arXiv subjects

Hanyu Zhu

Publications and source records attributed to Hanyu Zhu.

At least 19 recordsLinked to original sources

arXiv2026

Ultrafast Magnetization Induced from Raman-Active Axial Chiral Phonons

Axial chiral phonons, which carry angular momentum and exhibit unusually large magnetic moments, provide a new degree of freedom for controlling the time-reversal symmetry and magnetic properties of quantum materials. While infrared-active axial phonons are efficiently excited to large amplitudes by circularly polarized terahertz pulses, their application may be constrained by short lifetimes, small penetration depths, low spatial resolution, and limited availability of optical sources. Here, we report that an axial Raman-active phonon mode in CeF3 exhibits a significant magnetic moment and an exceedingly long lifetime that more closely matches the paramagnetic spin dynamics. The axial phonon population is resonantly driven by a near-infrared laser pulse with rotating linear polarization, known as an optical centrifuge, a coherent control scheme never applied to solids before. The phonon-driven magnetization observed by time-resolved Faraday rotation scales quadratically with incident power and rapidly decreases at high temperatures, consistent with phonon inverse Faraday effect from many-body spin-phonon coupling. Our findings open a new avenue for using shaped laser pulses from widely accessible light sources to manipulate coherent axial chiral phonons and ultrafast spintronics.

cond-mat.mtrl-sci↗

arXiv2026

Measuring chiral phonons

Chiral phonons are quantized vibrations where the atomic motion in a solid breaks improper rotation symmetries. In many cases, chiral phonons possess angular momenta and are therefore selective to circularly polarized light. Both fundamental and applied research efforts on chiral phonons have been gaining increasing attention owing to their importance in a variety of fields including spintronics, spin-selective chemical reactions, thermal transport, quantum information processing and biosensing, where the bi-directional spin-lattice coupling enabled by chiral phonons can be harnessed in new ways, and potentially lead to new functionalities. Thus far, the studies of chiral phonons across diverse materials platforms have evolved largely independently within these fields, but the experimental techniques are often interrelated. In this perspective, we present a detailed description, as well as advantages and disadvantages of the current approaches for experimentally measuring chiral phonons in chiral and achiral materials. We conclude with a discussion of new methods for measuring chiral phonons. Ultimately, this work seeks to offer an experimental guide for systematically investigating the properties of chiral phonons in various materials systems and applications.

cond-mat.mtrl-sci↗

arXiv2026

Quantum Dot Moiré from Crossed MoS2 Nanoribbons

Twisted atomically thin layers have attracted much attention for Moiré potential and correlated quantum phenomena. However, existing Moiré superlattices have largely been limited to extensive wavefunction without lateral confinement. Here we introduce a new platform where 1D nanoribbons of 2D MoS2 grown by vapor deposition can be easily superposed at various angles from stacking and transferring, to form Moiré quantum dots at their intersections with unique exciton physics. Angle-dependent Moiré intersections show enhanced exciton emission at commensurate angle 22 deg, which demonstrates faster relaxation at the cryogenic temperature. A size-dependent study further exhibits a reduced exciton energy and soften out-of-plane interlayer coupling for smaller Moiré areas. Our results reveal exciton physics turnability via precise overlapping of 1D nanoribbons.

cond-mat.mtrl-sci↗

arXiv2026

Optical Signature of Moiré Superlattices Formed by Twisted SrTiO$_3$ Membranes

Moiré superlattices formed at the interfaces of mismatched lattices have attracted significant interest over the past decade due to their large tunability of band parameters and interactions among electrons, spins, and lattices. Superlattices made from twisted perovskite oxides may have strong structure and potential modulation, but evidence of such modulation over macroscopic areas, particularly at large twisting angles, has not been clearly demonstrated so far. Here, we fabricated millimeter-scale twisted oxide bilayers at $36^\circ$ angle, close to the simple coincidence site lattice condition $\Sigma5$, from freestanding SrTiO$_3$ membranes. We discovered new low-frequency vibrational modes whose Raman activity, according to molecular dynamics simulations, is greatly enhanced by an asymmetric, twisted interface between the SrO and TiO$_2$ layers. Such an interface is energetically favorable from first-principles calculations and is corroborated by the observation of strong second harmonic generation from the interface comparable to that from the SrTiO$_3$ surface throughout the bilayer region. The results are consistent with interlayer coupling enhanced by high-temperature annealing and confirmed by cross-sectional scanning transmission electron microscopy imaging. Our work sheds light on the structural behavior of twisted oxides and provides directions for tuning their phononic and nonlinear optical properties in future studies.

