arXiv subjects

Haochen Zhu

Publications and source records attributed to Haochen Zhu.

10 recordsLinked to original sources

arXiv2026

Composition design of refractory compositionally complex alloys using machine learning models

Refractory compositionally complex alloys (RCCAs) are considered the next generation high-temperature materials. However, their high-dimensional composition spaces are too large to explore by traditional density functional theory or experimental means, making new RCCA discovery slow and cumbersome. This work has addressed these challenges with an integrated composition design framework that can efficiently and exhaustively explore the relationship between the compositions and two fundamental aspects: 1) the phase stability, including the target body-centered cubic (BCC) phase and its competing phases (hexagonal closed-pack (HCP) structures, Laves and B2 intermetallic phases), and 2) the mechanical properties. This framework is demonstrated with RCCAs within nine refractory metals (Ti, V, Cr, Zr, Nb, Mo, Hf, Ta, and W). Theory-guided machine learning (ML) models were employed to find the composition-mechanical property relationship of RCCAs, where the established theory is used to supplement the yield strength data at ultra-high temperature, and a forward sequential feature selection (SFS) is used to determine feature selection. The resulting ML model for temperature-dependent yield strength was found to have an R_squared value of 0.98 over the entire temperature range (from 0 to 2000 K). The impact of each constituent element on the six key properties is evaluated. The addition of Nb tends to stabilize the BCC phase and the addition of Ti improves the ductility of RCCAs. Combined with all methods involved in this framework, the on-demand designer allows the alloy designers to have all properties for any RCCA compositions and narrow down the composition space by applying custom screening criteria. The output from the predictor and screener provides valuable guidance for our experimental study of RCCAs and accelerates the pace of materials discovery.

cond-mat.mtrl-sci↗

arXiv2026

Autonomous Probe Microscopy with Robust Bag-of-Features Multi-Objective Bayesian Optimization: Pareto-Front Mapping of Nanoscale Structure-Property Trade-Offs

Combinatorial materials libraries are an efficient route to generate large families of candidate compositions, but their impact is often limited by the speed and depth of characterization and by the difficulty of extracting actionable structure-property relations from complex characterization data. Here we develop an autonomous scanning probe microscopy (SPM) framework that integrates automated atomic force and magnetic force microscopy (AFM/MFM) to rapidly explore magnetic and structural properties across combinatorial spread libraries. To enable automated exploration of systems without a clear optimization target, we introduce a combination of a static physics-informed bag-of-features (BoF) representation of measured surface morphology and magnetic structure with multi-objective Bayesian optimization (MOBO) to discover the relative significance and robustness of features. The resulting closed-loop workflow selectively samples the compositional gradient and reconstructs feature landscapes consistent with dense grid "ground truth" measurements. The resulting Pareto structure reveals where multiple nanoscale objectives are simultaneously optimized, where trade-offs between roughness, coherence, and magnetic contrast are unavoidable, and how families of compositions cluster into distinct functional regimes, thereby turning multi-feature imaging data into interpretable maps of competing structure-property trends. While demonstrated for Au-Co-Ni and AFM/MFM, the approach is general and can be extended to other combinatorial systems, imaging modalities, and feature sets, illustrating how feature-based MOBO and autonomous SPM can transform microscopy images from static data products into active feedback for real-time, multi-objective materials discovery.

cond-mat.mtrl-sci↗

arXiv2025

Accelerated Materials Discovery through Cost-Aware Bayesian Optimization of Real-World Indentation Workflows

