arXiv subjects

Ha-Leem Kim

Publications and source records attributed to Ha-Leem Kim.

7 recordsLinked to original sources

arXiv2026

Optical Voltage Profiling of 2D Semiconductors via Proximal Exciton Sensing

High contact resistances in atomically thin semiconductors often mask intrinsic electrical transport properties, particularly at low carrier densities where exotic correlated states emerge. We introduce optical voltage profiling, a noninvasive wide-field technique that replaces local voltage probes with a proximal monolayer MoSe$_2$ exciton sensor. Isolated by thin hexagonal boron nitride, this sensor converts the target's local electrostatic potential into spatially resolved modulations of exciton reflectance. Through pixel-wise in situ calibration, these signals yield quantitative two-dimensional voltage maps of an actively biased semiconductor device. Using this method, we demonstrate the carrier-density-driven metal-insulator transition in bilayer MoSe$_2$ and obtain channel resistances below 1 k$\Omega$ despite M$\Omega$-scale two-terminal resistances in the metallic region. The optically derived resistance exhibits a metal-insulator crossover near the resistance quantum $h/e^2$, and the voltage maps and reconstructed local conductivity reveal pronounced spatial heterogeneity in both insulating and metallic regimes. Beyond resolving channel resistance under high contact-resistance conditions, the technique provides spatially resolved access to microscopic transport heterogeneity in functional van der Waals devices.

cond-mat.mes-hall↗

arXiv2025

Contactless cavity sensing of superfluid stiffness in atomically thin 4Hb-TaS$_2$

The exceptional tunability of two-dimensional van der Waals materials offers unique opportunities for exploring novel superconducting phases. However, in such systems, the measurement of superfluid phase stiffness, a fundamental property of a superconductor, is challenging because of the mesoscopic sample size. Here, we introduce a contact-free technique for probing the electrodynamic response, and thereby the phase stiffness, of atomically thin superconductors using on-chip superconducting microwave resonators. We demonstrate this technique on 4Hb-TaS$_2$, a van der Waals superconductor whose gap structure under broken mirror symmetry is under debate. In our cleanest few-layer device, we observe a superconducting critical temperature comparable to that of the bulk. The temperature evolution of the phase stiffness features nodeless behavior in the presence of broken mirror symmetry, inconsistent with the scenario of nodal surface superconductivity. With minimal fabrication requirements, our technique enables microwave measurements across wide ranges of two-dimensional superconductors.

cond-mat.supr-con↗

arXiv2025

Visualizing the Impact of Quenched Disorder on 2D Electron Wigner Solids

Electron Wigner solids (WSs)1-12 provide an ideal system for understanding the competing effects of electron-electron and electron-disorder interactions, a central unsolved problem in condensed matter physics. Progress in this topic has been limited by a lack of single-defect-resolved experimental measurements as well as accurate theoretical tools to enable realistic experiment/theory comparison. Here we overcome these limitations by combining atomically-resolved scanning tunneling microscopy (STM) with neural-quantum-state quantum Monte Carlo (NQS-QMC) simulation of disordered 2D electron WSs to discover new disorder-induced physical regimes of correlated electron behavior. STM was used to image the electron density ($n_e$) dependent evolution of electron WSs in gate-tunable bilayer MoSe2 devices with varying long-range ($n_\mathrm{LR}$) and short-range ($n_\mathrm{SR}$) disorder densities. These images were compared to NQS-QMC simulations using realistic disorder maps extracted from experiment, thus allowing the roles of different disorder types to be disentangled. We identify two distinct physical regimes for disordered electron WSs that depend on $n_\mathrm{SR}$. For $n_\mathrm{SR} \lesssim n_e$ the WS behavior is dominated by long-range disorder and features extensive mixed solid-liquid phases, a new type of local re-entrant melting/crystallization, and prominent Friedel oscillations. In contrast, when $n_\mathrm{SR} \gg n_e$ these features are suppressed and a more robust amorphous WS phase emerges that persists to higher ne, highlighting the importance of short-range disorder in this regime. Our work establishes a powerful framework for studying disordered quantum solids via a combined experimental-theoretical approach.

