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Han-Chao Chen

Publications and source records attributed to Han-Chao Chen.

At least 19 recordsLinked to original sources

Observation of node-dependent Rydberg molecular bound states

Ultralong-range Rydberg molecules, formed by the interaction between a highly excited Rydberg atom and a ground-state atom, provide a unique platform for exploring quantum phenomena spanning nanometer-to-micrometer distances as well as exotic few-body interactions. The formation mechanisms and resultant physical properties differ markedly between s-wave and p-wave scattering channels. Here we report the experimental observation of node-dependent p-wave molecular signals in Rb(nS)-Rb(5S) Rydberg molecular spectra, where variations in the principal quantum number n directly reveal the shift of molecular binding energies induced by the moving nodal structure of the Rydberg electron wavefunction. This node-dependence is attributed to a cooperative effect between the local gradient of the nS-electron wavefunction and the energydependent p-wave scattering length. In addition, resolving two p-wave bound states associated with adjacent nodes highlights the remarkable sub-nanometer spatial resolution achieved in our experiment. Our findings reveal a more profound quantum control mechanism, wherein the principal quantum number acts as a switch for nodal-selective molecular bound states, and the reported method provides a sensitive spectroscopic probe of electron-atom scattering.

physics.atom-ph

Quantum Hashing via Constrained Rydberg Many-Body Dynamics

In this Letter, we show that constrained many-body dynamics in Rydberg atom arrays naturally gives rise to a quantum hashing mechanism. By encoding ternary strings into deterministic trajectories in the state space, the classical information space is mapped onto a quantum state ensemble in the Hilbert space with an induced geometric structure. Statistical analysis reveals that this ensemble exhibits high probability near-orthogonality, random-like distribution, and broad geometric coverage. These geometric features naturally give rise to the essential cryptographic properties of quantum hashing, including low collision probability, one-wayness, tamper sensitivity, and privacy preservation. Our results demonstrate that the cryptographic functionality of quantum hashing need not rely on deliberately engineered algorithms, but can instead emerge naturally from constrained many-body dynamics, identifying quantum dynamics itself as a physical resource for cryptographic information processing.

quant-ph

Fingerprint Recognition of Partial Discharge Signals in Deep Learning Enhanced Rydberg Atomic Sensors

Partial discharge originates from microscopic insulation imperfections in high-voltage apparatus and is widely considered a critical marker of incipient deterioration. Conventional partial discharge detection methods are typically constrained by limited bandwidth and often rely on predefined feature extraction, which impedes reliable recognition of broadband transient signals. In this work, we employ a Rydberg atomic sensor to directly capture time-domain responses of partial discharge emissions and construct distinctive spectral fingerprints for different types. A 1D ResNet deep learning model is then applied to recognize these fingerprints from time-domain signals without manual feature engineering. Under increased source-antenna distances, where spectral features are significantly attenuated, the model attains a recognition accuracy of approximately 94\% across four partial discharge categories, demonstrating robustness to attenuation and noise. We further validate the approach in a simulated early-warning scenario, where partial discharge signals mixed with noise are analyzed and the model successfully generates predictive alarms. These results underscore the potential of integrating Rydberg-based broadband sensing with data-driven analysis for non-invasive, high-sensitivity diagnostics of electrical insulation systems.

quant-ph

Dynamics of string breaking and revival in a Rydberg atomic chain

String breaking is one of the most representative non-perturbative dynamics processes in confinement theory, typically associated with the creation of particle-antiparticle pairs. In this paper, we take a one-dimensional Rydberg atomic chain to theoretically study the dynamical of finite-length string state. Under different string tension conditions, we find that the string dynamics exhibits two clearly distinguishable evolution characteristics: one is that the string breaks and the system enters a superposition state space containing multiple meson state configurations; the other is localized string dynamics, in which the string undergoes local breaking but can then recombine and return to a state close to the initial structure, with the breaking and recombination processes recurring over a long time scale. Through the analysis of the evolution of different meson state configurations, we visually depict the redistribution of configuration weights during the string breaking process, and reveal the observable recovery characteristics of the string after breaking. Further analysis shows that the enhancement of quantum fluctuations can increase the weight of the double-meson state configurations in the system wave function without changing the dominant dynamical behavior. The above results present a rich picture of string breaking dynamics in a one-dimensional Rydberg atomic chain and provide insights for studying confinement physics and related gauge field theory phenomena on quantum simulation platforms.

