arXiv subjects

H. R. Ott

Publications and source records attributed to H. R. Ott.

At least 37 records · Page 2Linked to original sources

arXiv2004

Evidence for s-wave superconductivity in the new beta-pyrochlore oxide RbOs2O6

We report the results of 87Rb NMR measurements on RbOs2O6, a new member of the family of the superconducting pyrochlore-type oxides with a critical temperature Tc = 6.4 K. In the normal state, the nuclear spin-lattice relaxation time T1 obeys the Korringa-type relation T1T = constant and the Knight shift is independent of temperature, indicating the absence of strong magnetic correlations. In the superconducting state, T1^{-1}(T) exhibits a tiny coherence enhancement just below Tc, and decreases exponentially with further decreasing temperatures. The value of the corresponding energy gap is close to that predicted by the conventional weak-coupling BCS theory. Our results indicate that RbOs2O6 is a conventional s-wave-type superconductor.

cond-mat.supr-con↗

arXiv2004

Kondo Behavior of U in CaB$_6$

Replacing U for Ca in semiconducting CaB$_6$ at the few at.% level induces metallic behaviour and Kondo-type phenomena at low temperatures, a rather unusual feature for U impurities in metallic hosts. For Ca$_{0.992}$U$_{0.008}$B$_6$, the resistance minimum occurs at $T$ = 17 K. The subsequent characteristic logarithmic increase of the resistivity with decreasing temperature merges into the expected $T^2$ dependence below 0.8 K. Data of the low-temperature specific heat and the magnetization are analyzed by employing a simple resonance-level model. Analogous measurements on LaB$_6$ with a small amount of U revealed no traces of Kondo behavior, above 0.4 K.

cond-mat.mtrl-sci↗

arXiv2004

Anisotropic field dependence of the magnetic transition in Cu2Te2O5Br2

We present the results of measurements of the thermal conductivity of Cu2Te2O5Br2, a compound where tetrahedra of Cu^{2+} ions carrying S=1/2 spins form chains along the c-axis of the tetragonal crystal structure. The thermal conductivity kappa was measured along both the c- and the a-direction as a function of temperature between 3 and 300 K and in external magnetic fields H up to 69 kOe, oriented both parallel and perpendicular to the c-axis. Distinct features of kappa(T) were observed in the vicinity of T_N=11.4 K in zero magnetic field. These features are unaltered in external fields which are parallel to the c-axis, but are more pronounced when a field is applied perpendicularly to the c-axis. The transition temperature increases upon enhancing the external field, but only if the field is oriented along the a-axis.

cond-mat.str-el↗

arXiv2004

On the interpretation of the equilibrium magnetization in the mixed state of high-Tc superconductors

We apply a recently developed scaling procedure to the analysis of equilibrium magnetization M(H) data that were obtained for T-2212 and Bi-2212single crystals and were reported in the literature. The temperature dependencies of the upper critical field and the magnetic field penetration depth resulting from our analysis are distinctly different from those obtained in the original publications. We argue that theoretical models, which are usually employed for analyses of the equilibrium magnetization in the mixed state of type-II superconductors are not adequate for a quantitative description of high-Tc superconductors. In addition, we demonstrate that the scaled equilibrium magnetization M(H) curve for a Tl-2212 sample reveals a pronounced kink, suggesting a phase transition in the mixed state.

cond-mat.supr-con↗

arXiv2004

Percolation and Colossal Magnetoresistance in Eu-based Hexaborides

Upon substituting Ca for Eu in the local-moment ferromagnet EuB$_6$, the Curie temperature $T_C$ decreases substantially with increasing dilution of the magnetic sublattice and is completely suppressed for $x$ $\leq$ 0.3. The Ca substitution leads to significant changes of the electronic properties across the Eu$_x$Ca$_{1-x}$B$_6$ series. Electron microscopy data for $x$ $\approx$ 0.27 indicate a phase separation into Eu- and Ca-rich clusters of 5 to 10 nm diameter, leading to percolation-type phenomena in the electrical transport properties. The related critical concentration $x_p$ is approximately 0.3. For $x$ $\approx$ 0.27, we observe colossal negative magnetoresistance effects at low temperatures, similar in magnitude as those reported for manganese oxides.

cond-mat.mtrl-sci↗

arXiv2004

Equilibrium magnetization in the vicinity of the first order phase transition in the mixed state of high-Tc superconductors

We present the results of a scaling analysis of isothermal magnetization M(H) curves measured in the mixed state of high-Tc superconductors in the vicinity of the established first order phase transition. The most surprising result of our analysis is that the difference between the magnetization above and below the transition may have either sign, depending on the particular chosen sample. We argue that this observation, based on M(H) data available in the literature, is inconsistent with the interpretation that the well known first order phase transition in the mixed state of high-Tc superconductors always represents the melting transition in the vortex system.

