arXiv subjects

Hannes Kempf

Publications and source records attributed to Hannes Kempf.

3 recordsLinked to original sources

arXiv2026

Ultrafast excitation of Bloch plasmon polaritons in hyperbolic metamaterials with an extreme ultra-violet transient grating

Manipulating materials properties with light drives advances in materials science and photonics. Hyperbolic metamaterials are promising candidates as next-generation quantum optical media. They support Bloch plasmon polaritons, which are characterized by potentially infinite wave-vectors and long lifetimes, but cannot be excited through direct light illumination due to momentum mismatch. Here, we experimentally show that a transient grating, formed via interference of fully coherent seeded free-electron laser pulses in a thin insulator film, enables the excitation of Bloch plasmon polaritons in an underlying hyperbolic metamaterial. Finite element simulations confirm the role of the transient grating in facilitating phase-matching and mode excitation. Our findings demonstrate a route to spatiotemporally excite Bloch plasmon polaritons modes, offering an alternative to permanently nanostructured gratings and potentially enabling ultrafast control of optical modes excitation.

physics.optics↗

arXiv2025

Polarization conversion using hybrid near-zero and high-index metamaterials

Near-zero-refractive index materials display unique optical properties such as perfect transmission through distorted waveguides, cloaking, and inhibited diffraction. Compared to conventional media, they can fundamentally behave differently to light impinging from air, owing to the phenomenon of total external reflection. This makes them attractive for evanescent wave phenomena without prism coupling or sub-wavelength air gaps. Here, we introduce a strategy for linear-to-circular polarization conversion based on this effect. Practically realizable device designs are presented using hybrid structures of near-zero index and high index materials in a simple planar geometry. Our results predict polarization conversion in both reflection and transmission configurations based on naturally available epsilon-near-zero materials and illustrate the role of loss in limiting performance. Although the operation wavelength is limited to the epsilon-near-zero region, the concept can be implemented from the terahertz to optical domains using tunable epsilon-near-zero materials.

physics.optics↗

arXiv2023

Few-femtosecond phase-sensitive detection of infrared electric fields with a third-order nonlinearity

Measuring an electric field waveform beyond radio frequencies is often accomplished via a second-order nonlinear interaction with a laser pulse shorter than half of the field's oscillation period. However, synthesizing such a gate pulse is extremely challenging when sampling mid- (MIR) and near- (NIR) infrared transients. Here, we demonstrate an alternative approach: a third-order nonlinear interaction with a relatively long multi-cycle pulse directly retrieves an electric-field transient whose central frequency is 156 THz. A theoretical model, exploring the different nonlinear frequency mixing processes, accurately reproduces our results. Furthermore, we demonstrate a measurement of the real part of a sample's dielectric function, information that is challenging to retrieve in time-resolved spectroscopy and is therefore often overlooked. The new method paves the way towards experimentally simple MIR-to-NIR time-resolved spectroscopy that simultaneously extracts the spectral amplitude and phase information, an important extension of optical pump-probe spectroscopy of, e.g., molecular vibrations and fundamental excitations in condensed-matter physics.

physics.optics↗