arXiv subjects

H. Tanaka

Publications and source records attributed to H. Tanaka.

At least 163 records · Page 9Linked to original sources

arXiv2006

Thermodynamic properties of the field-induced Neel order of TlCuCl3

TlCuCl3 shows a quantum phase transition from a spin-gap phase to a Neel-ordered ground state as a function of magnetic field around H_{C0}~4.8T. From measurements of the specific heat c and the linear thermal expansion alpha_i we calculate the Grueneisen parameter Gamma_i(T)=alpha_i/c. Close to H_{C0} we find a diverging Gamma_i(T->0, in qualitative agreement with theoretical predictions. However, the predicted individual temperature dependencies of alpha(T) and c(T) are not reproduced by our experimental data.

cond-mat.str-el↗

arXiv2006

Cu-NMR study on the disordered quantum spin magnet with the Bose-glass ground state

Cu-NMR study has been performed on the disordered spin-gap system Tl1-xKxCuCl3 In the high-field H > HC=Δ/μ_B, where Δis the spin-gap, the hyperfine field becomes extremely inhomogeneous at low temperatures due to the field-induced magnetic order, indicating that the ordered spin state must be different from the pure TlCuCl3. In the low field H < HC, a saturating behavior in the longitudinal nuclear spin relaxation rate 1/T1 was observed at low temperatures, indicating existence of the magnetic ground state proposed to be Bose-glass phase by Fisher.

cond-mat.str-el↗

arXiv2006

Thermodynamics of the coupled spin-dimer system TlCuCl3 close to a quantum phase transition

We present thermal expansion alpha, magnetostriction and specific heat C measurements of \tal, which shows a quantum phase transition from a spin-gap phase to a Neel-ordered ground state as a function of magnetic field around H_{C0}->4.8T. Using Ehrenfest's relation, we find huge pressure dependencies of the spin gap for uniaxial as well as for hydrostatic pressure. For T->0 and H->H_{C0} we observe a diverging Grueneisen parameter Gamma(T)=alpha/C, in qualitative agreement with theoretical predictions. However, the predicted individual temperature dependencies alpha(T) and C(T) are not reproduced by our experimental data.

cond-mat.str-el↗

arXiv2006

Magentic Ordering under Hydrostatic Pressure in Doped Spin Gap Systems ACu$_{1-x}$Mg$_x$Cl$_3$: A$=$Tl and K

Magnetic phase transitions under hydrostatic pressures in spin gap systems TlCu$_{0.988}$Mg$_{0.012}$Cl$_3$ and KCu$_{0.973}$Mg$_{0.027}$Cl$_3$ were investigated by magnetization measurements. The present doped systems exhibit impurity-induced magnetic orderings. With increasing pressure, ordering temperature $T_{\rm N}$ increases. With a further increase in pressure, the present systems undergo phase transitions to uniform antiferromagnetic phases due to the closing of the triplet gap in the intact dimers. The crossover from the impurity-induced ordered phase to the uniform antiferromagnetic phase occurs at $P \simeq 1.3$ kbar for TlCu$_{0.988}$Mg$_{0.012}$Cl$_3$.

cond-mat.str-el↗

arXiv2006

Magnetic-Field Induced Gap in One-Dimensional Antiferromagnet KCuGaF$_6$

Magnetic susceptibility and specific heat measurements in magnetic fields were performed on an $S=1/2$ one-dimensional antiferromagnet KCuGaF$_6$. Exchange interaction was evaluated as $J/k_{\rm B}\simeq 100$ K. However, no magnetic ordering was observed down to 0.46 K. It was found that an applied magnetic field induces a staggered magnetic susceptibility obeying the Curie law and an excitation gap, both of which should be attributed to the antisymmetric interaction of the Dzyaloshinsky-Moriya type and/or the staggered $g$-tensor. With increasing magnetic field $H$, the gap increases almost in proportion to $H^{2/3}$.

cond-mat.str-el↗

arXiv2006

Crossover from impurity-induced ordered phase to uniform antiferromagnetic phase under hydrostatic pressure in the doped spin-gap system TlCu$_{1-x}$Mg$_x$Cl$_3$

Magnetic phase transition under hydrostatic pressure in TlCu$_{0.988}$Mg$_{0.012}$Cl$_3$ was investigated by magnetization measurements. The parent compound TlCuCl$_3$ is a coupled spin dimer system, which undergoes a pressure-induced quantum phase transition from a gapped ground state to an antiferromagnetic state at $P_{\rm c} = 0.42$ kbar due to the shrinkage of the gap. At ambient pressure, the present doped system exhibits impurity-induced magnetic ordering at $T_{\rm N}=2.5$ K. With increasing pressure, $T_{\rm N}$ increases. This is because the effective exchange interaction $J_{\rm eff}$ between unpaired spins is enhanced by the shrinkage of the gap. With a further increase in pressure, the present system undergoes a phase transition to a uniform antiferromagnetic phase due to the closing of the triplet gap in the intact dimers. The crossover from the impurity-induced ordered phase to the uniform antiferromagnetic phase occurs at $P \simeq 1.3$ kbar.