cond-mat.mtrl-sci↗

arXiv2026

MAG-VLAQ: Multi-modal Aerial-Ground Query Aggregation for Cross-View Place Recognition

Multi-modal cross-view place recognition remains a fundamental challenge in computer vision and robotics due to the severe viewpoint, modality, and spatial-structure discrepancies between ground observations and aerial references. To address this challenge, we present MAG-VLAQ, a foundation-model-enhanced query aggregation framework for multi-modal aerial-ground cross-view place recognition. Specifically, our approach leverages pre-trained foundation models to extract dense visual tokens from both ground and aerial images, as well as expressive geometric tokens from ground LiDAR observations. These heterogeneous tokens are then projected into a shared embedding space for cross-modal alignment and fusion. As our main contribution, we propose ODE-conditioned VLAQ, which tightly couples neural ordinary differential equations (ODE)-based RGB-LiDAR fusion with vectors of locally aggregated queries (VLAQ). In this design, the VLAQ query centers are dynamically adapted according to the fused multi-modal state. This mechanism allows the final global descriptor to preserve globally learned retrieval prototypes while remaining responsive to scene-specific visual and geometric evidence, significantly improving aerial-ground matching. Extensive experiments on KITTI360-AG and nuScenes-AG validate the effectiveness of our proposed MAG-VLAQ. Notably, on KITTI360-AG, our MAG-VLAQ nearly doubles the state-of-the-art performance, achieving 61.1 Recall@1 in the satellite setting, compared with 34.5 from the closest competing approach.

cs.CV↗

arXiv2026

Chip-Scale Aligned Chiral Carbon Nanotubes Exhibiting Giant Second Harmonic Generation

Chiral carbon nanotubes (CNTs) are direct-gap semiconductors with optical properties governed by one-dimensional excitons with enormous oscillator strengths. Each species of chiral CNTs has an enantiomeric pair of left- and right-handed CNTs with nearly identical properties, but enantiomer-dependent phenomena can emerge, especially in nonlinear optical processes. Theoretical studies have predicted strong second-order nonlinearities in chiral CNTs, but no experimental quantitative verification has been reported due to the lack of macroscopically ordered assemblies of single-enantiomer chiral CNTs. Here, we report the synthesis of centimeter-scale, densely packed, aligned single-enantiomer chiral CNT films that are microfabrication-compatible. We observe giant second harmonic generation (SHG) emission from the chiral CNT film, which originates from the intrinsic chirality and inversion symmetry breaking of the atomic structure of chiral CNTs. The observed nonlinear susceptibility of the as-fabricated film reaches $4.9\times 10^2$\,pm/V at a pump wavelength of 1030\,nm, corresponding to the lowest-energy excitonic resonance, indicating $χ_{xyz} = 1.6\times 10^3$\,pm/V for a perfectly aligned CNT crystal. Our calculations based on many-body theory correctly estimate the spectrum and magnitude of such excitonically enhanced optical nonlinearity. These results are promising for the development of scalable chiral-CNT electronics and nonlinear photonics.

physics.app-ph↗

arXiv2026

A Wearable ECG Device for Differentiating Hypertrophic Cardiomyopathy from Acquired Left Ventricular Hypertrophy

Hypertrophic Cardiomyopathy (HCM) is a genetic heart disease affecting approximately 1 in 500 people and is the leading cause of sudden cardiac death in young athletes. Current diagnostic methods -- cardiovascular magnetic resonance (CMR), echocardiography, and genetic testing -- are limited by high costs, operator dependency, or insufficient accuracy, while standard electrocardiogram (ECG) analysis cannot reliably distinguish HCM from acquired left ventricular hypertrophy (LVH). This paper presents a wearable ECG device paired with a classification algorithm that differentiates HCM from acquired LVH using ECG signals alone. The portable device integrates a 3-lead electrode system, an AD8232 signal conditioning module, an Arduino Nano 33 BLE microcontroller, and a lithium polymer battery. The algorithm extracts two quantitative indices -- HCM Index~1 and HCM Index~2 -- from each heartbeat and classifies patients via dual statistical thresholds. Validation on 483 LVH patients (PhysioNet) and 29 HCM patients (digitized clinical records) yields 75.86\% sensitivity, 99.17\% specificity, and an F1-score of 80.00\%. Leave-one-out cross-validation confirms generalizability, with cross-validated sensitivity of 72.41\%, specificity of 98.96\%, and F1-score of 76.36\% (95\% confidence intervals reported). A digitization confound analysis demonstrates that the classification is driven by physiological cardiac features rather than data source artifacts. A simulated device acquisition chain analysis confirms that the wearable hardware's signal characteristics are compatible with the classification algorithm. The system offers a promising tool for affordable HCM screening in resource-limited settings.

