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H. Suzuki

Publications and source records attributed to H. Suzuki.

At least 19 recordsLinked to original sources

Coupled structural and electronic evolution under pressure in CuIr2Se4, CuRh2S4, and CuRh2Se4

Spinel chalcogenides provide a platform for investigating the interplay among metallic, superconducting, and pressure-induced insulating states. Here, we combine synchrotron powder X-ray diffraction and electrical-resistivity measurements to investigate the pressure evolution of CuIr2Se4, CuRh2S4, and CuRh2Se4 over pressure ranges extending beyond those previously explored. High-pressure diffraction reveals closely related monoclinic supercells in all three compounds. For CuIr2Se4 and CuRh2S4, constrained profile fits based on structural models relaxed using density functional theory are compatible with Phase-IV-type bond-disproportionated structures, whereas the data for CuRh2Se4 establish a compatible monoclinic unit cell without resolving its atomic-scale ordering pattern. Insulating-like transport develops abruptly over a narrow pressure range in CuIr2Se4 but more gradually over broader pressure ranges in the Rh-based compounds, in close correspondence with their respective structural transformations. We also establish previously unreported bulk superconductivity in CuIr2Se4 at ambient pressure: zero resistance is attained at 0.29 K, and the accompanying ac diamagnetic response is consistent with nearly complete superconducting shielding. These results establish a close relationship between the formation of the high-pressure monoclinic phases and the evolution toward insulating transport, and demonstrate that transition-metal and chalcogen substitutions tune the characteristic pressure scales and the competition with superconductivity within a closely related structural framework.

cond-mat.mtrl-sci

Femtoscopy Measurement with S$\pi$RIT TPC in Radioactive BeamHeavy-ion Collisions

Femtoscopy is a powerful tool for exploring the dynamic emitting structure in heavy-ion collisions, while radioactive beam heavy-ion collisions enable the investigation of nuclear matter under extreme isospin conditions. Here, we successfully perform femtoscopy measurements using the S$\pi$RIT Time Projection Chamber (TPC). A dedicated correction scheme for track merging and splitting is proposed, which is well applicable to rectangular TPCs housed inside dipole magnets and effectively improves the reconstructed correlation functions at small relative momenta. Focusing on the proton-proton (p-p) correlation function in the 270 MeV/u $^{132}\text{Sn}+^{124}\text{Sn}$ system, we successfully apply the track merging and splitting correction; additionally, the TPC angular acceptance exhibits a negligible impact on the correlation function. A systematic uncertainty quantification framework is established. The experimental results of the p-p correlation function confirm the feasibility of the S$\pi$RIT TPC for femtoscopy measurements and provide technical support for high-precision femtoscopy studies using rectangular TPCs in radioactive beam heavy-ion collisions.

physics.ins-det

Large amplification of the isospin-dependence of proton emitting source size in radioactive heavy-ion collisions: a signal of n-p correlation

We report proton-proton correlation function measurements in central $^{132}$Sn+$^{124}$Sn and $^{108}$Sn+$^{112}$Sn collisions at 270 MeV/nucleon. The proton emitting source sizes are extracted for the systems by using femtoscopic imaging technique. The fast dynamic core radius for the neutron-rich system is found to be $2.22 \pm 0.13\ \text{(stat.)} \pm 0.07\ \text{(syst.)}$ fm, which is approximately 24\% larger than that for the neutron-deficient system, $1.74 \pm 0.08\ \text{(stat.)} \pm 0.05\ \text{(syst.)}$ fm. This difference is an order of magnitude larger than the $\sim$3\% difference in the ground-state charge radii of the projectile nuclei. Transport model simulations based on mean-field dynamics cannot reproduce this amplification. The observation reveals a beyond-mean-field mechanism associated to short-range neutron-proton correlations, which dynamically enhance the proton emitting source in the neutron-rich environment. Our results demonstrate that heavy-ion collisions induced by radioactive beam, combined with femtoscopic precision, provide a new hadronic probe of short-range correlation, and that careful treatment of the beyond-mean-field interactions are required in modeling such processes.

nucl-ex

Three-dimensional zigzag correlations in the van der Waals Kitaev magnet RuBr$_3$