Accelerating the discovery of mechanical properties in combinatorial materials requires autonomous experimentation that accounts for both instrument behavior and experimental cost. Here, an automated nanoindentation (AE-NI) framework is developed and validated for adaptive mechanical mapping of combinatorial thin-film libraries. The method integrates heteroskedastic Gaussian-process modeling with cost-aware Bayesian optimization to dynamically select indentation locations and hold times, minimizing total testing time while preserving measurement accuracy. A detailed emulator and cost model capture the intrinsic penalties associated with lateral motion, drift stabilization, and reconfiguration-factors often neglected in conventional active-learning approaches. To prevent kernel-length-scale collapse caused by disparate time scales, a hierarchical meta-testing workflow combining local grid and global exploration is introduced. Implementation of the workflow is shown on a experimental Ta-Ti-Hf-Zr thin-film library. The proposed framework achieves nearly a thirty-fold improvement in property-mapping efficiency relative to grid-based indentation, demonstrating that incorporating cost and drift models into probabilistic planning substantially improves performance. This study establishes a generalizable strategy for optimizing experimental workflows in autonomous materials characterization and can be extended to other high-precision, drift-limited instruments.

cond-mat.mtrl-sci↗

arXiv2025

Lateral Ventricular Brain-Computer Interface System with Lantern-Inspired Electrode for Stable Performance and Memory Decoding

We present a lateral ventricular brain-computer interface (LV-BCI) that deploys an expandable, flexible electrode into the lateral ventricle through a minimally invasive external ventricular drainage pathway. Inspired by the framework of traditional Chinese lanterns, the electrode expands uniformly within the ventricle and conforms to the ependymal wall. Compared with conventional subdural ECoG electrodes, the LV-BCI shows superior signal stability and immunocompatibility. Resting-state spectral analyses revealed a maximum effective bandwidth comparable to subdural ECoG. In evoked potential tests, the LV-BCI maintained a consistently higher signal-to-noise ratio over 112 days without the decline typically associated with scarring or other immune responses. Immunohistochemistry showed only a transient, early microglial activation after implantation, returning to control levels and remaining stable through 168 days. We further designed an "action-memory T-maze" task and developed a microstate sequence classifier (MSSC) to predict rats' turn decisions. The LV-BCI achieved prediction accuracy up to 98%, significantly outperforming subdural ECoG, indicating enhanced access to decision-related information from deep structures such as the hippocampus. These results establish the lateral ventricle as a viable route for neural signal acquisition. Using a lantern-inspired flexible electrode, we achieve long-term stable recordings and robust memory decision decoding from within the ventricular system, opening new directions for BCI technology and systems neuroscience.

q-bio.NC↗

arXiv2024

Exploring Multi-view Pixel Contrast for General and Robust Image Forgery Localization

Image forgery localization, which aims to segment tampered regions in an image, is a fundamental yet challenging digital forensic task. While some deep learning-based forensic methods have achieved impressive results, they directly learn pixel-to-label mappings without fully exploiting the relationship between pixels in the feature space. To address such deficiency, we propose a Multi-view Pixel-wise Contrastive algorithm (MPC) for image forgery localization. Specifically, we first pre-train the backbone network with the supervised contrastive loss to model pixel relationships from the perspectives of within-image, cross-scale and cross-modality. That is aimed at increasing intra-class compactness and inter-class separability. Then the localization head is fine-tuned using the cross-entropy loss, resulting in a better pixel localizer. The MPC is trained on three different scale training datasets to make a comprehensive and fair comparison with existing image forgery localization algorithms. Extensive experiments on the small, medium and large scale training datasets show that the proposed MPC achieves higher generalization performance and robustness against post-processing than the state-of-the-arts. Code will be available at https://github.com/multimediaFor/MPC.

