arXiv subjects

H. Sato

Publications and source records attributed to H. Sato.

At least 91 records · Page 5Linked to original sources

arXiv2006

Evolution of superconductivity in Pr$_{1-x}$La$_{x}$Os$_{4}$Sb$_{12}$: Upper critical field measurements

Measurements of the upper critical field $H_{c2}$ near $T_c$ of Pr$_{1- x}$La$_{x}$Os$_{4}$Sb$_{12}$ were performed by specific heat. A positive curvature in $H_{c2}$ versus $T$ was observed in samples and concentrations exhibiting two superconducting transitions. These results argue against this curvature being due to two-band superconductivity. The critical field slope - $dH_{c2}/dT$ suggests the existence of a crossover concentration $x_{cr} \approx 0.25$, below which there is a rapid suppression of effective electron mass with La-alloying. This crossover concentration was previously detected in the measurement of the discontinuity of $C/T$ at $T_c$.

cond-mat.supr-con↗

arXiv2006

Drastic change in transport of entropy with quadrupolar ordering in PrFe$_{4}$P$_{12}$

The antiferroquadrupolar ordering of PrFe$_{4}$P$_{12}$ is explored by probing thermal and thermoelectric transport. The lattice thermal conductivity drastically increases with the ordering, as a consequence of a large drop in carrier concentration and a strong electron-phonon coupling. The low level of carrier density in the ordered state is confirmed by the anomalously large values of the Seebeck and Nernst coefficients. The results are reminiscent of URu$_{2}$Si$_{2}$ and suggest that both belong to the same class of aborted metal-insulator transitions. The magnitude of the Nernst coefficient, larger than in any other metal, indicates a new route for Ettingshaussen cooling at Kelvin temperatures.

cond-mat.str-el↗

arXiv2006

Electronic structure of semiconducting CeFe$_4$P$_{12}$: Strong hybridization and relevance of single-impurity Anderson model

Semiconducting skutterudite CeFe$_4$P$_{12}$ is investigated by synchrotron x-ray photoemission spectroscopy (PES) and x-ray absorption spectroscopy (XAS). Ce 3$d$ core-level PES and 3$d-4f$ XAS, in combination with single impurity Anderson model (SIAM) calculations, confirm features due to $f^0$, $f^1$ and $f^2$ configurations. The Ce 4$f$ density of states (DOS) indicates absence of a Kondo resonance at Fermi level, but can still be explained by SIAM with a small gap in non-$f$ DOS. While Ce 4$f$ partial DOS from band structure calculations are also consistent with the main Ce 4$f$ DOS, the importance of SIAM for core and valence spectra indicates Kondo semiconducting mixed valence for CeFe$_4$P$_{12}$, derived from strong hybridization between non-$f$ conduction and Ce 4$f$ DOS.

cond-mat.str-el↗

arXiv2005

Evidence for s-wave superconductivity with antiferromagnetic fluctuations in filled skutterudite LaFe$_{4}$P$_{12}$: $^{139}$La and $^{31}$P-NMR studies

We have performed $^{139}$La,$^{31}$P-NMR studies on a filled skutterudite superconductor LaFe$_{4}$P$_{12}$ with a critical temperature $T_c=4.1$ K. In the normal state, the presence of antiferromagnetic (AFM) fluctuations at finite wave vectors is suggested from the relation between the nuclear spin-lattice relaxation rate $1/T_1$ and the Knight shift. In the superconducting (SC) state, the distinct coherence peak was observed just below $T_c$, and is easily suppressed by the applied field. An exponential decrease of $1/T_1$ was observed, suggestive of the isotropic superconducting gap with $2Δ/k_{\rm B}T_c =3.8$. Besides, we observed the decrease of the Knight shift, indicative of the singlet-pair formation below $T_c$. These results are clear evidence that LaFe$_{4}$P$_{12}$ is a rare s-wave superconductor with significant AFM fluctuations.

cond-mat.str-el↗

arXiv2005

Design of a Polarised Positron Source Based on Laser Compton Scattering

We describe a scheme for producing polarised positrons at the ILC from polarised X-rays created by Compton scattering of a few-GeV electron beam off a CO2 or YAG laser. This scheme is very energy effective using high finesse laser cavities in conjunction with an electron storage ring.

