SearcharxivSearch

arXiv subjects

H. Q. Lin

Publications and source records attributed to H. Q. Lin.

At least 19 recordsLinked to original sources

Sign-Free Evidence for a d-Wave Superfluid Stiffness Dome in the Doped Hubbard Model

We construct an effective single-particle Hamiltonian $K_{\mathrm{eff}}$ from Monte Carlo--averaged matrix logarithms of the imaginary-time propagator in determinant quantum Monte Carlo (DQMC). The logarithm maps the multiplicative sign problem into an additive framework where the central limit theorem guarantees convergence, rendering $K_{\mathrm{eff}}$ sign-problem-free: both sign sectors yield identical dispersions to $<1\%$. $K_{\mathrm{eff}}$ captures the exact correlated single-particle spectrum, incorporating all self-energy effects non-perturbatively. Applied to the Hubbard model ($t'/t = -0.30$, $U/t = 4$), $K_{\mathrm{eff}}$ reveals a $d$-wave pseudogap with strong nodal-antinodal dichotomy below a computational phase transition at $T^*$. Three sign-free observables provide evidence consistent with spin-fluctuation pairing: (i) the gap ratio $R_g > 1$ confirms $d$-wave symmetry -- a temperature-independent property of the correlated band structure that provides the medium for pairing; (ii) the superfluid stiffness $\rho_s$ forms a dome across doping at $L = 8$, $10$, and $12$, exceeding the Berezinskii-Kosterlitz-Thouless threshold by $5$-$7\times$ at the dome peak; (iii) $S(\pi,\pi)$ is approximately flat across doping, establishing that the dome originates from Fermi-surface geometry responding to uniform spin-fluctuation glue. The pseudogap grows monotonically toward half-filling while $\rho_s$ forms a dome, mirroring cuprate phenomenology where $T_c$ is limited by the superfluid density (Uemura relation). Vertex corrections remain to be quantified.

cond-mat.str-el

Strong and tunable coupling between antiferromagnetic magnons and surface plasmons

Surface plasmons are the collective electron excitations in metallic systems and the associated electromagnetic wave usually has the transverse magnetic (TM) polarization. On the other hand, spin waves are the spin excitations perpendicular to the equilibrium magnetization and are usually circularly polarized in a ferromagnet. The direct coupling of these two modes is difficult due to the difficulty of matching electromagnetic boundary conditions at the interface of magnetic and non-magnetic materials. Here, we overcome this challenge by utilizing the linearly polarized spin waves in antiferromagnets (AFM) and show that a strong coupling between AFM magnons and surface plasmons can be realized in a hybrid 2D material/AFM structure, featuring a clear anticrossing spectrum at resonance. The coupling strength, characterized by the gap of anticrossing at resonance, can be tuned by electric gating on 2D materials and be probed by measuring the two reflection minima in the reflection spectrum. Further, as a potential application, we show that plasmonic modes can assist the coupling of two well-separated AFMs over several micrometers, featuring symmetric and antisymmetric hybrid modes. Our results may open a new platform to study antiferromagnetic spintronics and its interplay with plasmonic photonics.

cond-mat.mes-hall

Multipartite entanglement serves as a faithful detector for quantum phase transitions

We investigate quantum phase transitions in various spin chain systems using the multipartite entanglement measure $\tau_{SEF}$ based on the monogamy inequality of squared entanglement of formation. Our results demonstrate that $\tau_{SEF}$ is more effective and reliable than bipartite entanglement or bipartite correlation measures such as entanglement of formation, von Neumann entropy, and quantum discord in characterizing quantum phase transitions. $\tau_{SEF}$ not only detects critical points that may go unnoticed by other detectors but also avoids the issue of singularity at non-critical points encountered by other measures. Furthermore, by applying $\tau_{SEF}$, we have obtained the phase diagram for the XY spin chain with three and four interactions and discovered a new quantum phase.

quant-ph

Improved scaling of the entanglement entropy of quantum antiferromagnetic Heisenberg systems

