arXiv subjects
Publications and source records attributed to H. Suzuki.
The tetraneutron has been drawing the attention of the nuclear physics community for decades, but a firm conclusion on its existence and properties is still far from being reached despite many experimental and theoretical efforts. New measurements have recently been performed at RIBF with the SAMURAI spectrometer by applying complementary reaction probes, which will help to pin down the properties of this four-neutron system.
High resolution resonant inelastic x-ray scattering (RIXS) has proven particularly effective in the determination of crystal field and spin excitations in cuprates. Its strength lies in the large Cu $L_{3}$ resonance and in the fact that the scattering cross section follows quite closely the single-ion model predictions, both in the insulating parent compounds and in the superconducting doped materials. However, the spectra become increasingly broader with (hole) doping, hence resolving and assigning spectral features has proven challenging even with the highest energy resolution experimentally achievable. Here we have overcome this limitation by measuring the complete polarization dependence of the RIXS spectra as function of momentum transfer and doping in thin films of NdBa$_{2}$Cu$_{3}$O$_{7-δ}$. Besides confirming the previous assignment of $dd$ and spin excitations (magnon, bimagnon) in the antiferromagnetic insulating parent compound, we unequivocally single out the actual spin-flip contribution at all dopings. We also demonstrate that the softening of $dd$ excitations is mainly attributed to the shift of the $xy$ peak to lower energy loss. These results provide a definitive assessment of the RIXS spectra of cuprates and demonstrate that RIXS measurements with full polarization control are practically feasible and highly informative.
We report that the local Ising anisotropy in pyrochlore oxides - the crucial requirement for realizing the spin-ice state - can be broken by means of high magnetic fields. For the case of the well-established classical spin-ice compound Ho$_2$Ti$_2$O$_7$ the magnetization exceeds the angle-dependent saturation value of the Ising limit using ultra-high fields up to 120 T. However, even under such extreme magnetic fields full saturation cannot be achieved. Crystal-electric-field calculations reveal that a level crossing for two of the four ion positions leads to magnetization steps at 55 and 100 T. In addition, we show that by using a field sweep rate in the range of the spin-relaxation time the dynamics of the spin system can be probed. Exclusively at 25 ns/T a new peak of the susceptibility appears around 2 T. We argue, this signals the cross-over between spin-ice and polarized correlations.
Exotic nuclei are characterized by a number of neutrons (or protons) in excess relative to stable nuclei. Their shell structure, which represents single-particle motion in a nucleus, may vary due to nuclear force and excess neutrons, in a phenomenon called shell evolution. This effect could be counterbalanced by collective modes causing deformations of the nuclear surface. Here, we study the interplay between shell evolution and shape deformation by focusing on the magnetic moment of an isomeric state of the neutron-rich nucleus 75Cu. We measure the magnetic moment using highly spin-controlled rare-isotope beams and achieving large spin alignment via a two-step reaction scheme that incorporates an angular-momentum-selecting nucleon removal. By combining our experiments with numerical simulations of many-fermion correlations, we find that the low-lying states in 75Cu are, to a large extent, of single-particle nature on top of a correlated 74Ni core. We elucidate the crucial role of shell evolution even in the presence of the collective mode, and within the same framework, we consider whether and how the double magicity of the 78Ni nucleus is restored, which is also of keen interest from the perspective of nucleosynthesis in explosive stellar processes.
The most neutron-rich boron isotopes 20B and 21B have been observed for the first time following proton removal from 22N and 22C at energies around 230 MeV/nucleon. Both nuclei were found to exist as resonances which were detected through their decay into 19B and one or two neutrons. Two-proton removal from 22N populated a prominent resonance-like structure in 20B at around 2.5 MeV above the one-neutron decay threshold, which is interpreted as arising from the closely spaced 1-,2- ground-state doublet predicted by the shell model. In the case of proton removal from 22C, the 19B plus one- and two-neutron channels were consistent with the population of a resonance in 21B 2.47+-0.19 MeV above the two-neutron decay threshold, which is found to exhibit direct two-neutron decay. The ground-state mass excesses determined for 20,21B are found to be in agreement with mass surface extrapolations derived within the latest atomic-mass evaluations.