cond-mat.str-el↗

arXiv2025

Terahertz electrodynamics in a zero-field Wigner crystal

In clean two-dimensional (2D) systems, electrons are expected to self-organize into a regular lattice, a Wigner crystal, when their mutual Coulomb repulsion overwhelms kinetic energy. Understanding the Wigner crystal at zero magnetic field is a long-sought goal in physics, thanks to its fundamental simplicity and possible connection to the density-driven metal-insulator transition. To date, evidence for such a crystal has been reported across various platforms. However, the AC conductivity of a zero-field Wigner crystal, a key observable characterizing its electrodynamics, has never been measured. Here, we develop an ultrasensitive on-chip terahertz (THz) spectroscopy technique to probe the AC conductivity in electrostatically gated monolayer MoSe2 encapsulated in hexagonal boron nitride. We observe a sub-THz resonance corresponding to the pinning mode of a zero-field Wigner crystal, whose frequency is orders of magnitude higher than those under high magnetic fields. Using the pinning mode as an indicator, we reveal that moderate disorder notably stabilizes the Wigner crystal. With increasing density towards melting, we find that the pinning mode of the Wigner crystal coexists with a growing Drude component characteristic of an electron liquid, and the competition between these two components in the conductivity spectra leads to the insulator-metal transition of the 2D electron system. Our findings not only elucidate the low-energy electrodynamics of a zero-field Wigner crystal, but also establish on-chip THz spectroscopy as a powerful probe for correlated quantum phases in two-dimensional materials.

cond-mat.mes-hall↗

arXiv2023

Thermal Hall effects due to topological spin fluctuations in YMnO$_3$

The thermal Hall effect in magnetic insulators has been considered a powerful method for examining the topological nature of charge-neutral quasiparticles such as magnons. Yet, unlike the kagome system, the triangular lattice has received less attention for studying the thermal Hall effect because the scalar spin chirality cancels out between adjacent triangles. However, such cancellation cannot be perfect if the triangular lattice is distorted, which could open the possibility of a non-zero thermal Hall effect. Here, we report that the trimerized triangular lattice of multiferroic hexagonal manganite YMnO$_3$ produces a highly unusual thermal Hall effect due to topological spin fluctuations with the additional intricacy of a Dzyaloshinskii-Moriya interaction under an applied magnetic field. We conclude the thermal Hall conductivity arises from the system's topological nature of spin fluctuations. Our theoretical calculations demonstrate that the thermal Hall conductivity is also related in this material to the splitting of the otherwise degenerate two chiralities, left and right, of its 120$^{\circ}$ magnetic structure. Our result is one of the most unusual cases of topological physics due to this broken $Z_2$ symmetry of the chirality in the supposedly paramagnetic state of YMnO$_3$, with strong topological spin fluctuations. These new mechanisms in this important class of materials are crucial in exploring new thermal Hall physics and exotic excitations.

cond-mat.str-el↗

arXiv2020

Sizeable suppression of thermal Hall effect upon isotopic substitution in strontium titanate

We report measurements of the thermal Hall effect in single crystals of both pristine and isotopically substituted strontium titanate. We discovered a two orders of magnitude difference in the thermal Hall conductivity between $SrTi^{16}O_3$ and $^{18}O$-enriched $SrTi^{18}O_3$ samples. In most temperature ranges, the magnitude of thermal Hall conductivity ($κ_{xy}$) in $SrTi^{18}O_3$ is proportional to the magnitude of the longitudinal thermal conductivity ($κ_{xx}$), which suggests a phonon-mediated thermal Hall effect. However, they deviate in the temperature of their maxima, and the thermal Hall angle ratio ($|κ_{xy}/κ_{xx}|$) shows anomalously decreasing behavior below the ferroelectric Curie temperature $T_c$ ~$25 K$. This observation suggests a new underlying mechanism, as the conventional scenario cannot explain such differences within the slight change in phonon spectrum. Notably, the difference in magnitude of thermal Hall conductivity and rapidly decreasing thermal Hall angle ratio in $SrTi^{18}O_3$ is correlated with the strength of quantum critical fluctuations in this displacive ferroelectric. This relation points to a link between the quantum critical physics of strontium titanate and its thermal Hall effect, a possible clue to explain this example of an exotic phenomenon in non-magnetic insulating systems.

cond-mat.str-el↗

arXiv2018

Magnetic Excitations in Non-Collinear Antiferromagnetic Weyl Semimetal $\mathsf{Mn_{3}Sn}$

$\mathsf{Mn_{3}Sn}$ has recently attracted considerable attention as a magnetic Weyl semimetal exhibiting concomitant transport anomalies at room temperature. The topology of the electronic bands, their relation to the magnetic ground state and their nonzero Berry curvature lie at the heart of the problem. The examination of the full magnetic Hamiltonian reveals otherwise hidden aspects of these unusual physical properties. Here, we report the full spin wave spectra of $\mathsf{Mn_{3}Sn}$ measured over a wide momentum - energy range by the inelastic neutron scattering technique. Using a linear spin wave theory, we determine a suitable magnetic Hamiltonian which not only explains the experimental results but also stabilizes the low-temperature helical phase, consistent with our DFT calculations. The effect of this helical ordering on topological band structures is further examined using a tight-binding method, which confirms the elimination of Weyl points in the helical phase. Our work provides a rare example of the intimate coupling between the electronic and spin degrees of freedom for a magnetic Weyl semimetal system.

cond-mat.str-el↗