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Haitao Huang

Publications and source records attributed to Haitao Huang.

15 recordsLinked to original sources

4DGS-Fixer: Generative Sparse-View 4D Gaussian Splatting with Iterative Refinement Guided by Video Diffusion Priors

This paper addresses the challenges of dynamic scene synthesis from sparse-view videos. Existing methods employ geometric priors, adaptive optimization, or density-control strategies to improve 4D Gaussian modeling under sparse observations. However, they cannot fundamentally resolve the ill-posed problem caused by insufficient observations and missing scene information. Moreover, sparse-view 4D Gaussian Splatting (4DGS) often suffers from poor geometric initialization: with only a few input views, COLMAP typically reconstructs sparse and incomplete point clouds, leaving large scene regions without sufficient Gaussian support and making them difficult to recover through subsequent optimization. To address these limitations, we propose a novel iterative refinement framework based on a video diffusion model to improve the completeness and consistency of dynamic 4D scenes. Specifically, we first estimate multi-view depth maps and fuse them into dense point clouds to provide more complete geometric initialization for a dynamic 4DGS representation. We then employ a pretrained video restoration model to refine sequences rendered along novel camera trajectories at different time steps. The restored sequences serve as pseudo-supervision to regularize and iteratively refine the 4DGS representation. Experiments on a widely used benchmark dataset demonstrate that our method substantially outperforms existing baselines, achieving nearly a 2 dB PSNR improvement over the previous best-performing method.

cs.CV

Measuring Asteroid Rotation Periods Using the KMTNet Bulge Survey Data

Since 2015, the Korea Microlensing Telescope Network (KMTNet) has conducted high-cadence, near-continuous observations of the Galactic bulge for nearly nine months each year from three sites in Chile, South Africa, and Australia, and its wide field of view provides a unique opportunity to extract asteroid lightcurves from archival survey data. In this work, we performed photometric measurements of bright asteroids ($V< 20$~mag) identified within a one-square-degree field during the 2018 KMTNet bulge season. We derived reliable rotation periods for 96 asteroids, including 84 objects without previously published lightcurves. The reliable spin-rates of the asteroids in our sample are broadly consistent with those reported in the Asteroid Lightcurve Database. This archival mining approach can be readily extended to a much larger KMTNet footprint, and the existing $\sim12$~deg$^2$ high-cadence KMTNet dataset has the potential to yield reliable rotation periods (U $\geq 2+$) for more than 5,500 asteroids, substantially expanding the current database of asteroid rotational properties.

astro-ph.EP

DDSNet: Dual-domain Symmetry-aware Network for PCSEL Property Prediction

Efficient exploration of the photonic crystal (PhC) lattice design space is essential for developing photonic crystal surface-emitting lasers. While coupled-wave theory (CWT) provides an effective physical framework, its computational cost remains prohibitive for large-scale exploration, driving the demand for neural surrogates. However, existing AI models underexploit two key factors of PhC unit-cell dielectric patterns indicated by CWT: spectral components and asymmetric structures, which largely govern devices' physical properties. This mismatch weakens surrogate accuracy and screening reliability, especially in structure-sensitive regions. To address this, we propose the Dual-Domain Symmetry-Aware Network (DDSNet). It integrates translation-equivariant spectral filtering with a symmetry-induced structural prior. The spectral filtering injects a spectral inductive bias into vision model while preserving translation equivariance on lattices. Meanwhile, the structural prior decomposes lattice features into irreducible representation-associated, symmetry-resolved components and processes them in separate branches. Experiments demonstrate that DDSNet significantly outperforms existing AI baselines in property prediction and high-throughput screening, exhibiting superior reliability in structure-sensitive regions. Crucially, component masking analyses reveal that the network successfully learns property-specific dependencies aligned with physical priors. These results indicate that DDSNet effectively captures physically meaningful structure-property relationships, establishing a highly reliable neural surrogate for PhC design space exploration.

physics.app-ph

FluSplat: Sparse-View 3D Editing without Test-Time Optimization

Recent advances in text-guided image editing and 3D Gaussian Splatting (3DGS) have enabled high-quality 3D scene manipulation. However, existing pipelines rely on iterative edit-and-fit optimization at test time, alternating between 2D diffusion editing and 3D reconstruction. This process is computationally expensive, scene-specific, and prone to cross-view inconsistencies. We propose a feed-forward framework for cross-view consistent 3D scene editing from sparse views. Instead of enforcing consistency through iterative 3D refinement, we introduce a cross-view regularization scheme in the image domain during training. By jointly supervising multi-view edits with geometric alignment constraints, our model produces view-consistent results without per-scene optimization at inference. The edited views are then lifted into 3D via a feedforward 3DGS model, yielding a coherent 3DGS representation in a single forward pass. Experiments demonstrate competitive editing fidelity and substantially improved cross-view consistency compared to optimization-based methods, while reducing inference time by orders of magnitude.

