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H. Ott

Publications and source records attributed to H. Ott.

At least 19 recordsLinked to original sources
arXiv2018

Photoassociation of rovibrational Rydberg molecules

In this work we discuss the rotational structure of Rydberg molecules. We calculate the complete wave function in a laboratory fixed frame and derive the transition matrix elements for the pho- toassociation of free ground state atoms. We discuss the implications for the excitation of different rotational states as well as the shape of the angular nuclear wave function. We find a rather com- plex shape and unintuitive coupling strengths, depending on the angular momenta coupling that are relevant for the states. This work explains the different steps to calculate the wave functions and the transition matrix elements in a way, that they can be directly transferred to different molecular states, atomic species or molecular coupling cases.

physics.atom-ph↗
arXiv2017

The $c$-axis dimer and its electronic break-up: the insulator-to-metal transition in Ti$_2$O$_3$

We report on our investigation of the electronic structure of Ti$_2$O$_3$ using (hard) x-ray photoelectron and soft x-ray absorption spectroscopy. From the distinct satellite structures in the spectra we have been able to establish unambiguously that the Ti-Ti $c$-axis dimer in the corundum crystal structure is electronically present and forms an $a_{1g}a_{1g}$ molecular singlet in the low temperature insulating phase. Upon heating we observed a considerable spectral weight transfer to lower energies with orbital reconstruction. The insulator-metal transition may be viewed as a transition from a solid of isolated Ti-Ti molecules into a solid of electronically partially broken dimers where the Ti ions acquire additional hopping in the $a$-$b$ plane via the $e_g^{\pi}$ channel, the opening of which requires the consideration of the multiplet structure of the on-site Coulomb interaction.

cond-mat.str-el↗
arXiv2016

Mesoscopic Rydberg-blockaded ensembles in the superatom regime and beyond

Controlling strongly interacting many-body systems enables the creation of tailored quantum matter, with properties transcending those based solely on single particle physics. Atomic ensembles which are optically driven to a Rydberg state provide many examples of this, such as atom-atom entanglement, many-body Rabi oscillations, strong photon-photon interaction and spatial pair correlations. In its most basic form, Rydberg quantum matter consists of an isolated ensemble of strongly interacting atoms spatially confined to the blockade volume - a so-called superatom. Here we demonstrate the controlled creation and characterization of an isolated mesoscopic superatom by means of accurate density engineering and excitation to Rydberg $p$-states. Its variable size allows to investigate the transition from effective two-level physics for strong confinement to many-body phenomena in extended systems. By monitoring continuous laser-induced ionization we observe a strongly anti-bunched ion emission under blockade conditions and extremely bunched ion emission under off-resonant excitation. Our experimental setup enables in vivo measurements of the superatom, yielding insight into both excitation statistics and dynamics. We anticipate straightforward applications in quantum optics and quantum information as well as future experiments on many-body physics.

physics.atom-ph↗
arXiv2014

Scanning electron microscopy of Rydberg-excited Bose-Einstein condensates

We report on the realization of high resolution electron microscopy of Rydberg-excited ultracold atomic samples. The implementation of an ultraviolet laser system allows us to excite the atom, with a single-photon transition, to Rydberg states. By using the electron microscopy technique during the Rydberg excitation of the atoms, we observe a giant enhancement in the production of ions. This is due to $l$-changing collisions, which broaden the Rydberg level and therefore increase the excitation rate of Rydberg atoms. Our results pave the way for the high resolution spatial detection of Rydberg atoms in an atomic sample.

cond-mat.quant-gas↗
arXiv2012

Controlling the dynamics of an open many-body quantum system with localized dissipation

We experimentally investigate the action of a localized dissipative potential on a macroscopic matter wave, which we implement by shining an electron beam on an atomic Bose-Einstein condensate (BEC). We measure the losses induced by the dissipative potential as a function of the dissipation strength observing a paradoxical behavior when the strength of the dissipation exceeds a critical limit: for an increase of the dissipation rate the number of atoms lost from the BEC becomes lower. We repeat the experiment for different parameters of the electron beam and we compare our results with a simple theoretical model, finding excellent agreement. By monitoring the dynamics induced by the dissipative defect we identify the mechanisms which are responsible for the observed paradoxical behavior. We finally demonstrate the link between our dissipative dynamics and the measurement of the density distribution of the BEC allowing for a generalized definition of the Zeno effect. Due to the high degree of control on every parameter, our system is a promising candidate for the engineering of fully governable open quantum systems.