In this paper, we derive corrections to the subleading logarithmic term of the entanglement entropy in systems with spontaneous broken continuous symmetry. Using quantum Monte Carlo simulations, we show that the improved scaling formula leads to much better estimations of the number of Goldstone modes in the two-dimensional square lattice spin-1/2 Heisenberg model and bilayer spin-1/2 Heisenberg model in systems of rather small sizes, compared with previous results. In addition, the universal geometry-dependent finite constant in the entanglement entropy scaling is also obtained in good agreement with the theoretical value.

cond-mat.str-el

Band crossover and magnetic phase diagram of high-Tc superconducting compound Ba2CuO4-δ

We present the influences of electronic and magnetic correlations and doping evolution on the groundstate properties of recently discovered superconductor Ba$_{2}$CuO$_{4-δ}$ by utilizing the Kotliar-Ruckenstein slave boson method. Starting with an effective two-orbital Hubbard model (Scalapino {\it et al.} Phys. Rev. {\bf B 99}, 224515 (2019)), we demonstrate that with increasing doping concentration, the paramagnetic (PM) system evolves from two-band character to single-band ones around the electron filling n=2.5, with the band nature of the $d_{3z^{2}-r^{2}}$ and $d_{x^{2}-y^{2}}$ orbitals to the $d_{x^{2}-y^{2}}$ orbital, slightly affected when the electronic correlation U varies from 2 to 4 eV. Considering the magnetic correlations, the system displays one antiferromagnetically metallic (AFM) phase in $2 2.16$ at U=2 eV, or two AFM phases in $2 $2 eV, and crosses over to d-wave when U$>$2.2 eV.

cond-mat.supr-con

Topologically different spin disorder phases of the J1-J2 Heisenberg model on the honeycomb lattice

Searching for spin liquids on the honeycomb J1-J2 Heisenberg model has been attracting great attention in the past decade. In this Paper we investigate the topological properties of the J1-J2 Heisenberg model by introducing nearest-neighbour and next-nearest-neighbour bond parameters. We find that there exist two topologically different phases in the spin disordered regime 0.2 0.32, it is a pi-flux chiral spin liquid, which is topological nontrivial and gapped. These results suggest that there exist two topologically different spin disorder phases in honeycomb J1-J2 Heisenberg model.

cond-mat.str-el

The examination of stable charge states of vacancies in Cu2ZnSnS4

The stable charge states of vacancies in the solar cell absorber material Cu2ZnSnS4 are investigated using Kohn-Sham (KS) defect-induced single particle levels analysis by concerning the screened Coulomb hybrid functional. We found out that the Cu, Zn and S vacancies (denoted by VCu, VZn, VS) do not induce single particle defect levels in the vicinity of the band gap thus each of them has only one stable charge state corresponding to the fully occupied valence band VCu1-, VZn2- and VS0, respectively (and therefore cannot account for any defect transition energy levels). The Sn vacancy (VSn) has three stable charge states VSn2-, VSn3- and VSn4-, which may account for two charge transition energy levels. By comparing with previous charge transition energy levels studies, our results indicate that the examination of stable charge states is a necessary and important step which should be done before charge transition energy levels calculations.

cond-mat.mtrl-sci

Wilson ratio of Fermi gases in one dimension

We calculate the Wilson ratio of the one-dimensional Fermi gas with spin imbalance. The Wilson ratio of attractively interacting fermions is solely determined by the density stiffness and sound velocity of pairs and of excess fermions for the two-component Tomonaga-Luttinger liquid (TLL) phase. The ratio exhibits anomalous enhancement at the two critical points due to the sudden change in the density of states. Despite a breakdown of the quasiparticle description in one dimension, two important features of the Fermi liquid are retained, namely the specific heat is linearly proportional to temperature whereas the susceptibility is independent of temperature. In contrast to the phenomenological TLL parameter, the Wilson ratio provides a powerful parameter for testing universal quantum liquids of interacting fermions in one, two and three dimensions.

