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Hai-Yan Wang

Publications and source records attributed to Hai-Yan Wang.

4 recordsLinked to original sources

Liquid photonic-molecule microlasers for ultrasensitive biosensing

Droplet microlasers, as promising tools for biophotonics and biomedical sciences, have witnessed rapid advances due to their flexible reconfigurability, high sensitivity to stimuli, and label-free biosensing ability. However, designing these biosensors with simultaneously critical properties of low lasing threshold, high spectral purity, and ultimate sensitivity remains challenging. Here, we propose a versatile strategy to build liquid photonic molecules (LPMs) that combine all these features in a single device. We find that through tailoring the spectral Vernier overlap in size-mismatched droplets, this device enables single-mode lasing with a low threshold of ~610 nJ mm-2. The LPM lasers are engineered for dynamic tunability using a molecular isomerization strategy, which induces spectral mode hopping and thus yields a nearly ten-fold enhancement in spectral sensitivity over single droplets. Moreover, by leveraging the self-referenced intensity response of the LPM lasing modes, we demonstrate a three-orders-of-magnitude enhancement in biomolecular sensing, with a detection limit of 30 aM and a dynamic range spanning nine orders of magnitude. Our work offers exciting prospects for bio-integrated liquid sensors in diverse applications.

physics.optics

Straightforward computation of high-pressure elastic constants using Hooke's law: A prototype of metal Ru

In this paper, we did a systematic comparative study on the accuracy of two computational methods of elastic constants combined with the density functional theory (DFT), the stress-strain method and the energy-strain method. We took metal Ru as a prototype to compare its high-pressure elastic constants calculated by our present stress-strain method with the previous energy-strain results by others. Although the two methods yielded almost the same accuracy of high-pressure elastic constants for Ru, our stress-strain method directly based on the Hooke's law of elasticity theory is much straightforward and simple to implement. However, the energy-strain method needs complicated pressure corrections because of the pressure effects on the total energy. Various crystal systems have various pressure correction methods. Hence, the stress-strain method is preferred to calculate the high-pressure elastic constants of materials. Furthermore, we analyzed the variations of the elastic moduli, elastic anisotropy, sound velocities, Debye temperature of Ru with pressure.

cond-mat.mtrl-sci

Raman Response and Transport Properties of One-Dimensional van der Waals Tellurium Nanowires

Tellurium can form nanowires of helical atomic chains. Given their unique one-dimensional van der Waals structure, these nanowires are expected to show remarkably different physical and electronic properties than bulk tellurium. Here we show that few-chain and single-chain van der Waals tellurium nanowires can be isolated using carbon nanotube and boron nitride nanotube encapsulation. With the approach, the number of atomic chains can be controlled by the inner diameter of the nanotube. The Raman response of the structures suggests that the interaction between a single-atomic tellurium chain and a carbon nanotube is weak, and that the inter-chain interaction becomes stronger as the number of chains increases. Compared with bare tellurium nanowires on SiO2, nanowires encapsulated in boron nitride nanotubes exhibit a dramatically enhanced current-carrying capacity, with a current density of 1.5*10^8 A cm-2, which exceeds that of most semiconducting nanowires. We also use our tellurium nanowires encapsulated in boron nitride nanotubes to create field-effect transistors that have a diameter of only 2 nm.

cond-mat.mes-hall

Congruences for sequences analogous to Euler numbers

For a given real number $a$ we define the sequence $\{E_{n,a}\}$ by $E_{0,a}=1$ and $E_{n,a}=-a\sum_{k=1}^{[n/2]} \binom n{2k}E_{n-2k,a}$ $(n\ge 1)$, where $[x]$ is the greatest integer not exceeding $x$. Since $E_{n,1}=E_n$ is the n-th Euler number, $E_{n,a}$ can be viewed as a natural generalization of Euler numbers. In this paper we deduce some identities and an inversion formula involving $\{E_{n,a}\}$, and establish congruences for $E_{2n,a}\mod{2^{{\rm ord}_2n+8}}$, $E_{2n,a}\pmod{3^{{\rm ord}_3n+5}}$ and $E_{2n,a}\pmod{5^{{\rm ord}_5n+4}}$ provided that $a$ is a nonzero integer, where ${\rm ord}_pn$ is the least nonnegative integer $α$ such that $p^{\a}\mid n$ but $p^{\a+1}\nmid n$.

math.NT