arXiv subjects

H. O. U. Fynbo

Publications and source records attributed to H. O. U. Fynbo.

At least 19 recordsLinked to original sources

arXiv2026

Precision $β$-delayed charged-particle emission spectroscopy at FRIB: Proof of principle with the $β$-decay of $^{25}\mathrm{Si}$

We report on the $β$-delayed proton and $γ$-ray emission from $^{25}\mathrm{Si}$, measured at the Facility for Rare Isotope Beams (FRIB). Low-energy $^{25}\mathrm{Si}$ ions extracted from the Advanced Cryogenic Gas Stopper were implanted into a thin carbon foil surrounded by a compact, highly segmented array of silicon detector telescopes and two high-purity germanium detectors. This setup provides high-resolution charged-particle spectroscopy, establishing a proof of principle for precision stopped-beam decay studies at FRIB. We reconstruct the $^{25}\mathrm{Si}$ decay scheme, resolving new high-energy proton transitions and determining the feeding to excited states in $^{24}\mathrm{Mg}$. The observation of spectral interference patterns enables firm spin and parity assignments for highly excited states in $^{25}\mathrm{Al}$. The $^{25}\mathrm{Si}$ $β$-strength distribution is extracted and compared with large-scale shell-model calculations.

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arXiv2026

A ground state $^{22}$Al halo is unlikely

We report the decisive resolution of the ground state spin and parity of the proton-dripline nucleus $^{22}$Al, a prime candidate for a proton halo. The resolution stems from the first $β$-delayed charged particle emission experiment in the Gas Stopping Area at the Facility for Rare Isotope Beams (FRIB), leveraging high-intensity, low-energy beams extracted from the Advanced Cryogenic Gas Stopper (ACGS). The pristine beam quality from FRIB and the ACGS enabled a sensitive particle identification technique using thin silicon detectors, allowing for the suppression of the dominant proton background and the first observation of the weak $β$-delayed $α$ transition from the Isobaric Analog State in $^{22}$Mg to the $^{18}$Ne ground state. This observation uniquely fixes the $^{22}$Al ground state as $4^+$. The valence proton is confined by a dominant $d$-wave centrifugal barrier which, combined with the Coulomb repulsion, hinders the tunneling required for halo formation despite the exceptionally low proton separation energy of $^{22}$Al.

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arXiv2025

The 76Cu conundrum remains unsolved

Near the doubly-magic nucleus \nuc{Ni}{78} ($Z=28$, $N=50$), there has been a decades-long debate on the existence of a long-lived isomer in \nuc{Cu}{76}. A recent mass measurement claimed to have settled the debate, by measuring the energy of the isomer and shedding light on the structure of the nucleus. In this work, we present new, more accurate, and precise values of the half-lives of the isomeric and ground states in \nuc{Cu}{76}. Our findings suggest that both states have very similar half-lives, in the 600-700 ms range, in disagreement with the literature values, implying that they cannot be differentiated by their decay curves. These results raise more questions than they answer, reopening the debate and showing that the structures in \nuc{Cu}{76} are still not fully understood.

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arXiv2024

Revealing the nature of yrast states in neutron-rich polonium isotopes

Polonium isotopes having two protons above the shell closure at $Z=82$ show a wide variety of low-lying high-spin isomeric states across the whole chain. The structure of neutron-deficient isotopes up to $^{210}$Po ($N=126$) is well established as they are easily produced through various methods. However, there is not much information available for the neutron-rich counterparts for which only selective techniques can be used for their production. We report on the first fast-timing measurements of yrast states up to the 8$^+$ level in $^{214,216,218}$Po isotopes produced in the $β^-$ decay of $^{214,216,218}$Bi at ISOLDE, CERN. In particular, our new half-life value of 607(14) ps for the 8$_1^+$ state in $^{214}$Po is nearly 20 times shorter than the one available in literature and comparable with the newly measured half-lives of 409(16) and 628(25) ps for the corresponding 8$_1^+$ states in $^{216,218}$Po, respectively. The measured $B(E2;8_1^+ \to 6_1^+)$ transition probability values follow an increasing trend relative to isotope mass, reaching a maximum for $^{216}$Po. The increase contradicts the previous claims of isomerism for the $8^+$ yrast states in neutron-rich $^{214}$Po and beyond. Together with the other measured yrast transitions, the $B(E2)$ values provide a crucial test of the different theoretical approaches describing the underlying configurations of the yrast band. The new experimental results are compared to shell-model calculations using the KHPE and H208 effective interactions and their pairing modified versions, showing an increase in configuration mixing when moving towards the heavier isotopes.