The neutron-shell structure of $^{25}$F was studied using quasi-free (p,2p) knockout reaction at 270A MeV in inverse kinematics. The sum of spectroscopic factors of $π$0d$_{5/2}$ orbital is found to be $1.0 \pm 0.3$. However, the spectroscopic factor for the ground-state to ground-state transition ($^{25}$F, $^{24}$O$_{g.s.}$) is only $0.36\pm 0.13$, and $^{24}$O excited states are produced from the 0d$_{5/2}$ proton knockout. The result shows that the $^{24}$O core of $^{25}$F nucleus significantly differs from a free $^{24}$O nucleus, and the core consists of 35% $^{24}$O$_{g.s}$. and 65% excited $^{24}$O.
Incommensurate charge order (CO) has been identified as the leading competitor of high-temperature superconductivity in all major families of layered copper oxides, but the perplexing variety of CO states in different cuprates has confounded investigations of its impact on the transport and thermodynamic properties. The three-dimensional (3D) CO observed in YBa$_2$Cu$_3$O$_{6+x}$ in high magnetic fields is of particular interest, because quantum transport measurements have revealed detailed information about the corresponding Fermi surface. Here we use resonant X-ray scattering to demonstrate 3D-CO in underdoped YBa$_2$Cu$_3$O$_{6+x}$ films grown epitaxially on SrTiO$_3$ in the absence of magnetic fields. The resonance profiles indicate that Cu sites in the charge-reservoir layers participate in the CO state, and thus efficiently transmit CO correlations between adjacent CuO$_2$ bilayer units. The results offer fresh perspectives for experiments elucidating the influence of 3D-CO on the electronic properties of cuprates without the need to apply high magnetic fields.
A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.
We have used high-resolution resonant inelastic x-ray scattering (RIXS) to study a thin film of NdNiO$_3$, a compound whose unusual spin- and bond-ordered electronic ground state has been of long-standing interest. Below the magnetic ordering temperature, we observe well-defined collective magnon excitations along different high-symmetry directions in momentum space. The magnetic spectra depend strongly on the incident photon energy, which we attribute to RIXS coupling to different local electronic configurations of the expanded and compressed NiO$_6$ octahedra in the bond-ordered state. Both the noncollinear magnetic ground state and the observed site-dependent magnon excitations are well described by a model that assumes strong competition between the antiferromagnetic superexchange and ferromagnetic double-exchange interactions. Our study provides direct insight into the magnetic dynamics and exchange interactions of the rare-earth nickelates, and demonstrates that RIXS can serve as a site-selective probe of magnetism in these and other materials.
Charge order has now been observed in several cuprate high-temperature superconductors. We report a resonant inelastic x-ray scattering experiment on the electron-doped cuprate Nd$_{2-x}$Ce$_{x}$CuO$_4$ that demonstrates the existence of dynamic correlations at the charge order wave vector. Upon cooling we observe a softening in the electronic response, which has been predicted to occur for a d-wave charge order in electron-doped cuprates. At low temperatures, the energy range of these excitations coincides with that of the dispersive magnetic modes known as paramagnons. Furthermore, measurements where the polarization of the scattered photon is resolved indicate that the dynamic response at the charge order wave vector primarily involves spin-flip excitations. Overall, our findings indicate a coupling between dynamic magnetic and charge-order correlations in the cuprates.
In the polarised Drell-Yan experiment at the COMPASS facility in CERN pion beam with momentum of 190 GeV/c and intensity about $10^8$ pions/s interacted with transversely polarised NH$_3$ target. Muon pairs produced in Drel-Yan process were detected. The measurement was done in 2015 as the 1st ever polarised Drell-Yan fixed target experiment. The hydrogen nuclei in the solid-state NH$_3$ were polarised by dynamic nuclear polarisation in 2.5 T field of large-acceptance superconducting magnet. Large helium dilution cryostat was used to cool the target down below 100 mK. Polarisation of hydrogen nuclei reached during the data taking was about 80 %. Two oppositely polarised target cells, each 55 cm long and 4 cm in diameter were used. Overview of COMPASS facility and the polarised target with emphasis on the dilution cryostat and magnet is given. Results of the polarisation measurement in the Drell-Yan run and overviews of the target material, cell and dynamic nuclear polarisation system are given in the part II.