cond-mat.str-el↗

arXiv2006

Magentic-Field Induced Quantum Phase Transition and Critical Behavior in a Gapped Spin System TlCuCl$_3$

Magnetization measurements were performed on TlCuCl$_3$ with gapped ground state. The critical density and the magnetic phase diagram were obtained. The interacting constant was obtained as $U/k_{\rm B} = 313$ K. The experimental phase boundary for $T < 5$ K agrees perfectly with the magnon BEC theory based on the Hartree-Fock approximation with realistic dispersion relations and $U/k_{\rm B} = 320 $ K. The exponent $ϕ$ obtained with all the data points for $T < 5$ K is $ϕ= 1.99$, which is somewhat larger than theoretical exponent $ϕ_{\rm BEC} =3/2$. However, it was found that the exponent converges at $ϕ_{\rm BEC} =3/2$ with decreasing fitting window.

cond-mat.str-el↗

arXiv2006

S=1/2 Kagome antiferromagnets Cs$_2$Cu$_3MF$_{12}$ with M=Zr and Hf

Magnetization and specific heat measurements have been carried out on Cs$_2$Cu$_3$ZrF$_{12}$ and Cs$_2$Cu$_3$HfF$_{12}$ single crystals, in which Cu$^{2+}$ ions with spin-1/2 form a regular Kagomé lattice. The antiferromagnetic exchange interaction between neighboring Cu$^{2+}$ spins is $J/k_{\rm B}\simeq 360$ K and 540 K for Cs$_2$Cu$_3$ZrF$_{12}$ and Cs$_2$Cu$_3$HfF$_{12}$, respectively. Structural phase transitions were observed at $T_{\rm t}\simeq 210$ K and 175 K for Cs$_2$Cu$_3$ZrF$_{12}$ and Cs$_2$Cu$_3$HfF$_{12}$, respectively. The specific heat shows a small bend anomaly indicative of magnetic ordering at $T_\mathrm{N}= 23.5$ K and 24.5 K in Cs$_2$Cu$_3$ZrF$_{12}$ and Cs$_2$Cu$_3$HfF$_{12}$, respectively. Weak ferromagnetic behavior was observed below $T_\mathrm{N}$. This weak ferromagnetism should be ascribed to the antisymmetric interaction of the Dzyaloshinsky-Moriya type that are generally allowed in the Kagomé lattice.

cond-mat.str-el↗

arXiv2006

A simple model of reactor cores for reactor neutrino flux calculations for the KamLAND experiment

KamLAND is a reactor neutrino oscillation experiment with a very long baseline. This experiment successfully measured oscillation phenomena of reactor antineutrinos coming mainly from 53 reactors in Japan. In order to extract the results, it is necessary to accurately calculate time-dependent antineutrino spectra from all the reactors. A simple model of reactor cores and code implementing it were developed for this purpose. This paper describes the model of the reactor cores used in the KamLAND reactor analysis.

physics.data-an↗

arXiv2006

Attempt to distinguish the origins of self-similarity by natural time analysis

Self-similarity may originate from two origins, i.e., the process memory and the process' increments ``infinite'' variance. A distinction is attempted by employing the natural time χ. Concerning the first origin, we analyze recent data on Seismic Electric Signals, which support the view that they exhibit infinitely ranged temporal correlations. Concerning the second, slowly driven systems that emit bursts of various energies E obeying power-law distribution, i.e., P(E) ~ E^-γ, are studied. An interrelation between the exponent γand the variance κ_1(= <χ^2> - <χ>^2) is obtained for the shuffled (randomized) data. In the latter, the most probable value of κ_1 is approximately equal to that of the original data. Finally, it is found that the differential entropy associated with the probability P(κ_1) maximizes for γaround 1.6 to 1.7, which is comparable to the value determined experimentally in diverse phenomena, e.g., solar flares, icequakes, dislocation glide in stressed single crystals of ice e.t.c. It also agrees with the b-value in the Gutenberg-Richter law of earthquakes.

cond-mat.stat-mech↗

arXiv2006

Drastic Change of Magnetic Phase Diagram in Doped Quantum Antiferromagnet TlCu$_{1-x}$Mg$_x$Cl$_3$

TlCuCl$_3$ is a coupled spin dimer system, which has a singlet ground state with an excitation gap of $Δ/gμ_{\mathrm B}$ = 5.5 T. TlCu$_{1-x}$Mg$_x$Cl$_3$ doped with nonmagnetic Mg$^{2+}$ ions undergoes impurity-induced magnetic ordering. Because triplet excitation with a finite gap still remains, this doped system can also undergo magnetic-field-induced magnetic ordering. By specific heat measurements and neutron scattering experiments under a magnetic field, we investigated the phase diagram in TlCu$_{1-x}$Mg$_x$Cl$_3$ with $x\sim 0.01$, and found that impurity- and field-induced ordered phases are the same. The gapped spin liquid state observed in pure TlCuCl$_3$ is completely wiped out by the small amount of doping.

