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H. Rasiwala

Publications and source records attributed to H. Rasiwala.

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Design of a high voltage delivery system for noble liquid time projection chambers

Noble liquid time projection chambers (TPCs) are a leading technology in the detection of ionizing radiation, particularly in applications such as accelerator neutrino physics, dark matter detection, and neutrinoless double beta decay. This paper addresses the design considerations for implementing stable high voltage (HV) systems within large noble liquid TPCs, with a focus on the nEXO experiment. Utilizing insights from prior HV research and experimental investigations, we outline factors influencing HV stability and discuss design choices to improve stability and prevent electrical discharges. A novel HV delivery system concept is presented, tailored for the nEXO TPC, which incorporates these design considerations while also meeting the stringent radiopurity requirements of the nEXO neutrinoless double beta decay search. These design considerations and their specific implementation towards a HV delivery system offer guidance to future experiments applying high voltage in noble liquid environments.

physics.ins-det

Ultra-pure Nickel for Structural Components of Low-Radioactivity Instruments

The next generation of rare-event search experiments in nuclear and particle physics demand structural materials combining exceptional mechanical strength with ultra-low levels of radioactive contamination. This study evaluates chemical vapor deposition (CVD) nickel as a candidate structural material for such applications. Manufacturer-supplied CVD Ni grown on aluminum substrates underwent tensile testing before and after welding alongside standard Ni samples. CVD Ni exhibited a planar tensile strength of ~600 MPa, significantly surpassing standard nickel. However, welding and heat treatment were found to reduce the tensile strength to levels comparable to standard Ni, with observed porosity in the welds likely contributing to this reduction. Material assay via inductively coupled plasma mass spectrometry (ICP-MS) employing isotope-dilution produced measured bulk concentration of 232-Th, 238-U, and nat-K at the levels of ~70 ppq, <100 ppq, and ~900 ppt, respectively, which is the lowest reported in nickel. Surface-etch profiling uncovered higher concentrations of these contaminants extending ~10 micrometer beneath the surface, likely associated with the aluminum growth substrate. The results reported are compared to the one other well documented usage of CVD Ni in a low radioactive background physics research experiment and a discussion is provided on how the currently reported results may arise from changes in CVD fabrication or testing process. These results establish CVD Ni as a promising low-radioactivity structural material, while outlining the need for further development in welding and surface cleaning techniques to fully realize its potential in large-scale, low radioactive background rare-event search experiments.

nucl-ex

Sensitivity of nEXO to $^{136}$Xe Charged-Current Interactions: Background-free Searches for Solar Neutrinos and Fermionic Dark Matter

We study the sensitivity of nEXO to solar neutrino charged-current interactions, $\nu_e + ^{136}$Xe$\rightarrow ^{136}$Cs$^* + e^-$, as well as analogous interactions predicted by models of fermionic dark matter. Due to the recently observed low-lying isomeric states of $^{136}$Cs, these interactions will create a time-delayed coincident signal observable in the scintillation channel. Here we develop a detailed Monte Carlo of scintillation emission, propagation, and detection in the nEXO detector to model these signals under different assumptions about the timing resolution of the photosensor readout. We show this correlated signal can be used to achieve background discrimination on the order of $10^{-9}$, enabling nEXO to make background-free measurements of solar neutrinos above the reaction threshold of 0.668 MeV. We project that nEXO could measure the flux of CNO solar neutrinos with a statistical uncertainty of 25%, thus contributing a novel and competitive measurement towards addressing the solar metallicity problem. Additionally, nEXO could measure the mean energy of the $^7$Be neutrinos with a precision of $\sigma \leq 1.5$ keV and could determine the survival probability of $^{7}$Be and $pep$ solar $\nu_e$ with precision comparable to state-of-the-art. These quantities are sensitive to the Sun's core temperature and to non-standard neutrino interactions, respectively. Furthermore, the strong background suppression would allow nEXO to search for for charged-current interactions of fermionic dark matter in the mass range $m_\chi$ = $0.668$-$7$ MeV with a sensitivity up to three orders of magnitude better than current limits.

nucl-ex

Ultra-sensitive radon assay using an electrostatic chamber in a recirculating system

Rare event searches such as neutrinoless double beta decay and Weakly Interacting Massive Particle detection require ultra-low background detectors. Radon contamination is a significant challenge for these experiments, which employ highly sensitive radon assay techniques to identify and select low-emission materials. This work presents the development of ultra-sensitive electrostatic chamber (ESC) instruments designed to measure radon emanation in a recirculating gas loop, for future lower background experiments. Unlike traditional methods that separate emanation and detection steps, this system allows continuous radon transport and detection. This is made possible with a custom-built recirculation pump. A Python-based analysis framework, PyDAn, was developed to process and fit time-dependent radon decay data. Radon emanation rates are given for various materials measured with this instrument. A radon source of known activity provides an absolute calibration, enabling statistically-limited minimal detectable activities of 20 $\mu$Bq. These devices are powerful tools for screening materials in the development of low-background particle physics experiments.

physics.ins-det

Characterization of external cross-talk from silicon photomultipliers in a liquid xenon detector

