arXiv subjects

H. Sugawara

Publications and source records attributed to H. Sugawara.

At least 19 recordsLinked to original sources

arXiv2025

Simultaneous probes of pseudogap and disorder by hard x-ray photoemission applied for a candidate thermoelectric Al-Pd-Ru quasicrystal

The bulk electronic structure of Al-Pd-Ru quasicrystal (QC) have been investigated by hard X-ray photoemission spectroscopy (HAXPES). We have found an intrinsic pseudogap structure in which the spectral weight in the vicinity of the Fermi level (E_F) is remarkably suppressed at any photon energy. The valence-band HAXPES spectra and the asymmetry of the core-level peaks indicate a contribution of the Al sites to the electronic structure in the vicinity of E_F with less contributions from the Pd and Ru sites. The disorder effects are found in the core-level lineshapes of the Al-Pd-Ru QC, of which the widths are much broader than those of the other reference crystalline solids with less disorder.

cond-mat.mtrl-sci↗

arXiv2025

Hybridized and Localized 4f Electronic States of Nd-based Intermetallic Compounds in Cubic Symmetry Probed by High-Energy Photoemission

We have performed soft and hard X-ray photoemission spectroscopies on NdTi2Al20 and NdBe13 which show antiferromagnetic ordering at low temperatures. The Nd 3d core-level photoemission and Nd 3d-4f valence-band resonant photoemission spectra show finite 4f4 initial-state components in addition to the 4f3 configurations attributed to the c-f hybridization effects in NdTi2Al20, while the 4f3 initial-state components with localized character are dominant in NdBe13. These results imply the emergence of overscreening channel due to the two-channel Kondo effect in NdTi2Al20 through the the strong c-f hybridization effect.

cond-mat.str-el↗

arXiv2020

Isotropic parallel antiferromagnetism in the magnetic-field-induced charge-ordered state of SmRu$_4$P$_{12}$ caused by $p$-$f$ hybridization

Nature of the field-induced charge ordered phase (phase II) of SmRu$_4$P$_{12}$ has been investigated by resonant x-ray diffraction (RXD) and polarized neutron diffraction (PND), focusing on the relationship between the atomic displacements and the antiferromagnetic (AFM) moments of Sm. From the analysis of the interference between the non-resonant Thomson scattering and the resonant magnetic scattering, combined with the spectral function obtained from x-ray magnetic circular dichroism, it is shown that the AFM moment of Sm prefers to be parallel to the field ($m_{\text{AF}} \parallel H$), giving rise to large and small moment sites around which the P$_{12}$ and Ru cage contract and expand, respectively. This is associated with the formation of the staggered ordering of the $Γ_7$-like and $Γ_8$-like crystal-field states, providing a strong piece of evidence for the charge order. PND was also performed to obtain complementary and unambiguous conclusion. In addition, isotropic and continuous nature of the phase II is demonstrated by the field-direction invariance of the interference spectrum in RXD. Crucial role of the $p$-$f$ hybridization is shown by resonant soft x-ray diffraction at the P $K$-edge ($1s\leftrightarrow 3p$), where we detected a resonance due to the spin polarized $3p$ orbitals reflecting the AFM order of Sm.

cond-mat.str-el↗

arXiv2020

Helimagnetic Structure and Heavy-Fermion-Like Behavior in the Vicinity of the Quantum Critical Point in Mn$_3$P

Antiferromagnet Mn$_3$P with Neel temperature $T_N=30$ K is composed of Mn-tetrahedrons and zigzag chains formed by three inequivalent Mn sites. Due to the nearly frustrated lattice with many short Mn-Mn bonds, competition of the exchange interactions is expected. We here investigate the magnetic structure and physical properties including pressure effect in single crystals of this material, and reveal a complex yet well-ordered helimagnetic structure. The itinerant character of this materials is strong, and the ordered state with small magnetic moments is easily suppressed under pressure, exhibiting a quantum critical point at $\sim1.6$ GPa. The remarkable mass renormalization, even in the ordered state, and an incoherent-coherent crossover in the low-temperature region, characterize an unusual electronic state in Mn$_3$P, which is most likely effected by the underlying frustration effect.

cond-mat.str-el↗

arXiv2019

Nonsaturating large magnetoresistance in the high carrier density nonsymmorphic metal CrP