Ruthenium trihalides Ru$X_3$ ($X$ = Cl, Br, I) provide a tunable platform for Kitaev magnetism in two-dimensional van der Waals materials. Despite their similar crystal structures and zigzag antiferromagnetic order, RuBr$_3$ exhibits a higher N\'eel temperature ($T_N$) than RuCl$_3$, suggesting their distinct proximity to the Kitaev quantum spin liquid phase. Using Ru $L_3$-edge resonant x-ray scattering, we show that, while the long-range zigzag order in RuBr$_3$ disappears at $T_N$, the zigzag correlations that persist well above $T_N$ show a pronounced spectral weight redistribution along the interlayer direction. These results suggest that the enhanced interlayer magnetic interactions driven by the extended Br 4$p$ orbitals stabilize three-dimensional zigzag correlations in RuBr$_3$.

cond-mat.str-el

The dipole strength distribution of $^8$He and decay characteristics

The weak binding and spatially extended neutron densities characteristic of drip-line nuclei give rise to a distinctive low-energy dipole response. The drip-line nucleus $^8$He is the most neutron-rich bound nucleus with a mass-to-charge ratio of $A/Z=4$. We measure the dipole response of $^8$He, including for the first time the four-neutron decay channel. A total dipole strength of $\sum B(E1)(E^*<15$~MeV$)=0.95(16)~e^2$fm$^2$ and a dipole polarizability of $\alpha_D = 0.61(1)$~fm$^3$ are extracted from the differential Coulomb-excitation cross section and compared to state-of-the-art theoretical calculations employing coupled cluster and three-body approaches. We find that the dipole continuum is dominated, even at high excitation energies well above the $4n$ decay threshold, by two-neutron emission, pointing to a $^6$He$+2n$ structure of the excited dipole mode. No indication was found for a $4n$ final-state correlation, while pronounced $nn$ and $^6$He-$n$ final-state correlations are apparent.

nucl-ex

Single-particle strength toward N = 32: Spectroscopy of 51 Ca via the 50 Ca(d, p) reaction

States in the neutron-rich isotope 51 Ca were populated via the 50 Ca(d, p) transfer reaction in inverse kinematics at a beam energy of about 14 AMeV. The experiment was performed using a decelerated radioactive 50 Ca beam from the OEDO facility and the TiNA2 silicon array in combination with the SHARAQ magnetic spectrometer at RIBF/RIKEN. The energies of excited states in 51 Ca were reconstructed via missing mass spectroscopy, and angular distributions of protons were measured to extract differential cross sections. From a comparison with adiabatic distorted wave approximation (ADWA) calculations, spectroscopic factors were deduced for several states, including the ground state and excited states up to 4.2 MeV. These results are compared with shell-model calculations, as well as ab initio valence-space in-medium similarity renormalization group (VS-IMSRG) predictions. The data support the assignment of the 1/2- and 5/2- single-particle states and provide evidence for a candidate 9/2+ state with a structure consistent with neutron excitation into the 0g9/2 orbital. These findings contribute new constraints on the single-particle structure and shell evolution in neutron-rich calcium isotopes.

nucl-ex

Direct observation of three-neutron emission from $^7$He$^*$ and the search for the trineutron

Three-neutron emission from $^7$He has been directly measured for the first time, following neutron knockout from a $^8$He beam at 156 MeV/nucleon. A resonance-like structure at $2.08(4)$ MeV above the $^4$He+$3n$ threshold [$E_x=2.68(4)$ MeV] with a width of $3.9(2)$ MeV was observed and deduced to arise predominately from the predicted $J^{\pi}=3/2^{-}_2$ level. The three-neutron invariant-mass spectrum was reconstructed and found to peak at around 1 MeV and could, through complete simulations incorporating neutron-neutron correlations, be very well described by the sequential decay of $^7$He$^*$ via the $2_1^+$ excited state of $^6$He. No evidence was found for any significant three-neutron correlations beyond those expected from well-established two-body interactions, including a trineutron resonance.

nucl-ex

High-Precision Mass Measurements of Proton-Rich Rh, Pd, Cd isotopes in the vicinity of 100Sn and Impact on X-Ray Burst and Supernova Nucleosynthesis

Using the ZeroDegree multi-reflection time-of-flight mass spectrograph of the CRISMASS project at RIKEN Radioactive Isotope Beam Factory, we performed high-precision mass measurements of proton-rich nuclei near the doubly magic nucleus 100Sn, achieving uncertainties on the order of 10 keV. The masses of 91Rh, 92Pd, and 96Cd were determined for the first time with high precision, and the accuracy of several additional masses was substantially improved. Incorporating the new data into X-ray burst simulations significantly reduces the abundance uncertainties in the $A$ = 90-100 region, shifting the reaction flow toward $A$ = 90 production and suppressing the synthesis of heavier nuclei. Further investigation of the $\nu p$-process indicates that 99Rh plays a significant role in the reaction flow within the mass region studied. These high-precision mass measurements refine the mass surface near 100Sn and provide critical constraints on models of proton-rich nucleosynthesis.

