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Hadrien Vignaud

Publications and source records attributed to Hadrien Vignaud.

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Deep-UV bleaching of charge disorder in encapsulated graphene

Disorder masks much of the rich physics in two-dimensional electronic systems, with charged impurities often the limiting factor. In graphene, progress in reducing disorder has largely stagnated since boron nitride encapsulation was introduced a decade ago. Here we show that a brief deep-UV exposure enhances the electronic quality of encapsulated graphene - typically by two orders of magnitude - by neutralizing charged impurities within boron nitride. Following illumination, standard graphene devices exhibit numerous evendenominator fractional quantum Hall states, including non-Abelian candidates, and frequently reveal hidden superlattice minibands. Even macroscopically inhomogeneous devices, seemingly unusable for transport studies, recover after deep-UV illumination and display Landau quantization in millitesla fields. This finding provides a straightforward route to exceptional-quality graphene, enabling further exploration of interaction-driven, topological and other quantum phenomena.

cond-mat.mes-hall

Chiral-helical junctions in screened graphene

Reproducibility and quantization in quantum spin Hall platforms is a persisting challenge, limiting their use in hybrid realizations of topological superconductivity. We report robust and reproducible quantized transport in a graphene quantum Hall topological insulator, stabilized at low magnetic fields by screening long-range Coulomb interactions with a metallic Bi$_2$Se$_3$ back gate. Beyond quantized resistance plateaus, we demonstrate mode-resolved control via gate-defined chiral-helical junctions that selectively transmit or backscatter a single helical channel, a capability inaccessible in time-reversal symmetric quantum spin Hall systems. Targeted experiments and simulations identify contact-induced doping, effectively creating unintended chiral-helical interfaces, as a generic mechanism for quantization breakdown, which is mitigated by large area contacts that enhance edge-channel equilibration. Our findings establish metal screened graphene as a gate-tunable, interaction-driven helical system with quantized transport, spatially separable helical channels, and compatibility with superconducting proximity for topological devices.

cond-mat.mes-hall

Evidence for chiral supercurrent in quantum Hall Josephson junctions

Hybridizing superconductivity with the quantum Hall (QH) effects has major potential for designing novel circuits capable of inducing and manipulating non-Abelian states for topological quantum computation. However, despite recent experimental progress towards this hybridization, concrete evidence for a chiral QH Josephson junction -- the elemental building block for coherent superconducting-QH circuits -- is still lacking. Its expected signature is an unusual chiral supercurrent flowing in QH edge channels, which oscillates with a specific $2\phi_0$ magnetic flux periodicity ($\phi_0=h/2e$ is the superconducting flux quantum, $h$ the Planck constant and $e$ the electron charge). Here, we show that ultra-narrow Josephson junctions defined in encapsulated graphene nanoribbons exhibit such a chiral supercurrent, visible up to 8 teslas, and carried by the spin-degenerate edge channel of the QH plateau of resistance $h/2e^2\simeq 12.9$ k$\Omega$. We observe reproducible $2\phi_0$-periodic oscillation of the supercurrent, which emerges at constant filling factor when the area of the loop formed by the QH edge channel is constant, within a magnetic-length correction that we resolve in the data. Furthermore, by varying the junction geometry, we show that reducing the superconductor/normal interface length is pivotal to obtain a measurable supercurrent on QH plateaus, in agreement with theories predicting dephasing along the superconducting interface. Our findings mark a critical milestone along the path to explore correlated and fractional QH-based superconducting devices that should host non-Abelian Majorana and parafermion zero modes.

cond-mat.mes-hall

Imaging tunable quantum Hall broken-symmetry orders in graphene

When electrons populate a flat band their kinetic energy becomes negligible, forcing them to organize in exotic many-body states to minimize their Coulomb energy. The zeroth Landau level of graphene under magnetic field is a particularly interesting strongly interacting flat band because inter-electron interactions are predicted to induce a rich variety of broken-symmetry states with distinct topological and lattice-scale orders. Evidence for these stems mostly from indirect transport experiments that suggest that broken-symmetry states are tunable by boosting the Zeeman energy or by dielectric screening of the Coulomb interaction. However, confirming the existence of these ground states requires a direct visualization of their lattice-scale orders. Here, we image three distinct broken-symmetry phases in graphene using scanning tunneling spectroscopy. We explore the phase diagram by tuning the screening of the Coulomb interaction by a low or high dielectric constant environment, and with a magnetic field. In the unscreened case, we unveil a Kekul\'e bond order, consistent with observations of an insulating state undergoing a magnetic-field driven Kosterlitz-Thouless transition. Under dielectric screening, a sublattice-unpolarized ground state emerges at low magnetic fields, and transits to a charge-density-wave order with partial sublattice polarization at higher magnetic fields. The Kekul\'e and charge-density-wave orders furthermore coexist with additional, secondary lattice-scale orders that enrich the phase diagram beyond current theory predictions. This screening-induced tunability of broken-symmetry orders may prove valuable to uncover correlated phases of matter in other quantum materials.

cond-mat.mes-hall

A tunable Fabry-P\'erot quantum Hall interferometer in graphene

Electron interferometry with quantum Hall edge channels holds promise for probing and harnessing exotic exchange statistics of non-Abelian anyons. In semiconductor heterostructures, however, quantum Hall interferometry has proven challenging and often obscured by charging effects. Here we show that high-mobility monolayer graphene equipped with a series of gate-tunable quantum point contacts that act as electron beam-splitters provides a model system to perform Fabry-P\'{e}rot quantum Hall interferometry. We observe high-visibility Aharonov-Bohm interference free of charging effects and widely tunable through electrostatic gating or magnetic field, in remarkable agreement with theory. A coherence length of $\mathbf{10 \,\mu m}$ at a temperature of $0.02$ K allows us to further achieve coherently-coupled double Fabry-P\'{e}rot interferometry. Our results open a new avenue for quantum Hall interferometry and the exploitation of topological excitations for quantum computation.

cond-mat.mes-hall