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Hans Huebl

Publications and source records attributed to Hans Huebl.

At least 19 recordsLinked to original sources

Nonreciprocal Magnon Hanle Effect in Antiferromagnetic $\alpha$-Fe$_2$O$_3$

The precession of the magnon pseudospin about the equilibrium pseudofield, the latter capturing the nature of magnonic eigenexcitations in an antiferromagnet, gives rise to the magnon Hanle effect. Its realization via electrically injected and detected spin transport in an antiferromagnetic insulator demonstrates its high potential for devices and as a convenient probe for magnon eigenmodes and the underlying spin interactions in the antiferromagnet. Here, we observe a non-reciprocity in the Hanle signal measured in alpha-Fe2O3 using two spatially separated Pt electrodes as spin injector and detector. Interchanging their roles alters the detected magnon spin signal. The recorded difference depends on the applied magnetic field and reverses sign when the signal passes its nominal maximum at the so-called compensation field. Our findings unlock the high potential of antiferromagnetic magnonics towards the realization of electronics-inspired phenomena.

cond-mat.mes-hall

Spin Hall Magnetoresistance in Antiferromagnetic Insulators

Antiferromagnetic materials promise improved performance for spintronic applications, as they are robust against external magnetic field perturbations and allow for faster magnetization dynamics compared to ferromagnets. The direct observation of the antiferromagnetic state, however, is challenging due to the absence of a macroscopic magnetization. We show that the spin Hall magnetoresistance (SMR) is a versatile tool to probe the antiferromagnetic spin structure via simple electrical transport experiments by investigating the easy-plane antiferromagnetic insulators alpha-Fe2O3 (hematite) and NiO in bilayer heterostructures with a Pt heavy-metal top electrode. While rotating an external magnetic field in three orthogonal planes, we record the longitudinal and the transverse resistivities of Pt and observe characteristic resistivity modulations consistent with the SMR effect. We analyze both their amplitude and phase and compare the data to the results from a prototypical collinear ferrimagnetic Y3Fe5O12/Pt bilayer. The observed magnetic field dependence is explained in a comprehensive model, based on two magnetic sublattices and taking into account magnetic field-induced modifications of the domain structure. Our results show that the SMR effect allows to readout the spin configuration and to investigate magnetoelastic effects in antiferromagnetic multi-domain materials. We demonstrate that the SMR amplitude scales with the sum of the absolute sublattice magnetizations in ferrimagnetic and antiferromagnetic materials. In alpha-Fe2O3/Pt bilayers, we find an unexpectedly large SMR amplitude of 2.5E-3, twice as high as for prototype Y3Fe5O12/Pt bilayers, making the system particularly interesting for room-temperature antiferromagnetic spintronic applications.

cond-mat.mtrl-sci

Niobium Titanium Nitride as a High Tensile Stress Material for Nanomechanics

Over the past decades, high-coherence mechanical resonators have been continuously pushed to new limits, using techniques such as dissipation dilution and clamp-tapering to enhance their quality factor beyond intrinsic material limitations. Today, these mechanical resonators are often fabricated from silicon-nitride, silicon-carbide or aluminum. Recently, however, interest in novel material platforms has grown, especially those allowing for the integration within superconducting circuits. Among these, superconducting nitrides stand out as particularly promising due to their high transition temperatures compared to elementary superconductors. Here, we introduce them as nanomechanical resonators and report on the fabrication and characterization of highly stressed, doubly clamped niobium titanium nitride (NbTiN) nanostring resonators. Using optical interferometry, we determine the elastic properties and mechanical quality factor from room temperature to 13 K. We observe high tensile stress up to 0.81 GPa along with a Young's modulus of 181 GPa and an intrinsic mechanical quality factor up to 850. With these favorable mechanical properties, NbTiN constitutes a promising material platform for future applications in cavity electro- and nanomechanics.