The band structure of high carrier density metal CrP features an interesting crossing at the Y point of the Brillouin zone. The crossing, which is protected by the nonsymmorphic symmetry of the space group, results in a hybrid, semi-Dirac-like energy-momentum dispersion relation near Y. The linear energy-momentum dispersion relation along Y-$Γ$ is reminiscent of the observed band structure in several semimetallic extremely large magnetoresistance (XMR) materials. We have measured the transverse magnetoresistance of CrP up to 14 T at temperatures as low as $\sim$ 16 mK. Our data reveal a nonsaturating, quadratic magnetoresistance as well as the behaviour of the so-called `turn-on' temperature in the temperature dependence of resistivity. Despite the difference in the magnitude of the magnetoresistance and the fact that CrP is not a semimetal, these features are qualitatively similar to the observations reported for XMR materials. Thus, the high-field electrical transport studies of CrP offer the prospect of identifying the possible origin of the nonsaturating, quadratic magnetoresistance observed in a wide range of metals.

cond-mat.str-el↗

arXiv2016

Quasilinear quantum magnetoresistance in pressure-induced nonsymmorphic superconductor CrAs

In conventional metals, modification of electron trajectories under magnetic field gives rise to a magnetoresistance that varies quadratically at low field, followed by a saturation at high field for closed orbits on the Fermi surface. Deviations from the conventional behaviour, e.g. the observation of a linear magnetoresistance, or a non-saturating magnetoresistance, have been attributed to exotic electron scattering mechanisms. Recently, linear magnetoresistance has been observed in many Dirac materials, in which the electron-electron correlation is relatively weak. The strongly correlated helimagnet CrAs undergoes a quantum phase transition to a nonmagnetic superconductor under pressure. Near the magnetic instability, we observe a large and non-saturating quasilinear magnetoresistance from the upper critical field to 14 T at low temperatures. We show that the quasilinear magnetoresistance arises from an intricate interplay between a nontrivial band crossing protected by nonsymmorphic crystal symmetry and strong magnetic fluctuations

cond-mat.supr-con↗

arXiv2016

Atomic displacements and lattice distortion in the magnetic-field-induced charge ordered state of SmRu$_{4}$P$_{12}$

Structural properties of SmRu$_4$P$_{12}$ in the anomalous magnetic ordered phase between $T^*\sim 14 $ K and $T_{\text{N}}=16.5$ K in magnetic fields has been studied by x-ray diffraction. Atomic displacements of Ru and P, reflecting the field-induced charge order of the $p$ electrons, have been deduced by analyzing the intensities of the forbidden Bragg peaks, assuming a cubic space group $Pm\bar{3}$. Also, by utilizing high-resolution x-ray diffraction experiment, we observed a splitting of fundamental Bragg peaks, clarifying that the unit cell in the magnetic ordered phase is rhombohedral elongated along the $[1\, 1\, 1]$ axis. Responses of the rhombohedral domains to the magnetic field, which reflects the direction of the magnetic moment, is studied in detail.

cond-mat.str-el↗

arXiv2013

Pressure-Temperature-Magnetic Field Phase Diagram of Ferromagnetic Kondo Lattice CeRuPO

We report the temperature-pressure-magnetic field phase diagram made from electrical resistivity measurements for the ferromagnetic (FM) Kondo lattice CeRuPO. The ground state at zero field changes from the FM state to another state, which is suggested to be an antiferromagnetic (AFM) state, above ~0.7 GPa, and the magnetically ordered state is completely suppressed at ~2.8 GPa. In addition to the collapse of the AFM state under pressure and a magnetic field, a metamagnetic (MM) transition from a paramagnetic state to a polarized paramagnetic state appears. CeRuPO will give us a rich playground for understanding the mechanism of the MM transition under comparable FM and AFM correlations in the Kondo lattice.

cond-mat.str-el↗

arXiv2013

Nonmagnetic Impurity Effect of the S=1/2 Spin Ladder System (pipdH)_2Cu_{1-x}Zn_xBr_4

