Searcharxiv⌕ Search

arXiv subjects

Hanne S. Antila

Publications and source records attributed to Hanne S. Antila.

3 recordsLinked to original sources

Electrolyte density, diffusivity and conductivity in graphene nanoconfinement predicted by separating interfacial from genuine confinement effects

Confined aqueous electrolytes exhibit strong deviations from bulk behaviour, but it remains unclear which changes arise from genuine confinement-induced modification and which merely reflect the influence of interfaces. Here, we introduce an interfacial deficit-length framework, capable of decomposing density, diffusivity, and conductivity of confined electrolyte solutions into interfacial and confinement contributions. By applying the framework to molecular dynamics simulations of aqueous alkali halides in planar graphene nanoslits coupled to bulk reservoirs at variable electrolyte concentration, we show that genuine confinement effects emerge only for slit heights $H \lesssim 1$ nm; for larger H, deviations from bulk behaviour are quantitatively captured by interfacial deficit lengths. These deficit lengths are strongly ion-specific and generally positive for water and salt densities as well as for conductivities, meaning that graphene interfaces reduce the values of these observables, while diffusivity deficit lengths tend to be negative, corresponding to larger slit self-diffusivities relative to the corresponding bulk reference. Our deficit-length framework is applicable to any observable from experiments or simulations on nanoconfined electrolytes and predicts confined electrolyte properties for variable slit height H and reservoir electrolyte concentrations.

cond-mat.soft↗

Decoupling of dipolar and hydrophobic motions in biological membranes

Cells use homeostatic mechanisms to maintain an optimal composition of distinct types of phospholipids in cellular membranes. The hydrophilic dipolar layer at the membrane interface, composed of phospholipid headgroups, regulates the interactions between cell membranes and incoming molecules, nanoparticles, and viruses. On the other hand, the membrane hydrophobic core determines membrane thickness and forms an environment for membrane-bound molecules such as transmembrane proteins. A fundamental open question is to what extent the motions of these regions are coupled and, consequently, how strongly the interactions of lipid headgroups with other molecules depend on the properties and composition of the membrane hydrophobic core. We combine advanced solid-state nuclear magnetic resonance spectroscopy methodology with high-fidelity molecular dynamics simulations to demonstrate how the rotational dynamics of choline headgroups remain nearly unchanged (slightly faster) with incorporation of cholesterol into a phospholipid membrane, contrasting the well known extreme slowdown of the other phospholipid segments. Notably, our results suggest a new paradigm where phospholipid headgroups interact as quasi-freely rotating flexible dipoles at the interface, independent of the properties in the hydrophobic region.

cond-mat.soft↗

Dielectric modulation of ion transport near interfaces

Ion mobility and ionic conductance in nanodevices are known to deviate from bulk behavior, a phenomenon often attributed to surface effects. We demonstrate that dielectric mismatch between the electrolyte and the surface can qualitatively alter ionic transport in a counterintuitive manner. Instead of following the polarization-induced modulation of the concentration profile, mobility is enhanced or reduced by changes in the ionic atmosphere near the interface and affected by a polarization force parallel to the surface. In addition to revealing this mechanism, we explore the effect of salt concentration and electrostatic coupling.

cond-mat.soft↗