arXiv subjects

Hai-Hu Wen

Publications and source records attributed to Hai-Hu Wen.

At least 145 records · Page 8Linked to original sources

arXiv2015

Anisotropic Electronic Mobilities in the Nematic State of the Parent Phase NaFeAs

Hall effect and magnetoresistance have been measured on single crystals of the parent phase NaFeAs under a uniaxial pressure. Although significant difference of the in-plane resistivity $ρ_{xx}(I\parallel a)$ and $ρ_{xx}(I\parallel b)$ with the uniaxial pressure along $b$-axis was observed, the transverse resistivity $ρ_{xy}$ shows a surprisingly isotropic behavior. Detailed analysis reveals that the Hall coefficient $R_\mathrm{H}$ measured in the two orthogonal configurations ($I\parallel a$-axis and $I\parallel b$-axis) coincide very well and exhibit a deviation from the high temperature background at around the structural transition temperature $T_{\mathrm{s}}$. Furthermore, the magnitude of $R_\mathrm{H}$ increases remarkably below the structural transition temperature. This enhanced Hall coefficient is accompanied by the non-linear transverse resistivity versus magnetic field and enhanced magnetoresistance, which can be explained very well by the two band model with anisotropic mobilities of each band. Our results together with the two band model analysis clearly show that the anisotropic in-plane resistivity in the nematic state is closely related to the distinct quasiparticle mobilities when they are moving parallel or perpendicular to the direction of the uniaxial pressure.

cond-mat.supr-con↗

arXiv2015

Raman scattering in superconducting NdO1-xFxBiS2 crystals

The recently discovered layered BiS2-based superconductors have attracted a great deal of interest due to their structural similarity to cuprate and iron-pnictide superconductors. We have performed Raman scattering measurements on two superconducting crystals NdO0.5F0.5BiS2 (Tc = 4.5 K) and NdO0.7F0.3BiS2 (Tc = 4.8 K). The observed Raman phonon modes are assigned with the aid of first-principles calculations. The asymmetrical phonon mode around 118 cm-1 reveals a small electron-phonon (e-ph) coupling constant 0.16, which is insufficient to generate superconductivity at ~ 4.5 K. In the Raman spectra there exists a clear temperature-dependent hump around 100 cm-1, which can be well understood in term of inter-band vertical transitions around Fermi surface. The transitions get boosted when the particular rectangular-like Fermi surface meets band splitting caused by spin-orbit coupling. It enables a unique and quantitative insight into the band splitting.

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arXiv2014

Anisotropic Superconducting Gap and Elongated Vortices with Caroli-De-Gennes-Matricon States in the New Superconductor Ta4Pd3Te16

The superconducting state is formed by the condensation of a large number of Cooper pairs. The normal state electronic properties can give significant influence on the superconducting state. For usual type-II superconductors, the vortices are cylinder like with a round cross-section. For many two dimensional superconductors, such as Cuprates, 2H-NbSe$_2$ etc., albeit the in-plane anisotropy, the vortices generally have a round shape. In this paper we report results based on the scanning tunneling microscopy/spectroscopy measurements on a newly discovered superconductor Ta$_4$Pd$_3$Te$_{16}$. The chain like conducting channels of PdTe$_2$ in Ta$_4$Pd$_3$Te$_{16}$ make a significant anisotropy of the in-plane Fermi velocity. We suggest at least one anisotropic superconducting gap with gap minima or possible node exists in this multiband system. In addition, elongated vortices are observed with an anisotropy of $ξ_{\parallel b}/ξ_{\perp b}\approx 2.5$. Clear Caroli-de-Gennes-Matricon states are also observed within the vortex cores. Our results will initiate the study on the elongated vortices and superconducting mechanism in the new superconductor Ta$_4$Pd$_3$Te$_{16}$.

cond-mat.supr-con↗

arXiv2014

Simultaneous Vanishing of the Nematic Electronic State and the Structural Orthorhombicity in NaFe$_{1-x}$Co$_x$As Single Crystals

We have carried out in-plane resistivity measurements under a uniaxial pressure in NaFe$_{1-x}$Co$_x$As single crystals. A clear distinction of the in-plane resistivity $ρ_a$ and $ρ_b$ with the uniaxial pressure along $b$-axis was discovered in the parent and underdoped regime with the doping level up to about x=0.025$\pm$0.002. From the deviating point of $ρ_a$ and $ρ_b$, and the unique kinky structure of resistivity together with the published data we determined the temperatures for the nematic, structural and antiferromagnetic transitions. It is clearly shown that the nematic electronic state vanishes simultaneously with the structural transition. The antiferromagnetic state disappears however at a lower doping level. Our results, in combination with the data in BaFe$_{2-x}$Co$_x$As$_2$, indicate a close relationship between nematicity and superconductivity.