eess.IV↗

arXiv2026

Dicke materials as a resource for quantum squeezing

We study magnetic materials whose low energy physics can be effectively described by a Dicke model, which we term Dicke materials. We show how a Dicke model emerges in such materials due to a coexistence of fast-dispersing and slow-dispersing spins, which are strongly coupled. Analogous to the paradigmatic Dicke model describing light-matter interactions, these materials also exhibit signatures of a superradiant phase transition. The ground state near the superradiant phase transition is expected to be squeezed, making Dicke materials a resource for quantum metrology and witnessing entanglement in solid-state systems. However, as an entanglement measure, squeezing can be sensitive to perturbations that are otherwise irrelevant for usual correlation functions and order parameters. Motivated by the prospect of observing squeezing in such Dicke materials, we study the robustness of ground state squeezing under ubiquitous imperfections such as finite temperature, disorder, and local interactions. Using analytical and numerical techniques, we show that the squeezing obtained is perturbatively stable against these imperfections and quantitatively evaluate regimes promising for experimental observation.

quant-ph↗

arXiv2026

Exceptional Optical Phonon Coherence in Enriched Cubic Boron Arsenide via Suppression of Three-Phonon Scattering

Cubic boron arsenide (BAs) is a promising semiconductor for next-generation electronics due to its outstanding ambipolar mobility and thermal conductivity, the latter of which is attributed to the suppression of three-phonon scattering. However, precisely accounting for different high-order anharmonic scattering processes is challenging from both theory and experiment, so that questions remain open regarding the ultimate limit of phonon lifetime and thermal conductivity in BAs. Here we show that this gap nearly eliminates three-phonon scattering for zone-center optical phonons in a wide temperature range, leading to a record-high, isotope purity-limited phonon coherence with a quality factor above $3.7\times 10^3$ for >98% enriched $^{11}$BAs below 100 K. We discriminate three decoherence mechanisms by their temperature-dependent contribution to the damping rate using high-resolution Raman and Fourier transform infrared spectroscopy. For the as-synthesized crystals, we find that defect scattering has negligible contributions to the linewidth of optical phonons in comparison to isotope scattering. These results provide critical insights into the intrinsic and extrinsic scattering mechanisms of optical phonons in BAs, motivating further studies to quantify anharmonic effects and realize superior phonon transport.

cond-mat.mtrl-sci↗

arXiv2026

DC-VLAQ: Query-Residual Aggregation for Robust Visual Place Recognition

One of the central challenges in visual place recognition (VPR) is learning a robust global representation that remains discriminative under large viewpoint changes, illumination variations, and severe domain shifts. While visual foundation models (VFMs) provide strong local features, most existing methods rely on a single model, overlooking the complementary cues offered by different VFMs. However, exploiting such complementary information inevitably alters token distributions, which challenges the stability of existing query-based global aggregation schemes. To address these challenges, we propose DC-VLAQ, a representation-centric framework that integrates the fusion of complementary VFMs and robust global aggregation. Specifically, we first introduce a lightweight residual-guided complementary fusion that anchors representations in the DINOv2 feature space while injecting complementary semantics from CLIP through a learned residual correction. In addition, we propose the Vector of Local Aggregated Queries (VLAQ), a query--residual global aggregation scheme that encodes local tokens by their residual responses to learnable queries, resulting in improved stability and the preservation of fine-grained discriminative cues. Extensive experiments on standard VPR benchmarks, including Pitts30k, Tokyo24/7, MSLS, Nordland, SPED, and AmsterTime, demonstrate that DC-VLAQ consistently outperforms strong baselines and achieves state-of-the-art performance, particularly under challenging domain shifts and long-term appearance changes.

cs.CV↗

arXiv2026

NeuroGenPoisoning: Neuron-Guided Attacks on Retrieval-Augmented Generation of LLM via Genetic Optimization of External Knowledge

