arXiv subjects

Harald Herrmann

Publications and source records attributed to Harald Herrmann.

At least 19 recordsLinked to original sources

arXiv2025

Widely non-degenerate nonlinear frequency conversion in cryogenic titanium in-diffused lithium niobate waveguides

The titanium in-diffused lithium niobate waveguide platform is well-established for reliable prototyping and packaging of many quantum photonic components at room temperature. Nevertheless, compatibility with certain quantum light sources and superconducting detectors requires operation under cryogenic conditions. We characterize alterations in phase-matching and mode guiding of a non-degenerate spontaneous parametric down-conversion process emitting around 1556 nm and 950 nm, under cryogenic conditions. Despite the effects of pyroelectricity and photorefraction, the spectral properties match our theoretical model. Nevertheless, these effects cause small but significant variations within and between cooling cycles. These measurements provide a first benchmark against which other nonlinear photonic integration platforms, such as thin-film lithium niobate, can be compared.

quant-ph↗

arXiv2025

A ultrabright, two-colour photon pair source based on thin-film lithium niobate for bridging visible and telecom wavelengths

We present the design and characterisation of a guided-wave, bright and highly frequency non-degenerate parametric down-conversion source in thin-film lithium niobate. The source generates photon pairs with wavelengths of 815$\,\mathrm{nm}$ and 1550$\,\mathrm{nm}$ linking the visible wavelength regime with telecommunication wavelengths. We confirm the high quality of the generated single photons by determining a value for the heralded second-order correlation function as low as $g^{(2)}_h(0) = (6.7\pm1.1)\cdot10^{-3}$. Furthermore, we achieve a high spectral brightness of 0.44$\cdot$10$^{7}$$\frac{\text{pairs}}{\text{s} \cdot \text{mW} \cdot \text{GHz}}$ which is two orders of magnitude higher than sources based on weakly guiding waveguides. The almost perfect sinc-shape and the strong agreement between the effective and nominal bandwidth highlights the success of our integrated workflow, which begins with device design and continues through precise fabrication to detailed quantum-state characterization. This comprehensive approach enables targeted optimization of the source, resulting in excellent quantum state generation. Our results set a new standard for on-chip, non-degenerate photon-pair sources and represent a crucial step towards practical, scalable quantum communication networks and photonic quantum computing.

quant-ph↗

arXiv2025

Harnessing of temporal dispersion for integrated pump filtering in spontaneous heralded single-photon generation processes

Cointegration of heralded single-photon generation and on-chip detection requires the ability to differentiate between pump light and single photons. We explored the dispersion-induced temporal separation of optical pulses to reach this goal. Our method exploits the distinct group velocities of pump light and single photons, as well as single-photon detectors with high timing resolution. We simulate the propagation for photon pair generation by spontaneous parametric down-conversion in titanium in-diffused waveguides in lithium niobate and thin-film lithium niobate, and spontaneous four-wave mixing in silicon on insulator and silicon nitride. For the different integration platforms, we show the propagation distance required to sufficiently distinguish between pump and single photons for different timing resolutions, and demonstrate that this should be feasible with current superconducting nanowire single-photon detector technologies. Finally, we experimentally simulate our approach using the dispersion in the optical fiber.

quant-ph↗

arXiv2023

Pyroelectric Influence on Lithium Niobate During the Thermal Transition for Cryogenic Integrated Photonics

Lithium niobate has emerged as a promising platform for integrated quantum optics, enabling efficient generation, manipulation, and detection of quantum states of light. However, integrating single-photon detectors requires cryogenic operating temperatures, since the best performing detectors are based on narrow superconducting wires. While previous studies have demonstrated the operation of quantum light sources and electro-optic modulators in LiNbO3 at cryogenic temperatures, the thermal transition between room temperature and cryogenic conditions introduces additional effects that can significantly influence device performance. In this paper, we investigate the generation of pyroelectric charges and their impact on the optical properties of lithium niobate waveguides when changing from room temperature to 25K, and vice versa. We measure the generated pyroelectric charge flow and correlate this with fast changes in the birefringence acquired through the Senarmont method. Both electrical and optical influence of the pyroelectric effect occurs predominantly at temperatures above 100K.