nucl-ex

A XRISM/Resolve view of the dynamics in the hot gaseous atmosphere of M87

The XRISM/Resolve microcalorimeter directly measured the gas velocities in the core of the Virgo Cluster, the closest example of AGN feedback in a cluster. This proximity allows us to resolve the kinematic impact of feedback on scales down to 5 kpc. Our spectral analysis reveals a high velocity dispersion of $\sigma_v$=262 (+45 / -38) km/s near the AGN, which steeply declines to ~60 km/s between 5 and 25 kpc in the northwest direction. The observed line-of-sight bulk velocity in all regions is broadly consistent with the central galaxy, M87, with a mild trend toward blueshifted motions at larger radii. Systematic uncertainties have been carefully assessed and do not affect the measurements. The central velocities, if attributed entirely to isotropic turbulence, correspond to a transonic ICM at sub-6 kpc scales with three-dimensional Mach number 0.69 (+0.14 / -0.11) and a non-thermal pressure fraction of 21 (+7 / -5)%. Simple models of weak shocks and sound waves and calculations assuming isotropic turbulence both support the hypothesis that the velocity field reflects a mix of shock-driven expansion and turbulence. Compared to other clusters observed by XRISM to date, M87's central region stands out as the most kinematically disturbed, exhibiting both the highest velocity dispersion and the largest 3D Mach number, concentrated at the smallest physical scales.

astro-ph.GA

Translational symmetry breaking in the electronic nematic phase of BaFe2As2

The microscopic origin of the nematicity, namely, four-fold rotational symmetry breaking in iron-based superconductors has been controversial since its discovery. In particular, its relationship with the stripe-type spin-density-wave order and the orthorhombic lattice distortion in the antiferromagnetic orthorhombic (AFO) phase, which exists at temperatures below the electronic nematic phase, has been highly debated. Here, we report on the temperature evolution of angle-resolved photoemission spectra of the parent compound BaFe2As2, ranging from the AFO to nematic to paramagnetic phases. The Dirac cone feature, which is formed in the AFO phase, is found to persist in the nematic phase, suggesting that an antiferroic order of the same periodicity as the AFO phase persists in the nematic phase. Considering the relatively shallow d_xy orbital in BaFe2As2, we propose that an antiferro-orbital order involving the d_xy and other orbitals takes place in the nematic phase.

cond-mat.supr-con

The beta decay of Tz=-2 64Se and its descendants: the T=2 isobaric multiplet

In this paper we present our results on the decay of 64Se. It is the heaviest Tz=-2 nucleus that both beta decays and has a stable mirror partner Tz=+2, thus allowing comparison with charge exchange reaction studies. The beta decays of 64Se and its descendants were studied at the RIKEN Nishina Center (Tokyo, Japan) following their production in the fragmentation of 78Kr on a beryllium target. Beta-delayed gamma-ray and particle radiation was identified for each of the nuclei in the decay chain allowing us to obtain decay schemes for 64Se, 64As, and 63Ge. Thus new excited states could be found for the descendant nuclei, including the interesting case of the N=Z nucleus 64Ge. Furthermore we observed for the first time the beta-delayed proton emission of 64Se and 64As. Based on these results we obtained proton branching ratios of 48.0(9)% in 64Se decay and 4.4(1)% in 64As decay. We obtained a half-life value of 22.5(6) ms for 64Se decay and half-lives slightly more precise than those in the literature for each nucleus involved in the decay chain. Using our results on the excited levels of 64As and the mass excess in the literature for 63Ge we obtained -39588(50) keV for the mass excess of 64As. Then based on the IMME we obtained the mass excess of -27429(88) keV for 64Se by extrapolation. The mirror process of 64Se beta decay, the charge exchange reaction 64Zn(3He,t)64Ga, has already been measured allowing us to study the mirror symmetry through the comparison of the weak force (beta decay) and strong force (charge exchange reaction). An interpretation of the decay schemes based on the idea of the Anti Analogue State is proposed.