quant-ph

Second-Harmonic Imaging of Magnetic Domains in Thin Film Hematite

Hematite is an antiferromagnetic oxide and candidate altermagnetic insulator whose N\'eel order reorients from an easy-axis to an easy-plane phase at the Morin transition. Interpreting altermagnetic transport and symmetry sensitive optical responses requires knowledge of the N\'eel vector orientation relative to the crystal axes and of the domain structure within the probed device. Here, we show that polarization-resolved second-harmonic generation (SHG) microscopy resolves magnetic symmetry and domains in epitaxial (0001)-oriented hematite films. Across the Morin temperature, the SHG polarization anisotropy evolves from an approximately sixfold pattern consistent with the easy-axis orientation to pronounced twofold patterns consistent with the easy-plane orientation. A symmetry analysis based on magnetic-dipole and electric-quadrupole contributions reproduces this evolution. Importantly, the interference between SHG amplitudes that are odd and even under reversal of the magnetic order renders opposite N\'eel-vector orientations optically distinguishable. Consistently, opposite directions of an applied in-plane magnetic field produce distinct SHG responses in our experiments. Using this magnetic contrast, we image micrometer-scale domains, their reorganization across the Morin transition, and their reconfiguration under magnetic and thermal cycling, including a remanent change after cycling through the spin-flop transition. These results establish SHG microscopy as a local probe of magnetic symmetry, N\'eel-vector orientation, and domain evolution in hematite films.

cond-mat.mtrl-sci

GHz non-reciprocal optical conductivity in hematite ($\alpha$-$\text{Fe}_2\text{O}_3$)

We study the non-reciprocal properties of the iron oxide $\alpha$-Fe$_2$O$_3$ (hematite) in the canted easy-plane antiferromagnetic phase, specifically in the GHz to THz frequency range. First, using the the microscopic spin Hamiltonian, we obtain the correct classical ground state where the canting is induced by the Dzyaloshinskii-Moriya interactions (DMI). The magnon spectrum is simulated using linear spin wave theory. We then compute the polarizability and the sub-gap optical conductivities using linear response. We find that the conductivity tensor contains frequency peaks at the zero momentum magnon gaps of order $0.1~$meV which can be tuned by the DMI and on-site anisotropic spin interactions. Furthermore, we show that the canting-induced net magnetic moment $\mathbf{m}$ represents a measure for the effective time-reversal-symmetry breaking and non-reciprocity of the system: a finite $\mathbf{m}$ results in a non-zero Hall conductivity. Finally, we discuss the prospective application of hematite in non-reciprocal circulator design, by computing the non-reciprocal circulator transmission amplitude using the conductivities as input.

cond-mat.str-el

Temperature dependence of the magnon-phonon coupling in yttrium iron garnet/gadolinium gallium garnet high overtone bulk acoustic resonators

Weexperimentally study the temperature dependence of the magnon-phonon coupling in a yttrium iron garnet (YIG)/gadolinium gallium garnet (GGG) heterostructure. More specifically, we use broadband ferromagnetic resonance to investigate the magneto-elastic coupling between the Kittel mode of a YIG thin film and the transverse acoustic phonon modes of the YIG/GGG high overtone bulk acoustic wave acoustic resonator for in and out-of-plane field directions in the temperature range between T = 5K and 300K. We find that for a magnetic field applied normal to the film surface, magneto-elastic coupling decreases with decreasing temperature, whereas it increases for the in-plane magnetic field configuration. The observed temperature dependence differs from earlier observations on bulk YIG samples, which might be due to the temperature dependent stress imposed by the GGG substrate.

cond-mat.mtrl-sci

On-chip Dicke-type magnon polaritons in the ultrastrong coupling regime via spatially separated nanomagnets

Quantum electrodynamics lies at the heart of hybrid quantum systems essential for future technologies. The thermodynamic limit of the Dicke model, a fundamental model describing these systems, predicts exotic quantum phenomena, such as equilibrium superradiant phase transitions and ground-state two-mode squeezing. However, the experimental realization of genuine Dicke systems has remained elusive due to the inevitable existence of gauge-invariant self-interaction terms that hinder such phenomena. Here, we report on the on-chip realization of a Dicke-type system utilizing ultrastrong magnetic-dipole interactions between collective excitations in a spatially separated ferromagnetic array and a superconducting resonator, resulting in creation of magnon polaritons. Crucially, this spatially separated architecture allows the cooperative enhancement of the coupling strength without increasing the self-interaction energy. We experimentally confirm the Bloch-Siegert shift, originating from the counter-rotating terms, alongside the suppression of self-excitation terms required to observe critical Dicke physics. Our results establish a versatile platform, which provides the playground to explore quantum collective coupling physics and open pathways towards integrated quantum devices harnessing Dicke physics.