physics.optics↗

arXiv2023

Fully guided and phase locked Ti:PPLN waveguide squeezing for applications in quantum sensing

This work reports a fully guided setup for single-mode squeezing generation on integrated titanium-indiffused periodically poled nonlinear resonators. A continuous wave laser beam is delivered and the squeezed field is collected by single-mode fibers, where up to -3.17(9) dB of useful squeezing is available in fibers. To showcase the usefulness of such a fiber-coupled device, we applied the generated squeezed light in a fiber-based phase sensing experiment, showing a quantum enhancement in the signal-to-noise ratio of 0.35 dB. Moreover, our investigation of photorefraction's impact on the cavity resonance condition suggests that it causes system instabilities at high powers.

quant-ph↗

arXiv2023

Fiber-coupled plug-and-play heralded single photon source based on Ti:LiNbO$_3$ and polymer technology

A reliable, but cost-effective generation of single-photon states is key for practical quantum communication systems. For real-world deployment, waveguide sources offer optimum compatibility with fiber networks and can be embedded in hybrid integrated modules. Here, we present the first chip-size fully integrated fiber-coupled Heralded Single Photon Source (HSPS) module based on a hybrid integration of a nonlinear lithium niobate waveguide into a polymer board. Photon pairs at 810nm (signal) and 1550nm (idler) are generated via parametric down-conversion pumped at 532nm in the $\mathrm{LiNbO_3}$ waveguide. The pairs are splitted in the polymer board and routed to separate output ports. The module has a size of $(2 \times 1)\, \mathrm{cm^2}$ and is fully fiber-coupled with one pump input fiber and two output fibers. We measure a heralded second-order correlation function of $g_h^{(2)}=0.05$ with a heralding efficiency of $\eta_h=4.5\, \mathrm{\%}$ at low pump powers.

quant-ph↗

arXiv2022

Demonstration of Hong-Ou-Mandel interference in an LNOI directional coupler

Interference between single photons is key for many quantum optics experiments and applications in quantum technologies, such as quantum communication or computation. It is advantageous to operate the systems at telecommunication wavelengths and to integrate the setups for these applications in order to improve stability, compactness and scalability. A new promising material platform for integrated quantum optics is lithium niobate on insulator (LNOI). Here, we realise Hong-Ou-Mandel (HOM) interference between telecom photons from an engineered parametric down-conversion source in an LNOI directional coupler. The coupler has been designed and fabricated in house and provides close to perfect balanced beam splitting. We obtain a raw HOM visibility of (93.5+/-0.7)%, limited mainly by the source performance and in good agreement with off-chip measurements. This lays the foundation for more sophisticated quantum experiments in LNOI

quant-ph↗

arXiv2022

Lossy SU(1,1) interferometers in the single-photon-pair regime

The success of quantum technologies is intimately connected to the possibility of using them in real-world applications. To this aim, we study the sensing capabilities of quantum SU(1,1) interferometers in the single-photon-pair regime and in the presence of losses, a situation highly relevant to practical realistic measurements of extremely photosensitive materials. We show that coincidence measurement can be exploited to partially mitigate the effect of losses inside the interferometer. Finally, we find that quantum SU(1,1) interferometers are capable of outperforming classical SU(2) systems when analogous real-world conditions are considered.

quant-ph↗

arXiv2022

Cryogenic electro-optic modulation in titanium in-diffused lithium niobate waveguides