nucl-ex

Decay study of the most neutron-deficient Zn isotopes with the Warsaw Optical TPC detector

Results of decay studies of nuclei in the vicinity of 54Zn, which is the most neutron-deficient isotope of zinc and undergoes ground-state two-proton radioactivity (2p), are presented. The measurements were performed with a gaseous time projection chamber with optical readout which allowed us to record tracks of protons emitted in the decays. A new method of data analysis was used to reconstruct energies and emission angles of low-energy protons that were stopped within the active volume of the chamber. Half-lives and branching ratios for \b{eta}-delayed proton emission channels were determined for 56Zn, 55Zn, and 55Cu. The \b{eta}-delayed emission of two protons for 55Zn was observed for the first time. Five events of 2p radioactivity of 54Zn were detected and reconstructed. The distribution of the opening angle between momenta of the two protons is consistent with the findings published in [Ascher et al. PRL 107, 102502 (2011)]. The combination of all results suggests a flat angular distribution, in contrast to the one measured for 45Fe.

nucl-ex

The unusual spectrum of the X-ray transient source XRISM J174610.8-290021 near the Galactic center

The Galactic center region was observed with the XRISM X-ray observatory during the performance verification phase in 2024 and a point-like X-ray source was detected with the X-ray imager Xtend at a position of (RA, Dec)=(17h46m10.8s, -29{\deg}00'21''), which is thus named XRISM J174610.8-290021. This source was bright in February to March and showed time variations in count rate by more than one order of magnitude in one week. The 2-10 keV X-ray luminosity was ~$10^{35}$ erg/s for the assumed distance of 8 kpc. However, after six months, it was below the detection limit. We found a hint of periodicity of 1537 s from timing analysis. The XRISM/Xtend spectrum has emission lines from helium-like iron (Fe He$\alpha$) at 6.7 keV and hydrogen-like iron (Fe Ly$\alpha$) at 6.97 keV; their intensity ratio is unusual with the latter being four times stronger than the former. If the emission is of thermal origin, the ionization temperature estimated from the iron-line intensity ratio is ~30 keV, which is inconsistent with the electron temperature estimated from the thermal bremsstrahlung, ~7 keV. Spectral models of magnetic cataclysmic variables, which are often seen in the Galactic center in this luminosity range, are found to fail to reproduce the obtained spectrum. By contrast, we found that the spectrum is well reproduced with the models of low-mass X-ray binaries containing a neutron star plus two narrow Gaussian lines. We consider that the source is intrinsically bright reaching $10^{37}$ erg/s, but is blocked from direct view due to a high inclination and only the scattered emission is visible. The photoionized plasma above the accretion disk with an ionization parameter of ~$10^{5}$ may explain the unusual iron line ratio. We further discuss the potential contribution of point sources of the type of XRISM J174610.8-290021 to the diffuse Galactic center X-ray emission.

astro-ph.HE

New limit on the \mu+->e+\gamma decay with the MEG II experiment

This letter reports the result of the search for the decay \mu+->e+\gamma undertaken at the Paul Scherrer Institut in Switzerland with the MEG II experiment using the data collected in the 2021- 2022 physics runs. The sensitivity of this search is 2.2x10-13, a factor of 2.4 better than that of the full MEG dataset and obtained in a data taking period of about one fourth that of MEG, thanks to the superior performances of the new detector. The result is consistent with the expected background, yielding an upper limit on the branching ratio of B(\mu+->e+\gamma)<1.5 x 10-13 (90 % C.L.). Additional improvements are expected with the data collected during the years 2023-2024. The data-taking will continue in the coming years.

hep-ex

LHCspin: a Polarized Gas Target for LHC

The goal of the LHCspin project is to develop innovative solutions for measuring the 3D structure of nucleons in high-energy polarized fixed-target collisions at LHC, exploring new processes and exploiting new probes in a unique, previously unexplored, kinematic regime. A precise multi-dimensional description of the hadron structure has, in fact, the potential to deepen our understanding of the strong interactions and to provide a much more precise framework for measuring both Standard Model and Beyond Standard Model observables. This ambitious task poses its basis on the recent experience with the successful installation and operation of the SMOG2 unpolarized gas target in front of the LHCb spectrometer. Besides allowing for interesting physics studies ranging from astrophysics to heavy-ion physics, SMOG2 provides an ideal benchmark for studying beam-target dynamics at the LHC and demonstrates the feasibility of simultaneous operation with beam-beam collisions. With the installation of the proposed polarized target system, LHCb will become the first experiment to simultaneously collect data from unpolarized beam-beam collisions at $\sqrt{s}$=14 TeV and polarized and unpolarized beam-target collisions at $\sqrt{s_{NN}}\sim$100 GeV. LHCspin has the potential to open new frontiers in physics by exploiting the capabilities of the world's most powerful collider and one of the most advanced spectrometers. This document also highlights the need to perform an R\&D campaign and the commissioning of the apparatus at the LHC Interaction Region 4 during the Run 4, before its final installation in LHCb. This opportunity could also allow to undertake preliminary physics measurements with unprecedented conditions.