quant-ph

Practical quantum tokens: challenges and perspectives

The concept of quantum tokens dates back alongside quantum cryptography to Stephen Wiesner's seminal work in 1983[1]. Already this initial work proposes society-relevant applications such as secure quantum banknotes, which can be exchanged between a bank and a customer. This quantum currency is based on various physical states that can be easily verified but is protected from being copied by the fundamental quantum laws. Four decades later, these ideas have flourished in the field of quantum information, and the concept of quantum banknotes has not only adopted many varying names, such as quantum money, quantum coins, quantum-digital payments, and quantum tokens, but also reached its first experimental demonstrations. In this perspective article, we discuss the current state-of-the-art of quantum tokens in the field of quantum information, as well as their future perspectives. We present a number of physical realizations of quantum tokens with integrated quantum memories and their applicability scenarios in detail. Finally, we discuss how quantum tokens fit into the information security ecosystem and consider their relationship to post-quantum cryptography.

quant-ph

Resolving Abrikosov vortex entry in superconducting nano-string resonators via displacement-noise spectroscopy in cavity-optomechanics

Abrikosov vortices in type-II superconductors critically influence current flow and coherence, thereby imposing fundamental limits on superconducting quantum technologies. Quantum circuits employ superconducting elements at micro- and mesoscopic scales, where individual vortices can significantly impact device performance, necessitating investigation of vortex entry, motion, and pinning in these constrained geometries. Cavity-optomechanical platforms combining flux-tunable microwave resonators with superconducting nanomechanical elements offer a promising route to the single-photon strong-coupling regime and enable highly sensitive probing of the mechanical degree of freedom under elevated magnetic fields. Here, we exploit this platform to investigate vortex entry processes at the single-event level. We observe discrete jumps of the mechanical resonance frequency attributable to individual vortex entry, corresponding to attonewton-scale forces and allowing quantitative extraction of single-vortex pinning energies. These signatures are superimposed on a smooth power-law background characteristic of the collective Campbell-regime of vortex elasticity. Our results establish optomechanics-inspired sensing as a powerful method for exploring fundamental superconducting properties and identifying decoherence pathways in quantum circuits. Beyond advancing vortex physics, this work opens new opportunities for integrating mechanical sensing into superconducting device architectures, bridging condensed matter physics and quantum information science.

cond-mat.mes-hall

Influence of Platinum Thin Films on the Photophysical and Quantum Properties of Near-Surface NV Centers

Nitrogen-vacancy (NV) centers in diamond are optically addressable spin defects with great potential for nanoscale quantum sensing. A key application of NV centers is the detection of external spins at the diamond surface. Among metals, platinum thin films - widely used in spintronics, catalysis and electrochemistry - provide a particularly interesting system for such studies. However, the interaction between NV centers and metals is known to affect their quantum sensing capabilities. In this work, we study five platinum-covered diamond samples containing shallow NVs created via nitrogen implantation with different energies (2.5-60 keV) and investigate the optical and quantum properties of NV ensembles beneath the metal films. We find a substantial reduction of the photoluminescence lifetime and a pronounced decrease of the NV$^{-}$ population for NV ensembles located near the platinum layer. As a result, optically detected magnetic resonance experiments could only be efficiently performed on diamonds implanted with at least 20 keV, where we observed a strong increase in the T$_{2}$ coherence time beneath the platinum thin films. Our study describes the various processes affecting NV centers near platinum films and provides guidance for the integration of thin metal films with near-surface NV centers.

