arXiv subjects

Hai-Jun Liao

Publications and source records attributed to Hai-Jun Liao.

At least 19 recordsLinked to original sources

arXiv2026

Optimized Tensor-Network Renormalization for Quantum Dynamics: Resolving the Spectral Function of $\mathrm{K_2Co(SeO_3)_2}$

Tensor-network methods have opened a powerful route for the study of dynamical spectral functions in two-dimensional quantum systems. However, existing approaches within the framework of infinite projected entangled-pair states construct the required renormalization tensors solely from the ground-state environment and can suffer from severe numerical instability. We identify the origin of this instability and introduce an excitation-tailored corner-transfer-matrix renormalization-group (ET-CTMRG) method to resolve it. By incorporating excitation tensors into the renormalization procedure, the method constructs a substantially more accurate effective Hamiltonian matrix and thereby yields reliable and well-converged excitation spectra. For Heisenberg antiferromagnets, it reduces truncation errors by orders of magnitude and for the particularly complex case of the supersolid phase in the triangular-lattice XXZ magnet $\mathrm{K_2Co(SeO_3)_2}$, it achieves excellent quantitative agreement with inelastic neutron-scattering measurements. ET-CTMRG therefore provides a robust framework for investigating the dynamical properties of strongly correlated quantum systems.

cond-mat.str-el↗

arXiv2026

Dynamical Spectral Function of the Kagome Quantum Spin Liquid

Quantum spin liquids (QSLs) host exotic fractionalized magnetic and gauge-field excitations whose microscopic origins and experimental verification remain frustratingly elusive. In the absence of static magnetic order, the spin excitation spectrum constitutes the crucial probe of QSL behavior, but its theoretical computation is a serious challenge. Here we employ state-of-the-art tensor-network methods to obtain the full dynamical spectral function of the $J_1$-$J_2$ kagome Heisenberg model and benchmark our results by tracking their evolution across the magnetically ordered and QSL phases. Reducing $|J_2|/J_1$ causes increasingly strong spin-wave renormalization, flattening these modes then merging them into a continuum characteristic of deconfined spinons at all finite energies in the QSL. The low-energy continuum and the occurrence of gap closure at multiple high-symmetry points identify this gapless QSL as the U(1) Dirac spin liquid. These results establish a unified understanding of spin excitations in highly frustrated quantum magnets and provide clear spectral fingerprints for experimental detection in candidate kagome QSL materials.

cond-mat.str-el↗

arXiv2026

Exact Neural-Network Representations of the Motzkin States

Motzkin spin chains are paradigmatic frustration-free one-dimensional quantum systems whose ground states feature exactly solvable combinatorial structures and exotic, area-law-violating entanglement scaling. Specifically, colorless Motzkin states exhibit critical logarithmic entanglement divergence $\log N$ with system size $N$, while their colorful counterparts host supercritical sublinear $\sqrt{N}$ entanglement growth. Such unconventional entanglement behaviors place these states well beyond the expressive capability of standard matrix product states, which are fundamentally constrained by the entanglement area law. Here, we systematically construct exact, training-free neural-network representations for both colorless and colorful Motzkin states across four mainstream architectures, including recurrent, feedforward, convolutional, and transformer networks. Our core design leverages a causal prefix-sum module, implementable via recurrent updates, feedforward mappings, or masked attention layers, combined with position-selective rectified linear gates that enforce the Motzkin height constraints. For the colorful states, we further introduce a dedicated causal stack module that explicitly encodes the last-in-first-out color-matching rule. Our results demonstrate that neural architectures can accurately capture highly non-trivial entanglement features inaccessible to conventional tensor networks, providing prototypic examples for benchmarking and a constructive design framework for future neural-network quantum state developments targeting strongly entangled quantum systems.