cs.CV

Decoupling Precipitation and Surface Complexation during Mn(II) Removal by Biochar via Experiments and Atomistic Simulations

Manganese(II) mobilised by mining activity poses a persistent water-quality challenge, yet the mechanisms by which low-cost sorbents, such as biochar, sequester Mn(II) remain poorly resolved. This study identifies the specific chemical drivers of Mn(II) sequestration by combining fixed-bed column and batch experiments with atomistic molecular dynamics simulations. Oilseed rape straw biochars, produced at 350\textdegree C, 550\textdegree C, and 700\textdegree C, removed 20-50% of dissolved Mn from acidic influent (pH 4, 5 ppm). High-temperature biochar achieved the greatest removal ($\sim$50%) and rapidly increased effluent pH to 9, triggering alkaline precipitation. Conversely, lower-temperature biochars removed 20-30% of Mn while maintaining a near-neutral pH (7-7.5). Enhanced \ce{K+} release in these systems indicates significant cation exchange and non-precipitative pathways. Molecular simulations confirmed that while neutral surfaces show weak Mn(II) association, deprotonated sites drive strong adsorption through inner-sphere complexation ($\sim$50% removal) and outer-sphere association ($\sim$10%). These results establish a mechanistic framework to distinguish between precipitation-led and surface-complexation-led removal. By providing specific chemical criteria for Mn-targeted sequestration, this work enables the rational design of engineered biochars for sustainable water remediation.

cond-mat.mtrl-sci

Optically driven thermodynamic transition from free- to locked-epitaxy

Controlling crystallographic orientation in quasi-van der Waals (vdW) epitaxy remains a fundamental challenge, especially for material systems located near the boundary between weakly and strongly coupled growth regimes. In such marginal systems, epitaxial selection is governed by a delicate thermodynamic competition between surface-energy penalties and interfacial interaction gains, giving rise to two archetypal limits: vdW-dominated free-epitaxy and strong interfacial coupling dominated locked-epitaxy. However, dynamically driving transitions between these regimes has remained elusive. Here, we demonstrate that external light irradiation can deterministically induce such a transition. Using the thermodynamically frustrated Fe4N/mica interface as a model system, we show that photo-excited carriers act as a chemical potentiator, significantly enhancing the interfacial chemical affinity. Within a quantitative thermodynamic description, this optical modulation increases the locking criterion (I_lock)-defined as the ratio of interfacial energy gain to surface-energy cost-beyond its critical threshold. As a result, the system switches from vdW-dominated free-epitaxy with (001) orientation to chemically locked-epitaxy with (111) orientation. Our findings establish light as a non-invasive and switchable control knob to dynamically reconfigure the interfacial energy landscape in quasi-vdW epitaxy, enabling programmable access to distinct epitaxial states beyond intrinsic material limitations.

cond-mat.mtrl-sci

Universal thermodynamic framework for quasi-van der Waals epitaxy

van der Waals (vdW) epitaxy is conventionally regarded as a rotation-free and strain-free growth mode driven by weak, isotropic interactions, yet many interfaces paradoxically exhibit strictly locked orientations that defy standard surface-energy models. We resolve this inconsistency by establishing a unified quantitative framework for 2D-3D systems, in which strong electrostatic and chemical interactions compete with entropic forces. We introduce a two-tier descriptor set-the predictive index (I_pre) and the thermodynamic locking criterion (I_lock)-to quantify the energetic sufficiency for locked epitaxy. Our theory accurately predicted the competitive interactions at the interface within the 2D-3D system, precisely characterized whether the epitaxial layer underwent free growth or was constrained in a locked growth mode, demonstrating robust consistency with diverse experimental observations. This framework unifies orientation selection in 3D-on-2D films and rotational locking in 2D-on-3D layers within a single-phase diagram. Our work provides a generalizable, predictive route to controlling epitaxial orientation across a broad spectrum of layered heterostructure

