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H. Schröder

Publications and source records attributed to H. Schröder.

3 recordsLinked to original sources

Two-XUV-photon double ionization of Neon studied at the Extreme Light Infrastructure (ELI-ALPS)

Two XUV-photon double ionization of Ne, induced by an intense few-pulse attosecond train with a ~ 4 fs envelope duration is investigated experimentally and theoretically. The experiment is performed at ELI-ALPS utilizing the recently constructed 10 Hz gas phase high-order harmonic generation SYLOS GHHG-COMPACT beamline. A total pulse energy up to ~1 μJ generated in Argon in conjunction with high reflectivity optics in the XUV region, allowed the observation of the doubly charged state of Ne induced by 40 eV central XUV photon energies. The interaction of the intense attosecond pulse train with Ne is also theoretically studied via a second-order time dependent perturbation theory equations-of-motion. The results of this work, combined with the feasibility of conducting XUV-pump-XUV-probe experiments, constitute a powerful tool for many potential applications. Those include attosecond pulse metrology as well as time resolved investigations of the dynamics underlying direct and sequential double ionization and their electron correlation effects.

physics.atom-ph↗

Time gated ion microscopy of light-atom interactions

The development of ultra-short intense laser sources in the visible and extreme ultraviolet (XUV) spectral range led to fascinating studies in laser-matter interactions and attosecond science. In the majority of these studies the system under investigation interacts with a focused laser beam, which ionizes the system. The ionization products are usually measured by devices, which spatiotemporally integrate the ionization signal originating from the entire focal area, discarding in this way valuable information about the ionization dynamics that take place in the interaction volume. Here, we review a recently developed approach in measuring the spatially resolved photoionization yields resulting from the interaction of infrared (IR)/XUV ultra-short laser pulses in gas phase media. We show how this approach enables a) the in-situ focus diagnostic, b) quantitative studies of linear and non-linear ionization processes in the IR/XUV regime, c) single-shot XUV-pump-XUV-probe studies and d) single-shot 2nd-order XUV autocorrelation measurements. The article has been published in J. Opt. 20, 024018 (2018) (doi.org/10.1088/2040-8986/aaa326).

physics.atom-ph↗

Revealing quantum path details in high-field physics

The tunnelling of an electron through a suppressed atomic potential followed by its motion in the continuum, is the fundamental mechanism underlying strong-field laser-atom/molecule interactions. Due to its quantum nature, the interaction is governed by the phase of the released electron wave-packets. Thus, detailed mapping of the electron wave-packet interferences provides essential insight into the physics underlying the interaction. A process which is providing access to the intricacies of the interaction is the generation of high order harmonics of the laser frequency. The phase-amplitude distribution of the emitted extreme-ultraviolet (EUV), carries the complete information about the harmonic generation process and vice-versa. Thus, the visualization of the EUV-spatial-amplitude-distribution, as it results from interfering electron wave-packet contributions, is of crucial importance. Restrictions to this accomplishment are due to the spatially integrating measurement approaches applied so far, that average out the phase effects in the generation process. In this work, we demonstrate a method which overcomes this obstacle. An EUV-spatial-amplitude-distribution-image is induced from the imprint on the measured spatial distribution of ions, produced through EUV-photon ionization of atoms. Interference extremes in the image carry phase information about the interfering electron wave-packets. The present approach provides detailed insight on the strong-field laser-atom interaction mechanism, while establishing the era of phase selective interaction studies. Furthermore, it paves the way for substantial enhancement of the spectral and temporal precision of measurements by in-situ controlling the phase distribution of the emitted radiation and/or spatially selecting the EUV-radiation-atom interaction products.

physics.atom-ph↗