physics.acc-ph↗

arXiv2005

Direct Observation of Quadrupolar Excitons in the Heavy-Fermion Superconductor PrOs$_{4}$Sb$_{12}$

We report inelastic neutron scattering experiments performed to investigate the low energy magnetic excitations on single crystals of the heavy-fermion superconductor PrOs$_{4}$Sb$_{12}$. The observed excitation clearly softens at a wave vector Q = (1,0,0), which is the same as the modulation vector of the field-induced antiferro-quadrupolar ordering, and its intensity at Q = (1,0,0) is smaller than that around the zone center. This result directly evidences that this excitonic behavior is derived mainly from nonmagnetic quadrupolar interactions. Furthermore, the narrowing of the linewidths of the excitations below the superconducting transition temperature indicates the close connection between the superconductivity and the excitons.

cond-mat.str-el↗

arXiv2005

Transport properties of the heavy fermion superconductor PrOs$_{4}$Sb$_{12}$

We have measured the electrical resistivity, thermoelectric power, Hall coefficient, and magnetoresistance (MR) on single crystals of PrOs$_{4}$Sb$_{12}$, LaOs$_{4}$Sb$_{12}$ and NdOs$_{4}$Sb$_{12}$. All the transport properties in PrOs$_{4}$Sb$_{12}$ are similar to those in LaOs$_{4}$Sb$_{12}$ and NdOs$_{4}$Sb$_{12}$ at high temperatures, indicating the localized character of 4$f$-electrons. The transverse MR both in LaOs$_{4}$Sb$_{12}$ and PrOs$_{4}$Sb$_{12}$ tends to saturate for wide field directions, indicating these compounds to be uncompensated metals with no open orbit. We have determined the phase diagram of the field induced ordered phase by the MR measurement for all the principle field directions, which indicates an unambiguous evidence for the $Γ_{\rm 1}$ singlet crystalline electric field ground state.

cond-mat.str-el↗

arXiv2005

Novel features in the flux-flow resistivity of the heavy fermion superconductor PrOs$_{4}$Sb$_{12}$

We have investigated the electrical resistivity of the heavy fermion superconductor PrOs$_{4}$Sb$_{12}$ in the mixed state. We found unusual double minima in the flux-flow resistivity as a function of magnetic field below the upper critical field for the first time, indicating double peaks in the pinning force density ($F_{\rm P}$). Estimated $F_{\rm P}$ at the peak exhibits apparent dependence on applied field direction; composed of two-fold and four-fold symmetries mimicking the reported angular dependence of thermal conductivity ($κ$). The result is discussed in correlation with the double step superconducting (SC) transition in the specific heat and the multiple SC-phases inferred from the angular dependence of $κ$.

cond-mat.str-el↗

arXiv2005

Silver-assisted growth of NdBa2Cu3O7-d thin films: A novel approach for the growth of superior quality ceramic oxide films

We have grown NdBa2Cu3O7-d films under silver atomic flux by molecular beam epitaxy, which show a drastic improvement in microstructure and also crystallinity leading to 30 % enhancement in critical current density. The most remarkable point is that the final film is free from silver. The key to our process in achieving a silver-free film was the use of RF-activated oxygen that oxidizes silver, nonvolatile, to silver oxide, volatile at the deposition temperature. This process enables one to utilize the beneficial effects of silver in the growth of oxide films and at the same time ensures that the final film be free from silver, which is important for high-frequency applications. This method can be made use in the growth of thin films of other complex oxide materials.

cond-mat.supr-con↗

arXiv2005

Fermi surface of the filled-skutterudite superconductor LaRu4P12: A clue to the origin of the metal-insulator transition in PrRu4P12

We report the de Haas-van Alphen (dHvA) effect and magnetoresistance in the filled-skutterudite superconductor LaRu4P12, which is a reference material of PrRu4P12 that exhibits a metal-insulator (M-I) transition at T_MI~60 K. The observed dHvA branches for the main Fermi surface (FS) are well explained by the band-structure calculation, using the full potential linearized augmented-plane-wave method with the local-density approximation, suggesting a nesting instability with q =(1,0,0) in the main multiply connected FS as expected also in PrRu4P12. Observed cyclotron effective masses of (2.6-11.8)m_0, which are roughly twice the calculated masses, indicate the large mass enhancement even in the La-skutterudites. Comparing the FS between LaRu4P12 and PrRu4P12, an essential role of c-f hybridization cooperating with the FS nesting in driving the the M-I transition in PrRu4P12 has been clarified.