cond-mat.mes-hall

Charge, heat, and spin transport phenomena in metallic conductors

In solid state materials, gradients of the electro-chemical potential, the temperature, or the spin-chemical potential drive the flow of charge, heat, and spin angular momentum, resulting in a net transport of energy. Beyond the primary transport processes - such as the flow of charge, heat, and spin angular momentum driven by gradients in their respective potentials - a wide range of coupled or cross-linked transport responses can occur, giving rise to a rich variety of transport phenomena. These transport phenomena are commonly categorized under (anomalous) thermoelectric, thermomagnetic, and galvanomagnetic effects, along with their spin-dependent counterparts. However, establishing a systematic classification and comparison among them remains a complex and nontrivial task. This paper attempts a didactic overview of the different transport phenomena, by categorizing and briefly discussing each of them based on charge, heat, and spin transport in conducting solids. The phenomena are structured in three categories: collinear, transverse, and so-called `planar' transport effects. The resulting overview attempts to categorize all effects in a consistent manner.

cond-mat.mtrl-sci

Theory of polarization-dependent phonon pumping in ferromagnetic/non-magnetic bilayers

We develop a theoretical model for polarization-selective phonon pumping induced by magnon-phonon coupling in a ferromagnetic/non-magnetic acoustic bilayer structure, focusing on the effects arising from a misalignment between the magnetic and crystallographic symmetry axes. Our model considers the coupled equations of motion describing uniform magnetization dynamics (the Kittel mode) and elastic waves in both layers, incorporating phonon pumping and boundary conditions at the interface. We show that even small misalignments lift the degeneracy of transverse shear elastic modes, resulting in phononic birefringence characterized by distinct propagation velocities for linearly polarized modes. Furthermore, our analysis reveals that magnon-phonon hybridization gives magnetic-field-dependent properties to otherwise non-magnetic phonons. We show that the polarization transfer between linearly polarized phonons and the circularly polarized Kittel mode can be tuned with an external magnetic field. Our theoretical results quantitatively reproduce recent experimental findings [1].

cond-mat.mes-hall

Broadband electron paramagnetic resonance spectroscopy of $^{167}$Er:$^{7}$LiYF$_4$ at mK temperatures

Rare-earth spin ensembles are a promising platform for microwave quantum memory applications due to their hyperfine transitions, which can exhibit exceptionally long coherence times when using an operation point with zero first-order Zeeman (ZEFOZ) shift. In this work, we use broadband electron paramagnetic resonance (EPR) spectroscopy on $^{167}$Er:$^{7}$LiYF$_4$ single crystals at sub-Kelvin temperatures. By fitting the spin Hamiltonian to the zero-field spectrum, we obtain refined parameters of the magnetic field-independent interactions, such as the hyperfine and quadrupole interaction. We also study the influence of the quadrupole interaction on the hyperfine splitting in the zero and low magnetic field range by analyzing EPR-spectra between 0 mT and 50 mT. Our findings highlight the broadband EPR spectroscopy approach as a powerful tool for the precise determination of the spin Hamiltonian parameters and for the characterization of hyperfine transitions in terms of their selection rules and linewidth.

quant-ph

Emergence of giant spin-orbit torque in a two-dimensional hole gas on the hydrogen-terminated diamond surface

Two-dimensional (2D) carrier systems exhibit various significant physical phenomena for electronics and spintronics, where one of the most promising traits is efficient spin-to-charge conversion stemming from their Rashba-type spin-orbit interaction. Meanwhile, a nuisance in quests of promising materials for spintronics application is that vast majority of the investigated platforms consists of rare and/or toxic elements, such as Pt and Te, which hinders progress of spin conversion physics in view of element strategy and green technology. Here, we show the emergence of giant spin-orbit torque driven by 2D hole gas at the surface of hydrogen-terminated diamond, where the constituent substances are ubiquitous elements, carbon and hydrogen. The index of its spin torque efficiency at room temperature is several times greater than that of rare metal, Pt, the benchmark system/element for spin-to-charge conversion. Our finding opens a new pathway for more sustainable spintronics and spin-orbitronics applications, with efficient spin-orbit torque employing ubiquitous non-toxic elements.

cond-mat.mes-hall

Remote sensing of a levitated superconductor with a flux-tunable microwave cavity