Retrieval-Augmented Generation (RAG) empowers Large Language Models (LLMs) to dynamically integrate external knowledge during inference, improving their factual accuracy and adaptability. However, adversaries can inject poisoned external knowledge to override the model's internal memory. While existing attacks iteratively manipulate retrieval content or prompt structure of RAG, they largely ignore the model's internal representation dynamics and neuron-level sensitivities. The underlying mechanism of RAG poisoning has not been fully studied and the effect of knowledge conflict with strong parametric knowledge in RAG is not considered. In this work, we propose NeuroGenPoisoning, a novel attack framework that generates adversarial external knowledge in RAG guided by LLM internal neuron attribution and genetic optimization. Our method first identifies a set of Poison-Responsive Neurons whose activation strongly correlates with contextual poisoning knowledge. We then employ a genetic algorithm to evolve adversarial passages that maximally activate these neurons. Crucially, our framework enables massive-scale generation of effective poisoned RAG knowledge by identifying and reusing promising but initially unsuccessful external knowledge variants via observed attribution signals. At the same time, Poison-Responsive Neurons guided poisoning can effectively resolves knowledge conflict. Experimental results across models and datasets demonstrate consistently achieving high Population Overwrite Success Rate (POSR) of over 90% while preserving fluency. Empirical evidence shows that our method effectively resolves knowledge conflict.

cs.AI↗

arXiv2025

Lattice-induced spin dynamics in Dirac magnet CoTiO3

Spin-lattice coupling is crucial for understanding the spin transport and dynamics for spintronics and magnonics applications. Recently, cobalt titanate (CoTiO3), an easy-plane antiferromagnet, has been found to host axial phonons with a large magnetic moment, which may originate from spin-lattice coupling. Here, we investigate the effect of light-driven lattice dynamics on the magnetic properties of CoTiO3 using time-resolved spectroscopy with a THz pump and a magneto-optic probe. We found resonantly driven Raman active phonons, phonon-polariton-induced excitation of the antiferromagnetic magnons, and a slow increase in the polarization rotation of the probe, all indicating symmetry breaking that is not intrinsic to the magnetic space group. The temperature dependence confirmed that the observed spin dynamics is related to the magnetic order, and we suggest surface effects as a possible mechanism. Our results of THz-induced spin-lattice dynamics signify that extrinsic symmetry breaking may contribute strongly and unexpectedly to light-driven phenomena in bulk complex oxides.

cond-mat.mtrl-sci↗

arXiv2025

Quantum Vacuum in Matter

An intriguing consequence of quantum field theory is that vacuum is not empty space; it is full of quantum fluctuating electromagnetic fields, or virtual photons, corresponding to their zero-point energy, even though the average number of photons is zero. These short-lived vacuum fluctuations are behind some of the most fascinating physical processes in the universe, including spontaneous emission, the Lamb shift, and the Casimir force. Recent theory and experiments indicate that the properties of materials placed in photonic cavities may be altered, even in the complete absence of any external fields, through interaction with the fluctuating vacuum electromagnetic fields. Judicious engineering of the quantum vacuum surrounding the matter inside a cavity can lead to significant and nonintuitive modifications of electronic and vibrational states, producing a ``vacuum dressed'' material. These exciting new ideas have stimulated discussions regarding the fundamental physics of vacuum-matter interactions and also broadened the scope of potential applications using zero-point fluctuations to engineer materials. This Perspective will first discuss recent experimental and theoretical developments on vacuum-modified condensed matter systems, which usually require the realization of the so-called ultrastrong light-matter coupling regime. Then, we will overview some of the most promising cavity designs for enhancing vacuum electromagnetic fields in materials with various energy scales. Finally, we will discuss urgent open questions and technical challenges to be solved in this emerging field.

quant-ph↗

arXiv2025

Unconventional Temperature Dependence of Exciton Diamagnetism in 2D Ruddlesden-Popper Lead Halide Perovskites

Layered hybrid perovskites containing larger organic cations have demonstrated superior environmental stability, but the presence of these insulating spacers also strengthens the exciton binding energy, which contributes to reduced carrier separation. The consequences of increased binding energy on device efficiency are still not fully documented, and binding energy measurements are often conducted at cryogenic temperatures where linewidths are decreased and a series of hydrogen-like bound states can be identified, but not under ambient conditions where devices are expected to operate. In contrast to the quenching observed in 3D perovskites such as methylammonium lead iodide, where exciton binding energies are thought to decrease at higher temperatures, we present evidence for a smaller excitonic radius at higher temperatures in the $n=5$ member of butylammonium-spaced methylammonium lead iodide, (BA)$_2$(MA)$_{n-1}$Pb$_n$I$_{3n+1}$. We measured the temperature-dependent diamagnetic shift coefficient in magnetic fields up to 40\,T, which is one-third as large at room temperature as those at cryogenic temperatures. In both the ideal 2D and 3D hydrogen models, this trend would indicate that the exciton binding energy more than triples at room temperature.

