irregular particle shapes require a DFF similar to that of a Gaussian random sphere with sigma=0.3, whereas roundish grain shapes are best fitted with that of a fractal aggregate of a fractal dimension 2.4-1.8. In addition we used a fitting algorithm to obtain the best-fit DFFs for the various laboratory samples. In this way we can independently derive information on the shape of the grains from their infrared spectra. For anisotropic materials, different DFFs are needed for the different crystallographic axes. This is due to a theoretical problem, which is inherent to all models that are simply averaging the contributions of the crystallographic directions.

astro-ph.IM↗

arXiv2009

Morphological effects on IR band profiles: Experimental spectroscopic analysis with application to observed spectra of oxygen-rich AGB stars

To trace the source of the unique 13, 19.5, and 28 $μ$m emission features in the spectra of oxygen-rich circumstellar shells around AGB stars, we have compared dust extinction spectra obtained by aerosol measurements. We have measured the extinction spectra for 19 oxide powder samples of eight different types, such as Ti-compounds (TiO, TiO$_2$, Ti$_2$O$_3$, Ti$_3$O$_5$, Al$_2$TiO$_5$, CaTiO$_3$), $α$-, $γ$-, $χ$-$δ$-$κ$-Al$_2$O$_3$, and MgAl$_2$O$_4$ in the infrared region (10 - 50 $μ$m) paying special attention to the morphological (size, shape, and agglomeration) effects and the differences in crystal structure. Anatase (TiO$_2$) particles with rounded edges are the possible 13, 19.5 and 28 $μ$m band carriers as the main contributor in the spectra of AGB stars, and spherically shaped nano-sized spinel and Al$_2$TiO$_5$ dust grains are possibly associated with the anatase, enhancing the prominence of the 13 $μ$m feature and providing additional features at 28 $μ$m. The extinction data sets obtained by the aerosol and CsI pellet measurements have been made available for public use at http://elbe.astro.uni-jena.de

astro-ph.IM↗

arXiv2009

Spectral properties of gas-phase condensed fullerene-like carbon nanoparticles from far-ultraviolet to infrared wavelengths

Carbon solids are ubiquitous material in the interstellar space. However, the formation pathway of carbonaceous matter in astrophysical environments as well as in terrestrial gas-phase condensation reactions is not yet understood. Laser ablation of graphite in different quenching gas atmospheres such as pure He, He/H$_2$, and He/H$_2$O at varying pressures is used to synthesize very small, fullerene-like carbon nanoparticles. The particles are characterized by very small diameters between 1 and 4 nm and a disturbed onion-like structure. The soot particles extracted from the condensation zone obviously represent a very early stage of particle condensation. The spectral properties have been measured from the far-ultraviolet (FUV) ($λ$=120 nm) to the mid-infrared (MIR) ($λ$=15 ~$μ$m). The seed-like soot particles show strong absorption bands in the 3.4 ~$μ$m range. The profile and the intensity pattern of the 3.4 ~$μ$m band of the diffuse interstellar medium can be well reproduced by the measured 3.4 ~$μ$m profile of the condensed particles, however, all the carbon which is left to form solids is needed to fit the intensity of the interstellar bands. In contrast to the assumption that onion-like soot particles could be the carrier of the interstellar ultraviolet (UV) bump, our very small onion-like carbon nanoparticles do not show distinct UV bands due to ($π-π$*) transitions.

astro-ph.GA↗

arXiv2009

Formation of PAHs and Carbonaceous Solids in Gas-Phase Condensation Experiments

Carbonaceous grains represent a major component of cosmic dust. In order to understand their formation pathways, they have been prepared in the laboratory by gas-phase condensation reactions such as laser pyrolysis and laser ablation. Our studies demonstrate that the temperature in the condensation zone determines the formation pathway of carbonaceous particles. At temperatures lower than 1700 K, the condensation by-products are mainly polycyclic aromatic hydrocarbons (PAHs), that are also the precursors or building blocks for the condensing soot grains. The low-temperature condensates contain PAH mixtures that are mainly composed of volatile 3-5 ring systems. At condensation temperatures higher than 3500 K, fullerene-like carbon grains and fullerene compounds are formed. Fullerene fragments or complete fullerenes equip the nucleating particles. Fullerenes can be identified as soluble components. Consequently, condensation products in cool and hot astrophysical environments such as cool and hot AGB stars or Wolf Rayet stars should be different and should have distinct spectral properties.

astro-ph.GA↗

arXiv2008

Far-infrared spectra of hydrous silicates at low temperatures - Providing laboratory data for Herschel and ALMA