cond-mat.quant-gas

Superconducting Resonance and paring symmetry in electron-doped cuprates

The magnetic excitations in the superconducting electron-doped cuprates are studied in the framework of spin-density-wave description. The superconducting resonance is a natural product of the superconductivity due to the opening of d-wave gap. Its resonance energy exhibits well linear scaling with superconducting gap as $E_{res}/2Δ\sim 0.6$, quantitatively consisting with the experimental discovery. This ratio is insensitive to the selected parameters, manifesting its universality. Another lower-energy peak below resonance energy is predicted when the hole pocket emerges due to suppression of spin-density wave. We further verify that the ratio of linear scales is intimately related to the pairing symmetry. Distinct ratio can be found with respective pairing symmetry. In comparison with the inelastic neutron scattering data, the monotonic d-wave superconductivity is the most likely candidate in the electron-doped cuprates. Furthermore, we proposed a new method to check the pairing symmetry by the inelastic neutron scattering measurements.

cond-mat.supr-con

Origin of the pseudogap and its influence on superconducting state

When holes move in the background of strong antiferromagnetic correlation, two effects with different spatial scale emerge, leading to a much reduced hopping integral with an additional phase factor. An effective Hamiltonian is then proposed to investigate the underdoped cuprates. We argue that the pseudogap is the consequence of dressed hole moving in the antiferromagnetic background and has nothing to do with the superconductivity. The momentum distributions of the gap are qualitatively consistent with the recent ARPES measurements both in the pseudogap and superconducting state. Two thermal qualities are further calculated to justify our model. A two-gap scenario is concluded to describe the relation between the two gaps.

cond-mat.str-el

Interlayer magnetic frustration driven quantum spin disorder in honeycomb compound In$_{3}$Cu$_{2}$VO$_{9}$

We present electronic and magnetic properties of a honeycomb compound In$_{3}$Cu$_{2}$VO$_{9}$ in this paper. We find that the parent phase is a charge transfer insulator with an energy gap of about 1.5 eV. Singly occupied d$_{3z^{2}-r^{2}}$ electrons of copper ions contribute an $S$ = 1/2 spin, while vanadium ions show nonmagnetism. Oxygen 2$p$ orbitals hybridizing with a small fraction of Cu 3$d$ orbitals dominate the density of states near $E_{F}$. The planar nearest-neighbor, next-nearest-neighbor and interplane superexchange couplings of Cu spins are $J_{1}$ $\approx$ 16.2 meV, $J_{2}$ $\approx$ 0.3 meV and $J_{z}$ $\approx$ 1.2 meV, suggesting a low-dimensional antiferromagnet \cite{Sondhi10}. We propose that the magnetic frustration along the c-axis leads to a quantum spin disorder in In$_{3}$Cu$_{2}$VO$_{9}$, in accordance with the recent experiments. {abstract}

cond-mat.supr-con

The commensurate magnetic excitations induced by band-splitting and Fermi surface topology in n-type Cuprates

The antiferromagnetic correlation plays an important role in high-T$_{c}$ superconductors. Considering this effect, the magnetic excitations in n-type cuprates near the optimal doping are studied within the spin density wave description. The magnetic excitations are commensurate in the low energy regime and further develop into spin wave-like dispersion at higher energy, well consistent with the inelastic neutron scattering measurements. We clearly demonstrate that the commensurability originates from the band splitting and Fermi surface topology. The commensurability is a normal state property, and has nothing to do with d-wave superconductivity. The distinct behaviors of magnetic excitation between the n-type and p-type cuprates are further discussed. Our results strongly suggest the essential role of antiferromagnetic correlations in the cuprates.

cond-mat.str-el

Indirect exchange of magnetic impurities in zigzag graphene ribbon

We use quantum Monte Carlo method to study the indirect coupling between two magnetic impurities on the zigzag edge of graphene ribbon, with respect to the chemical potential $μ$. We find that the spin-spin correlation between two adatoms located on the nearest sites in the zigzag edge are drastically suppressed around the zero-energy. As we switch the system away from half-filling, the antiferromagnetic correlation is first enhanced and then decreased. If the two adatoms are adsorbed on the sites belonging to the same sublattice, we find similar behavior of spin-spin correlation except for a crossover from ferromagnetic to antiferromagentic correlation in the vicinity of zero-energy. We also calculated the weight of different components of d-electron wave function and local magnet moment for various values of parameters, and all the results are consistent with those of spin-spin correlation between two magnetic impurities.

