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Hai-Hu Wen

Publications and source records attributed to Hai-Hu Wen.

At least 181 records · Page 10Linked to original sources

Anomalous Properties in the Normal and Superconducting States of LaRu$_3$Si$_2$

Superconductivity in LaRu$_3$Si$_2$ with the honeycomb structure of Ru atoms has been investigated. It is found that the normal state specific heat C/T exhibits a deviation from the Debye model down to the lowest temperature. A relation $C/T = γ_n+βT^2-ATlnT$ which concerns the electron correlations can fit the data very well. The suppression to the superconductivity by the magnetic field is not the mean-field like, which is associated well with the observation of strong superconducting fluctuations. The field dependence of the induced quasiparticle density of states measured by the low temperature specific heat shows a non-linear feature, indicating the significant contributions given by the delocalized quasiparticles.

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Anisotropic resistivity in underdoped single crystals (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$, $0 \leq x<0.35$

Temperature-dependent in-plane, $ρ_a(T)$, and inter-plane, $ρ_c(T)$, resistivities were measured for the iron-arsenide superconductor (Ba$_{1-x}$K$_x$)Fe $_2$As$_2$ over a broad doping range from parent compound to optimal doping $T_c\approx 38 K$, $0\leq x \leq 0.35$. The coupled magnetic/structural transition at $T_{SM}$ is clearly observed for samples with $T_c <$26 K ($x <0.25$), however its effect on resistivity is much weaker than in the electron-doped Ba(Fe$_{1-x}$Co$_x$)Fe $_2$As$_2$, and the transition leads only to a decrease of resistivity. In addition to the feature at $T_{SM}$, the inter-plane resistivity shows a maximum at $T^*\sim$200 K, which moves slightly to higher temperature with doping, revealing a trend opposite to the electron-doped materials. A smeared feature at about the same temperature is seen in $ρ_a(T)$. For $T<T^*$, the temperature dependence of resistivity shows systematic evolution and is close to linear at optimal doping. This feature, being most pronounced for $ρ_c(T)$, suggests the existence of a quantum critical point close to optimal doping.

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Transport properties and anisotropy of Rb0.8Fe2Se2 single crystals

Single crystals of Rb{0.8}Fe2Se2 are successfully synthesized with the superconducting transition temperatures T_c{onset}= 31 K and T_c{zero}= 28 K. A clear anomaly of resistivity was observed in the normal state at about 150 K, as found in a similar system KxFe2Se2. The upper critical field has been determined with the magnetic field along ab-plane and c-axis, yielding an anisotropy of about 3.5. The angle dependent resistivity measured below T_c allow a perfect scaling feature based on the anisotropic Ginzburg-Landau theory, leading to a consistent value of the anisotropy which decreases from about 3.6 at around T_c to 2.9 at 27 K. Comparing to the anisotropy determined for Ba0.6K0.4Fe2As2 and Ba(Fe0.92Co0.08)2As2 using the same method, we find that the present sample is more anisotropic and the Fermi surfaces with stronger two dimensional characters are expected.

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Highly anisotropic superconducting gap in underdoped Ba$_{1-x}$K$_x$Fe$_2$As$_2$

The in-plane London penetration depth, $Δλ(T)$, was measured using a tunnel diode resonator in single crystals of Ba$_{1-x}$K$_x$Fe$_2$As$_2$ for five doping levels $x$ ranging from underdoped, $T_c$=11 K ($x$=0.17), to optimally doped, $T_c=$38 K ($x_\textmd{\scriptsize opt}$= 0.35). In the optimally doped samples, $Δλ(T)$ shows exponential saturation in $T \to 0$ limit suggesting a fully gapped superconductivity. The lowest-$T_c$ samples show much stronger non-exponential variation of $Δλ(T)$. Fitting the data to a power-law, $Δλ(T)= AT^n$, reveals a monotonic decrease of the exponent $n$ with $x$ towards the underdoped edge of the superconducting dome. Comparison with $n \approx 1.2$ reported in KFe$_2$As$_2$ ($T_c$=3.5 K, $x=$ 1), suggests a dome-like variation of $n$ with $x$, implying an evolution of the topology of the superconducting gap from full and isotropic in the center of the dome towards strongly anisotropic and, eventually, nodal at the dome edges.