cond-mat.quant-gas

Observation of non-Hermitian topology in cold Rydberg quantum gases

The pursuit of topological phenomena in non-Hermitian systems has unveiled new physics beyond the conventional Hermitian paradigm, yet their realization in interacting many-body platforms remains a critical challenge. Exploring this interplay is essential to understand how strong interactions and dissipation collectively shape topological phases in open quantum systems. Here, we experimentally demonstrate non-Hermitian spectra topology in a dissipative Rydberg atomic gas and characterize parameters-dependent winding numbers. By increasing the interaction strength, the system evolves from Hermitian to non-Hermitian regime, accompanying emergence of trajectory loop in the complex energy plane. As the scanning time is varied, the spectra topology becomes twisted in the complex energy plane manifesting as a topology phase transition with the sign winding number changed. When preparing the system in different initial states, we can access a nontrivial fractional phase within a parameter space that globally possesses an integer winding. Furthermore, by changing the scanning direction, we observe the differentiated loops, revealing the breaking of chirality symmetry. This work establishes cold Rydberg gases as a versatile platform for exploring the rich interplay between non-Hermitian topology, strong interactions, and dissipative quantum dynamics.

cond-mat.quant-gas

Quantum Zeno Effect in the Spatial Evolution of a Single Atom

The quantum Zeno effect (QZE) reveals that frequent measurements can suppress quantum evolution, but the detailed dynamics of the system under finite-duration measurements in experiments remain insufficiently explored. Here, we employ an optical dipole trap as a projective measurement to study the motion of a single cold atom in free space. By monitoring atomic loss, we directly observe the QZE in single-atom motion in free space and find that the effect of dipole measurements on the atom comprises a short-time collapse followed by subsequent periodic unitary evolution, thereby providing an intuitive physical picture of measurement backaction across different timescales. We further investigate the effects of measurement frequency, strength, and spatial position, demonstrating that measurements not only suppress the spreading of quantum states but also enable deterministic preparation of distinct motional states. Furthermore, by dynamically controlling the measurement position, we achieve measurement-induced directional transport of a single atom without imparting additional momentum. Our results provide a direct experimental demonstration of the QZE in real space and establish a versatile framework for measurement-based control of atomic motion, paving the way for motional-state engineering in cold-atom platforms.

quant-ph

Observation of Discrete Time Quasicrystal in Rydberg Atomic Gases

Discrete time quasicrystals (DTQC) constitute a class of non-equilibrium matter characterized by temporal order without strict periodicity, in contrast to conventional time crystals. Investigating these phenomena is essential for expanding our fundamental understanding of far-from-equilibrium quantum matter and spontaneous symmetry breaking beyond periodic regimes. Here, we experimentally observe a DTQC in a driven-dissipative ensemble of strongly interacting Rydberg atoms, displaying non-equilibrium dynamical response with a different finite Abelian group symmetry $\mathbb{Z}{_m} \times \mathbb{Z}{_n}$. By applying a quasi-periodic drive using a dual-frequency drive with incommensurate frequencies, we demonstrate that the system exhibits a robust subharmonic response at multiple incommensurate frequencies, signifying the emergence of a DTQC phase. We map the full phase diagram of the system, which includes the DTQC phase, and demonstrated its rigidity against perturbations in both RF field intensity and laser detuning. Moreover, we observe a cyclic group symmetry effect that constrains the construction of $\mathbb{Z}{_2} \times \mathbb{Z}{_3}$-symmetric DTQC. This work establishes a versatile platform for studying non-equilibrium phases of matter and provides insights into the dynamics of time-translation symmetry breaking in quantum many-body systems.

cond-mat.quant-gas

Fragmented quantum phases in anti-blockade regime of Rydberg atom array

In this Letter, we report a parameter-dependent Hilbert space fragmentation in a one-dimensional Rydberg atom array under anti-blockade conditions. We identify distinct non-equilibrium dynamical phases and show that their quasi-periodic behavior arises from the interplay of multi-path interference and multi-photon cascaded excitations, reflecting fundamental differences in state connectivity and effective dimensionality. By constructing a complete phase diagram, we reveal the transition from thermalization to fragmentation, and further demonstrate a secondary fragmentation process enabled by local constraints. Our results highlight the potential of anti-blockade mechanisms for programmable non-thermal dynamics in many-body systems.

quant-ph

Diatomic and Polyatomic Heteronuclear Ultralong-Range Rydberg Molecules

Ultra-long-range Rydberg molecules (ULRMs) have attracted significant interest due to their unique electronic properties and potential applications in quantum technologies. We theoretically investigate the formation and characteristics of heteronuclear ULRMs, focusing on Rb-Cs systems. We explore the vibrational energy levels of heteronuclear nD ULRMs and compare them with homonuclear counterparts. We also predict the formation of polyatomic heteronuclear ULRMs, discussing how the binding energy and spectral features evolve as the number of ground-state atoms increases. Our theoretical predictions are presented in terms of molecular spectra and provide insight into the formation dynamics of these systems. The study further explores the potential applications of heteronuclear ULRMs in quantum information processing, quantum simulation, and precision measurements, offering new avenues for future research in many-body physics and quantum technologies.

