arXiv subjects

H. Y. Huang

Publications and source records attributed to H. Y. Huang.

26 records · Page 2Linked to original sources

arXiv2017

Coulomb correlations intertwined with spin and orbital excitations in LaCoO$_3$

We carried out temperature-dependent (20 - 550 K) measurements of resonant inelastic X-ray scattering on LaCoO$_3$ to investigate the evolution of its electronic structure across the spin-state crossover. In combination with charge-transfer multiplet calculations, we accurately quantized the renormalized crystal-field excitation energies and spin-state populations. We show that the screening of the on-site Coulomb interaction of 3d electrons is orbital selective and coupled to the spin-state crossover in LaCoO$_3$. The results establish that the gradual spin-state crossover is associated with a relative change of Coulomb energy versus bandwidth, leading to a Mott-type insulator-to-metal transition.

cond-mat.str-el↗

arXiv2016

Jahn-Teller distortion driven magnetic polarons in magnetite

The first known magnetic mineral, magnetite (Fe$_3$O$_4$), has unusual properties which have fascinated mankind for centuries; it undergoes the Verwey transition at $T_{\rm V}$ $\sim$120 K with an abrupt change in structure and electrical conductivity. The mechanism of the Verwey transition however remains contentious. Here we use resonant inelastic X-ray scattering (RIXS) over a wide temperature range across the Verwey transition to identify and separate out the magnetic excitations derived from nominal Fe$^{2+}$ and Fe$^{3+}$ states. Comparison of the RIXS results with crystal-field multiplet calculations shows that the spin-orbital $dd$ excitons of the Fe$^{2+}$ sites arise from a tetragonal Jahn-Teller active polaronic distortion of the Fe$^{2+}$O$_6$ octahedra. These low-energy excitations, which get weakened for temperatures above 350 K but persist at least up to 550 K, are distinct from optical excitations and best explained as magnetic polarons.

cond-mat.str-el↗

arXiv2015

Raman and fluorescence characteristics of resonant inelastic X-ray scattering from doped superconducting cuprates

Measurements of spin excitations are essential for an understanding of spin-mediated pairing for superconductivity; and resonant inelastic X-ray scattering (RIXS) provides a considerable opportunity to probe high-energy spin excitations. However, whether RIXS correctly measures the collective spin excitations of doped superconducting cuprates remains under debate. Here we demonstrate distinct Raman- and fluorescence-like RIXS excitations of Bi$_{1.5}$Pb$_{0.6}$Sr$_{1.54}$CaCu$_{2}$O$_{8+δ}$ in the mid-infrared energy region. Combining photon-energy and momentum dependent RIXS measurements with theoretical calculations using exact diagonalization provides conclusive evidence that the Raman-like RIXS excitations correspond to collective spin excitations, which are magnons in the undoped Mott insulators and evolve into paramagnons in doped superconducting compounds. In contrast, the fluorescence-like shifts are due primarily to the continuum of particle-hole excitations in the charge channel. Our results show that under the proper experimental conditions RIXS indeed can be used to probe paramagnons in doped high-$T_c$ cuprate superconductors.

cond-mat.supr-con↗

arXiv1997

New sum rule identities and duality relation for the Potts $n$-point correlation function

It is shown that certain sum rule identities exist which relate correlation functions for $n$ Potts spins on the boundary of a planar lattice for $n\geq 4$. Explicit expressions of the identities are obtained for $n=4,5$. It is also shown that the identities provide the missing link needed for a complete determination of the duality relation for the $n$-point correlation function. The $n=4$ duality relation is obtained explicitly. More generally we deduce the number of correlation identities for any $n$ as well as an inversion relation and a conjecture on the general form of the duality relation.

cond-mat.stat-mech↗

arXiv1997

Lattice Statistics in Three Dimensions: Exact Solution of Layered Dimer and Layered Domain Wall Models

Exact analyses are given for two three-dimensional lattice systems: A system of close-packed dimers placed in layers of honeycomb lattices and a layered triangular-lattice interacting domain wall model, both with nontrivial interlayer interactions. We show that both models are equivalent to a 5-vertex model on the square lattice with interlayer vertex-vertex interactions. Using the method of Bethe ansatz, a closed-form expression for the free energy is obtained and analyzed. We deduce the exact phase diagram and determine the nature of the phase transitions as a function of the strength of the interlayer interaction.

cond-mat.stat-mech↗

arXiv1996

Exact Solution of a Three-Dimensional Dimer System

We consider a three-dimensional lattice model consisting of layers of vertex models coupled with interlayer interactions. For a particular non-trivial interlayer interaction between charge-conserving vertex models and using a transfer matrix approach, we show that the eigenvalues and eigenvectors of the transfer matrix are related to those of the two-dimensional vertex model. The result is applied to analyze the phase transitions in a realistic three-dimensional dimer system.

cond-mat.stat-mech↗

arXiv1995

Interacting dimers on the honeycomb lattice: An exact solution of the five-vertex model

The problem of close-packed dimers on the honeycomb lattice was solved by Kasteleyn in 1963. Here we extend the solution to include interactions between neighboring dimers in two spatial lattice directions. The solution is obtained by using the method of Bethe ansatz and by converting the dimer problem into a five-vertex problem. The complete phase diagram is obtained and it is found that a new frozen phase, in which the attracting dimers prevail, arises when the interaction is attractive. For repulsive dimer interactions a new first-order line separating two frozen phases occurs. The transitions are continuous and the critical behavior in the disorder regime is found to be the same as in the case of noninteracting dimers characterized by a specific heat exponent $\a=1/2$.

cond-mat↗

arXiv1994

A Soluble Free-Fermion Model in d Dimensions

We consider a vertex model in d dimensions characterized by lines which run in a preferred direction. We show that this vertex model is soluble if the weights of vertices with intersecting lines are given by a free-fermion condition, and that a fugacity -1 is associated to each loop of lines. The solution is obtained by mapping the model into a dimer problem and by evaluating a Pfaffian. We also determine the critical point and the singular behavior of the free energy.

cond-mat↗