cond-mat.quant-gas↗
arXiv2012

Spatio-temporal Fermionization of Strongly Interacting 1D Bosons

Building on the recent experimental achievements obtained with scanning electron microscopy on ultracold atoms, we study one-dimensional Bose gases in the crossover between the weakly (quasi-condensate) and the strongly interacting (Tonks-Girardeau) regime. We measure the temporal two-particle correlation function and compare it with calculations performed using the Time Evolving Block Decimation algorithm. More pronounced antibunching is observed when entering the more strongly interacting regime. Even though this mimics the onset of a fermionic behavior, we highlight that the exact and simple duality between 1D bosons and fermions does not hold when such dynamical response is probed. The onset of fermionization is also reflected in the density distribution, which we measure \emph{in situ} to extract the relevant parameters and to identify the different regimes. Our results show agreement between experiment and theory and give new insight into the dynamics of strongly correlated many-body systems.

cond-mat.quant-gas↗
arXiv2012

Macroscopic Zeno effect and stationary flows in nonlinear waveguides with localized dissipation

We theoretically demonstrate the possibility to observe the macroscopic Zeno effect for nonlinear waveguides with a localized dissipation. We show the existence of stable stationary flows, which are balanced by the losses in the dissipative domain. The macroscopic Zeno effect manifests itself in the non-monotonic dependence of the stationary flow on the strength of the dissipation. In particular, we highlight the importance of the parameters of the dissipation to observe the phenomenon. Our results are applicable to a large variety of systems, including condensates of atoms or quasi-particles and optical waveguides.

nlin.PS↗
arXiv2011

Continuous Coupling of Ultracold Atoms to an Ionic Plasma via Rydberg Excitation

We characterize the two-photon excitation of an ultracold gas of Rubidium atoms to Rydberg states analysing the induced atomic losses from an optical dipole trap. Extending the duration of the Rydberg excitation to several ms, the ground state atoms are continuously coupled to the formed positively charged plasma. In this regime we measure the $n$-dependence of the blockade effect and we characterise the interaction of the excited states and the ground state with the plasma. We also investigate the influence of the quasi-electrostatic trapping potential on the system, confirming the validity of the ponderomotive model for states with $20\leq n\leq 120$.

physics.atom-ph↗
arXiv2011

Magnetic domain fluctuations in an antiferromagnetic film observed with coherent resonant soft x-ray scattering

We report the direct observation of slow fluctuations of helical antiferromagnetic domains in an ultra-thin holmium film using coherent resonant magnetic x-ray scattering. We observe a gradual increase of the fluctuations in the speckle pattern with increasing temperature, while at the same time a static contribution to the speckle pattern remains. This finding indicates that domain-wall fluctuations occur over a large range of time scales. We ascribe this non-ergodic behavior to the strong dependence of the fluctuation rate on the local thickness of the film.

cond-mat.other↗
arXiv2011

Intrinsic and extrinsic x-ray absorption effects in soft x-ray diffraction from the superstructure in magnetite

We studied the (001/2) diffraction peak in the low-temperature phase of magnetite (Fe3O4) using resonant soft x-ray diffraction (RSXD) at the Fe-L2,3 and O-K resonance. We studied both molecular-beam-epitaxy (MBE) grown thin films and in-situ cleaved single crystals. From the comparison we have been able to determine quantitatively the contribution of intrinsic absorption effects, thereby arriving at a consistent result for the (001/2) diffraction peak spectrum. Our data also allow for the identification of extrinsic effects, e.g. for a detailed modeling of the spectra in case a "dead" surface layer is present that is only absorbing photons but does not contribute to the scattering signal.

cond-mat.str-el↗
arXiv2010

Local electronic structure of Fe$^{2+}$ impurities in MgO thin films: Temperature-dependent soft x-ray absorption spectroscopy study

We report on the local electronic structure of Fe impurities in MgO thin films. Using soft x-ray absorption spectroscopy (XAS) we verified that the Fe impurities are all in the 2+ valence state. The fine details in the line shape of the Fe $L_{2,3}$ edges provide direct evidence for the presence of a dynamical Jahn-Teller distortion. We are able to determine the magnitude of the effective $D_{4h}$ crystal field energies. We also observed a strong temperature dependence in the spectra which we can attribute to the thermal population of low-lying excited states that are present due to the spin-orbit coupling in the Fe 3d. Using this Fe$^{2+}$ impurity system as an example, we show that an accurate measurement of the orbital moment in Fe$_3$O$_4$ will provide a direct estimate for the effective local low-symmetry crystal fields on the Fe$^{2+}$ sites, important for the theoretical modeling of the formation of orbital ordering.