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arXiv2024

Detailed study of the decay of $^{21}$Mg

Beta-delayed proton and gamma emission in the decay of $^{21}$Mg has been measured at ISOLDE, CERN with the ISOLDE Decay Station (IDS) set-up. The existing decay scheme is updated, in particular what concerns proton transitions to excited states in $^{20}$Ne. Signatures of interference in several parts of the spectrum are used to settle spin and parity assignments to highly excited states in $^{21}$Na. The previously reported $β$p$α$ branch is confirmed. A half-life of 120.5(4) ms is extracted for $^{21}$Mg. The revised decay scheme is employed to test mirror symmetry in the decay and to extract the beta strength distribution of $^{21}$Mg that is compared with theory.

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arXiv2023

Simultaneous $γ$-ray and electron spectroscopy of $^{182,184,186}$Hg isotopes

Background: The mercury isotopes around $N=104$ are a well-known example of nuclei exhibiting shape coexistence. Mixing of configurations can be studied by measuring the monopole strength $ρ^2(E0)$, however, currently the experimental information is scarce and lacks precision, especially for the $I^π\rightarrow I^π$ ($I \neq 0$) transitions. Purpose: The goals of this study were to increase the precision of the known branching ratios and internal conversion coefficients, to increase the amount of available information regarding excited states in $^{182,184,186}$Hg and to interpret the results in the framework of shape coexistence using different models. Method: The low-energy structures in $^{182,184,186}$Hg were populated in the $β$ decay of $^{182,184,186}$Tl, produced at ISOLDE and purified by laser ionization and mass separation. The $γ$-ray and internal conversion electron events were detected by five germanium clover detectors and a segmented silicon detector, respectively, and correlated in time to build decay schemes. Results: In total, 193, 178 and 156 transitions, including 144, 140 and 108 observed for the first time in a $β$-decay experiment, were assigned to $^{182,184,186}$Hg, respectively. Internal conversion coefficients were determined for 23 transitions, out of which 12 had an $E0$ component. Extracted branching ratios allowed the sign of the interference term in $^{182}$Hg as well as $ρ^2(E0;0^+_2\rightarrow 0^+_1)$ and $B(E2;0^+_2\rightarrow 2^+_1)$ in $^{184}$Hg to be determined. By means of electron-electron coincidences, the $0^+_3$ state was identified in $^{184}$Hg. The experimental results were qualitatively reproduced by five theoretical approaches, the IBM with configuration mixing with two different parametrizations, the General Bohr Hamiltonian, the BMF model and the SCCM model. However, a quantitative description is lacking.

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arXiv2023

133In: A Rosetta Stone for decays of r-process nuclei

The $β$ decays from both the ground state and a long-lived isomer of $^{133}$In were studied at the ISOLDE Decay Station (IDS). With a hybrid detection system sensitive to $β$, $γ$, and neutron spectroscopy, the comparative partial half-lives (logft) have been measured for all their dominant $β$-decay channels for the first time, including a low-energy Gamow-Teller transition and several First-Forbidden (FF) transitions. Uniquely for such a heavy neutron-rich nucleus, their $β$ decays selectively populate only a few isolated neutron unbound states in $^{133}$Sn. Precise energy and branching-ratio measurements of those resonances allow us to benchmark $β$-decay theories at an unprecedented level in this region of the nuclear chart. The results show good agreement with the newly developed large-scale shell model (LSSM) calculations. The experimental findings establish an archetype for the $β$ decay of neutron-rich nuclei southeast of $^{132}$Sn and will serve as a guide for future theoretical development aiming to describe accurately the key $β$ decays in the rapid-neutron capture (r-) process.

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arXiv2023

Beta-delayed neutron spectroscopy of $^{133}$In

The decay properties of $^{133}$In were studied in detail at the ISOLDE Decay Station (IDS). The implementation of the Resonance Ionization Laser Ion Source (RILIS) allowed separate measurements of its $9/2^+$ ground state ($^{133g}$In) and $1/2^-$ isomer ($^{133m}$In). With the use of $β$-delayed neutron and $γ$ spectroscopy, the decay strengths above the neutron separation energy were quantified in this neutron-rich nucleus for the first time. The allowed Gamow-Teller transition $9/2^+\rightarrow7/2^+$ was located at 5.92 MeV in the $^{133g}$In decay with a logft = 4.7(1). In addition, several neutron-unbound states were populated at lower excitation energies by the First-Forbidden decays of $^{133g,m}$In. We assigned spins and parities to those neutron-unbound states based on the $β$-decay selection rules, the logft values, and systematics.

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arXiv2023

Active target TPC for study of photonuclear reactions at astrophysical energies

A setup designed to study photonuclear reactions at astrophysical energies - an active target Time Projection Chamber was developed and constructed at the Faculty of Physics, University of Warsaw. The device was successfully employed in two experiments at the Institute of Nuclear Physics Polish Academy of Sciences in Cracow, in which γ- and neutron-induced reactions with CO2 gas target were measured. The reaction products were detected and their momenta reconstructed. Preliminary results are shown.