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Reversibly tuning the insulating and superconducting state in KxFe2-ySe2 crystals by post-annealing

Since the discovery of superconductivity at 26 K in oxy-pnictide LaFeAsO1-xFx, enormous interests have been stimulated in the field of condensed matter physics and material sciences. Among the many kind of structures in the iron pnictide superconductors, FeSe with the PbO structure has received special attention since there is not poisonous pnictogen element in chemical composition and its structure is the simplest one. However, the superconducting transition temperature (Tc) in iron chalcogenide compounds is not enhanced as high as other iron pnictide superconductors under ambient pressure until the superconductivity at above 30 K in potassium intercalated iron selenide KxFe2-ySe2 was discovered. The insulating and the superconducting state are both observed in KxFe2-ySe2 with different stoichiometries and some groups have tuned the system from insulating to superconducting state by varying the ratio of starting materials[10, 11]. The recent data from neutron scattering suggest that the superconductivity may be built upon an ordered state of Fe vacancies as well as the antiferromagnetic state with a very strong ordered magnetic moment 3.4 B. Here we show that the superconductivity can actually be tuned on a single sample directly from an insulating state by post-annealing and fast quenching. Upon waiting for some days at room temperatures, the superconductivity will disappear and the resistivity exhibits an insulating behavior again. The spatial distribution of the compositions of the as-grown sample and the post-annealed-quenched one was analyzed by the Energy Dispersive X-ray Spectrum (EDXS) and found to be very close to each other. Therefore it is tempting to conclude that the superconductivity is achieved when the Fe-vacancies are in a random (disordered) state. Once they arrange in an ordered state by relaxation or slow cooling, the system turns out to be an insulator.

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Determination of the superconducting gap in near optimally doped Bi_2Sr_{2-x}La_xCuO_{6+δ} (x ~ 0.4) from low-temperature specific heat

Low-temperature specific heat of the monolayer high-Tc superconductor Bi_2Sr_{2-x}La_xCuO_{6+δ} has been measured close to the optimal doping point (x ~ 0.4) in different magnetic fields. The identification of both a T^2 term in zero field and a \sqrt{H} dependence of the specific heat in fields is shown to follow the theoretical prediction for d-wave pairing, which enables us to extract the slope of the superconducting gap in the vicinity of the nodes (v_Δ, which is proportional to the superconducting gap Δ_0 at the antinodes according to the standard d_{x^2-y^2} gap function). The v_Δ or Δ_0 (~ 12 meV) determined from this bulk measurement shows close agreement with that obtained from spectroscopy or tunneling measurements, which confirms the simple d-wave form of the superconducting gap.

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Nodeless superconductivity in K$_x$Fe$_{2-y}$Se$_2$ single crystals revealed by low temperature specific heat

Low temperature specific heat (SH) has been measured in K$_x$Fe$_{2-y}$Se$_2$ single crystals with T$_c$ = 32 K. The SH anomaly associated with the superconducting transition is moderate and sharp yielding a value of $ΔC/T \mid_{T_c}$ = 11.6 $\pm$ 1.0 $mJ/mol K^2$. The residual SH coefficient $γ(0)$ in the superconducting state at T$\rightarrow$ 0 is very small with a value of about 0.39 $mJ/mol K^2$. The magnetic field induced enhancement of the low-T SH exhibits a rough linear feature indicating a nodeless gap. This is further supported by the scaling based on the s-wave approach of the low-T data at different magnetic fields. A rough estimate tells that the normal state SH coefficient $γ_n$ is about 6 $\pm$ 0.5 $mJ/mol K^2$ leading to $ΔC/γ_nT\mid_{T_c}$ = 1.93 and placing this new superconductor in the strong coupling region.

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Static magnetic order of Sr$_{4}$A$_{2}$O$_{6}$Fe$_{2}$As$_{2}$ (A = Sc and V) revealed by local probes

Static magnetic order of quasi two-dimensional FeAs compounds Sr4A2O6-xFe2As2, with A = Sc and V, has been detected by 57Fe Moessbauer and muon spin relaxation (μSR) spectroscopies. The non-superconducting stoichiometric (x = 0) A = Sc system exhibits a static internal/hyperfine magnetic field both at the 57Fe and μ+ sites, indicating antiferromagnetic order of Fe moments below TN = 35 K with ~ 0.1 Bohr magneton per Fe at T = 2 K. The superconducting and oxygen deficient (x = 0.4) A = V system exhibits a static internal field only at the μ+ site below TN ~ 40 K, indicating static magnetic order of V moments co-existing with superconductivity without freezing of Fe moments. These results suggest that the 42622 FeAs systems belong to the same paradigm with the 1111 and 122 FeAs systems with respect to magnetic behavior of Fe moments.

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Anomalous Meissner effect in pnictide superconductors

The Meissner effect has been studied in Ba(Fe0.926Co0.074)2As2 and Ba0.6K0.4Fe2As2 single crystals and compared to well known, type-II superconductors LuNi2B2C and V3Si. Whereas flux penetration is mostly determined by the bulk pinning (and, perhaps, surface barrier) resulting in a large negative magnetization, the flux expulsion upon cooling in a magnetic field is very small, which could also be due to pinning and/or surface barrier effects. However, in stark contrast with the expected behavior, the amount of the expelled flux increases almost linearly with the applied magnetic field, at least up to our maximum field of 5.5 T, which far exceeds the upper limit for the surface barrier. One interpretation of the observed behavior is that there is a field-driven suppression of magnetic pair-breaking.

