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Haixiao Wang

Publications and source records attributed to Haixiao Wang.

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Non-Hermitian-induced higher-order topological phases in acoustic fractal lattices

For fractal (non-integer-dimension) geometries in Hermitian system, high-order topological phases were realized in the past few years, for which, it is difficult to tune the energy concentration degree of topological states flexibly and smoothly. Non-Hermiticity method is expected to solve this problem. However, in non-integer-dimension system, the non-Hermitian-fractal coupled topological mechanism is unclear and topological phases induced by non-Hermiticity remain unrealized. By introducing a loss contrast in a fractal lattice, this study proposes a non-Hermitian route to realize higher-order topological phases in acoustic fractal lattices with good tunability. Based on the tight-binding approximation, calculations on the Hamiltonian of the system yield the wave-function distribution of the zero-energy modes, revealing the formation mechanisms and conditions for the topological phase transitions induced by non-Hermiticity in acoustic fractal lattices. We numerically and experimentally realize non-Hermitian-induced topological edge and corner states in a fractal structure. Furthermore, a tunable acoustic energy concentrator has been realized, namely, the degree of acoustic energy localization can be tuned conveniently by merely adjusting the loss contrast, rather than redesigning the structure parameters. This work not only establishes an effective mechanism for manipulating higher-order topology in complex fractal geometries through non-Hermiticity but also provides a theoretical framework for exploring exotic topological states of matter in non-integer dimensions.

physics.app-ph

Ni-O-Ag catalyst enables 103-m$^2$ artificial photosynthesis with >16% solar-to-chemical energy conversion efficiency

Herein, NiO nanosheets supported with Ag single atoms are synthesized for photothermal CO2 hydrogenation to achieve 1065 mmol g$^{-1}$ h$^{-1}$ of CO production rate under 1 sun irradiation, revealing the unparalleled weak sunlight driven reverse water-gas shift reaction (RWGS) activity. This performance is attributed to the coupling effect of Ag-O-Ni sites to enhance the hydrogenation of CO$_2$ and weaken the CO adsorption, resulting in 1434 mmol g$^{-1}$ h$^{-1}$ of CO yield at 300$^\circ$ C, surpassing any low-temperature RWGS performances ever reported. Building on this, we integrated the 2D Ni$_1$Ag$_{0.02}$O$_1$ supported photothermal RWGS with commercial photovoltaic electrolytic water splitting, leading to the realization of 103 m$^2$ scale artificial photosynthesis system (CO$_2$+H$_2$$\to$CO+H$_2$O) with a daily CO yield of 18.70 m$^3$, a photochemical energy conversion efficiency of >16%, over 90% H$_2$ ultilization efficiency, outperforming other types of artificial photosynthesis. The results of this research chart a promising course for designing practical, natural sunlight-driven artificial photosynthesis systems and highly efficient platinum-free CO$_2$ hydrogenation catalysts. This work is a significant step towards harnessing solar energy more efficiently and sustainably, opening exciting possibilities for future research and development in this area.

cond-mat.mtrl-sci