Lithium niobate is a promising platform for integrated quantum optics. In this platform we aim to efficiently manipulate and detect quantum states by combining superconducting single photon detectors and modulators. The cryogenic operation of a superconducting single photon detector dictates the optimisation of the electro-optic modulators under the same operating conditions. To that end, we characterise a phase modulator, directional coupler, and polarisation converter at both ambient and cryogenic temperatures. The operation voltage $V_{\pi/2}$ of these modulators increases due to the decrease of the electro-optic effect by 74% for the phase modulator, 84% for the directional coupler and 35% for the polarisation converter below 8.5$\,\mathrm{K}$. The phase modulator preserves its broadband nature and modulates light in the characterised wavelength range. The unbiased bar state of the directional coupler changed by a wavelength shift of 85$\,\mathrm{nm}$ while cooling the device down to 5$\,\mathrm{K}$. The polarisation converter uses periodic poling to phasematch the two orthogonal polarisations. The phasematched wavelength of the used poling changes by 112$\,\mathrm{nm}$ when cooling to 5$\,\mathrm{K}$

physics.optics↗

arXiv2020

Spectrally multimode integrated SU(1,1) interferometer

Nonlinear SU(1,1) interferometers are fruitful and promising tools for spectral engineering and precise measurements with phase sensitivity below the classical bound. Such interferometers have been successfully realized in bulk and fiber-based configurations. However, rapidly developing integrated technologies provide higher efficiencies, smaller footprints, and pave the way to quantum-enhanced on-chip interferometry. In this work, we theoretically realised an integrated architecture of the multimode SU(1,1) interferometer which can be applied to various integrated platforms. The presented interferometer includes a polarization converter between two photon sources and utilizes a continuous-wave (CW) pump. Based on the potassium titanyl phosphate (KTP) platform, we show that this configuration results in almost perfect destructive interference at the output and supersensitivity regions below the classical limit. In addition, we discuss the fundamental difference between single-mode and highly multimode SU(1,1) interferometers in the properties of phase sensitivity and its limits. Finally, we explore how to improve the phase sensitivity by filtering the output radiation and using different seeding states in different modes with various detection strategies.

quant-ph↗

arXiv2020

Waveguide Resonator with Integrated Phase Modulator for Second Harmonic Generation

We report second harmonic generation from a titanium indiffused lithium niobate waveguide resonator device whose cavity length is locked to the fundamental pump laser using an on-chip phase modulator. The device remains locked for more than 5 minutes, producing more than 80\% of the initial second harmonic power. The stability of the system is seen to be limited by DC-drift, a known effect in many lithium niobate systems that include deposited electrodes. The presented device explores the suitability of waveguide resonators in this platform for use in larger integrated networks.

physics.optics↗

arXiv2020

Two-photon phase-sensing with single-photon detection

Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realising this experimentally is technologically demanding, as it requires coincident single-photon detection proportional to the number of photons involved, which represents a severe challenge for achieving a practical quantum advantage over classical methods. Here, we exploit advanced quantum state engineering based on superposing two photon-pair creation events to realise a new approach that bypasses this issue. In particular, optical phase shifts are probed with a two-photon quantum state whose information is subsequently effectively transferred to a single-photon state. Notably, without any multiphoton detection, we infer phase shifts by measuring the average intensity of the single-photon beam on a photodiode, in analogy to standard classical measurements. Importantly, our approach maintains the quantum advantage: twice as many interference fringes are observed for the same phase shift, corresponding to N=2 path-entangled photons. Our results demonstrate that the advantages of quantum-enhanced phase-sensing can be fully exploited in standard intensity measurements, paving the way towards resource-efficient and practical quantum optical metrology.

quant-ph↗

arXiv2020

Cryogenic Electro-Optic Polarisation Conversion in Titanium in-diffused Lithium Niobate Waveguides

Many technologies in quantum photonics require cryogenic conditions to operate. However, the underlying platform behind active components such as switches, modulators and phase shifters must be compatible with these operating conditions. To address this, we demonstrate an electro-optic polarisation converter for 1550nm light at 0.8K in titanium in-diffused lithium niobate waveguides. To do so, we exploit the electro-optic properties of lithium niobate to convert between orthogonal polarisation modes with a fiber-to-fiber transmission >43%. We achieve a modulation depth of 23.6 +/-3.3dB and a conversion voltage-length product of 28.8 V cm. This enables the combination of cryogenic photonics and active components on a single integration platform.