cond-mat.str-el↗
arXiv2010

AC-Stark shift and photoionization of Rydberg atoms in an optical dipole trap

We have measured the AC-Stark shift of the $14D_{5/2}$ Rydberg state of rubidium 87 in an optical dipole trap formed by a focussed CO$_2$-laser. We find good quantitative agreement with the model of a free electron experiencing a ponderomotive potential in the light field. In order to reproduce the observed spectra we take into account the broadening of the Rydberg state due to photoionization. The extracted cross-section is compatible with previous measurements on neighboring Rydberg states.

physics.atom-ph↗
arXiv2010

Ultracold Atoms as a Target: Absolute Scattering Cross-Section Measurements

We report on a new experimental platform for the measurement of absolute scattering cross-sections. The target atoms are trapped in an optical dipole trap and are exposed to an incident particle beam. The exponential decay of the atom number directly yields the absolute total scattering cross-section. The technique can be applied to any atomic or molecular species that can be prepared in an optical dipole trap and provides a large variety of possible scattering scenarios.

physics.atom-ph↗
arXiv2009

Static and fluctuating stripe order observed by resonant soft x-ray diffraction in La1.8Sr0.2NiO4

We studied the stripe phase of La1.8Sr0.2NiO4 using neutron diffraction, resonant soft x-ray diffraction (RSXD) at the Ni L2,3 edges, and resonant x-ray diffraction (RXD) at the Ni K threshold. Differences in the q-space resolution of the different techniques have to be taken into account for a proper evaluation of diffraction intensities associated with the spin and charge order superstructures. We find that in the RSXD experiment the spin and charge order peaks show the same temperature dependence. In the neutron experiment by contrast, the spin and charge signals follow quite different temperature behaviors. We infer that fluctuating magnetic order contributes considerably to the magnetic RSXD signal and we suggest that this result may open an interesting experimental approach to search for fluctuating order in other systems by comparing RSXD and neutron diffraction data.

cond-mat.str-el↗
arXiv2008

Atomic multiplet calculation of 3d_{5/2} -> 4f resonant x-ray diffraction from Ho metal

We compare for Ho metal the x-ray absorption spectrum and the resonant soft x-ray diffraction spectra obtained at the $3d_{5/2} \to 4f$ ($M_5$) resonance for the magnetic 1st and 2nd order diffraction peaks $(0,0,τ)$ and $(0,0,2τ)$ with the result of an atomic multiplet calculation. We find a good agreement between experiment and simulation giving evidence that this kind of simulation is well suited to quantitatively analyze resonant soft x-ray diffraction data from correlated electron systems.

cond-mat.str-el↗
arXiv2008

Resonant soft x-ray scattering from stepped surfaces of SrTiO3

We studied the resonant diffraction signal from stepped surfaces of SrTiO3 at the Ti 2p -> 3d (L2,3) resonance in comparison with x-ray absorption (XAS) and specular reflectivity data. The steps on the surface form an artificial superstructure suited as a model system for resonant soft x-ray diffraction. A small step density on the surface is sufficient to produce a well defined diffraction peak, showing the high sensitivity of the method. At larger incidence angles, the resonant diffraction spectrum from the steps on the surface resembles the spectrum for specular reflectivity. Both deviate from the XAS data in the relative peak intensities and positions of the peak maxima. We determined the optical parameters of the sample across the resonance and found that the differences between the XAS and scattering spectra reflect the different quantities probed in the different signals. When recorded at low incidence or detection angles, XAS and specular reflectivity spectra are distorted by the changes of the angle of total reflection with energy. Also the step peak spectra, though less affected, show an energy shift of the peak maxima in grazing incidence geometry.

cond-mat.str-el↗
arXiv2007

Direct observation of t2g orbital ordering in magnetite

Using soft-x-ray diffraction at the site-specific resonances in the Fe L23 edge, we find clear evidence for orbital and charge ordering in magnetite below the Verwey transition. The spectra show directly that the (001/2) diffraction peak (in cubic notation) is caused by t2g orbital ordering at octahedral Fe2+ sites and the (001) by a spatial modulation of the t2g occupation.

cond-mat.str-el↗