arXiv subjects

Hans-Georg Babin

Publications and source records attributed to Hans-Georg Babin.

6 recordsLinked to original sources

arXiv2025

Optical and magnetic response by design in GaAs quantum dots

Quantum networking technologies use spin qubits and their interface to single photons as core components of a network node. This necessitates the ability to co-design the magnetic- and optical-dipole response of a quantum system. These properties are notoriously difficult to design in many solid-state systems, where spin-orbit coupling and the crystalline environment for each qubit create inhomogeneity of electronic g-factors and optically active states. Here, we show that GaAs quantum dots (QDs) obtained via the quasi-strain-free local droplet etching epitaxy growth method provide spin and optical properties predictable from assuming the highest possible QD symmetry. Our measurements of electron and hole g-tensors and of transition dipole moment orientations for charged excitons agree with our predictions from a multiband k.p simulation constrained only by a single atomic-force-microscopy reconstruction of QD morphology. This agreement is verified across multiple wavelength-specific growth runs at different facilities within the range of 730 nm to 790 nm for the exciton emission. Remarkably, our measurements and simulations track the in-plane electron g-factors through a zero-crossing from -0.1 to 0.3 and linear optical dipole moment orientations fully determined by an external magnetic field. The robustness of our results demonstrates the capability to design - prior to growth - the properties of a spin qubit and its tunable optical interface best adapted to a target magnetic and photonic environment with direct application for high-quality spin-photon entanglement.

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arXiv2025

Robust biexciton preparation for entangled photon-pair generation by single-shot Floquet driving

Quantum emitters driven by resonant two-photon excitation are a leading source for deterministically generated entangled photon pairs, essential for scalable photonic quantum technologies. However, conventional excitation schemes pose various constraints, limiting their scalability and practicability. Here, we demonstrate how biexciton preparation schemes with significantly improved robustness and reduced experimental demands can be identified using a novel design principle: ultrafast single-shot Floquet driving. This is achieved by employing two strongly and symmetrically detuned dichromatic pulses, whose superposition generates a stroboscopic Hamiltonian that enables direct coupling between ground and biexciton states. Moreover, a pulse delay serves as a tuning knob, introducing an effective magnetic field making biexciton preparation particularly robust. Experimentally, we achieve a biexciton occupation exceeding 96% and preserve photon-pair entanglement with a fidelity of 93.4%. Our work opens avenues for designing a class of quantum control protocols with superior performance across diverse quantum emitters and qubit platforms.

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arXiv2024

All-optical ultrafast arbitrary rotation of hole orbital qubits with direct phase control

Complete quantum control of a stationary quantum bit embedded in a quantum emitter is crucial for photonic quantum information technologies. Recently, the orbital degree of freedom in optically active quantum dots has emerged as a promising candidate. However, the essential ability to perform arbitrary rotations on orbital qubits remains elusive. Here, we demonstrate arbitrary rotation of a hole orbital qubit with direct phase control using picosecond optical pulses. This is achieved by successfully inducing stimulated Raman transitions within $Λ$ systems coupled via radiative Auger processes. The new capability enables direct control of polar and azimuth angles of the Bloch vector without requiring timed precession. Our results establish orbital states in solid-state quantum emitters as a viable resource for applications in high-speed quantum information processing.

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arXiv2024

Wavelength-tunable high-fidelity entangled photon sources enabled by dual Stark effects

The construction of a large-scale quantum internet requires quantum repeaters containing multiple entangled photon sources with identical wavelengths. Semiconductor quantum dots can generate entangled photon pairs deterministically with high fidelity. However, realizing wavelength-matched quantum-dot entangled photon sources faces two difficulties: the non-uniformity of emission wavelength and exciton fine-structure splitting induced fidelity reduction. Typically, these two factors are not independently tunable, making it challenging to achieve simultaneous improvement. In this work, we demonstrate wavelength-tunable entangled photon sources based on droplet-etched GaAs quantum dots through the combined use of AC and quantum-confined Stark effects. The emission wavelength can be tuned by ~1 meV while preserving an entanglement fidelity f exceeding 0.955(1) in the entire tuning range. Based on this hybrid tuning scheme, we finally demonstrate multiple wavelength-matched entangled photon sources with f>0.919(3), paving a way towards robust and scalable on-demand entangled photon sources for quantum internet and integrated quantum optical circuits.

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arXiv2023

Coherent control of a high-orbital hole in a semiconductor quantum dot

Coherently driven semiconductor quantum dots are one of the most promising platforms for non-classical light sources and quantum logic gates which form the foundation of photonic quantum technologies. However, to date, coherent manipulation of single charge carriers in quantum dots is limited mainly to their lowest orbital states. Ultrafast coherent control of high-orbital states is obstructed by the demand for tunable terahertz pulses. To break this constraint, we demonstrate an all-optical method to control high-orbital states of a hole via stimulated Auger process. The coherent nature of the Auger process is proved by Rabi oscillation and Ramsey interference. Harnessing this coherence further enables the investigation of single-hole relaxation mechanism. A hole relaxation time of 161 ps is observed and attributed to the phonon bottleneck effect. Our work opens new possibilities for understanding the fundamental properties of high-orbital states in quantum emitters and developing new types of orbital-based quantum photonic devices.

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arXiv2023

Enhanced Electron Spin Coherence in a GaAs Quantum Emitter

A spin-photon interface should operate with both coherent photons and a coherent spin to enable cluster-state generation and entanglement distribution. In high-quality devices, self-assembled GaAs quantum dots are near-perfect emitters of on-demand coherent photons. However, the spin rapidly decoheres via the magnetic noise arising from the host nuclei. Here, we address this drawback by implementing an all-optical nuclear-spin cooling scheme on a GaAs quantum dot. The electron-spin coherence time increases 156-fold from $T_2^*$ = 3.9 ns to 0.608 $μ$s. The cooling scheme depends on a non-collinear term in the hyperfine interaction. The results show that such a term is present even though the strain is low and no external stress is applied. Our work highlights the potential of optically-active GaAs quantum dots as fast, highly coherent spin-photon interfaces.

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