cond-mat.mtrl-sci

Continuous-variable Quantum Diffusion Model for State Generation and Restoration

The generation and preservation of complex quantum states against environmental noise are paramount challenges in advancing continuous-variable (CV) quantum information processing. This paper introduces a novel framework based on continuous-variable quantum diffusion principles, synergizing them with CV quantum neural networks (CVQNNs) to address these dual challenges. For the task of state generation, our Continuous-Variable Quantum Diffusion Generative model (CVQD-G) employs a physically driven forward diffusion process using a thermal loss channel, which is then inverted by a learnable, parameter-efficient backward denoising process based on a CVQNN with time-embedding. This framework's capability is further extended for state recovery by the Continuous-Variable Quantum Diffusion Restoration model (CVQD-R), a specialized variant designed to restore quantum states, particularly coherent states with unknown parameters, from thermal degradation. Extensive numerical simulations validate these dual capabilities, demonstrating the high-fidelity generation of diverse Gaussian (coherent, squeezed) and non-Gaussian (Fock, cat) states, typically with fidelities exceeding 99%, and confirming the model's ability to robustly restore corrupted states. Furthermore, a comprehensive complexity analysis reveals favorable training and inference costs, highlighting the framework's efficiency, scalability, and its potential as a robust tool for quantum state engineering and noise mitigation in realistic CV quantum systems.

quant-ph

Quantum Complex-Valued Self-Attention Model

Self-attention has revolutionized classical machine learning, yet existing quantum self-attention models underutilize quantum states' potential due to oversimplified or incomplete mechanisms. To address this limitation, we introduce the Quantum Complex-Valued Self-Attention Model (QCSAM), the first framework to leverage complex-valued similarities, which captures amplitude and phase relationships between quantum states more comprehensively. To achieve this, QCSAM extends the Linear Combination of Unitaries (LCUs) into the Complex LCUs (CLCUs) framework, enabling precise complex-valued weighting of quantum states and supporting quantum multi-head attention. Experiments on MNIST and Fashion-MNIST show that QCSAM outperforms recent quantum self-attention models, including QKSAN, QSAN, and GQHAN. With only 4 qubits, QCSAM achieves 100% and 99.2% test accuracies on MNIST and Fashion-MNIST, respectively. Furthermore, we evaluate scalability across 3-8 qubits and 2-4 class tasks, while ablation studies validate the advantages of complex-valued attention weights over real-valued alternatives. This work advances quantum machine learning by enhancing the expressiveness and precision of quantum self-attention in a way that aligns with the inherent complexity of quantum mechanics.

quant-ph

High-efficient Bloch simulation of magnetic resonance imaging sequences based on deep learning

Objective: Bloch simulation constitutes an essential part of magnetic resonance imaging (MRI) development. However, even with the graphics processing unit (GPU) acceleration, the heavy computational load remains a major challenge, especially in large-scale, high-accuracy simulation scenarios. This work aims to develop a deep learning-based simulator to accelerate Bloch simulation. Approach: The simulator model, called Simu-Net, is based on an end-to-end convolutional neural network and is trained with synthetic data generated by traditional Bloch simulation. It uses dynamic convolution to fuse spatial and physical information with different dimensions and introduces position encoding templates to achieve position-specific labeling and overcome the receptive field limitation of the convolutional network. Main Results: Compared with mainstream GPU-based MRI simulation software, Simu-Net successfully accelerates simulations by hundreds of times in both traditional and advanced MRI pulse sequences. The accuracy and robustness of the proposed framework were verified qualitatively and quantitatively. Besides, the trained Simu-Net was applied to generate sufficient customized training samples for deep learning-based T2 mapping and comparable results to conventional methods were obtained in the human brain. Significance: As a proof-of-concept work, Simu-Net shows the potential to apply deep learning for rapidly approximating the forward physical process of MRI and may increase the efficiency of Bloch simulation for optimization of MRI pulse sequences and deep learning-based methods.

eess.IV

Unravelling Distance-Dependent Inter-Site Interactions and Magnetic Transition Effects of Heteronuclear Single Atom Catalysts on Electrochemical Oxygen Reduction

Inter-site interactions between single atom catalysts (SACs) in the high loading regime are critical to tuning the catalytic performance. However, the understanding on such interactions and their distance dependent effects remains elusive, especially for the heteronuclear SACs. In this study, we reveal the effects of the distance-dependent inter-site interaction on the catalytic performance of SACs. Using the density functional theory calculations, we systematically investigate the heteronuclear iron and cobalt single atoms co-supported on the nitrogen-doped graphene (FeN4-C and CoN4-C) for oxygen reduction reaction (ORR). We find that as the distance between Fe and Co SACs decreases, FeN4-C exhibits a reduced catalytic activity, which can be mitigated by the presence of an axial hydroxyl ligand, whereas the activity of CoN4-C shows a volcano-like evolution with the optimum reached at the intermediate distance. We further unravel that the transition towards the high-spin state upon adsorption of ORR intermediate adsorbates is responsible for the decreased activity of both FeN4-C and CoN4-C at short inter-site distance. Such high-spin state transition is also found to significantly shift the linear relation between hydroxyl (*OH) and hydroperoxyl (*OOH) adsorbates. These findings not only shed light on the SAC-specific effect of the distance-dependent inter-site interaction between heteronuclear SACs, but also pave a way towards shifting the long-standing linear relations observed in multiple-electron chemical reactions.