cond-mat.str-el↗

arXiv2026

Statistical mechanics of the $N$-queens problem

We investigate the $N$-queens problem as a lattice gas -- a model in which $N$ queens are placed on an $N \times N$ chessboard with pairwise repulsive interactions along shared rows, columns, and diagonals -- from the perspective of statistical mechanics. The ground states are exactly the $Q(N)$ solutions of the classical $N$-queens problem, with entropy per queen $s_0 \approx \ln N - γ$ ($γ\approx 1.944$). This entropy reflects a characteristic constraint hierarchy: each successive geometric constraint -- columns, then diagonals -- reduces the entropy from the free-placement value $\ln N$ by a definite constant. We derive the exact high-temperature energy $E/N \to 5/3$ as $N \to \infty$. Extensive Monte Carlo simulations with $10^8$ sweeps per temperature point for $N = 8$--$1024$ reveal that the specific heat per queen $C_v/N$ converges to a universal function of $T$ as $N \to \infty$. The converged curve features a non-divergent peak $C_v^{\max}/N \approx 1.63$ at $T^* \approx 0.235\,J$, establishing the absence of a thermodynamic phase transition. Combined with the trivially exact high-temperature entropy $S(\infty)/N = (1/N) \ln \binom{N^2}{N}$, the convergence of $C_v/N$ enables a thermodynamic integration of $C_v/T$ from $T = \infty$ to $T = 0$ that recovers the ground-state entropy -- and hence the Simkin constant $γ$ -- purely from Monte Carlo data. This provides an independent thermodynamic route to a fundamental combinatorial constant. Thermodynamic integration yields $γ_{\rm MC} = 1.946 \pm 0.003$ at $N = 1024$, within $0.1\%$ of the precise combinatorial value $γ= 1.94400(1)$. We further present a transfer-matrix-based tensor network formulation that encodes the non-attacking constraints into a rank-9 site tensor with 17 nonzero elements, providing a complementary exact-enumeration route.

cond-mat.stat-mech↗

arXiv2025

Possible Observation of Quadrupole Waves in Spin Nematics

Discovery of new states of matter is a key objective in modern condensed matter physics, which often leads to revolutionary technological advancements such as superconductivity. Quantum spin nematic, a ``hidden order'' that evades conventional magnetic probes, is one such state. Na$_2$BaNi(PO$_4$)$_2$ is a potential spin nematic material, suggested by the observation of a two-magnon Bose-Einstein condensation from above the saturation field. However, direct confirmation of the spin nematicity remains elusive. This Letter presents inelastic neutron scattering spectra from the putative spin nematic phases of Na$_2$BaNi(PO$_4$)$_2$, revealing low-energy quadrupole waves that are absent in the neighboring conventional magnetic phases. A spin-one model quantitatively captures the full details of the spin excitation spectra across all low-temperature phases, providing direct evidence of the spin nematic orders. Additionally, we show evidence of the three-magnon continuum and two-magnon bound states in the $1/3$-magnetization plateau, revealing condensation of the two-magnon bound state as the origin of the low-field spin nematic supersolid phase.

cond-mat.str-el↗

arXiv2025

Thermodynamics of the Hubbard Model on the Bethe Lattice

We investigate the thermodynamic properties of the Hubbard model on the Bethe lattice with a coordination number of 3 using the thermal canonical tree tensor network method. Our findings reveal two distinct thermodynamic phases: a low-temperature antiferromagnetic phase, where spin SU(2) symmetry is broken, and a high-temperature paramagnetic phase. A key feature of the system is the separation of energy scales for charge and spin excitations, which is reflected in the temperature dependence of thermodynamic quantities and the disparity between spin and charge gaps extracted from their respective susceptibilities. At the critical point, both spin and charge susceptibilities exhibit singularities, suggesting that charge excitations are not fully decoupled from their spin counterparts. Additionally, the double occupancy number exhibits a non-monotonic temperature dependence, indicative of an entropy-driven Pomeranchuk effect. These results demonstrate that the loopless Bethe lattice effectively captures the essential physics of the Hubbard model while providing a computationally efficient framework for studying strongly correlated electronic systems.

cond-mat.str-el↗

arXiv2025

Fractionalization Signatures in the Dynamics of Quantum Spin Liquids

We investigate the signatures of fractionalization in quantum spin liquids by studying different phases of the Kitaev honeycomb model in the presence of an out-of-plane magnetic field through which the model becomes non-integrable. Using the infinite projected entangled pair states (iPEPS) ansatz, along with analytical calculations and exact diagonalization, we calculate dynamical signatures of fractionalized particles through spin-spin and dimer-dimer correlations. Our analysis demonstrates the ability of these correlations to discern distinct fractionalized quantum sectors, namely Majorana fermions and the emergent $Z_2$ fluxes, in both the chiral spin liquid (CSL) phase under weak field and the emergent intermediate gapless phase (IGP) under moderate field. Importantly, our calculation reveals the nature of IGP observed at moderate fields, a region of ongoing debate, indicating that this phase is a Majorana metal induced by strong flux fluctuations.

