arXiv subjects

Hanoh Lee

Publications and source records attributed to Hanoh Lee.

12 recordsLinked to original sources

arXiv2025

Coexisting Kagome and Heavy Fermion Flat Bands in YbCr$_6$Ge$_6$

Flat bands, emergent in strongly correlated electron systems, stand at the frontier of condensed matter physics, providing fertile ground for unconventional quantum phases. Recent observations of dispersionless bands at the Fermi level in kagome lattice open the possibility of unifying the disjoint paradigms of topology and correlation-driven heavy fermion liquids. Here, we report the unprecedented coexistence of these mechanisms in the layered kagome metal YbCr6Ge6. At high temperatures, an intrinsic kagome flat band-arising from the frustrated hopping on the kagome lattice-dominates the Fermi level. Upon cooling, localized Yb 4f-states hybridize with the topological kagome flat bands, transforming this state into the Kondo resonance states that are nearly dispersionless across the entire Brillouin zone. Crystalline symmetry forbids hybridization along specific high-symmetry lines, which stabilizes Dirac crossings of heavy-fermion character. Topological analysis of the resulting gaps reveals both trivial and nontrivial Z2 invariants, establishing the emergence of a Dirac-Kondo semimetal phase. Taken together, these results identify YbCr6Ge6 as a prototype of a topological heavy-fermion system and a platform where geometric frustration, strong correlations, and topology converge, with broad implications for correlated quantum matter.

cond-mat.str-el↗

arXiv2021

Emergent nematicity and intrinsic vs. extrinsic electronic scattering processes in the kagome metal CsV$_3$Sb$_5$

Fermi surface fluctuations and lattice instabilities in the 2D metallic kagome superconductor CsV$_3$Sb$_5$ are elucidated via polarization-resolved Raman spectroscopy. The presence of a weak electronic continuum in high-quality samples marks the cross-over into the charge-density-wave (CDW) ordered phase, while impurity-rich samples promote strong defect-induced electronic scattering processes that affect the coherence of the CDW phase. CDW-induced phonon anomalies appear below $T_{\mathrm{CDW}}$, with emergent $C2$ symmetry for one of the CDW amplitude modes, alluding to nematicity. In conjunction with symmetry-breaking lattice distortions, a kink-like hardening of the A$_{1g}$ phonon energy at $T_{\mathrm{CDW}}$ signifies a concerted interplay of electronic correlations and electron-phonon coupling in the exotic CDW order.

cond-mat.str-el↗

arXiv2020

Structural and magnetic properties of antiferromagnetic Ce$_2$IrGa$_{12}$

We report a study of the structural and magnetic properties of single crystals of Ce$_2$IrGa$_{12}$. Ce$_2$IrGa$_{12}$ crystallizes in a layered tetragonal structure, and undergoes an antiferromagnetic transition below 3.1 K. We characterize the temperature-field phase diagrams of Ce$_2$IrGa$_{12}$ for fields both within the $ab$-plane and along the $c$-axis, where the presence of a field-induced magnetic phase is found for in-plane fields. The ordering temperature is moderately enhanced upon the application of pressures up to 2.3~GPa, suggesting that Ce$_2$IrGa$_{12}$ corresponds to the well localized region of the Doniach phase diagram.

cond-mat.str-el↗

arXiv2019

Strange metal behavior in a pure ferromagnetic Kondo lattice

The strange metal phases found to develop in a wide range of materials near a quantum critical point (QCP), have posed a long-standing mystery. The frequent association of strange metals with unconventional superconductivity and antiferromagnetic QCPs has led to a belief that they are highly entangled quantum states. Ferromagnets, by contrast are regarded as an unlikely setting for strange metals, for they are weakly entangled and their QCPs are often interrupted by competing phases or first order phase transitions. Here, we provide compelling evidence that the stoichiometric heavy fermion ferromagnet CeRh$_6$Ge$_4$ becomes a strange metal at a pressure-induced QCP: specific heat and resistivity measurements demonstrate that the FM transition is continuously suppressed to zero temperature revealing a strange metal phase. We argue that strong magnetic anisotropy plays a key role in this process,injecting entanglement, in the form of triplet resonating valence bonds (tRVBs) into the ordered ferromagnet. We show that the singular transformation from tRVBs into Kondo singlets that occurs at the QCP causes a jump in the Fermi surface volume: a key driver of strange metallic behavior. Our results open up a new direction for research into FM quantum criticality, while also establishing an important new setting for the strange metal problem. Most importantly, strange metallic behavior at a FM quantum critical point suggests that it is quantum entanglement rather than the destruction of antiferromagnetism that is the common driver of the many varied examples of strange metallic behavior.

cond-mat.str-el↗

arXiv2018

Structural and magnetic properties of CeZnAl$_3$ single crystals

We have synthesized single crystals of CeZnAl$_3$, which is a new member of the family of the Ce-based intermetallics Ce$TX_3$ ($T$ = transition metal, $X$= Si, Ge, Al), crystallizing in the non-centrosymmetric tetragonal BaNiSn$_3$-type structure. Magnetization, specific heat and resistivity measurements all show that CeZnAl$_3$ orders magnetically below around 4.4 K. Furthermore, magnetization measurements exhibit a hysteresis loop at low temperatures and fields, indicating the presence of a ferromagnetic component in the magnetic state. This points to a different nature of the magnetism in CeZnAl$_3$ compared to the other isostructural Ce$T$Al$_3$ compounds. Resistivity measurements under pressures up to 1.8 GPa show a moderate suppression of the ordering temperature with pressure, suggesting that measurements to higher pressures are required to look for quantum critical behavior.