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arXiv2023

Three-body calculations of beta decay applied to $^{11}$Li

A novel practical few-body method is formulated to include isospin symmetry for nuclear halo structures. The method is designed to describe beta decay, where the basic concept of isospin symmetry facilitates a proper understanding. Both isobaric analogue and anti-analogue states are treated. We derive general and explicit formulas for three-body systems using hyperspherical coordinates. The example of the beta decaying $^{11}$Li ($^{9}$Li+$n$+$n$) is chosen as a challenging application for numerical calculations of practical interest. The detailed results are compared to existing experimental data and good agreement is found at high excitation energies, where the isobaric analogue and anti-analogue states are situated in the daughter nucleus. An interpretation of the decay pattern at lower excitation energies is suggested. Decays of the $^{9}$Li-core and the two halo-neutrons are individually treated and combined to the daughter system with almost unique isospin, which we predict to be broken by about $0.4\%$ probability. Properties of decay products are predicted as possible future tests of this model.

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arXiv2021

New experimental $^{23}$Na($α,p$)$^{26}$Mg Reaction Rate for Massive Star and Type-Ia Supernova models

The $^{23}$Na($α,p$)$^{26}$Mg reaction has been identified as having a significant impact on the nucleosynthesis of several nuclei between Ne and Ti in type-Ia supernovae, and of $^{23}$Na and $^{26}$Al in massive stars. The reaction has been subjected to renewed experimental interest recently, motivated by high uncertainties in early experimental data and in the statistical Hauser-Feshbach models used in reaction rate compilations. Early experiments were affected by target deterioration issues and unquantifiable uncertainties. Three new independent measurements instead are utilizing inverse kinematics and Rutherford scattering monitoring to resolve this. In this work we present directly measured angular distributions of the emitted protons to eliminate a discrepancy in the assumptions made in the recent reaction rate measurements, which results in cross sections differing by a factor of 3. We derive a new combined experimental reaction rate for the $^{23}$Na($α,p$)$^{26}$Mg reaction with a total uncertainty of 30% at relevant temperatures. Using our new $^{23}$Na($α,p$)$^{26}$Mg rate, the $^{26}$Al and $^{23}$Na production uncertainty is reduced to within 8%. In comparison, using the factor of 10 uncertainty previously recommended by the rate compilation STARLIB, $^{26}$Al and $^{23}$Na production was changing by more than a factor of 2. In type-Ia supernova conditions, the impact on production of $^{23}$Na is constrained to within 15%.

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arXiv2021

Unveiling the Two-Proton Halo Character of 17Ne: Exclusive Measurement of Quasi-free Proton-Knockout Reactions

The proton drip-line nucleus 17Ne is investigated experimentally in order to determine its two-proton halo character. A fully exclusive measurement of the 17Ne(p,2p)16F->15O+p quasi-free one-proton knockout reaction has been performed at GSI at around 500 MeV/nucleon beam energy. All particles resulting from the scattering process have been detected. The relevant reconstructed quantities are the angles of the two protons scattered in quasi-elastic kinematics, the decay of 16F into 15O (including gamma decays from excited states) and a proton, as well as the 15O+p relative-energy spectrum and the 16F momentum distributions. The latter two quantities allow an independent and consistent determination of the ratio of l=0 and l=2 motion of the valence protons in 17Ne. With a resulting relatively small l=0 component of only around 35(3)%, it is concluded that 17Ne exhibits a rather modest halo character only. The quantitative agreement of the two values deduced from the energy spectrum and the momentum distributions supports the theoretical treatment of the calculation of momentum distributions after quasi-free knockout reactions at high energies by taking into account distortions based on the Glauber theory. Moreover, the experimental data allow the separation of valence-proton knockout and knockout from the 15O core. The latter process contributes with 11.8(3.1) mb around 40% to the total proton-knockout cross section of 30.3(2.3) mb, which explains previously reported contradicting conclusions derived from inclusive cross sections.

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arXiv2021

Detailed study of the decay of 32Ar

In an experiment performed at the SPIRAL1 facility of GANIL, the beta decay of 32Ar has been studied by means of the "Silicon Cube" device associated with germanium clover detectors from the EXOGAM array. Beta-delayed protons and gamma rays have been observed and allowed the determination of all relevant decay branches. The Gamow-Teller strength distribution is compared to shell-model calculations and excellent agreement is found. The Fermi strength is inline with expectations. A quasi-complete decay scheme of 32Ar is established.