cond-mat.str-el↗

arXiv2024

Universal scaling behavior of resistivity under two-dimensional superconducting phase fluctuations

In superconductors with relatively low superfluid density, such as cuprate high-$T_c$ superconductors, the phase fluctuations of the superconducting order parameter are remarkable, presumably playing a nonnegligible role in shaping many distinctive physical properties. This work systematically investigates the electrical transport properties arising from thermal superconducting phase fluctuations in two-dimensional superconductors. Employing the Monte Carlo procedure, we access the numerically exact properties of a microscopic model of superconductivity, in which the classical XY model governs the thermal phase fluctuations of the superconducting order parameter. For both $s$-wave and $d_{x^2-y^2}$-wave pairings, the electrical resistivity exhibits a universal scaling behavior in the temperature range above $T_c$. Our numerical results demonstrate that the scaling behavior of the quasiparticle lifetime is associated with the correlation length of the superconducting order parameter, yielding the universal scaling behavior of electrical resistivity determined by the Berezinskii-Kosterlitz-Thouless critical scaling of the correlation length. Furthermore, we discuss the dependence of the electrical resistivity coefficient on the pairing amplitude and the possible implication on recent transport experiments.

cond-mat.str-el↗

arXiv2024

Dynamical Spectra of Spin Supersolid States in Triangular Antiferromagnets

We employ tensor network renormalization to explore the dynamical spectra of the easy-axis triangular-lattice antiferromagnet (TLAF) in a magnetic field. Our analysis identifies two distinct low-energy magnon excitations: a gapless Goldstone mode and a gapped mode. At zero field, the spectra display two nearly degenerate roton modes near the M point. With the increase of the magnetic field within the Y-shape superfluid phase, these modes diverge, with the roton excitation vanishing from the Goldstone mode branch, suggesting that the roton dip in this mode may just result from the energy-level repulsion imposed by the roton excitation in the gapped mode. Moreover, the in-plane spectral function shows substantial weight in high energies in the same spin excitation channel where the low-energy roton excitation appears. However, these roton excitations are absent in the V-shape supersolid phase.

cond-mat.str-el↗

arXiv2023

Simulation of IBM's kicked Ising experiment with Projected Entangled Pair Operator

We perform classical simulations of the 127-qubit kicked Ising model, which was recently emulated using a quantum circuit with error mitigation [Nature 618, 500 (2023)]. Our approach is based on the projected entangled pair operator (PEPO) in the Heisenberg picture. Its main feature is the ability to automatically identify the underlying low-rank and low-entanglement structures in the quantum circuit involving Clifford and near-Clifford gates. We assess our approach using the quantum circuit with 5+1 trotter steps which was previously considered beyond classical verification. We develop a Clifford expansion theory to compute exact expectation values and use them to evaluate algorithms. The results indicate that PEPO significantly outperforms existing methods, including the tensor network with belief propagation, the matrix product operator, and the Clifford perturbation theory, in both efficiency and accuracy. In particular, PEPO with bond dimension $χ=2$ already gives similar accuracy to the CPT with $K=10$ and MPO with bond dimension $χ=1024$. And PEPO with $χ=184$ provides exact results in $3$ seconds using a single CPU. Furthermore, we apply our method to the circuit with 20 Trotter steps. We observe the monotonic and consistent convergence of the results with $χ$, allowing us to estimate the outcome with $χ\to\infty$ through extrapolations. We then compare the extrapolated results to those achieved in quantum hardware and with existing tensor network methods. Additionally, we discuss the potential usefulness of our approach in simulating quantum circuits, especially in scenarios involving near-Clifford circuits and quantum approximate optimization algorithms. Our approach is the first use of PEPO in solving the time evolution problem, and our results suggest it could be a powerful tool for exploring the dynamical properties of quantum many-body systems.