The Light-only Liquid Xenon experiment (LoLX) employs a small-scale detector equipped with 96 Hamamatsu VUV4 silicon photomultipliers (SiPMs) submerged in 5 kg of liquid xenon (LXe) to perform characterization measurements of light production, transport and detection in xenon. In this work, we perform a novel measurement of the "external cross-talk" (ExCT) of SiPMs, where photons produced in the avalanche process escape the device and produce correlated signals on other SiPMs. SiPMs are the photodetector technology of choice for next generation rare-event search experiments; understanding the sources and effects of correlated noise in SiPMs is critical for producing accurate estimates of detector performance and sensitivity projections. We measure the probability to observe ExCT through timing correlation of detected photons in low-light conditions within LoLX. Measurements of SiPM ExCT are highly detector dependent; thus the ExCT process is simulated and modelled using the Geant4 framework. Using the simulation, we determine the average transport and detection efficiency for ExCT photons within LoLX, a necessary input to extract the expected ExCT probability from the data. For an applied overvoltage of 4 V and 5 V, we measure a mean number of photons emitted into the LXe per avalanche of $0.5^{+0.3}_{-0.2}$ and $0.6^{+0.3}_{-0.2}$, respectively. Using an optical model to describe photon transmission through the SiPM surface, this corresponds to an estimated photon yield inside the bulk silicon of $20^{+11}_{-9}$ and $25^{+12}_{-9}$ photons per avalanche. The relative increase in intensity of SiPM ExCT emission between 4 V and 5 V is consistent with expectation for the linear increase of gain with respect to overvoltage.

physics.ins-det

Imaging of single barium atoms in a second matrix site in solid xenon for barium tagging in a $^{136}$Xe double beta decay experiment

Neutrinoless double beta decay is one of the most sensitive probes for new physics beyond the Standard Model of particle physics. One of the isotopes under investigation is $^{136}$Xe, which would double beta decay into $^{136}$Ba. Detecting the single $^{136}$Ba daughter provides a sort of ultimate tool in the discrimination against backgrounds. Previous work demonstrated the ability to perform single atom imaging of Ba atoms in a single-vacancy site of a solid xenon matrix. In this paper, the effort to identify signal from individual barium atoms is extended to Ba atoms in a hexa-vacancy site in the matrix and is achieved despite increased photobleaching in this site. Abrupt fluorescence turn-off of a single Ba atom is also observed. Significant recovery of fluorescence signal lost through photobleaching is demonstrated upon annealing of Ba deposits in the Xe ice. Following annealing, it is observed that Ba atoms in the hexa-vacancy site exhibit antibleaching while Ba atoms in the tetra-vacancy site exhibit bleaching. This may be evidence for a matrix site transfer upon laser excitation. Our findings offer a path of continued research toward tagging of Ba daughters in all significant sites in solid xenon.

physics.atom-ph

'Searching for a needle in a haystack;' A Ba-tagging approach for an upgraded nEXO experiment

nEXO is a proposed experiment that will search for neutrinoless double-beta decay (0$νββ$) in 5-tonnes of liquid xenon (LXe), isotopically enriched in $^{136}$Xe. A technique called Ba-tagging is being developed as a potential future upgrade for nEXO to detect the $^{136}$Xe double-beta decay daughter isotope, $^{136}$Ba. An efficient Ba-tagging technique has the potential to boost nEXO's 0$νββ$ sensitivity by essentially suppressing non-double-beta decay background events. A conceptual approach for the extraction from the detector volume, trapping, and identification of a single Ba ion from 5 tonnes of LXe is presented, along with initial results from the commissioning of one of its subsystems, a quadrupole mass filter.

nucl-ex

Development of a $^{127}$Xe calibration source for nEXO

We study a possible calibration technique for the nEXO experiment using a $^{127}$Xe electron capture source. nEXO is a next-generation search for neutrinoless double beta decay ($0νββ$) that will use a 5-tonne, monolithic liquid xenon time projection chamber (TPC). The xenon, used both as source and detection medium, will be enriched to 90% in $^{136}$Xe. To optimize the event reconstruction and energy resolution, calibrations are needed to map the position- and time-dependent detector response. The 36.3 day half-life of $^{127}$Xe and its small $Q$-value compared to that of $^{136}$Xe $0νββ$ would allow a small activity to be maintained continuously in the detector during normal operations without introducing additional backgrounds, thereby enabling in-situ calibration and monitoring of the detector response. In this work we describe a process for producing the source and preliminary experimental tests. We then use simulations to project the precision with which such a source could calibrate spatial corrections to the light and charge response of the nEXO TPC.

physics.ins-det

Characterization of a Spatially Resolved Multi-Element Laser Ablation Ion Source

A laser ablation ion source (LAS) is a powerful tool by which diverse species of ions can be produced for mass spectrometer calibration, or surface study applications. It is necessary to frequently shift the laser position on the target to selectively ablate materials in a controlled manner, and to mitigate degradation of the target surface caused by ablation. An alternative to mounting the target onto a rotation wheel or $x-y$ translation stage, is to shift the laser position with a final reflection from a motorized kinematic mirror mount. Such a system has been developed, assembled and characterized with a two axis motorized mirror and various metal targets. In the system presented here, ions are ablated from the target surface and guided by a 90 degree quadrupole bender to a Faraday cup where the ion current is measured. Spatially resolved scans of the target are produced by actuating the mirror motors, thus moving the laser spot across the target, and performing synchronous measurements of the ion current to construct 2D images of a target surface which can be up to 50~mm in diameter. The spatial resolution of the system has been measured by scanning the interfaces between metals such as steel and niobium, where it was demonstrated that the LAS can selectively ablate an area of diameter $\approx$50 $μ$m. This work informs the development of subsequent LAS systems, that are intended to serve as multi-element ion sources for commercial and custom-built time-of-flight mass spectrometers, or to selectively study surface specific regions of samples.

physics.ins-det