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Precision Microwave Electrodynamic Measurements of K- and Co-doped BaFe$_2$As$_2$

We have studied the microwave electrodynamics of single crystal iron-based superconductors Ba$_{0.72}$K$_{0.28}$Fe$_2$As$_2$ (hole-doped, $T_\mathrm{c}$ $\approx $30 K) and Ba(Fe$_{0.95}$Co$_{0.05}$)$_2$As$_2$ (electron-doped, $T_\mathrm{c}$ $\approx$20 K), by cavity perturbation and broadband spectroscopy. SQUID magnetometry was used to confirm the quality and homogeneity of the samples under study. Through cavity perturbation techniques, the temperature dependence of the in-plane London penetration depth $Δλ(T)$, and therefore the superfluid phase stiffness $λ^2(0)/λ^2(T)$ was measured. Down to 0.4 K, the data do not show the exponential saturation at low temperatures expected from a singly-, fully-gapped superconductor. Rather, both the electron- and the hole-doped systems seem to be best described by a power law behavior, with $λ^2(0)/λ^2(T)$ $\sim$ $T^n$ and \emph{n} $\approx$ 2.5. In the three samples we studied, a weak feature near the sensitivity limit of our measurements appears near $T/T_\mathrm{c}$ =~0.04, hinting at a corresponding low energy feature in the superconducting density of states. The data can also be relatively well-described by a simple two-gap s-wave model of the order parameter, but this yields parameters which seem unrealistic and dependent on the fit range. Broadband surface resistance measurements reveal a sample dependent residual loss whose origin is unclear. The data from the \FeAs samples can be made to scale as $ω^2$ if the extrinsic loss is treated as an additive component, indicating large scattering rates. Finally, the temperature dependence of the surface resistance at 13 GHz obeys a power law very similar to those observed for $Δλ(T)$.

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Flux-dynamics associated with the Second Magnetisation Peak in iron-pnictide Ba_{1-x}K_xFe_2As_2

We report on isofield magnetic relaxation data on a single crystal of $Ba_{1-x}K_xFe_2As_2$ with superconducting transition temperature $T_c$= 32.7 K which exhibit the so called fish-tail effect. A surface map of the superconducting transition temperature shows that the superconducting properties are close to homogeneous across the sample. Magnetic relaxation data, M(t), was used to obtain the activation energy U(M) in order to study different vortex dynamics regimes. Results of this analysis along with time dependent measurements as a function of field and temperature extended to the reversible region of some M(H) curves demonstrate that the irreversibility as well the second magnetization peak position, $H_p(T)$, are time dependent and controlled by plastic motion of the vortex state. In the region delimited by a characteristic field Hon (well below $H_p$), and $H_p$, the vortex dynamics is controlled by collective pinning. For fields below Hon the activation energy, $U_0$, increases with field as expected for collective pinning, but the pinning mechanism is likely to be in the single vortex limit.

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Low Temperature Specific Heat of Optimally Doped BaFe$_{2-x}$$TM_x$As$_{2}$ ($TM$ = Co and Ni) Single Crystals: Constraint on the Pairing Gap

Low temperature specific heat has been measured in optimally doped and highly overdoped non-superconducting BaFe$_{2-x}$TM$_x$As$_{2}$ ($TM$ = Co and Ni) single crystals. By using the data of the overdoped samples, we successfully removed the phonon contribution of the optimally doped ones, and derived the electronic specific heat coefficient $γ_e$. Remarkably, we found a continuing temperature dependent $γ_e(T)$ which follows the quadratic relation $γ_e=γ_0+αT^2$ in the low temperature limit. Together with the very small residual term $γ_0$, linear magnetic field dependence of $γ_e$, it is concluded that there are either small segments of nodal lines, or point-like nodes in these samples.

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Multi-band effect in the noncentrosymmetric superconductors Mg_{12-δ}Ir_{19}B_{16} revealed by Hall effect and magnetoresistance measurements

We report the longitudinal resistivity and Hall effect measurements on the noncentrosymmetric superconducting Mg$_{12-δ}$Ir$_{19}$B$_{16}$ samples with different critical transition temperatures. A strong temperature dependence of the Hall coefficient $R_H$ and nonlinear magnetic field dependence of the Hall resistivity $ρ_{xy}$ in wide temperature region are observed, suggesting a strong multi-band effect in this system. Moreover, a large magnetoresistance up to 20% is found at the field of 9 T. We also observe the violation of the Kohler's rule from our magnetoresistance data, further confirming the presence of multi-band effect in our samples. A detailed analysis shows that the data can't be simply described within the two-band scenario at low temperatures, so we argue that there may be more than two bands contributing to the conduction of the samples.