quant-ph↗

arXiv2023

Differentiable programming tensor networks for Kitaev magnets

We present a general computational framework to investigate ground state properties of quantum spin models on infinite two-dimensional lattices using automatic differentiation-based gradient optimization of infinite projected entangled-pair states. The approach exploits the variational uniform matrix product states to contract infinite tensor networks with unit-cell structure and incorporates automatic differentiation to optimize the local tensors. We applied this framework to the Kitaev-type model, which involves complex interactions and competing ground states. To evaluate the accuracy of this method, we compared the results with exact solutions for the Kitaev model and found that it has a better agreement for various observables compared to previous tensor network calculations based on imaginary-time projection. Additionally, by finding out the ground state with lower variational energy compared to previous studies, we provided convincing evidence for the existence of nematic paramagnetic phases and 18-site configuration in the phase diagram of the $K$-$Γ$ model. Furthermore, in the case of the realistic $K$-$J$-$Γ$-$Γ'$ model for the Kitaev material $α$-RuCl$_3$, we discovered a non-colinear zigzag ground state. Lastly, we also find that the strength of the critical out-of-plane magnetic field that suppresses such a zigzag state has a lower transition field value than the previous finite-cylinder calculations. The framework is versatile and will be useful for a quick scan of phase diagrams for a broad class of quantum spin models.

physics.comp-ph↗

arXiv2023

Projected d-wave superconducting state: a fermionic projected entangled pair state study

We investigate the physics of projected d-wave pairing states using their fermionic projected entangled pair state (fPEPS) representation. First, we approximate a d-wave Bardeen-Cooper-Schrieffer state using the Gaussian fPEPS. Next, we translate the resulting state into fPEPS tensors and implement the Gutzwiller projection which removes double occupancy by modifying the local tensor elements. The tensor network representation of the projected d-wave pairing state allows us to evaluate physical quantities in the thermodynamic limit without employing the Gutzwiller approximation. Despite having very few variational parameters, such physically motivated tensor network states are shown to exhibit competitive energies for the doped t-J model. We expect that such construction offers useful initial states and guidance for variational tensor network calculations.

cond-mat.str-el↗

arXiv2022

Spin Excitation Spectra of Anisotropic Spin-$1/2$ Triangular Lattice Heisenberg Antiferromagnets

Investigation of dynamical excitations is difficult but crucial to the understanding of many exotic quantum phenomena discovered in quantum materials. This is particularly true for highly frustrated quantum antiferromagnets whose dynamical properties deviate strongly from theoretical predictions made based on the spin-wave or other approximations. Here we present a large-scale numerical calculation on the dynamical correlation functions of spin-$1/2$ triangular Heisenberg model using a state-of-the-art tensor network renormalization group method. The calculated results allow us to gain for the first time a comprehensive picture on the nature of spin excitation spectra in this highly frustrated quantum system. It provides a quantitative account for all the key features of the dynamical spectra disclosed by inelastic neutron scattering measurements for $\rm Ba_3CoSb_2O_9$, revealing the importance of the interplay between low- and high-energy excitations and its renormalization effect to the low-energy magnon bands and high-energy continuums. We identify the longitudinal Higgs modes in the intermediate-energy scale and predict the energy and momentum dependence of spectral functions along the three principal axes that can be verified by polarized neutron scattering experiments. Furthermore, we find that the spin excitation spectra weakly depend on the anisotropic ratio of the antiferromagnetic interaction.

cond-mat.str-el↗

arXiv2022

Variational determination of arbitrarily many eigenpairs in one quantum circuit

The state-of-the-art quantum computing hardware has entered the noisy intermediate-scale quantum (NISQ) era. Having been constrained by the limited number of qubits and shallow circuit depth, NISQ devices have nevertheless demonstrated the potential of applications on various subjects. One example is the variational quantum eigensolver (VQE) that was first introduced for computing ground states. Although VQE has now been extended to the study of excited states, the algorithms previously proposed involve a recursive optimization scheme which requires many extra operations with significantly deeper quantum circuits to ensure the orthogonality of different trial states. Here we propose a new algorithm to determine many low energy eigenstates simultaneously. By introducing ancillary qubits to purify the trial states so that they keep orthogonal to each other throughout the whole optimization process, our algorithm allows these states to be efficiently computed in one quantum circuit. Our algorithm reduces significantly the complexity of circuits and the readout errors, and enables flexible post-processing on the eigen-subspace from which the eigenpairs can be accurately determined. We demonstrate this algorithm by applying it to the transverse Ising model. By comparing the results obtained using this variational algorithm with the exact ones, we find that the eigenvalues of the Hamiltonian converge quickly with the increase of the circuit depth. The accuracies of the converged eigenvalues are of the same order, which implies that the difference between any two eigenvalues can be more accurately determined than the eigenvalues themselves.