physics.chem-ph

Age-Energy Tradeoff in Fading Channels with Packet-Based Transmissions

The optimal transmission strategy to minimize the weighted combination of age of information (AoI) and total energy consumption is studied in this paper. It is assumed that the status update information is obtained and transmitted at fixed rate over a Rayleigh fading channel in a packet-based wireless communication system. A maximum transmission round on each packet is enforced to guarantee certain reliability of the update packets. Given fixed average transmission power, the age-energy tradeoff can be formulated as a constrained Markov decision process (CMDP) problem considering the sensing power consumption as well. Employing the Lagrangian relaxation, the CMDP problem is transformed into a Markov decision process (MDP) problem. An algorithm is proposed to obtain the optimal power allocation policy. Through simulation results, it is shown that both age and energy efficiency can be improved by the proposed optimal policy compared with two benchmark schemes. Also, age can be effectively reduced at the expense of higher energy cost, and more emphasis on energy consumption leads to higher average age at the same energy efficiency. Overall, the tradeoff between average age and energy efficiency is identified.

cs.IT

Transition Metal-Tetracyanoquinodimethane Monolayers as Single-Atom Catalysts for Electrocatalytic Nitrogen Reduction Reaction

Converting earth-abundant dinitrogen into value-added chemical ammonia is a significant yet challenging topic. Electrocatalytic nitrogen reduction reaction (NRR), compared with conventional Haber-Bosch process, is an energy-saving and environmentally friendly approach. The major task of electrocatalytic NRR is to find electrocatalysts which can activate dinitrogen effectively and exhibit high selectivity and stability. Single atom catalysts can act as a good solution. In this work, by means of first-principles density functional theory, molecular dynamics calculations, and a two-step screening process, we confirm that single Sc and Ti atom supported on tetracyanoquinodimethane monolayers (Sc,Ti-TCNQ) are excellent candidates for NRR electrocatalysts. N2 adsorption and activation are effective due to the acceptance-donation mechanism and outstanding electronic structure of TM-TCNQ, and Gibbs free energy diagram shows that Sc-TCNQ and Ti-TCNQ exhibit low NRR overpotential of 0.33 and 0.22 V through enzymatic-consecutive mixed pathway, respectively. In addition, selectivity over HER and stability of Sc/Ti-TCNQ monolayers are also validated. This work opens a new avenue for designing novel single atom catalysts for NRR as well as other catalytic applications.

physics.chem-ph

Theoretical investigation of two-dimensional phosphorus carbides as promising anode materials for lithium-ion batteries

Employing two-dimensional (2D) materials as anodes for lithium-ion batteries (LIBs) is believed to be an effective approach to meet the growing demands of high-capacity next-generation LIBs. In this work, the first-principles density functional theory (DFT) calculations are employed to evaluate the potential application of two-dimensional phosphorus carbide (2D PCx, x=2, 5, and 6) monolayers as anode materials for lithium-ion batteries. The 2D PCx systems are predicted to show outstanding structural stability and electronic properties. From the nudge elastic band calculations, the Li atoms show extreme high diffusivities on the PCx monolayer with low energy barriers of 0.18 eV for PC2, 0.47 eV for PC5, and 0.44 eV for PC6. We further demonstrate that the theoretical specific capacity of monolayer PC5 and PC6 can reach up to 1251.7 and 1235.9 mAh g-1, respectively, several times that of graphite anode used in commercial LIBs. These results suggest that both PC5 and PC6 monolayer are promising anode materials for LIBs. Our work opens a new avenue to explore novel 2D materials in energy applications, where phosphorus carbides could be used as high-performance anode in LIBs.

physics.app-ph

Generation of 30-fs pulses from a diode-pumped graphene mode-locked Yb:CaYAlO4 laser

Stable 30 fs pulses centered at 1068 nm (less than 10 optical cycles) are demonstrated in a diode pumped Yb:CaYAlO4 laser by using high-quality chemical vapor deposited monolayer graphene as the saturable absorber. The mode locked 8.43 optical-cycle pulses have a spectral bandwidth of ~ 50 nm and a pulse repetition frequency of ~ 113.5 MHz. To our knowledge, this is the shortest pulse ever reported for graphene mode-locked lasers and mode-locked Yb-doped bulk lasers. Our experimental results demonstrate that graphene mode locking is a very promising practical technique to generate few-cycle optical pulses directly from a laser oscillator.

physics.optics