cond-mat.str-el↗

arXiv2017

Enhancement of the effective mass at high magnetic fields in CeRhIn$_5$

The Kondo-lattice compound CeRhIn$_5$ displays a field-induced Fermi surface reconstruction at $B^*\approx30$ T, which occurs within the antiferromagnetic state, prior to the quantum critical point at $B_{c0}\approx50$ T. Here, in order to investigate the nature of the Fermi surface change, we measured the magnetostriction, specific heat, and magnetic torque of CeRhIn$_5$ across a wide range of magnetic fields. Our observations uncover the field-induced itineracy of the $4f$ electrons, where above $B_{\rm onset}\approx17$ T there is a significant enhancement of the Sommerfeld coefficient, and spin-dependent effective cyclotron masses determined from quantum oscillations. Upon crossing $B_{\rm onset}$, the temperature dependence of the specific heat also shows distinctly different behavior from that at low fields. Our results indicate that the Kondo coupling is remarkably robust upon increasing the magnetic field. This is ascribed to the delocalization of the $4f$ electrons at the Fermi surface reconstruction at $B^*$.

cond-mat.str-el↗

arXiv2017

Antiferromagnetism with divalent Eu in EuNi$_5$As$_3$

We have successfully synthesized single crystals of EuNi$_5$As$_3$ using a flux method and we present a comprehensive study of the physical properties using magnetic susceptibility, specific heat, electrical resistivity, thermoelectric power and x-ray absorption spectroscopy (XAS) measurements. EuNi$_5$As$_3$ undergoes two close antiferromagnetic transitions at respective temperatures of $T_{N1}$ = 7.2 K and $T_{N2}$ = 6.4 K, which are associated with the Eu$^{2+}$ moments. Both transitions are suppressed upon applying a field and we map the temperature-field phase diagrams for fields applied parallel and perpendicular to the easy $a$ axis. XAS measurements reveal that the Eu is strongly divalent, with very little temperature dependence, indicating the localized Eu$^{2+}$ nature of EuNi$_5$As$_3$, with a lack of evidence for heavy fermion behavior.

cond-mat.str-el↗

arXiv2013

Pressure phase diagram and quantum criticality of CePt2In7 single crystals

We report the temperature-pressure (T-P) phase diagram of CePt2In7 single crystals, especially the pressure evolution of the antiferromagnetic order and the emergence of superconductivity, which have been studied by electrical resistivity and ac calorimetry under nearly hydrostatic environments. Compared with its polycrystalline counterpart, bulk superconductivity coexists with antiferromagnetism in a much narrower pressure region. The possible existence of textured superconductivity and local quantum criticality also are observed in CePt2In7, exhibiting a remarkable similarity with CeRhIn5.

cond-mat.str-el↗

arXiv2011

Heat-Capacity Measurements of Energy-Gap Nodes of the Heavy-Fermion Superconductor CeIrIn5 Deep inside the Pressure-Dependent Dome Structure of its Superconducting Phase Diagram

We use heat capacity measurements as a function of field rotation to identify the nodal gap structure of CeIrIn5 at pressures to 2.05 GPa, deep inside its superconducting dome. A four-fold oscillation in the heat capacity at 0.3 K is observed for all pressures but with its sign reversed between 1.50 and 0.90 GPa. On the basis of recent theoretical models for the field-angle dependent specific heat, all data, including the sign reversal, imply a d{x^2-y^2} order parameter with nodes along [110], which constrains theoretical models of the pairing mechanism in CeIrIn5.

cond-mat.supr-con↗

arXiv2009

Presure-Induced Superconducting State of Antiferromagnetic CaFe$_2$As$_2$

The antiferromagnet CaFe$_2$As$_2$ does not become superconducting when subject to ideal hydrostatic pressure conditions, where crystallographic and magnetic states also are well defined. By measuring electrical resistivity and magnetic susceptibility under quasi-hydrostatic pressure, however, we find that a substantial volume fraction of the sample is superconducting in a narrow pressure range where collapsed tetragonal and orthorhombic structures coexist. At higher pressures, the collapsed tetragonal structure is stabilized, with the boundary between this structure and the phase of coexisting structures strongly dependent on pressure history. Fluctuations in magnetic degrees of freedom in the phase of coexisting structures appear to be important for superconductivity.

cond-mat.supr-con↗

arXiv2008

Pressure-induced superconductivity in single crystal CaFe2As2

We report pressure-induced superconductivity in a single crystal of CaFe2As2. At atmospheric pressure, this material is antiferromagnetic below 170 K but under an applied pressure of 0.69 GPa becomes superconducting, with a transition temperature Tc exceeding 10 K. The rate of Tc suppression with applied magnetic field is -0.7 K/T, giving an extrapolated zero-temperature upper critical field of 10-14T.

cond-mat.supr-con↗

arXiv2006

Pressure-tuned First-order Phase Transition and Accompanying Resistivity Anomaly in CeZn_{1-δ}Sb_{2}

The Kondo lattice system CeZn_{0.66}Sb_{2} is studied by the electrical resistivity and ac magnetic susceptibility measurements at several pressures. At P=0 kbar, ferromagnetic and antiferromagnetic transitions appear at 3.6 and 0.8 K, respectively. The electrical resistivity at T_N dramatically changes from the Fisher-Langer type (ferromagnetic like) to the Suzaki-Mori type near 17 kbar, i.e., from a positive divergence to a negative divergence in the temperature derivative of the resistivity. The pressure-induced SM type anomaly, which shows thermal hysteresis, is easily suppressed by small magnetic field (1.9 kOe for 19.8 kbar), indicating a weakly first-order nature of the transition. By subtracting a low-pressure data set, we directly compare the resistivity anomaly with the SM theory without any assumption on backgrounds, where the negative divergence in dρ/dT is ascribed to enhanced critical fluctuations in the presence of superzone gaps.

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