cond-mat.str-el↗

arXiv2005

Specific heat of the $S = 1$ spin-dimer antiferromagnet Ba$_3$Mn$_2$O$_8$ in high magnetic fields

We have measured the specific heat of the coupled spin-dimer antiferromagnet Ba$_3$Mn$_2$O$_8$ to 50 mK in temperature and to 29 T in the magnetic field. The experiment extends to the midpoint of the field region (25.9 T $\leq H \leq$ 32.3 T) of the magnetization plateau at 1/2 of the saturation magnetization, and reveals the presence of three ordered phases in the field region between that of the magnetization plateau and the low-field spin-liquid region. The exponent of the phase boundary with the thermally disordered region is smaller than the theoretical value based on the Bose-Einstein condensation of spin triplets. At zero field and 29 T, the specific-heat data show gapped behaviors characteristic of spin liquids. The zero-field data indicate that the gapped triplet excitations form two levels whose energies differ by nearly a factor of two. At least the lower level is well localized. The data at 29 T reveal that the low-lying excitations at the magnetization plateau are weakly delocalized.

cond-mat.str-el↗

arXiv2005

EMR Measurements of Field-Induced Superconductor lamda-(BETS)2FexGa1-xCl4

We have performed high-field Electron Magnetic Resonance (EMR) measurements of lamda-(BETS)2FexGa1-xCl4 to clarify the role of Pi- and d-electrons in the paramagnetic (PM) and field-induced superconducting (FISC) phases. We found that this system has a non-negligible Pi-d interaction that is very sensitive to the sample cooling rate. The Pi-d interaction is weaker when the sample is rapidly cooled which might affect its FISC phase. The results of the organic alloy lamda-(BETS)2FexGa1-xCl4 (x=0.6) will be presented in this paper.

cond-mat.supr-con↗

arXiv2005

Parametric control of a superconducting flux qubit

Parametric control of a superconducting flux qubit has been achieved by using two-frequency microwave pulses. We have observed Rabi oscillations stemming from parametric transitions between the qubit states when the sum of the two microwave frequencies or the difference between them matches the qubit Larmor frequency. We have also observed multi-photon Rabi oscillations corresponding to one- to four-photon resonances by applying single-frequency microwave pulses. The parametric control demonstrated in this work widens the frequency range of microwaves for controlling the qubit and offers a high quality testing ground for exploring nonlinear quantum phenomena.

cond-mat.mes-hall↗

arXiv2005

Uniaxial pressure dependencies of the phase boundary of TlCuCl_3

We present a thermal expansion and magnetostriction study of TlCuCl_3, which shows a magnetic-field induced transition from a spin gap phase to a Neel ordered phase. Using Ehrenfest relations we derive huge and strongly anisotropic uniaxial pressure dependencies of the respective phase boundary, e.g. the transition field changes by about $\pm 185$ GPa depending on the direction of uniaxial pressure.

cond-mat.str-el↗

arXiv2005

Optimality of Natural Time Representation of Complex Time Series

The concept of natural time turned out to be useful in revealing dynamical features behind complex time series including electrocardiograms, ionic current fluctuations of membrane channels, seismic electric signals, and seismic event correlation. However, the origin of this empirical usefulness is yet to be clarified. Here, it is shown that this time domain is in fact optimal for enhancing the signals in time-frequency space by employing the Wigner function and measuring its localization property.

cond-mat.other↗

arXiv2004

Magnetoelastic Coupling in the Spin-Dimer System TlCuCl$_3$

We present high-resolution measurements of the thermal expansion and the magnetostriction of TlCuCl$_{3}$ which shows field-induced antiferromagnetic order. We find pronounced anomalies in the field and temperature dependence of different directions of the lattice signaling a large magnetoelastic coupling. The phase boundary is extremely sensitive to pressure, e.g. the transition field would change by about +/- 185$%/GPa under uniaxial pressure applied along certain directions. This drastic effect can unambiguously be traced back to changes of the intradimer coupling under uniaxial pressure. The interdimer couplings remain essentially unchanged under pressure, but strongly change when Tl is replaced by K.

cond-mat.str-el↗

arXiv2004

A theoretical analysis of flux-qubit measurements with a dc-SQUID

The readout process of a superconducting flux-qubit is theoretically analyzed in terms of the quantum dynamics of a qubit-SQUID coupled system during measurement. The quantity directly observed by the measurement is the switching current (Isw) of the dc-SQUID placed around the qubit ring. In order to clarify the relation between the Isw and the qubit state, we calculated the time evolution of the density operator of the qubit-SQUID system while increasing the SQUID bias current until switching events occur and obtained the switching current distributions. This clarifies what information of the qubit is obtained by a dc-SQUID switching current measurement under specific conditions, for example, when the qubit eigenstate is a superposition of two different flux states.

cond-mat.supr-con↗