cond-mat.str-el↗

arXiv2005

Transport properties in CeOs$_{4}$Sb$_{12}$: Possibility of the ground state being semiconducting

We have measured both magnetoresistance and Hall effect in CeOs$_4$Sb$_{12}$ to clarify the large resistivity state ascribed to the Kondo insulating one and the origin of the phase transition near 0.9 K reported in the specific heat measurement. We found unusual temperature ($T$) dependence both in the electrical resistivity $ρ\sim T^{-1/2}$ and the Hall coefficient $R_{\rm H}\sim T^{\rm -1}$ over the wide temperature range of about two order of magnitude below $\sim30$ K, which can be explained as a combined effect of the temperature dependences of carrier density and carrier scattering by spin fluctuation. An anomaly related with the phase transition has been clearly observed in the transport properties, from which the $H-T$ phase diagram is determined up to 14 T. Taking into account the small entropy change, the phase transition is most probably the spin density wave one. Both the electrical resistivity and Hall resistivity at 0.3 K is largely suppressed about an order of magnitude by magnetic fields above $\sim3$ T, suggesting a drastic change of electronic structure and a suppression of spin fluctuations under magnetic fields.

cond-mat.str-el↗

arXiv2004

Evolution of superconducting order in Pr(Os$_{1-x}$Ru$_{x}$)$_{4}$Sb$_{12}$

We report measurements of the magnetic penetration depth $λ$ in single crystals of Pr(Os$_{1-x}$Ru$_{x}$)$_{4}$Sb$_{12}$ down to 0.1 K. Both $λ$ and superfluid density $ρ_{s}$ exhibit an exponential behavior for the $x$$\geq$0.4 samples, going from weak ($x$=0.4,0.6), to moderate, coupling ($x$=0.8). For the $x$$\leq$0.2 samples, both $λ$ and $ρ_{s}$ vary as $T^{2}$ at low temperatures, but $ρ_{s}$ is s-wave-like at intermediate to high temperatures. Our data are consistent with a three-phase scenario, where a fully-gapped phase at $T_{c1}$ undergoes two transitions: first to an unconventional phase at $T_{c2}$$\lesssim$$T_{c1}$, then to a nodal low-$T$ phase at $T_{c3}$$<$$T_{c2}$, for small values of $x$.

cond-mat.supr-con↗

arXiv2004

Possible Kondo resonance in PrFe4P12 studied by bulk-sensitive photoemission

Pr 4f electronic states in Pr-based filled skutterudites PrT4X12(T=Fe and Ru; X=P and Sb) have been studied by high-resolution bulk-sensitive Pr 3d-4f resonance photoemission. A very strong spectral intensity is observed just below the Fermi level in the heavy-fermion system PrFe4P12. The increase of its intensity at lower temperatures is observed. We speculate that this is the Kondo resonance of Pr, the origin of which is attributed to the strong hybridization between the Pr 4f and the conduction electrons.

cond-mat.str-el↗

arXiv2004

Electronic structures of Cr$_{1-δ}$X (X=S, Te) studied by Cr 2p soft x-ray magnetic circular dichroism

Cr 2p core excited XAS and XMCD spectra of ferromagnetic Cr$_{1-δ}$Te with several concentrations of $δ$=0.11-0.33 and ferrimagnetic Cr$_{5}$S$_{6}$ have been measured. The observed XMCD lineshapes are found to very weakly depend on $δ$ for Cr$_{1-δ}$Te. The experimental results are analyzed by means of a configuration-interaction cluster model calculation with consideration of hybridization and electron correlation effects. The obtained values of the spin magnetic moment by the cluster model analyses are in agreement with the results of the band structure calculation.The calculated result shows that the doped holes created by the Cr deficiency exist mainly in the Te 5porbital of Cr$_{1-δ}$Te, whereas the holes are likely to be in Cr 3d state for Cr$_{5}$S$_{6}$.