physics.optics↗

arXiv2020

Cryogenic second harmonic generation in periodically-poled lithium niobate waveguides

Prospective integrated quantum optical technologies will combine nonlinear optics and components requiring cryogenic operating temperatures. Despite the prevalence of integrated platforms exploiting $\chi^{(2)}$-nonlinearities for quantum optics, for example used for quantum state generation and frequency conversion, their material properties at low temperatures are largely unstudied. Here, we demonstrate the first second harmonic generation in a fiber-coupled lithium niobate waveguide at temperatures down to 4.4K. We observe a reproducible shift in the phase-matched pump wavelength within the telecom band, in addition to transient discontinuities while temperature cycling. Our results establish lithium niobate as a versatile nonlinear photonic integration platform compatible with cryogenic quantum technologies.

physics.optics↗

arXiv2020

Counter-propagating photon pair generation in a nonlinear waveguide

Counter-propagating parametric conversion processes in non-linear bulk crystals have been shown to feature unique properties for efficient narrowband frequency conversion. In quantum optics, the generation of photon pairs with a counter-propagating parametric down-conversion process (PDC) in a waveguide, where signal and idler photons propagate in opposite directions, offers unique material-independent engineering capabilities. However, realizing counter-propagating PDC necessitates quasi-phase-matching (QPM) with extremely short poling periods. Here, we report on the generation of counter-propagating single-photon pairs in a self-made periodically poled lithium niobate waveguide with a poling period on the same order of magnitude as the generated wavelength. The single photons of the biphoton state bridge GHz and THz bandwidths with a separable joint temporal-spectral behavior. Furthermore, they allow the direct observation of the temporal envelope of heralded single photons with state-of-the art photon counters.

quant-ph↗

arXiv2019

Metasurface interferometry towards quantum sensors

Optical metasurfaces open new avenues for precise wavefront control of light for integrated quantum technology. Here, we demonstrate a hybrid integrated quantum photonic system that is capable to entangle and disentangle two-photon spin states at a dielectric metasurface. By interfering single-photon pairs at a nanostructured dielectric metasurface, a path-entangled two-photon NOON state with circular polarization is generated that exhibits a quantum HOM interference visibility of 86 $\pm$ 4%. Furthermore, we demonstrate nonclassicality and phase sensitivity in a metasurface-based interferometer with a fringe visibility of 86.8 $\pm$ 1.1 % in the coincidence counts. This high visibility proves the metasurface-induced path entanglement inside the interferometer. Our findings provide a promising way to hybrid-integrated quantum technology with high-dimensional functionalities in various applications like imaging, sensing, and computing.

physics.optics↗

arXiv2019

The Role of Stickiness in the Rheology of Semiflexible Polymers

Semiflexible polymers form central structures in biological material. Modeling approaches usually neglect influences of polymer-specific molecular features aiming to describe semiflexible polymers universally. Here, we investigate the influence of molecular details on networks assembled from filamentous actin, intermediate filaments, and synthetic DNA nanotubes. In contrast to prevalent theoretical assumptions, we find that bulk properties are affected by various inter-filament interactions. We present evidence that these interactions can be merged into a single parameter in the frame of the glassy wormlike chain model. The interpretation of this parameter as a polymer specific stickiness is consistent with observations from macro-rheological measurements and reptation behavior. Our findings demonstrate that stickiness should generally not be ignored in semiflexible polymer models.

cond-mat.soft↗

arXiv2018

Integrated transition edge sensors on lithium niobate waveguides

We show the proof-of-principle detection of light at 1550 nm coupled evanescently from a titanium in-diffused lithium niobate waveguide to a superconducting transition edge sensor. The coupling efficiency strongly depends on the polarization, the overlap between the evanescent field, and the detector structure. We experimentally demonstrate polarization sensitivity of this coupling as well as photon-number resolution of the integrated detector. The combination of transition edge sensors and lithium niobate waveguides can open the field for a variety of new quantum optics experiments.

physics.ins-det↗