We report the synthesis and the magnetic susceptibility of (pipdH)2Cu1-xZnxBr4, which is a nonmagnetic impurity-doped S=1/2 spin ladder system. The samples were synthesized from a solution by using a slow evaporation method. Samples were confirmed to be in a single phase and to have the same crystal structure as the pure system (pipdH)2CuBr4 by using X-ray diffraction measurements. To check the magnetic properties, we performed magnetic susceptibility and magnetization measurements with a SQUID magnetometer. A plot of the inverse magnetic susceptibility indicates the presence of dominant antiferromagnetic coupling. The magnetic susceptibility shows a broad maximum due to low dimensionality and a spin gap behavior related to the two-leg spin ladder at low temperature. The spin gap and the Curie constants of Zn-doped samples, as estimated from an analysis of the magnetic susceptibility, monotonically decrease as the Zn concentration decreases. A nonmagnetic impurity of S=1/2 spin ladder system affects the spin gap.

cond-mat.mtrl-sci↗

arXiv2013

Pressure suppression of spin-density-wave gap in the optical conductivity of SrFe2As2

Optical reflectance R(w) of a pressure-induced superconductor SrFe2As2 has been measured under external pressure to 6 GPa and at temperatures to 8 K. Optical conductivity s(w) has been derived from the measured R(w). At ambient pressure, in the antiferromagnetic state below T_N=198 K, a pronounced feature develops in s(w) due to the opening of a spin density wave (SDW) gap, as already reported in the literature. With increasing pressure, the SDW gap feature in s(w) is progressively suppressed. At 4 GPa, where the sample is superconducting, the SDW gap feature in s(w) is strongly reduced than that at ambient pressure, but is still clearly observed. At 6 GPa, the SDW gap is completely suppressed. The pressure evolutions of the SDW gap magnitude and the spectral weight closely follow the pressure evolution of T_N.

cond-mat.str-el↗

arXiv2012

Penetration depth study of LaOs$_4$Sb$_{12}$: Multiband s-wave superconductivity

We measured the magnetic penetration depth $λ(T)$ in single crystals of LaOs$_{4}$Sb$_{12}$ ($T_c$=0.74 K) down to 85 mK using a tunnel diode oscillator technique. The observed low-temperature exponential dependence indicates a s-wave gap. Fitting the low temperature data to BCS s-wave expression gives the zero temperature gap value $Δ(0)= (1.34 \pm 0.07) k_B T_c$ which is significantly smaller than the BCS value of 1.76$k_B T_c$. In addition, the normalized superfluid density $ρ(T)$ shows an unusually long suppression near $T_c$, and are best fit by a two-band s-wave model.

cond-mat.supr-con↗

arXiv2012

Pressure suppression of unconventional charge-density-wave state in PrRu4P12 studied by optical conductivity

Optical conductivity s(w) of PrRu4P12 has been studied under high pressure to 14 GPa, at low temperatures to 8 K, and at photon energies 12 meV-1.1 eV. The energy gap in s(w) at ambient pressure, caused by a metal-insulator transition due to an unconventional charge-density-wave formation at 63 K, is gradually filled in with increasing pressure to 10 GPa. At 14 GPa and below 30 K, s(w) exhibits a pronounced Drude-type component due to free carriers. This indicates that the initial insulating ground state at zero pressure has been turned into a metallic one at 14 GPa. This is consistent with a previous resistivity study under pressure, where the resistivity rapidly decreased with cooling below 30 K at 14 GPa. The evolution of electronic structure with pressure is discussed in terms of the hybridization between the 4f and conduction electrons.

cond-mat.str-el↗

arXiv2012

Optical Conductivity and Electronic Structure of CeRu4Sb12 under High Pressure

Optical conductivity [s(w)] of Ce-filled skutterudite CeRu4Sb12 has been measured at high pressure to 8 GPa and at low temperature, to probe the pressure evolution of its electronic structures. At ambient pressure, a mid-infrared peak at 0.1 eV was formed in s(w) at low temperature, and the spectral weight below 0.1 eV was strongly suppressed, due to a hybridization of the f electron and conduction electron states. With increasing external pressure, the mid-infrared peak shifts to higher energy, and the spectral weight below the peak was further depleted. The obtained spectral data are analyzed in comparison with band calculation result and other reported physical properties. It is shown that the electronic structure of CeRu4Sb12 becomes similar to that of a narrow-gap semiconductor under external pressure.

cond-mat.str-el↗

arXiv2011

Suppression of time reversal symmetry breaking superconductivity in Pr(Os,Ru)_4Sb_12 and (Pr,La)Os_4Sb_12