Hydrous silicates occur in various cosmic environments, and are among the minerals with the most pronounced bands in the far infrared (FIR) spectral region. Given that Herschel and ALMA will open up new possibilities for astronomical FIR and sub-mm spectroscopy, data characterizing the dielectric properties of these materials at long wavelengths are desirable. We aimed at examining the FIR spectra of talc, picrolite, montmorillonite, and chamosite, which belong to four different groups of phyllosilicates. We tabulated positions and band widths of the FIR bands of these minerals depending on the dust temperature. By means of powder transmission spectroscopy, spectra of the examined materials were measured in the wavelength range 25-500 mum at temperatures of 300, 200, 100, and 10 K. Room-temperature measurements yield the following results. For talc, a previously unknown band, centered at 98.5 mum, was found, in addition to bands at 56.5 and 59.5 mum. For montmorillonite, several bands at wavelengths <110 mum were detected, including a band at 105 mum with an FWHM of about 10 mum. Picrolite shows a sharp 77 mum FIR band. Chamosite is characterized by bands in the 72-92 mum range, and a prominent band at 277 mum. At decreasing temperature, most of the bands shift to shorter wavelengths. Examining a potential counterpart of the 105mum band in the spectra of HD 142527 and HD 100546, we find that the broad band in the spectra of these young stars - extending from 85 to 125 mum - cannot be due to montmorillonite or any of the hydrous silicates we studied, since these materials have sharper bands in the FIR wavelength range than previously assumed, especially at low temperatures.

astro-ph↗

arXiv2007

Carbonates in space - The challenge of low temperature data

Carbonates have repeatedly been discussed as possible carriers of stardust emission bands. However, the band assignments proposed so far were mainly based on room temperature powder transmission spectra of the respective minerals. Since very cold calcite grains have been claimed to be present in protostars and in Planetary Nebulae such as NGC 6302, the changes of their dielectric functions at low temperatures are relevant from an astronomical point of view. We have derived the IR optical constants of calcite and dolomite from reflectance spectra - measured at 300, 200, 100 and 10K - and calculated small particle spectra for different grain shapes, with the following results: i) The absorption efficiency factors both of calcite and dolomite are extremely dependent on the particle shapes. This is due to the high peak values of the optical constants of CaCO3 and CaMg[CO3]2. ii) The far infrared properties of calcite and dolomite depend also very significantly on the temperature. Below 200K, a pronounced sharpening and increase in the band strengths of the FIR resonances occurs. iii) In view of the intrinsic strength and sharpening of the 44 mum band of calcite at 200-100K, the absence of this band -- inferred from Infrared Space Observatory data -- in PNe requires dust temperatures below 45K. iv) Calcite grains at such low temperatures can account for the '92' mum band, while our data rule out dolomite as the carrier of the 60-65 mum band. The optical constants here presented are publicly available in the electronic database http://www.astro.uni-jena.de/Laboratory/OCDB

astro-ph↗

arXiv2006

The 10 $μ$m infrared band of silicate dust: A laboratory study comparing the aerosol and KBr pellet techniques

The profile of the silicate 10 $μ$m IR band contains important information about the evolutional stage of dust in circumstellar environments and the possible ongoing process of planetesimal formation. In order to extract this information, the observed band profiles are compared with calculated or laboratory-measured absorption cross sections of amorphous and crystalline grains with different sizes and compositions. We present in this study the first laboratory measurements of the 10 $μ$m band profiles of nonembedded, i.e. free-flying, particles of amorphous and crystalline Mg$_2$SiO$_4$ (with two different particle shapes), amorphous and crystalline MgSiO$_3$, and crystalline olivine. We compare the spectra with those measured on embedded grains and discuss the potential of the new experimental method for comparison with observed spectra, as well as for future studies of agglomeration and surface manipulation of the grains.

astro-ph↗

arXiv2005

Nanodiamond dust and the energy distribution of quasars

The spectral energy distribution of quasars shows a sharp steepening of the continuum shortward of ~ 1100 A. The steepening could be a result of dust absorption. We present a dust extinction model which considers crystalline carbon grains and compare it with SMC-like dust extinction consisting of a mixture of silicate grains with graphite or amorphous carbon grains. We show that the sharp break seen in individual quasar spectra of intermediate redshif \~ 1-2 can be reproduced by dust absorption provided the extinction curve consists of nanodiamonds, composed of terrestial cubic diamonds or of diamonds similar to the presolar nanodiamonds found in primitive meteorites.

astro-ph↗