quant-ph

A Rb-Cs dual-species magneto-optical trap

We describe a three-dimensional (3D) magneto-optical trap (MOT) capable of simultaneously capturing 85Rb and 133Cs atoms. Unlike conventional setups, our system utilizes two separate laser systems that are combined before entering the vacuum chamber, enabling the simultaneous trapping of two different atomic species. Additionally, in our 3D MOT configuration, two (of three) pairs of laser beams are not orthogonal to the chamber surfaces but are aligned at a 45{\deg} angle. With a total trapping laser power of 8 mW and repump laser power of 4 mW for Rb atoms, and a total trapping laser power of 7.5 mW and repump laser power of 1.5 mW for Cs atoms, we achieve optical depths (OD) of 3.71 for Rb and 3.45 for Cs, demonstrating efficient trapping for both species. Our 3D MOT setup allows full horizontal optical access to the trapped atomic ensembles without spatial interference from the trapping or repump laser beams. Moreover, the red detuning for trapping both atomic species is smaller than in traditional configurations. This system offers a versatile platform for exploring complex phenomena in ultracold atom physics, such as Rydberg molecule formation and interspecies interactions.

physics.atom-ph

Observation of Higgs and Goldstone modes in U(1) symmetry-broken Rydberg atomic systems

Higgs and Goldstone modes manifest as fluctuations in the order parameter of system, offering insights into its phase transitions and symmetry properties. Exploring the dynamics of these collective excitations in a Rydberg atoms system advances various branches of condensed matter, particle physics, and cosmology. Here, we report an experimental signature of Higgs and Goldstone modes in a U(1) symmetry-broken Rydberg atomic gases. By constructing two probe fields to excite atoms, we observe the distinct phase and amplitude fluctuations of Rydberg atoms collective excitations under the particle-hole symmetry. Due to the van der Waals interactions between the Rydberg atoms, we detect a symmetric variance spectrum divided by the divergent regime and phase boundary, capturing the full dynamics of the additional Higgs and Goldstone modes. Studying the Higgs and Goldstone modes in Rydberg atoms allows us to explore fundamental aspects of quantum phase transitions and symmetry breaking phenomena, while leveraging the unique properties of these highly interacting systems to uncover new physics and potential applications in quantum simulation.

cond-mat.quant-gas

Quantum enhanced metrology based on flipping trajectory of cold Rydberg gases

The dynamical trajectory of a dissipative Rydberg many-body system could be flipped under a microwave field driving, displaying an enhanced sensitivity. This is because the intersection of the folded hysteresis trajectories exhibits a sharp peak near the phase transition, amplifying the response to small changes in the microwave field. Here, we demonstrate an experiment of enhanced metrology through flipping the hysteresis trajectory in a cold atomic system, displaying an approach to improve sensitivity near the gap-closing points. By measuring the intersection points of hysteresis trajectories versus Rabi frequency of the microwave field, we quantify the equivalent sensitivity to be 1.6(5) nV cm-1 Hz-1/2. The measurement is also dependent on the interaction time, optical depth and principal quantum number since the long-range interaction between Rydberg atoms could dramatically change the shape of hysteresis trajectories. The reported results suggest that flipping trajectory features in cold Rydberg many-body systems could advance sensing and metrology applications.

cond-mat.quant-gas

Folded multistability and hidden critical point in microwave-driven Rydberg atoms

The interactions between Rydberg atoms and microwave fields provide a valuable framework for studying the complex dynamics out of equilibrium, exotic phases, and critical phenomena in many-body physics. This unique interplay allows us to explore various regimes of nonlinearity and phase transitions. Here, we observe a phase transition from the state in the regime of bistability to that in multistability in strongly interacting Rydberg atoms by varying the microwave field intensity, accompanying with the breaking of Z3-symmetry. During the phase transition, the system experiences a hidden critical point, in which the multistable states are difficult to be identified. Through changing the initial state of system, we can identify a hidden multistable state and reveal a hidden trajectory of phase transition, allowing us to track to a hidden critical point. In addition, we observe multiple phase transitions in spectra, suggesting higher-order symmetry breaking. The reported results shed light on manipulating multistability in dissipative Rydberg atoms systems and hold promise in the applications of non-equilibrium many-body physics.