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arXiv2020

Decay studies of the long-lived states in $^{186}$Tl

Decay spectroscopy of the long-lived states in $^{186}$Tl has been performed at the ISOLDE Decay Station at ISOLDE, CERN. The $α$ decay from the low-spin $(2^-)$ state in $^{186}$Tl was observed for the first time and a half-life of $3.4^{+0.5}_{-0.4}$ s was determined. Based on the $α$-decay energy, the relative positions of the long-lived states were fixed, with the $(2^-)$ state as the ground state, the $7^{(+)}$ state at 77(56)~keV and the $10^{(-)}$ state at 451(56) keV. The level scheme of the internal decay of the $^{186}$Tl($10^{(-)}$) state ($T_{1/2} = 3.40(9)$ s), which was known to decay solely through emission of 374 keV $γ$-ray transition, was extended and a lower-limit for the $β$-decay branching $b_β> 5.9(3)\%$ was determined. The extracted retardation factors for the $γ$ decay of the $10^{(-)}$ state were compared to the available data in neighboring odd-odd thallium isotopes indicating the importance of the $πd_{3/2}$ shell in the isomeric decay and significant structure differences between $^{184}$Tl and $^{186}$Tl.

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arXiv2020

A stringent upper limit on the direct 3$α$ decay of the Hoyle State in $^{12}$C

We investigate an implication of the most recent observation of a second $J^π= 2^+$ state in $^{12}$C, which was measured using the $^{12}$C($γ$,$α$)$^8$Be$_{\textrm{(g.s.)}}$ reaction. In addition to the dissociation of $^{12}$C to an $α$-particle and $^8$Be in its ground state, a small fraction of events (2%) were identified as direct decays and decays to excited states in $^8$Be. This allowed a limit on the direct 3$α$ partial decay width to be determined as $Γ_{3α} < 32(4)$ keV. Since this 2$^+$ state is predicted by all theoretical models to be a collective excitation of the Hoyle state, the 3$α$ partial width of the Hoyle state is calculable from the ratio of 3$α$ decay penetrabilities of the Hoyle and 2$^+$ states. This was calculated using the semi-classical WKB approach and we deduce a stringent upper limit for the direct decay branching ratio of the Hoyle state of ${Γ_{3α} \over Γ} < 5.7 \times 10^{-6}$, over an order of magnitude lower than previously reported. This result places the direct measurement of this rare decay mode beyond current experimental capabilities.

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arXiv2020

Search for beta-delayed proton emission from $^{11}$Be

We report on an attempt to reproduce the observation of $β^-$-delayed proton emission from $^{11}$Be through detection of the final state nucleus $^{10}$Be with accelerator mass spectrometry. Twelve samples were collected at the ISOLDE facility at CERN at different separator settings, allowing tests of different sources of contamination to be carried out. The observed amounts of $^{10}$Be per collected $^{11}$Be rule out several contamination sources, but do not agree internally. Formation of BeH molecular ions in the ion source may explain our data, in which case an upper limit of the $β$p branching ratio of $2.2 \cdot 10^{-6}$ can be derived.

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arXiv2019

Comment on "Direct Observation of Proton Emission in $^{11}$Be"

We argue that conclusions of [PRL 123, 082501 (2019)] are incorrect. The authors present the direct observation of beta-delayed proton emission in the beta decay of 11Be. From the determined branching ratio for this process and from the energy spectrum of emitted protons the existence of a so far unobserved narrow resonance in 11Be was deduced. The given beta strength for the transition to this state is however wrong. In addition, we show that the combination of peak position and branching ratio is in strong disagreement with models considered by the authors. Furthermore, we identify several deficiencies in the analysis, and we provide possible sources of background, that could explain the error.

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arXiv2019

Measurement of the $2^+\rightarrow 0^+$ ground-state transition in the $β$ decay of $^{20}$F

We report the first detection of the second-forbidden, non-unique, $2^+\rightarrow 0^+$, ground-state transition in the $β$ decay of $^{20}$F. A low-energy, mass-separated $^{20}\rm{F}^+$ beam produced at the IGISOL facility in Jyväskylä, Finland, was implanted in a thin carbon foil and the $β$ spectrum measured using a magnetic transporter and a plastic-scintillator detector. The $β$-decay branching ratio inferred from the measurement is $b_β = [ 0.41\pm 0.08\textrm{(stat)}\pm 0.07\textrm{(sys)}] \times 10^{-5}$ corresponding to $\log ft = 10.89(11)$, making this one of the strongest second-forbidden, non-unique $β$ transitions ever measured. The experimental result is supported by shell-model calculations and has significant implications for the final evolution of stars that develop degenerate oxygen-neon cores. Using the new experimental data, we argue that the astrophysical electron-capture rate on $^{20}$Ne is now known to within better than 25% at the relevant temperatures and densities.

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