cond-mat.supr-con↗

arXiv2003

Unconventional Charge Ordering in Na0.70CoO2 below 300 K

We present the results of measurements of the dc-magnetic susceptibility chi(T) and the 23Na-NMR response of Na_{0.70}CoO_{2} at temperatures between 50 and 340 K. The chi(T) data suggest that for T > 75 K, the Co ions adopt an effective configuration of Co^{3.4+}. The 23Na-NMR response reveals pronounced anomalies near 250 and 295 K, but no evidence for magnetic phase transitions is found in chi(T). Our data suggest the onset of a dramatic change in the Co 3d-electron spin dynamics at 295 K. This process is completed at 230 K. Our results maybe interpreted as evidence for either a tendency to electron localization or an unconventional charge-density wave phenomenon within the cobalt oxide layer, CoO_2, 3d electron system near room temperature.

cond-mat.str-el↗

arXiv2003

Electronic transport in EuB$_6$

EuB$_6$ is a magnetic semiconductor in which defects introduce charge carriers into the conduction band with the Fermi energy varying with temperature and magnetic field. We present experimental and theoretical work on the electronic magnetotransport in single-crystalline EuB$_6$. Magnetization, magnetoresistance and Hall effect data were recorded at temperatures between 2 and 300 K and in magnetic fields up to 5.5 T. The negative magnetoresistance is well reproduced by a model in which the spin disorder scattering is reduced by the applied magnetic field. The Hall effect can be separated into an ordinary and an anomalous part. At 20 K the latter accounts for half of the observed Hall voltage, and its importance decreases rapidly with increasing temperature. As for Gd and its compounds, where the rare-earth ion adopts the same Hund's rule ground state as Eu$^{2+}$ in EuB$_{6}$, the standard antisymmetric scattering mechanisms underestimate the $size$ of this contribution by several orders of magnitude, while reproducing its $shape$ almost perfectly. Well below the bulk ferromagnetic ordering at $T_C$ = 12.5 K, a two-band model successfully describes the magnetotransport. Our description is consistent with published de Haas van Alphen, optical reflectivity, angular-resolved photoemission, and soft X-ray emission as well as absorption data, but requires a new interpretation for the gap feature deduced from the latter two experiments.

cond-mat.str-el↗

arXiv2003

Magneto-optical Kerr effect in $Eu_{1-x}Ca_{x}B_{6}$

We have measured the magneto-optical Kerr rotation of ferromagnetic $Eu_{1-x}Ca_{x}B_{6}$ with x=0.2 and 0.4, as well as of $YbB_{6}$ serving as the non-magnetic reference material. As previously for $EuB_{6}$, we could identify a feature at 1 $eV$ in the Kerr response which is related with electronic transitions involving the localized 4f electron states. The absence of this feature in the data for $YbB_{6}$ confirms the relevance of the partially occupied 4f states in shaping the magneto-optical features of $Eu$-based hexaborides. Disorder by $Ca$-doping broadens the itinerant charge carrier contribution to the magneto-optical spectra.

cond-mat.str-el↗

arXiv2003

Ambivalence of the anisotropy of the vortex lattice in an anisotropic type-II superconductor

We present a geometry-based discussion of possible vortex configurations in the mixed state of anisotropic type-II superconductors. It is shown that, if energy considerations assign six nearest neighbors to each vortex, two distinct modifications of the vortex lattice are possible. It is expected that certain conditions lead to a first order phase transition from one modification of the vortex lattice to the other upon varying the external magnetic field.

cond-mat.supr-con↗

arXiv2003

Optical evidence for a spin-filter effect in the charge transport of $Eu_{0.6}Ca_{0.4}B_{6}$

We have measured the optical reflectivity $R(ω)$ of $Eu_{0.6}Ca_{0.4}B_{6}$ as a function of temperature between 1.5 and 300 $K$ and in external magnetic fields up to 7 $T$. The slope at the onset of the plasma edge feature in $R(ω)$ increases with decreasing temperature and increasing field but the plasma edge itself does not exhibit the remarkable blue shift that is observed in the binary compound $EuB_{6}$. The analysis of the magnetic field dependence of the low temperature optical conductivity spectrum confirms the previously observed exponential decrease of the electrical resistivity upon increasing, field-induced bulk magnetization at constant temperature. In addition, the individual exponential magnetization dependences of the plasma frequency and scattering rate are extracted from the optical data.

cond-mat.str-el↗

arXiv2003

Diffusive energy transport in the S=1 Haldane chain compound AgVP2S6

We present the results of measurements of the thermal conductivity $κ$ of the spin S=1 chain compound AgVP_2S_6 in the temperature range between 2 and 300 K and with the heat flow directed either along or perpendicular to the chain direction. The analysis of the anisotropy of the heat transport allowed for the identification of a small but non-negligible magnon contribution $κ_m$ along the chains, superimposed on the dominant phonon contribution $κ_ph$. At temperatures above about 100 K the energy diffusion constant D_E(T), calculated from the $κ_m(T)$ data, exhibits similar features as the spin diffusion constant D_S(T), previously measured by NMR. In this regime, the behaviour of both transport parameters is consistent with a diffusion process that is caused by interactions inherent to one-dimensional S=1 spin systems.