Charge modulations are considered as a leading competitor of high-temperature superconductivity in the underdoped cuprates, and their relationship to Fermi surface reconstructions and to the pseudogap state is an important subject of current research. Overdoped cuprates, on the other hand, are widely regarded as conventional Fermi liquids without collective electronic order. For the overdoped (Bi,Pb)2.12Sr1.88CuO6+δ (Bi2201) high-temperature superconductor, here we report resonant x-ray scattering measurements revealing incommensurate charge order reflections, with correlation lengths of 40-60 lattice units, that persist up to at least 250K. Charge order is markedly more robust in the overdoped than underdoped regime but the incommensurate wave vectors follow a common trend; moreover it coexists with a single, unreconstructed Fermi surface, without pseudogap or nesting features, as determined from angle-resolved photoemission spectroscopy. This re-entrant charge order is reproduced by model calculations that consider a strong van Hove singularity within a Fermi liquid framework.
We have constructed a nuclear equation of state (EOS) that includes a full nuclear ensemble for use in core-collapse supernova simulations. It is based on the EOS for uniform nuclear matter that two of the authors derived recently, applying a variational method to realistic two- and there-body nuclear forces. We utilize an extended liquid drop model of heavy nuclei and a quantum-theoretical mass evaluation for light nuclei. In addition to realistic nuclear forces, the inclusion of in-medium effects on the full ensemble of nuclei makes the new EOS one of the most realistic EOS's for supernova simulations. We make comparisons with the FYSS EOS, which is based on the same formulation for the nuclear ensemble but adopts the relativistic mean field (RMF) theory with the TM1 parameter set for uniform nuclear matter. The new EOS is softer than the FYSS EOS around and above nuclear saturation densities. We find that neutron-rich nuclei with small mass numbers are more abundant in the new EOS than in the FYSS EOS because of the larger saturation densities and smaller symmetry energy of nuclei in the former. We apply the two EOS's to 1D supernova simulations and find that the new EOS gives lower electron fractions and higher temperatures in the collapse phase owing to the smaller symmetry energy. As a result, the inner core has smaller masses for the new EOS. It is more compact, on the other hand, due to the softness of the new EOS and bounces at higher densities. The ensuing outward propagations of the shock wave in the outer core are very similar in the two simulations, which may be an artifact, though, caused by the use of the same tabulated electron capture rates for heavy nuclei ignoring differences in the nuclear composition between the two EOS's in these computations.
The $β$ decay of the odd-odd nucleus $^{70}$Br has been investigated with the BigRIPS and EURICA setups at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center. The $T=0$ ($J^π=9^+$) and $T=1$ ($J^π=0^+$) isomers have both been produced in in-flight fragmentation of $^{78}$Kr with ratios of 41.6(8)\% and 58.4(8)\%, respectively. A half-life of $t_{1/2}=2157^{+53}_{-49}$ ms has been measured for the $J^π=9^+$ isomer from $γ$-ray time decay analysis. Based on this result, we provide a new value of the half-life for the $J^π=0^+$ ground state of $^{70}$Br, $t_{1/2}=78.42\pm0.51$ ms, which is slightly more precise, and in excellent agreement, with the best measurement reported hitherto in the literature. For this decay, we provide the first estimate of the total branching fraction decaying through the $2^+_1$ state in the daughter nucleus $^{70}$Se, $R(2^+_1)=1.3\pm1.1\%$. We also report four new low-intensity $γ$-ray transitions at 661, 1103, 1561, and 1749 keV following the $β$ decay of the $J^π=9^+$ isomer. Based on their coincidence relationships, we tentatively propose two new excited states at 3945 and 4752 keV in $^{70}$Se with most probable spins and parities of $J^π=(6^+)$ and $(8^+)$, respectively. The observed structure is interpreted with the help of shell-model calculations, which predict a complex interplay between oblate and prolate configurations at low excitation energies.