cs.CV↗

arXiv2023

Progressive Feedback-Enhanced Transformer for Image Forgery Localization

Blind detection of the forged regions in digital images is an effective authentication means to counter the malicious use of local image editing techniques. Existing encoder-decoder forensic networks overlook the fact that detecting complex and subtle tampered regions typically requires more feedback information. In this paper, we propose a Progressive FeedbACk-enhanced Transformer (ProFact) network to achieve coarse-to-fine image forgery localization. Specifically, the coarse localization map generated by an initial branch network is adaptively fed back to the early transformer encoder layers, which can enhance the representation of positive features while suppressing interference factors. The cascaded transformer network, combined with a contextual spatial pyramid module, is designed to refine discriminative forensic features for improving the forgery localization accuracy and reliability. Furthermore, we present an effective strategy to automatically generate large-scale forged image samples close to real-world forensic scenarios, especially in realistic and coherent processing. Leveraging on such samples, a progressive and cost-effective two-stage training protocol is applied to the ProFact network. The extensive experimental results on nine public forensic datasets show that our proposed localizer greatly outperforms the state-of-the-art on the generalization ability and robustness of image forgery localization. Code will be publicly available at https://github.com/multimediaFor/ProFact.

cs.CV↗

arXiv2023

Transferable Adversarial Attack on Image Tampering Localization

It is significant to evaluate the security of existing digital image tampering localization algorithms in real-world applications. In this paper, we propose an adversarial attack scheme to reveal the reliability of such tampering localizers, which would be fooled and fail to predict altered regions correctly. Specifically, the adversarial examples based on optimization and gradient are implemented for white/black-box attacks. Correspondingly, the adversarial example is optimized via reverse gradient propagation, and the perturbation is added adaptively in the direction of gradient rising. The black-box attack is achieved by relying on the transferability of such adversarial examples to different localizers. Extensive evaluations verify that the proposed attack sharply reduces the localization accuracy while preserving high visual quality of the attacked images.

cs.CV↗

arXiv2023

Effective Image Tampering Localization via Enhanced Transformer and Co-attention Fusion

Powerful manipulation techniques have made digital image forgeries be easily created and widespread without leaving visual anomalies. The blind localization of tampered regions becomes quite significant for image forensics. In this paper, we propose an effective image tampering localization network (EITLNet) based on a two-branch enhanced transformer encoder with attention-based feature fusion. Specifically, a feature enhancement module is designed to enhance the feature representation ability of the transformer encoder. The features extracted from RGB and noise streams are fused effectively by the coordinate attention-based fusion module at multiple scales. Extensive experimental results verify that the proposed scheme achieves the state-of-the-art generalization ability and robustness in various benchmark datasets. Code will be public at https://github.com/multimediaFor/EITLNet.

cs.CV↗

arXiv2023

Single and coupled cavity mode sensing schemes using a diagnostic field

Precise optical mode matching is of critical importance in experiments using squeezed-vacuum states. Automatic spatial-mode matching schemes have the potential to reduce losses and improve loss stability. However, in quantum-enhanced coupled-cavity experiments, such as gravitational-wave detectors, one must also ensure that the sub-cavities are also mode matched. We propose a new mode sensing scheme, which works for simple and coupled cavities. The scheme requires no moving parts, nor tuning of Gouy phases. Instead a diagnostic field tuned to the HG20/LG10 mode frequency is used. The error signals are derived to be proportional to the difference in waist position, and difference in Rayleigh ranges, between the sub-cavity eigenmodes. The two error signals are separable by 90 degrees of demodulation phase. We demonstrate reasonable error signals for a simplified Einstein Telescope optical design. This work will facilitate routine use of extremely high levels of squeezing in current and future gravitational-wave detectors.

physics.optics↗

arXiv2022

Effective Image Tampering Localization with Multi-Scale ConvNeXt Feature Fusion

With the widespread use of powerful image editing tools, image tampering becomes easy and realistic. Existing image forensic methods still face challenges of low generalization performance and robustness. In this letter, we propose an effective image tampering localization scheme based on ConvNeXt network and multi-scale feature fusion. Stacked ConvNeXt blocks are used as an encoder to capture hierarchical multi-scale features, which are then fused in decoder for locating tampered pixels accurately. Combined loss and effective data augmentation are adopted to further improve the model performance. Extensive experimental results show that localization performance of our proposed scheme outperforms other state-of-the-art ones. The source code will be available at https://github.com/ZhuHC98/ITL-SSN.

cs.CV↗