cond-mat.str-el

Magnetic impurity in the vicinity of a vacancy in bilayer graphene

We use quantum Monte Carlo method to study a magnetic impurity located next to a vacancy in bilayer graphene with Bernal stacking. Due to the broken symmetry between two sublattices in bilayer system, there exist two different types of vacancy induced localized state. We find that the magnetic property of the adatom located on the adjacent site of the vacancy depends on whether the vacancy belongs to A or B sublattice. In general, local moment is more strongly suppressed if the vacancy belongs to the sublattice A when $μ\sim 0$. We switch the values of the chemical potential and study the basic thermodynamic quantities and the correlation functions between the magnetic adatom and the carbon sites.

cond-mat.str-el

Magnetic Impurity in Bernal Stacked Bilayer Graphene

We investigate a magnetic impurity in Bernal stacked bilayer graphene by a non-perturbative numerical exact approach. In the two cases we study, impurity is placed on the top of two different sublattices (A and B) in bilayer graphene. We find that similar to the monolayer case, magnet moment of the impurity could still be tuned in a wide range through changing the chemical potential. However, the property of the impurity depends strongly on its location due to the broken symmetry between sublattices A and B caused by the Bernal stacking. This difference becomes more apparent with the increase in the hybridization and decrease in the on-site Coulomb repulsion. Additionally, we calculate the impurity spectral densities and the correlation functions between the impurity and the conduction-band electrons. All the computational results show the same spatial dependence on the location of the impurity.

cond-mat.str-el

KAgF3: quasi-one-dimensional magnetism in three-dimensional magnetic ions sublattice

The electronic structure and magnetic properties of the Jahn-Teller-distorted perovskite KAgF3 have been investigated using the full-potential linerized aug- mented plane-wave method. It is found that KAgF3 exhibits significant quasi-one- dimensional antiferromagnetism with the ratio of exchange constant jJ?j (perpen- dicular to the z axis) and J (along the z axis) about 0.04, although the sublattice of magnetic ion is three-dimensional. The strong quasi-one-dimensional antiferromag- netism originates from the C-antiferro-distortive orbital ordering of the Ag2+ 4d9 ions. The orbital ordered antiferromagnetic insulating state in KAgF3 is determined by on-site Coulomb repulsion to a large extent.

cond-mat.str-el

Strong enhancement of d-wave superconducting state in the three-band Hubbard model coupled to an apical oxygen phonon

We study the hole binding energy and pairing correlations in the three-band Hubbard model coupled to an apical oxygen phonon, by exact diagonalization and constrained-path Monte Carlo simulations. In the physically relevant charge-transfer regime, we find that the hole binding energy is strongly enhanced by the electron-phonon interaction, which is due to a novel potential-energy-driven pairing mechanism involving reduction of both electronic potential energy and phonon related energy. The enhancement of hole binding energy, in combination with a phonon-induced increase of quasiparticle weight, leads to a dramatic enhancement of the long-range part of d-wave pairing correlations. Our results indicate that the apical oxygen phonon plays a significant role in the superconductivity of high-$T_c$ cuprates.

cond-mat.str-el

The spin states of Co ions in La1.5Ca0.5CoO4 from first-principles

The spin states and electronic structure of layered perovskite La1.5Ca0.5CoO4 are investigated using fullpotential linearized augmented plane-wave method. All the computational results indicate that the Co2+ ion is in a high-spin state and the Co3+ in a low-spin state. The Co2+ t2g orbitals with a small crystal-field splitting are mixed by spin-orbit coupling, which accounts for the observed easy in-plane magnetism. The nonmagnetic LS-Co3+ state, which is stabilized by a strong crystal field, provides a natural explanation for the observed low magnetic ordering temperature and a spin-blockade phenomenon of the electron hopping. Furthermore, we find that the intermediate-spin state of Co3+ has a large multiplet splitting. But the lowest-lying IS state of Co3+ is still higher in energy than the LS ground state by a few hundred millielectron volts and the HS state of Co3+ is even less stable, both in sharp contrast to a recent experimental study which suggested the HS+IS mixed Co3+ ground state. We note that either the IS-Co3+ or HS-Co3+ states or their mixture would produce a wrong out-of-plane magnetic anisotropy and a much higher magneticordering temperature than observed. Thus, the present work sheds light on this material concerning its electronic and magnetic structure, and it would stimulate different experiments to settle this intriguing spin-state issue.

cond-mat.str-el