cond-mat.str-el↗

arXiv2003

Unusual magnetic field-induced phase transition in the mixed state of superconducting NbSe2

The thermal conductivity κin the basal plane of single-crystalline hexagonal NbSe2 has been measured as a function of magnetic field H, oriented both along and perpendicular to the c-axis, at several temperatures below T_c. With the magnetic field in the basal plane and oriented parallel to the heat flux we observed, in fields well below H_c2, an unexpected hysteretic behavior of κ(H) with all the generic features of a first order phase transition. The transition is not manifest in the κ(H) curves, if H is still in the basal plane but oriented perpendicularly to the heat-flux direction. The origin of the transition is not yet understood.

cond-mat.supr-con↗

arXiv2003

Temperature dependence of the upper critical field of high-Tc superconductors from isothermal magnetization data. Influence of a temperature dependent Ginzburg-Landau parameter

We show that the scaling procedure, recently proposed for the evaluation of the temperature variation of the normalized upper critical field of type-II superconductors, may easily be modified in order to take into account a possible temperature dependence of the Ginzburg-Landau parameter kappa. As an example, we consider kappa (T) as it follows from the microscopic theory of superconductivity.

cond-mat.supr-con↗

arXiv2003

Inhomogeneous magnetism in decagonal Al$_{69.8}$Pd$_{12.1}$Mn$_{18.1}$

We report the results of measurements of $^{27}$Al and $^{55}$Mn NMR spectra, the related spin-lattice relaxation rates, and the dc magnetic susceptibility of the stable decagonal quasicrystal Al$_{69.8}$Pd$_{12.1}$Mn$_{18.2}$. The temperature-variation of the magnetic susceptibility $χ(T)$ reveals that the Mn ions carry only an average magnetic moment of approximately $2μ_{\mathrm{B}}$, and confirms a spin-glass type freezing of the Mn-moments at $T_f=12$K. The NMR spectra reveal two partially resolved lines for the $^{27}$Al-nuclei, indicating that there are two different sets of environments for the Al-sites. The integrated intensity of the Mn line in the spectra suggests that about half of the Mn ions carry no magnetic moment. Below 50K, and upon decreasing the temperature, the $^{27}$Al NMR-linewidth $w$ and the spin-lattice relaxation rate $T_1^{-1}$ both grow with an increasingly negative slope, as it is often observed and interpreted as a critical "slowing down" of magnetic moments in systems approaching a spin-glass transition. Various features, such as a broad maximum in $T_1^{-1}(T)$ and a slope change in the $w(χ)$ plot, both around 120K, suggest a gradual reduction of the number of Mn moments with decreasing temperature below 120K.

cond-mat.mtrl-sci↗

arXiv2003

Universal behavior of spin-mediated energy transport in S=1/2 chain cuprates: BaCu2Si2O7 as an example

The thermal conductivity of the spin-1/2 chain cuprate BaCu2Si2O7 was measured along different crystallographic directions in the temperature region between 0.5 and 300 K. The thermal conductivity along the chain direction considerably exceeds that along perpendicular directions. Near the antiferromagnetic transition at T_N = 9.2 K the data indicates enhanced scattering of phonons by critical fluctuations in the spin system. A comparison of the data above T_N with available results on similar materials reveals similarities in the main features of the temperature dependence of the mean free path of itinerant spin excitations. This universal behavior is most likely caused by the spin-lattice interaction.

cond-mat.str-el↗

arXiv2002

Reinterpretation of the equilibrium magnetization of a Tl-based single crystal. Another phase transition in the mixed state of high-Tc superconductors?

We apply a recently developed scaling procedure for the analysis of the equilibrium magnetization M that was measured on a Tl-based single crystal and was recently reported in the literature. The results of our analysis are distinctly different from those obtained in the original publication where the Hao-Clem model served to analyze the magnetization data. We argue that the Hao-Clem model is not adequate for a quantitative description of the mixed state in high-Tc superconductors especially in high magnetic fields. The scaled equilibrium magnetization data reveal a pronounced kink in the M(H) dependence that might be indicative of a phase transition in the mixed state.

cond-mat.supr-con↗

arXiv2002

On the equilibrium magnetization of high-Tc superconductors below the irreversibility line

By scaling isothermal magnetization data measured at different temperatures in the mixed state of high-Tc superconductors, we show that in some cases the sample magnetization, measured in increasing magnetic field below the irreversibility line, is identical with the equilibrium magnetization even in magnetic fields well within the irreversible regime. This surprising behavior can hardly be explained in terms of traditional models of vortex pinning in the bulk of the sample.

cond-mat.supr-con↗