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Observation of Lattice and Andreev Bound States of Vortices in Ba0.6K0.4Fe2As2 Single Crystals with Scanning Tunneling Microscopy/Spectroscopy

For a type-II superconductor, when the applied magnetic field is higher than the lower critical value Hc1, the magnetic flux will penetrate into the superconductor and form quantized vortices, which usually are arranged in an Abrikosov lattice. For the newly discovered iron pnictide superconductors, previous measurements have shown that, in electron-doped BaFe2As2, the vortices form a highly disordered structure. In addition, the density of states (DOS) within the vortex cores1 do not exhibit the Andreev bound states in conventional superconductors. In this Letter, we report the observation of a triangular vortex lattice and the Andreev bound states in hole-doped BaFe2As2 by using a low temperature scanning tunneling microscope (STM). Detailed study of the vortex cores reveals that the spectrum of the Andreev bound states inside the vortex core exhibits a distinct spatial evolution: at the center of the vortex core, it appears as a single peak at 0.5 mV below the Fermi-energy; away from the core center, it gradually evolves into two sub-peaks and they eventually fade out. The drastic differences between the vortex cores of the electron-doped and hole-doped counterparts are illusive to the pairing mechanism of the iron pnictide superconductors.

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Contrasting Pair-Breaking Effects by Doping Mn and Zn in Ba0.5K0.5Fe2As2

Resistivity, Hall effect, magnetoresistance and DC magnetization were measured in Mn and Zn doped Ba$_{0.5}$K$_{0.5}$Fe$_{2}$As$_{2}$ samples. It is found that the Mn-doping can depress the superconducting transition temperature drastically with a rate of $ΔT_c$/Mn-1% = -4.2 K, while that by Zn-doping is negligible. Detailed analysis reveals that the Mn-doping enhances the residual resistivity ($ρ_0$) significantly, and induces strong local magnetic moments ($\sim$ 2.58 $μ_B$) which play as pair breakers. While the impurity scattering measured by $ρ_0$ in the Zn-doped samples is much weaker, accompanied by a negligible pair breaking effect. A possible explanation is that the impurity scattering by the Zn impurities are mainly small angle scattering (or small momentum transfer), therefore it cannot break the pairing induced by the interpocket scattering and thus affect the superconducting transition temperature weakly.

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Superconductivity induced by doping Platinum in BaFe2As2

By substituting Fe with the 5d-transition metal Pt in BaFe2As2, we have successfully synthesized the superconductors BaFe2-xPtxAs2. The systematic evolution of the lattice constants indicates that the Fe ions were successfully replaced by Pt ions. By increasing the doping content of Pt, the antiferromagnetic order and structural transition of the parent phase is suppressed and superconductivity emerges at a doping level of about x = 0.02. At a doping level of x = 0.1, we get a maximum transition temperature Tc of about 25 K. The synchrotron powder x-ray diffraction shows that the resistivity anomaly is in good agreement with the structural transition. The superconducting transitions at different magnetic fields were also measured at the doping level of about x = 0.1, yielding a slope of -dHc2/dT = 5.4 T/K near Tc. A phase diagram was established for the Pt doped 122 system. Our results suggest that superconductivity can also be easily induced in the FeAs family by substituting the Fe with Pt, with almost the similar maximum transition temperatures as doping Ni, Co, Rh and Ir.

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Low temperature specific heat in BaFe1.9Ni0.1As2 single crystals

Low-temperature specific heat was measured on the BaFe1.9Ni0.1As2 single crystals with critical transi-tion temperature Tc = 20.1 K. A clear specific heat jump with the value \DeltaC/T|Tc \approx 23 mJ/mol K^2 has been observed. In addition, a roughly linear magnetic field dependence of the electronic specific heat coefficient Δγ(H) is found in the zero-temperature limit, suggesting that at least one Fermi pocket, probably the hole derivative one, is fully gapped with a small anisotropy in the present sample. A slight curvature of the curve Δγ(H) may suggest a complex gap structure (anisotropic gap or nodes) at other Fermi surfaces.

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Suppression of the critical temperature of superconducting NdFeAs(OF) single crystals by Kondo-like defect sites induced by alpha-particle irradiation

We report a comprehensive investigation of the suppression of the critical temperature Tc of NdFeAs(OF) single crystal by alpha-particle irradiation. Our data indicate that irradiation defects produce both nonmagnetic and magnetic scattering, resulting in the Kondo-like excess resistance $Δρ(T)\propto ln T$ over 2 decades in temperatures above $T_c$. Despite high densities of irradiation defects, the dose at which $T_c$ is suppressed to zero is comparable to that for MgB2 but is well above the corresponding values for cuprates.

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