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arXiv2014

Critical current oscillations in the intrinsic hybrid vortex state of SmFeAs(O,F)

In layered superconductors the order parameter may be modulated within the unit cell, leading to non-trivial modifications of the vortex core if the interlayer coherence length $ξ_c(T)$ is comparable to the interlayer distance. In the iron-pnictide SmFeAs(O,F) ($T_c \approx 50$K) this occurs below a cross-over temperature $T^\star \approx 41$K, which separates two regimes of vortices: anisotropic Abrikosov-like at high and Josephson-like at low temperatures. Yet in the transition region around $T^\star$, hybrid vortices between these two characteristics appear. Only in this region around $T^\star$ and for magnetic fields well aligned with the FeAs layers, we observe oscillations of the c-axis critical current $j_c(H)$ periodic in $\frac{1}{\sqrt{H}}$ due to a delicate balance of intervortex forces and interaction with the layered potential. $j_c(H)$ shows pronounced maxima when a hexagonal vortex lattice is commensurate with the crystal structure. The narrow temperature window in which oscillations are observed suggests a significant suppression of the order parameter between the superconducting layers in SmFeAs(O,F), despite its low coherence length anisotropy ($γ_ξ\approx 3-5$).

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arXiv2014

A balancing act: Evidence for a strong subdominant d-wave pairing channel in ${\rm Ba_{0.6}K_{0.4}Fe_2As_2}$

We present an analysis of the Raman spectra of optimally doped ${\rm Ba_{0.6}K_{0.4}Fe_2As_2}$ based on LDA band structure calculations and the subsequent estimation of effective Raman vertices. Experimentally a narrow, emergent mode appears in the $B_{1g}$ ($d_{x^2-y^2}$) Raman spectra only below $T_c$, well into the superconducting state and at an energy below twice the energy gap on the electron Fermi surface sheets. The Raman spectra can be reproduced quantitatively with estimates for the magnitude and momentum space structure of the s$_{+-}$ pairing gap on different Fermi surface sheets, as well as the identification of the emergent sharp feature as a Bardasis-Schrieffer exciton, formed as a Cooper pair bound state in a subdominant $d_{x^2-y^2}$ channel. The binding energy of the exciton relative to the gap edge shows that the coupling strength in this subdominant $d_{x^2-y^2}$ channel is as strong as 60% of that in the dominant $s_{+-}$ channel. This result suggests that $d_{x^2-y^2}$ may be the dominant pairing symmetry in Fe-based sperconductors which lack central hole bands.

cond-mat.str-el↗

arXiv2014

Lower critical field and SNS-Andreev spectroscopy of 122-arsenides: Evidence of nodeless superconducting gap

Using two experimental techniques, we studied single crystals of the 122-FeAs family with almost the same critical temperature, Tc. We investigated the temperature dependence of the lower critical field of a single crystal under static magnetic fields parallel to the axis. The temperature dependence of the London penetration depth can be described equally well either by a single anisotropic -wave-like gap or by a two-gap model, while a d-wave approach cannot be used to fit the London penetration depth data. Intrinsic multiple Andreev reflection effect spectroscopy was used to detect bulk gap values in single crystals of the intimate compound, with the same Tc. We estimated the range of the large gap value 6-8 meV (depending on small variation of and its a space anisotropy of about 30%, and the small gap 1.7 meV. This clearly indicates that the gap structure of our investigated systems more likely corresponds to a nodeless s-wave two gaps.

cond-mat.supr-con↗

arXiv2014

Pressure Tuned Enhancement of Superconductivity and Change of Ground State Properties in LaO0.5F0.5BiSe2 Single Crystals

By using a hydrostatic pressure, we have successfully tuned the ground state and superconductivity in LaO0.5F0.5BiSe2 single crystals. It is found that, with the increase of pressure, the original superconducting phase with Tc about 3.5 K can be tuned to a state with lower Tc, and then a new superconducting phase with Tc about 6.5 K emerges. Accompanied by this crossover, the ground state is switched from a semiconducting state to a metallic one. Accordingly, the normal state resistivity also shows a nonmonotonic change with the external pressure. Furthermore, by applying a magnetic field, the new superconducting state under pressure with Tc about 6.5 K is suppressed, and the normal state reveals a weak semiconducting feature again. These results illustrate a non-trivial relationship between the normal state property and superconductivity in this newly discovered superconducting system.