cond-mat.mtrl-sci↗

arXiv2004

Superconducting phase diagram of the filled skuterrudite PrOs4Sb12

We present new measurements of the specific heat of the heavy fermion superconductor PrOs4Sb12, on a sample which exhibits two sharp distinct anomalies at Tc1= 1.89K and Tc2= 1.72K. They are used to draw a precise magnetic field-temperature superconducting phase diagram of PrOs4Sb12 down to 350 mK. We discuss the superconducting phase diagram of PrOs4Sb12 and its possible relation with an unconventional superconducting order parameter. We give a detailed analysis of Hc2(T), which shows paramagnetic limitation (a support for even parity pairing) and multiband effects.

cond-mat.supr-con↗

arXiv2004

Complex magnetic phase diagram of CePd_{2-x}Ni_xAl_3 around its critical concentration

Thermal, magnetic and transport measurements are reported on CePd_{2-x}Ni_xAl_3 in the 0<= x <= 1 range, including the effect of pressure (p) and magnetic field on some selected samples. The low temperature results indicate that long range antiferromagnetic order is stable up to x=0.2, while between 0.25 and 0.5 magnetic disorder gives rise to non-Fermi-liquid (NFL) behavior. In this region, the low temperature specific heat can be described by the sum of two components, the major one showing a C_P/T=gamma_0 -gamma_1 T^(1/2) dependence, while the minor one includes a decreasing number of degrees of freedom related to a residue of short range order. The latter extrapolates to zero between 0.45<x_{cr}<0.5. Electrical resistivity (rho) studies performed under pressure for x=0.5 allow to investigate the evolution of the NFL state right above the critical point, where the exponent of rho ~ T^n is found to increase from n=1 (for p=0) up to n=2 (for p=12 kbar). The latter is observed for x=1.0 already at normal pressure, indicating the onset of the Fermi Liquid behavior. Doping and pressure effects are compared by fitting high temperature resistivity data employing a unique function which allows to describe the evolution of the characteristic energy of this series through a large range of concentration and pressure.

cond-mat.str-el↗

arXiv2004

Probing the superconducting gap symmetry of PrRu$_{4}$Sb$_{12}$: A comparison with PrOs$_{4}$Sb$_{12}$

We report measurements of the magnetic penetration depth $λ$ in single crystals of PrRu$_{4}$Sb$_{12}$ down to 0.1 K. Both $λ$ and superfluid density $ρ_{s}$ exhibit an exponential behavior for $T$ $<$ 0.5$T_{c}$, with parameters $Δ$(0)/\textit{k}$_{B}$\textit{T}$_{c}$ = 1.9 and $λ(0)$ = 2900 Å. The value of $Δ$(0) is consistent with the specific-heat jump value of $ΔC/γT_{c}$ = 1.87 measured elsewhere, while the value of $λ(0)$ is consistent with the measured value of the electronic heat-capacity coefficient $γ$. Our data are consistent with PrRu$_{4}$Sb$_{12}$ being a moderate-coupling, fully-gapped superconductor. We suggest experiments to study how the nature of the superconducting state evolves with increasing Ru substitution for Os.

cond-mat.supr-con↗

arXiv2003

Probing the superconducting gap symmetry of PrOs$_{4}$Sb$_{12}$: A penetration depth study

We report measurements of the magnetic penetration depth $λ$ in single crystals of PrOs$_{4}$Sb$_{12}$ down to $\sim$0.1 K using a tunnel-diode based, self-inductive technique at 21 MHz, with the ac field applied along the \textit{a}, \textit{b} and \textit{c} directions. In all three field orientations the penetration depth and superfluid density $ρ_{s}$ tend to follow a power law, $λ\sim \mathit{T}^{2}, ρ_{s} \sim \mathit{T}% ^{2}$ at low temperatures. $ρ_{s}$ for various gap functions have been calculated, and data is best fit by the $^{3}$He A-phase-like gap with multidomains, each having two point nodes along a cube axis, and parameter $Δ_{0}$(0)/\textit{k}$_{B}$\textit{T}$_{c}$ = 2.6. This suggests that PrOs$_{4}$Sb$_{12}$ is a strong-coupling superconductor with two point nodes on the Fermi surface. We also confirm the observation of the double transitions at 1.75 K and 1.85 K seen in other measurements.

cond-mat.supr-con↗