Zero-field muon spin relaxation experiments have been carried out in the Pr(Os_{1-x}Ru_x)_4Sb_12 and Pr_{1-y}La_yOs_4Sb_12 alloy systems to investigate broken time-reversal symmetry (TRS) in the superconducting state, signaled by the onset of a spontaneous static local magnetic field B_s. In both alloy series B_s initially decreases linearly with solute concentration. Ru doping is considerably more efficient than La doping, with a ~50% faster initial decrease. The data suggest that broken TRS is suppressed for Ru concentration x >~ 0.6, but persists for essentially all La concentrations. Our data support a crystal-field excitonic Cooper pairing mechanism for TRS-breaking superconductivity.

cond-mat.supr-con↗

arXiv2010

Comment on "Pronounced Enhancement of the Lower Critical Field and Critical Current Deep in the Superconducting State of PrOs4Sb12"

Cichorek et al. [Phys. Rev. Lett. 94, 107002 (2005)] reported enhancements of the lower critical field Hc1(T) and critical current in superconducting PrOs4Sb12 below a transition temperature Tc3 ~ 0.6 K, and speculated that this reflects a transition between superconducting phases. Features have been observed near Tc3 in other properties, but not in the specific heat. We report muon spin rotation measurements of the penetration depth in the vortex state of PrOs4Sb12 near Hc1(T), that to high accuracy exhibit no anomaly Tc3 and therefore cast doubt on the putative phase transition.

cond-mat.supr-con↗

arXiv2009

Anomalous properties in the low-carrier ordered phase of PrRu4P12: Consequence of hybridization between conduction and Pr 4f electrons

The low-carrier ordered phase below the metal-non-metal transition temperature T_MI ~ 63 K of PrRu4P12 is explored by probing magnetoresistance, magnetic susceptibility, thermoelectric power, and Hall effect on high quality single crystals. All the measured properties exhibit the signature of decimation of the Fermi surface below T_MI and anomalous behaviors below 30 K including a large thermoelectric power ~-200 uV/K and a giant negative magnetoresistance (93% at ~0.4 K). The results indicate an additional structure below 30 K and a semimetal-like ground state. The observed anomalous behaviors are most likely associated with the novel role of c-f hybridization between conduction electrons and Pr 4f electrons, whose crystalline electric field level schemes show drastic change below T_MI.

cond-mat.str-el↗

arXiv2009

Effect of Uniaxial Stress for Pressure-Induced Superconductor SrFe_2As_2

We report that the pressure-temperature phase diagram of single-crystalline SrFe$_2$As$_2$ is easily affected by the hydrostaticity of a pressure-transmitting medium. For all of the three mediums we used, superconductivity with zero resistance appears, accompanied by the suppression of an antiferromagnetic (orthorhombic) phase, but the critical pressure $P_c$ was found to depend on the type of medium. $P_c$ was estimated to be 4.4 GPa under almost hydrostatic condition, but it decreased to $3.4-3.7$ GPa with the use of the medium already solidified at room temperature. The uniaxial stress along the c-axis is suggested to aid in the suppression of the antiferromagnetic (orthorhombic) phase. The pressure effect of BaFe$_2$As$_2$ is also reported.

cond-mat.supr-con↗

arXiv2009

Superconducting Gap Structure of LaFePO Studied by Thermal Conductivity

The superconducting gap structure of LaFePO ($T_c=7.4 $K) is studied by thermal conductivity ($κ$) at low temperatures in fields $H$ parallel and perpendicular to the c axis. A clear two-step field dependence of $κ(H)$ with a characteristic field $H_s(\sim 350$ Oe) much lower than the upper critical field $H_{c2}$ is observed. In spite of large anisotropy of $H_{c2}$, $κ(H)$ in both $H$-directions is nearly identical below $H_s$. Above $H_s$, $κ(H)$ grows gradually with $H$ with a convex curvature, followed by a steep increase with strong upward curvature near $H_{c2}$. These results indicate the multigap superconductivity with active two-dimensional (2D) and passive 3D bands having contrasting gap values. Together with the recent penetration depth results, we suggest that the 2D bands consist of nodal and nodeless ones, consistent with the extended s-wave symmetry.

cond-mat.supr-con↗