hep-ex

Precision mass measurements around ${}^{84}$Mo rule out ZrNb cycle formation in the rapid proton-capture process at type I X-ray bursts

The rapid proton-capture ($rp$-) process is one of the primary, explosive thermonuclear burning processes that drive type I X-ray bursts. A possible termination of the $rp$-process at around ${}^{84}$Mo was previously suggested by the formation of a ZrNb cycle. We report here precision mass measurements at around ${}^{84}$Mo, which have concluded the possibility of the cycle. The experiment was conducted using the multi-reflection time-of-flight spectrograph at RIKEN RI Beam Factory, and the masses of ${}^{79}$Y, ${}^{83}$Nb, ${}^{84}$Mo, ${}^{88}$Ru, and an isomer in ${}^{78}$Y were measured. For ${}^{84}$Mo, and ${}^{88}$Ru, and the isomeric state of ${}^{78}$Y, their masses are experimentally determined for the first time with uncertainties of $\delta m \approx 20~{\rm keV/c^2}$. The mass precision of ${}^{79}$Y and ${}^{83}$Nb is improved to $13~{\rm keV/c^2}$ and $9.6~{\rm keV/c^2}$, respectively. The new $\alpha$-separation energy of ${}^{84}$Mo, 1.434(83) MeV, unambiguously rules out the possibility of forming the ZrNb cycle. The X-ray burst simulation with the new masses shows that our measurements effectively remove the large final abundance uncertainties in the $A=80-90$ mass region. The new mass values improve the prediction power for the composition of the nuclear ashes in X-ray bursts.

nucl-ex

Impact of newly measured $\beta$\nobreakdash-delayed neutron emitters around \myisoSimp{78}{Ni} on light element nucleosynthesis in the neutrino-wind following a neutron star merger

Neutron emission probabilities and half-lives of 37 beta-delayed neutron emitters from 75Ni to 92Br were measured at the RIKEN Nishina Center in Japan, including 11 one-neutron and 13 two-neutron emission probabilities and 6 half-lives measured for the first time, which supersede theoretical estimates. These nuclei lie in the path of the weak r-process occurring in neutrino-driven winds from the accretion disk formed after the merger of two neutron stars, synthesizing elements in the A~80 abundance peak. The presence of such elements dominates the accompanying kilonova emission over the first few days and has been identified in the AT2017gfo event, associated with the gravitational wave detection GW170817. Abundance calculations based on over 17000 simulated trajectories describing the evolution of matter properties in the merger outflows show that the new data lead to an increase of 50-70 percent in the abundance of Y, Zr, Nb, and Mo. This enhancement is large compared to the scatter of relative abundances observed in old very metal-poor stars and is therefore significant in the comparison with other possible astrophysical processes contributing to light-element production. These results underline the importance of including experimental decay data for very neutron-rich beta-delayed neutron emitters into r-process models.

nucl-ex

Circular Dichroism in Resonant Inelastic X-ray Scattering: Probing Altermagnetic Domains in MnTe

X-ray magnetic circular dichroism provides a means to identify ferromagnetic, chiral, and altermagnetic orders via their time-reversal-symmetry ($\mathcal{T}$) breaking. However, differentiating magnetic domains related by crystallographic symmetries remains a technical challenge. Here we reveal a circular dichroism (CD) in the resonant inelastic x-ray scattering (RIXS) spectra from the altermagnetic MnTe. The azimuthal dependence of the RIXS-CD intensity of the magnon excitations indicates a dominant occupation of a single altermagnetic domain. The RIXS-CD in our scattering geometry is ascribed to the mirror-symmetry breaking associated with the $\mathcal{T}$-broken altermagnetic order. Our results establish RIXS-CD as a domain-sensitive probe of elementary excitations in quantum materials.

cond-mat.str-el