cond-mat.supr-con↗

arXiv2014

Strong and nonmonotonic temperature dependence of Hall coefficient in superconducting K$_x$Fe$_{2-y}$Se$_2$ single crystals

In-plane resistivity, magnetoresistance and Hall effect measurements have been conducted on quenched K$_x$Fe$_{2-y}$Se$_2$ single crystals in order to analysis the normal-state transport properties. It is found that the Kohler's rule is well obeyed below about 80 K, but clearly violated above 80 K. Measurements of the Hall coefficient reveal a strong but non-monotonic temperature dependence with a maximum at about 80 K, in contrast to any other FeAs-based superconductors. With the two-band model analysis on the Hall coefficient, we conclude that a gap may open below 65 K. The data above 65 K are interpreted as a temperature induced crossover from a metallic state at a low temperature to an orbital-selective Mott phase at a high temperature. This is consistent with the recent data of angle resolved photoemission spectroscopy. These results call for a refined theoretical understanding, especially when the hole pockets are absent or become trivial in K$_x$Fe$_{2-y}$Se$_2$ superconductors.

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arXiv2014

Competition between superconductivity and magnetic/nematic order as a source of anisotropic superconducting gap in underdoped Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$

The in-plane London penetration depth, $Δλ(T)$, was measured using a tunnel diode resonator technique in single crystals of Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$ with doping levels $x$ ranging from heavily underdoped, $x$=0.16 ($T_{c}$=7~K) to nearly optimally doped, $x$= 0.34 ($T_{c}=$39 K). Exponential saturation of $Δλ(T)$ in the $T\to0$ limit is found in optimally doped samples, with the superfluid density $ρ_{s}(T)\equiv(λ(0)/λ(T))^{2}$ quantitatively described by a self-consistent $γ$-model with two nodeless isotropic superconducting gaps. As the doping level is decreased towards the extreme end of the superconducting dome at $x$=0.16, the low-temperature behavior of $Δλ(T)$ becomes non-exponential and best described by the power-law $Δλ(T)\propto T^{2}$, characteristic of strongly anisotropic gaps. The change between the two regimes happens within the range of coexisting magnetic/nematic order and superconductivity, $x<0.25$, and is accompanied by a rapid rise in the absolute value of $Δλ(T)$ with underdoping. This effect, characteristic of the competition between superconductivity and other ordered states, is very similar to but of significantly smaller magnitude than what is observed in the electron-doped Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ compounds. Our study suggests that the competition between superconductivity and magnetic/nematic order in hole-doped compounds is weaker than in electron-doped compounds, and that the anisotropy of the superconducting state in the underdoped iron pnictides is a consequence of the anisotropic changes in the pairing interaction and in the gap function promoted by both magnetic and nematic long-range order.

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arXiv2014

Intrinsic Josephson junctions in the iron-based multi-band superconductor (V2Sr4O6)Fe2As2

In layered superconductors, Josephson junctions may be formed within the unit cell due to sufficiently low interlayer coupling. These intrinsic Josephson junction (iJJ) systems have attracted considerable interest for their application potential in quantum computing as well as efficient sources of THz radiation, closing the famous "THz gap". So far, iJJ have been demonstrated in single-band, copper-based high-Tc superconductors, mainly in Ba-Sr-Ca-Cu-O. Here we report clear experimental evidence for iJJ behavior in the iron-based superconductor (V2Sr4O6)Fe2As2. The intrinsic junctions are identified by periodic oscillations of the flux flow voltage upon increasing a well aligned in-plane magnetic field. The periodicity is well explained by commensurability effects between the Josephson vortex lattice and the crystal structure, which is a hallmark signature of Josephson vortices confined into iJJ stacks. This finding adds (V2Sr4O6)Fe2As2 as the first iron-based, multi-band superconductor to the copper-based iJJ materials of interest for Josephson junction applications, and in particular novel devices based on multi-band Josephson coupling may be realized.

cond-mat.supr-con↗

arXiv2014

Magnetism and superconductivity in Sr$_2$VFeAsO$_3$ revealed by $^{75}$As- and $^{51}$V-NMR under elevated pressures