We present a cavity-electromechanical system comprising a superconducting quantum interference device which is embedded in a microwave resonator and coupled via a pick-up loop to a 6 $μ$g magnetically-levitated superconducting sphere. The motion of the sphere in the magnetic trap induces a frequency shift in the SQUID-cavity system. We use microwave spectroscopy to characterize the system, and we demonstrate that the electromechanical interaction is tunable. The measured displacement sensitivity of $10^{-7} \, \mathrm{m} / \sqrt{\mathrm{Hz}}$, defines a path towards ground-state cooling of levitated particles with Planck-scale masses at millikelvin environment temperatures.

quant-ph

Inductive magnon noise spectroscopy

State tomography allows to characterize quantum states, and was recently applied to reveal the dynamic magnetization state of a parametrically driven magnet. The identification of non-classical states, such as squeezed states, relies on a careful analysis of their emission and their distinction from thermal and vacuum fluctuations. A technique allowing to detect equilibrium magnetization fluctuations is a crucial first step in this regard. In this Letter, we show that inductive magnon noise spectroscopy (iMNS) allows to characterize the thermal magnetization fluctuations of a ferromagnetic thin film in a broadband coplanar waveguide-based scheme. Relative to a cold microwave background, the microwaves emitted by the equilibrium magnetization fluctuations can be detected via spectrum analysis. We provide a comprehensive picture of our microwave system by quantitatively modeling its response, including the thermalizing influence of the cables. The model allows for direct comparison to low-power broadband ferromagnetic resonance measurements with excellent agreement, corroborating the equilibrium character of the iMNS measurement by probing the linear response of the equilibrium state. Our work thus demonstrates broadband access to the equilibrium properties of magnetization fluctuations using a purely inductive approach.

cond-mat.mes-hall

Temperature dependence of the magnon-phonon interaction in high overtone bulk acoustic resonator-ferromagnetic thin film hybrids

Tailored magnon-phonon hybrid systems, where high overtone bulk acoustic resonators couple resonantly to the magnonic mode of a ferromagnetic thin film, are considered optimal for the creation of acoustic phonons with a defined circular polarization. This class of devices is therefore ideal for the investigation of phonon propagation properties and assessing their capacity to transport angular momentum in the classical and potentially even in the quantum regime. Here, we study the coupling between the magnons in a ferromagnetic \ch{Co25Fe75} thin film and the transverse acoustic phonons in a bulk acoustic wave resonators formed by the sapphire substrate onto which the film is deposited. Using broadband ferromagnetic resonance experiments as a function of temperature, we investigate the strength of the coherent magnon-phonon interaction and the individual damping rates of the magnons and phonons participating in the process. This demonstrates that this coupled magnon-phonon system can reach a cooperativity $C\approx 1$ at cryogenic temperatures. Our experiments also showcase the potential of strongly coupled magnon-phonon systems for strain sensing applications.

cond-mat.mes-hall

Electrically induced angular momentum flow between separated ferromagnets

Converting angular momentum between different degrees of freedom within a magnetic material results from a dynamic interplay between electrons, magnons and phonons. This interplay is pivotal to implementing spintronic device concepts that rely on spin angular momentum transport. We establish a new concept for long-range angular momentum transport that further allows to address and isolate the magnonic contribution to angular momentum transport in a nanostructured metallic ferromagnet. To this end, we electrically excite and detect spin transport between two parallel and electrically insulated ferromagnetic metal strips on top of a diamagnetic substrate. Charge-to-spin current conversion within the ferromagnetic strip generates electronic spin angular momentum that is transferred to magnons via electron-magnon coupling. We observe a finite angular momentum flow to the second ferromagnetic strip across a diamagnetic substrate over micron distances, which is electrically detected in the second strip by the inverse charge-to-spin current conversion process. We discuss phononic and dipolar interactions as the likely cause to transfer angular momentum between the two strips. Moreover, our work provides the experimental basis to separate the electronic and magnonic spin transport and thereby paves the way towards magnonic device concepts that do not rely on magnetic insulators.

cond-mat.mes-hall