The low-lying unbound level structure of the halo nucleus $^{19}\textrm{C}$ has been investigated using single-neutron knockout from $^{20}\textrm{C}$ on a carbon target at 280 MeV/nucleon. The invariant mass spectrum, derived from the momenta of the forward going beam velocity $^{18}\textrm{C}$ fragment and neutrons, was found to be dominated by a very narrow near threshold ($E_\textrm{rel}$ = 0.036(1) MeV) peak. Two less strongly populated resonance-like features were also observed at $E_\textrm{rel}$ = 0.84(4) and 2.31(3) MeV, both of which exhibit characteristics consistent with neutron $p$-shell hole states. Comparisons of the energies, measured cross sections and parallel momentum distributions to the results of shell-model and eikonal reaction calculations lead to spin-parity assignments of $5/2^+_1$ and $1/2^-_1$ for the levels at $E_x$ = 0.62(9) and 2.89(10) MeV with $S_n$ = 0.58(9) MeV. Spectroscopic factors were also deduced and found to be in reasonable accord with shell-model calculations. The valence neutron configuration of the $^{20}\textrm{C}$ ground state is thus seen to include, in addition to the known $1s^2_{1/2}$ component, a significant $0d^2_{5/2}$ contribution. The level scheme of $^{19}\textrm{C}$, including significantly the $1/2^-_1$ cross-shell state, is well accounted for by the YSOX shell-model interaction developed from the monopole-based universal interaction.
A new table of the nuclear equation of state (EOS) based on realistic nuclear potentials is constructed for core-collapse supernova numerical simulations. Adopting the EOS of uniform nuclear matter constructed by two of the present authors with the cluster variational method starting from the Argonne v18 and Urbana IX nuclear potentials, the Thomas-Fermi calculation is performed to obtain the minimized free energy of a Wigner-Seitz cell in non-uniform nuclear matter. As a preparation for the Thomas-Fermi calculation, the EOS of uniform nuclear matter is modified so as to remove the effects of deuteron cluster formation in uniform matter at low densities. Mixing of alpha particles is also taken into account following the procedure used by Shen et al. (1998, 2011). The critical densities with respect to the phase transition from non-uniform to uniform phase with the present EOS are slightly higher than those with the Shen EOS at small proton fractions. The critical temperature with respect to the liquid-gas phase transition decreases with the proton fraction in a more gradual manner than in the Shen EOS. Furthermore, the mass and proton numbers of nuclides appearing in non-uniform nuclear matter with small proton fractions are larger than those of the Shen EOS. These results are consequences of the fact that the density derivative coefficient of the symmetry energy of our EOS is smaller than that of the Shen EOS.
We have investigated the superconducting gap of optimally doped Ba(Fe$_{0.65}$Ru$_{0.35}$)$_2$As$_2$ by angle-resolved photoemission spectroscopy (APRES) using bulk-sensitive 7 eV laser and synchrotron radiation. It was found that the gap is isotropic in the $k_x$-$k_y$ plane both on the electron and hole Fermi surfaces (FSs). The gap magnitudes of two resolved hole FSs show similar $k_z$ dependences and decrease as $k_z$ approaches $\sim$ 2$π$/$c$ (i.e., around the Z point) unlike the other Fe-based superconductors reported so far, where the superconducting gap of only one hole FS shows a strong $k_z$ dependence. This unique gap structure can be understood in the scenario that the $d_{z^2}$ orbital character is mixed into both hole FSs due to the finite spin-orbit coupling between almost degenerate FSs and is reproduced by calculations within the random phase approximation including the spin-orbit coupling.
Transient single-particle spectral function of BaFe$_{2}$As$_{2}$, a parent compound of iron-based superconductors, has been studied by time- and angle-resolved photoemission spectroscopy with an extreme-ultraviolet laser generated by higher harmonics from Ar gas, which enables us to investigate the dynamics in the entire Brillouin zone. We observed electronic modifications from the spin-density-wave (SDW) ordered state within $\sim$ 1 ps after the arrival of a 1.5 eV pump pulse. We observed optically excited electrons at the zone center above $E_{F}$ at 0.12 ps, and their rapid decay. After the fast decay of the optically excited electrons, a thermalized state appears and survives for a relatively long time. From the comparison with the density-functional theory band structure for the paramagnetic and SDW states, we interpret the experimental observations as the melting of the SDW. Exponential decay constants for the thermalized state to recover back to the SDW ground state are $\sim$ 0.60 ps both around the zone center and the zone corner.