We report $^{75}$As- and $^{51}$V-nuclear magnetic resonance (NMR) measurements on the iron-based superconductor Sr$_2$VFeAsO$_3$ with alternating stacks structure. We find that the $^{75}$As nuclear spin-spin relaxation rate ($1/T_2$) shows a pronounced peak at $T_N$ = 165 K, below which the resonance peak shifts to a higher frequency due to the onset of an internal magnetic field. The $^{51}$V spectrum does not shift, but is broadened below $T_N$. We conclude that the Fe electrons oder antiferromagnetically below $T_N$ with a magnetic moment $m_{Fe}$ $\sim$ 0.4 $μ_B$. Application of external pressure up to 2.4 GPa reduces $T_N$ in a rate of $-$40 K/GPa, and enhances the superconducting transition temperature $T_c$ in a rate of 2 K/GPa. The pressure-temperature phase diagram for Sr$_2$VFeAsO$_3$ shows that superconductivity coexists with antiferromagnetism over a wide pressure range with an unprecedented high $T_c$ up to 36.5 K.

cond-mat.supr-con↗

arXiv2014

Interplane resistivity of underdoped single crystals (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$, $0 \leq x<0.34$

Temperature-dependent inter-plane resistivity, $ρ_c(T)$, was measured in hole-doped iron-arsenide superconductor (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$ over a doping range from parent compound to optimal doping $T_c\approx 38~K$, $0\leq x \leq 0.34$. Measurements were undertaken on high-quality single crystals grown from FeAs flux. The coupled magnetic/structural transition at $T_{SM}$ leads to clear accelerated decrease of $ρ_c(T)$ on cooling in samples with $T_c <$26~K ($x <0.25$). This decrease in hole-doped material is in notable contrast to an increase in $ρ_c(T)$ in the electron-doped Ba(Fe$_{1-x}$Co$_x$)Fe $_2$As$_2$ and iso-electron substituted BaFe$_2$(As$_{1-x}$P$_x$)$_2$. The $T_{SM}$ decreases very sharply with doping, dropping from $T_s$=71~K to zero on increase of $T_c$ from approximately 25 to 27~K. The $ρ_c(T)$ becomes $T$-linear close to optimal doping. The broad crossover maximum in $ρ_c(T)$, found in the parent BaFe$_2$As$_2$ at around $T_{max} \sim$200~K, shifts to higher temperature $\sim$250~K with doping $x$=0.34. The maximum shows clear correlation with the broad crossover feature found in the temperature-dependent in-plane resistivity $ρ_a(T)$. The doping evolution of $T_{max}$ in (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$ is in notable contrast with both rapid suppression of $T_{max}$ found in Ba(Fe$_{1-x}TM_x$)$_2$As$_2$ ($TM$=Co,Rh,Ni,Pd) and its rapid increase BaFe$_2$(As$_{1-x}$P$_x$)$_2$. This observation suggest that pseudogap features are much stronger in hole-doped than in electron-doped iron-based superconductors, revealing significant electron-hole doping asymmetry similar to the cuprates. This paper replaces: cond-mat:1106.0533.

cond-mat.supr-con↗

arXiv2014

The spectroscopic signature of Kondo screening on single adatoms in Na(Fe0.96Co0.03Mn0.01)As

The electronic states of surface adatoms in Na(Fe0.96Co0.03Mn0.01)As have been studied by low temperature scanning tunneling spectroscopy. The spectra recorded on the adatoms display both superconducting coherence peaks and an asymmetric resonance in a larger energy scale. The Fano-type line shape of the spectra points towards a possible Kondo effect at play. The apparent energy position of the resonance peak shifts about 5 meV to the Fermi level when measured across the critical temperature, supporting that the Bogoliubov quasiparticle is responsible for the Kondo screening in the superconducting state. The tunneling spectra do not show the subgap bound states, which is explained as the weak pair breaking effect given by the weak and broad scattering potential after the Kondo screening.