cond-mat.mtrl-sci↗

arXiv2024

Angle-resolved photoemission spectroscopy with an $\textit{in situ}$ tunable magnetic field

Angle-resolved photoemission spectroscopy (ARPES) is a powerful tool for probing the momentum-resolved single-particle spectral function of materials. Historically, $\textit{in situ}$ magnetic fields have been carefully avoided as they are detrimental to the control of photoelectron trajectory during the photoelectron detection process. However, magnetic field is an important experimental knob for both probing and tuning symmetry-breaking phases and electronic topology in quantum materials. In this paper, we introduce an easily implementable method for realizing an $\textit{in situ}$ tunable magnetic field at the sample position in an ARPES experiment and analyze magnetic field induced artifacts in ARPES data. Specifically, we identified and quantified three distinct extrinsic effects of a magnetic field: Fermi surface rotation, momentum shrinking, and momentum broadening. We examined these effects in three prototypical quantum materials, i.e., a topological insulator (Bi$_2$Se$_3$), an iron-based superconductor (LiFeAs), and a cuprate superconductor (Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$), and demonstrate the feasibility of ARPES measurements in the presence of a controllable magnetic field. Our studies lay the foundation for the future development of the technique and interpretation of ARPES measurements of field-tunable quantum phases.

cond-mat.str-el↗

arXiv2024

Challenges and Opportunities in Searching for Rashba-Dresselhaus Materials for Efficient Spin-Charge Interconversion at Room Temperature

Spintronic logic devices require efficient spin-charge interconversion: converting charge current to spin current and spin current to charge current. In spin-orbit materials that are regarded as the most promising candidate for spintronic logic devices, one mechanism that is responsible for spin-charge interconversion is Edelstein and inverse Edelstein effects based on spin-momentum locking in materials with Rashba-type spin-orbit coupling. Over last decade, there has been rapid progresses for increasing interconversion efficiencies due to the Edelstein effect in a few Rashba-Dresselhaus materials and topological insulators, making Rashba spin-momentum locking a promising technological solution for spin-orbit logic devices. However, despite the rapid progress that leads to high spin-charge interconversion efficiency at cryogenic temperatures, the room-temperature efficiency needed for technological applications is still low. This paper presents our understanding on the challenges and opportunities in searching for Rashba-Dresselhaus materials for efficient spin-charge interconversion at room temperature by focusing on materials properties such as Rashba coefficients, momentum relaxation times, spin-momentum locking relations and electrical conductivities.

cond-mat.mtrl-sci↗

arXiv2023

Non-linear optics at twist interfaces in h-BN/SiC heterostructures

Understanding the emergent electronic structure in twisted atomically thin layers has led to the exciting field of twistronics. However, practical applications of such systems are challenging since the specific angular correlations between the layers must be precisely controlled and the layers have to be single crystalline with uniform atomic ordering. Here, we suggest an alternative, simple and scalable approach where nanocrystalline two-dimensional (2D) film on three-dimensional (3D) substrates yield twisted-interface-dependent properties. Ultrawide-bandgap hexagonal boron nitride (h-BN) thin films are directly grown on high in-plane lattice mismatched wide-bandgap silicon carbide (4H-SiC) substrates to explore the twist-dependent structure-property correlations. Concurrently, nanocrystalline h-BN thin film shows strong non-linear second-harmonic generation and ultra-low cross-plane thermal conductivity at room temperature, which are attributed to the twisted domain edges between van der Waals stacked nanocrystals with random in-plane orientations. First-principles calculations based on time-dependent density functional theory manifest strong even-order optical nonlinearity in twisted h-BN layers. Our work unveils that directly deposited 2D nanocrystalline thin film on 3D substrates could provide easily accessible twist-interfaces, therefore enabling a simple and scalable approach to utilize the 2D-twistronics integrated in 3D material devices for next-generation nanotechnology.

cond-mat.mtrl-sci↗

arXiv2023

CVPR 2023 Text Guided Video Editing Competition

Humans watch more than a billion hours of video per day. Most of this video was edited manually, which is a tedious process. However, AI-enabled video-generation and video-editing is on the rise. Building on text-to-image models like Stable Diffusion and Imagen, generative AI has improved dramatically on video tasks. But it's hard to evaluate progress in these video tasks because there is no standard benchmark. So, we propose a new dataset for text-guided video editing (TGVE), and we run a competition at CVPR to evaluate models on our TGVE dataset. In this paper we present a retrospective on the competition and describe the winning method. The competition dataset is available at https://sites.google.com/view/loveucvpr23/track4.

cs.CV↗