quant-ph↗

arXiv2021

Entanglement Entropy of Non-Hermitian Free Fermions

We study the entanglement properties of non-Hermitian free fermionic models with translation symmetry using the correlation matrix technique. Our results show that the entanglement entropy has a logarithmic correction to the area law in both one-dimensional and two-dimensional systems. For any one-dimensional one-band system, we prove that each Fermi point of the system contributes exactly 1/2 to the coefficient c of the logarithmic correction. Moreover, this relation between c and Fermi point is verified for more general one-dimensional and two-dimensional cases by numerical calculations and finite-size scaling analysis. In addition, we also study the single-particle and density-density correlation functions.

cond-mat.mes-hall↗

arXiv2021

Abnormal Critical Fluctuations Revealed by Magnetic Resonance in the Two-Dimensional Ferromagnetic Insulators

Phase transitions and critical phenomena, which are dominated by fluctuations and correlations, are one of the fields replete with physical paradigms and unexpected discoveries. Especially for two-dimensional magnetism, the limitation of the Ginzburg criterion leads to enhanced fluctuations breaking down the mean-field theory near a critical point. Here, by means of magnetic resonance, we investigate the behavior of critical fluctuations in the two-dimensional ferromagnetic insulators $\rm CrXTe_3 (X=Si, Ge)$. After deriving the classical and quantum models of magnetic resonance, we deem the dramatic anisotropic shift of the measured $g$ factor to originate from fluctuations with anisotropic interactions. The deduction of the $g$ factor behind the fluctuations is consistent with the spin-only state (${g\approx}$ 2.050(10) for $\rm CrSiTe_3$ and 2.039(10) for $\rm CrGeTe_3$). Furthermore, the abnormal enhancement of $g$ shift, supplemented by specific heat and magnetometry measurements, suggests that $\rm CrSiTe_3$ exhibits a more typical two-dimensional nature than $\rm CrGeTe_3$ and may be closer to the quantum critical point.

cond-mat.mes-hall↗

arXiv2020

Automatic Differentiation for Second Renormalization of Tensor Networks

Tensor renormalization group (TRG) constitutes an important methodology for accurate simulations of strongly correlated lattice models. Facilitated by the automatic differentiation technique widely used in deep learning, we propose a uniform framework of differentiable TRG ($\partial$TRG) that can be applied to improve various TRG methods, in an automatic fashion. Essentially, $\partial$TRG systematically extends the concept of second renormalization [PRL 103, 160601 (2009)] where the tensor environment is computed recursively in the backward iteration, in the sense that given the forward process of TRG, $\partial$TRG automatically finds the gradient through backpropagation, with which one can deeply "train" the tensor networks. We benchmark $\partial$TRG in solving the square-lattice Ising model, and demonstrate its power by simulating one- and two-dimensional quantum systems at finite temperature. The deep optimization as well as GPU acceleration renders $\partial$TRG manybody simulations with high efficiency and accuracy.

cond-mat.str-el↗

arXiv2020

Critical properties of the two-dimensional $q$-state clock model

We perform the state-of-the-art tensor network simulations directly in the thermodynamic limit to clarify the critical properties of the $q$-state clock model on the square lattice. We determine accurately the two phase transition temperatures through the singularity of the classical analog of the entanglement entropy, and provide extensive numerical evidences to show that both transitions are of the Berezinskii-Kosterlitz-Thouless (BKT) type for $q\ge 5$ and that the low-energy physics of this model is well described by the $\mathbb{Z}_q$-deformed sine-Gordon theory. We also determine the characteristic conformal parameters, especially the compactification radius, that govern the critical properties of the intermediate BKT phase.

cond-mat.stat-mech↗