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arXiv2014

Power Law Like Correlation between Condensation Energy and Superconducting Transition Temperatures in Iron Pnictide/Chalcogenide Superconductors: Beyond the BCS Understanding

Superconducting condensation energy $U_0^{int}$ has been determined by integrating the electronic entropy in various iron pnictide/chalcogenide superconducting systems. It is found that $U_0^{int}\propto T_c^n$ with $n$ = 3 to 4, which is in sharp contrast to the simple BCS prediction $U_0^{BCS}=1/2N_FΔ_s^2$ with $N_F$ the quasiparticle density of states at the Fermi energy, $Δ_s$ the superconducting gap. A similar correlation holds if we compute the condensation energy through $U_0^{cal}=3γ_n^{eff}Δ_s^2/4π^2k_B^2$ with $γ_n^{eff}$ the effective normal state electronic specific heat coefficient. This indicates a general relationship $γ_n^{eff} \propto T_c^m$ with $m$ = 1 to 2, which is not predicted by the BCS scheme. A picture based on quantum criticality is proposed to explain this phenomenon.

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arXiv2013

In-Gap Quasiparticle Excitations Induced by Non-Magnetic Cu Impurities in Na(Fe0.96Co0.03Cu0.01)As Revealed by Scanning Tunneling Spectroscopy

The pairing mechanism in the iron pnictides remains unresolved yet. One of the central issues is the structure of the superconducting order parameter which classifies the community into two different and highly disputed camps. On one hand the picture of pairing based on the magnetic origin predicts a sign reversal gap on the electron and hole Fermi pockets, leading to the S+- pairing. On the other hand, a more conventional S++ pairing gap was suggested based on the phonon or orbital fluctuation mediated pairing. In the superconducting state, the impurities may generate a unique pattern of local density of states in space and energy, which are regarded as the fingerprints for checking the structure of the pairing gap. In this study, we successfully identified the non-magnetic and magnetic impurities in Na(Fe0.97-xCo0.03Tx)As (T=Cu, Mn) and investigated the spatial resolved scanning tunneling spectroscopy. We present clear evidence of the in-gap quasiparticle states induced by the nonmagnetic Cu impurities, giving decisive evidence of the S+- pairing. This is corroborated by the consistency between the experimental data and the first-principles calculations based on the S+- pairing gap with a scalar scattering potential.

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arXiv2013

Close relationship between superconductivity and the bosonic mode in Ba0.6K0.4Fe2As2 and Na(Fe0.975Co0.025)As

Since the discovery of high temperature superconductivity in the iron pnictides and chalcogenides in early 2008, a central issue has been the microscopic origin of the superconducting pairing. Although previous experiments suggest that the pairing may be induced by exchanging the antiferromagnetic spin fluctuations and the superconducting order parameter has opposite signs in the electron and hole pockets as predicted by the S+- pairing model, it remains unclear whether there is a bosonic mode from the tunneling spectrum which has a close and universal relationship with superconductivity as well as the spin excitation. In this paper, based on the measurements of scanning tunneling spectroscopy, we show the clear evidence of a bosonic mode with the energy identical to that of the neutron spin resonance in two completely different systems Ba0.6K0.4Fe2As2 and Na(Fe0.975Co0.025)As with different superconducting transition temperatures. In both samples, the superconducting coherence peaks and the mode feature vanish simultaneously inside the vortex core or above Tc, indicating a close relationship between superconductivity and the bosonic mode. Our data also demonstrate a universal ratio between the mode energy and superconducting transition temperature, that is [mode energy]/kBTc ~ 4.3, which underlines the unconventional mechanism of superconductivity in the iron pnictide superconductors.

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arXiv2013

Unexpected Giant Superconducting Fluctuation and Anomalous Semiconducting Normal State in NdO1-xFxBi1-yS2 Single Crystals

The BiS2-based superconductors were discovered recently. The superconductivity has been proved by many other groups. Since the previous experiments were all done on polycrystalline samples, therefore there remains a concern whether the superconductivity is really derived from the materials intrinsically or from some secondary phases. Experiments on single crystals are highly desired. In this paper, we report the successful growth of the NdO1-xFxBi1-yS2 single crystals. Resistive and magnetic measurements reveal that the bulk superconducting transition occurs at about 5 K, while an unexpected giant superconducting fluctuation appears at temperatures as high as 2-4 kBTC. Analysis based on the anisotropic Ginzbaug-Landau theory gives an anisotropy of 30-45. Two gap features with magnitudes of about 3.5+-0.3 meV and 7.5+-1 meV were observed by scanning tunneling spectroscopy. The smaller gap is associated with the bulk superconducting transition at about 5 K yielding a huge ratio 2Delta_s/kBTc =16.8, the larger gap remains up to about 26 K. The normal state recovered by applying a high magnetic field shows an anomalous semiconducting behavior. All these suggest that the superconductivity in this newly discovered superconductor cannot be formatted into the BCS theory.

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