cond-mat.quant-gas

Exceptional point and hysteresis trajectories in cold Rydberg atomic gases

The interplay between strong long-range interactions and the coherent driving contribute to the formation of complex patterns, symmetry, and novel phases of matter in many-body systems. However, long-range interactions may induce an additional dissipation channel, resulting in non-Hermitian many-body dynamics and the emergence of exceptional points in spectrum. Here, we report experimental observation of interaction-induced exceptional points in cold Rydberg atomic gases, revealing the breaking of charge-conjugation parity symmetry. By measuring the transmission spectrum under increasing and decreasing probe intensity, the interaction-induced hysteresis trajectories are observed, which give rise to non-Hermitian dynamics. We record the area enclosed by hysteresis loops and investigate the dynamics of hysteresis loops. The reported exceptional points and hysteresis trajectories in cold Rydberg atomic gases provide valuable insights into the underlying non-Hermitian physics in many-body systems, allowing us to study the interplay between long-range interactions and non-Hermiticity.

cond-mat.quant-gas

Quantum synchronization at the critical point of Floquet driven Rydberg atoms

The criticality enhanced correlations and susceptibility allow weak periodic driving to induce collective synchronization due to critical slowing down, providing a unique platform to study non-equilibrium order emergence. This establishes a powerful paradigm for investigating non-equilibrium order formation, yet the fundamental mechanisms of critical-point synchronization remain poorly understood. Here, we utilize a microwave pulse as a seed to induce quantum synchronization at the critical point of Floquet driven Rydberg atoms. In the experiment, the microwave periodic driving on Rydberg states acts as a seeded temporal order in subspace, which triggers synchronization across the entire ensemble. The behavior of the emergent synchronized oscillation is elaborately linked to alterations in the seed, such as the relative phase shift and the frequency difference, which result in phase-dependent seeding and embryonic synchronization. This result opens up new possibilities for studying and harnessing time-dependent quantum many-body phenomena, offering insight into the behavior of complex many-body systems under seeding.

cond-mat.quant-gas

Early warning signals of the tipping point in strongly interacting Rydberg atoms

The identification of tipping points is essential for prediction of collapses or other sudden changes in complex systems. Applications include studies of ecology, thermodynamics, climatology, and epidemiology. However, detecting early signs of proximity to a tipping is made challenging by complexity and non-linearity. Strongly interacting Rydberg atom gases offer model systems that offer both complexity and non-linearity, including phase transition and critical slowing down. Here, via an external probe we observe prior warning of the proximity of a phase transition of Rydberg thermal gases. This warning signal is manifested as a deviation from linear growth of the variance with increasing probe intensity. We also observed the dynamics of the critical slowing down behavior versus different time scales, and atomic densities, thus providing insights into the study of a Rydberg atom system's critical behavior. Our experiment suggests that the full critical slowing down dynamics of strongly-interacting Rydberg atoms can be probed systematically, thus providing a benchmark with which to identify critical phenomena in quantum many-body systems.

cond-mat.quant-gas

Floquet engineering Rydberg sub-THz frequency comb spectroscopy

Engineering a Terahertz (THz) frequency comb spectroscopy at atomic level advances the precisely measurement in spectroscopy and sensing. Current progresses on THz frequency comb rely on difference-frequency generation, optical parametric oscillation, and other methods. Generating a THz frequency comb poses challenges in source stability and achieving a narrow bandwidth, which traditional THz devices are difficult to achieve. Furthermore, accurately measuring the generated THz frequency comb necessitates a high-performance THz detector. Rydberg atoms are well-suited for electric field sensing due to their ultra-wide radio frequency transition energy levels, making them especially sensitive to external electric fields in the DC to THz bandwidth. However, there have been no reports about generating THz frequency comb spectroscopy at the atomic level until now. This work presents a THz frequency comb spectroscopy with Rydberg atoms, in which a Floquet comb-like transition is engineered through a time-periodic drive field. Our approach simplifies the setup required for THz frequency comb spectroscopy while extending the working bandwidth for Rydberg atomic sensors. The THz frequency comb spectroscopy at the atomic level reported in this article shows great potential for various applications in astronomy, remote sensing, spectral detection of biological samples, and other related fields.

physics.atom-ph

Cavity-enhanced Rydberg atom microwave receiver

Developing microwave electric field sensing based on Rydberg atom has received significant attention due to its unique advantages. However, achieving effective coupling between Rydberg atom and the microwave electric field in the sensing process is a challenging problem that greatly impacts the sensitivity. To address this, we propose the use of a microwave resonant cavity to enhance the effective coupling between the Rydberg atoms and the microwave electric field. In our experiment, we use a three-photon excitation scheme to prepare Rydberg atoms, make measurements of electric fields without and with a microwave cavity in which the vapor cell is put inside. Through experimental testing, we achieve an 18 dB enhancement of power sensitivity. The experiment shows an effective enhancement in electric field pulse signal detection. This result provides a promising direction for enhancing the sensitivity of Rydberg atomic electric field sensors and paves the way for their application in precision electric field measurements.

physics.atom-ph