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Harald Plank

Publications and source records attributed to Harald Plank.

8 recordsLinked to original sources

Transmissive extreme ultraviolet metagrating

Extreme ultraviolet (EUV) radiation is a key tool for attosecond physics and lithography. However, strong material absorption limits the availability of transmissive optical elements at these wavelengths. Metaoptics exploit geometry to control the wavefront of transmitted light on the nanoscale and, due to their minimal thickness, promise to fill this gap. Here, we demonstrate the first EUV metaoptics for broadband applications: we design, fabricate, and experimentally investigate a blazed transmissive EUV metagrating and compare it with a focused-ion-beam-milled sawtooth-blazed grating serving as an in-situ reference. The metagrating achieves an angular dispersion of 0.04{\deg}/nm with a directionality (the ratio of the +1st and -1st diffraction order efficiency) of up to 5.8. The device shows phase-based operation up to 50 eV photon energy (down to 25 nm vacuum wavelength) and an octave-spanning bandwidth of 25 eV, doubling the previous spectral window addressable by metasurfaces. Comparing both gratings' performance reveals that, when accounting for fabrication constraints, EUV metasurfaces are competitive with free-form optics while offering scalability to large apertures and arbitrary phase profiles. Broadband transmissive operation removes the need for grazing incidence optics, defeating a major source of aberrations, and allows polarization-insensitive spectral analysis, enabling energy-resolved ultrafast spectroscopy in compact experimental configurations.

physics.optics

Towards practical mass spectrometry with nanomechanical pillar resonators by surface acoustic wave transduction

Nanoelectromechanical systems (NEMS) have proven outstanding performance in the detection of small masses down to single proton sensitivity. To obtain a high enough throughput for the application in practical mass spectrometry, NEMS resonators have to be arranged in two-dimensional (2D) arrays. However, all state-of-the-art electromechanical transduction methods rely on electrical lines placed close to the mechanical resonators, which drastically restricts the density of 2D resonator arrays. An exception is the transduction by surface acoustic waves (SAWs), which has so far only been shown for the transduction of single nanomechanical pillar resonators. Here, we demonstrate the transduction of pillar pairs by surface acoustic waves. The pillars have a diameter of 700 nm and show a mass responsivity of -588$\pm$98 ng$^{-1}$. The distances between the pillar pairs are 70 nm and 14.3 $\mu$m. SAW transduction enabled us to measure both pillars of each pair with electrical lines no closer than 300 $\mu$m, illustrating the potential of SAWs to transduce dense arrays of pillar resonators, a crucial step towards practical mass spectrometry with NEMS.

physics.app-ph

Transduction of single nanomechanical pillar resonators by scattering of surface acoustic waves

One of the challenges of nanoelectromechanical systems (NEMS) is the effective transduction of the tiny resonators. Vertical structures, such as nanomechanical pillar resonators, which are exploited in a wide range of fields, such as optomechanics, acoustic metamaterials, and nanomechanical sensing, are particularly challenging to transduce. Existing electromechanical transduction methods are ill-suited as they complicate the pillars' fabrication process, put constraints on the pillars' material, and do not enable a transduction of freestanding pillars. Here, we present an electromechanical transduction method for single nanomechanical pillar resonators based on surface acoustic waves (SAWs). We demonstrate the transduction of freestanding nanomechanical platinum-carbon pillars in the first-order bending and compression mode. Since the principle of the transduction method is based on resonant scattering of a SAW by a nanomechanical resonator, our transduction method is independent of the pillar's material and not limited to pillar-shaped geometries. It represents a general method to transduce vertical mechanical resonators with nanoscale lateral dimensions.

physics.app-ph

Analyzing Nanogranularity of Focused Electron-Beam-Induced Deposited (FEBID) Materials by Electron Tomography

Nanogranular material systems are promising for a variety of applications in research and development. Their physical properties are often determined by grain sizes, shapes, mutual distances and by the chemistry of the embedding matrix With focused electron beam induced deposition arbitrarily shaped nanocomposite materials can be designed, where metallic, nanogranular structures are embedded in a carbonaceous matrix. Using "post-growth" electron beam curing, these materials can be tuned for improved electric transport or mechanical behavior. Such an optimization necessitates a thorough understanding and characterization of the internal changes in chemistry and morphology, which is where conventional projection based imaging techniques fall short. Here, we apply scanning transmission electron tomography to get a comprehensive picture of the distribution and morphology degree of embedded Pt nanograins after initial fabrication, and we demonstrate the impact of electron beam curing, which leads to condensed regions of interconnected metal nanograins.

cond-mat.mtrl-sci

Direct-write of free-form 3D nanostructures with controlled magnetic frustration

Building nanotechnological analogues of naturally occurring magnetic structures has proven to be a powerful approach to studying topics like geometry-induced magnetic frustration and to provide model systems for statistical physics. Moreover, it practically allows to engineer novel physical properties by realizing artificial lattice geometries that are not accessible via natural crystallization or chemical synthesis. This has been accomplished with great success in the field of two-dimensional artificial spin ice systems with important branches reaching into the field of magnetic logic devices. Although first proposals have been made to advance into three dimensions (3D), established nanofabrication pathways based on electron beam lithography have not been adapted to obtain free-form 3D nanostructures. Here we demonstrate the direct-write fabrication of freestanding ferromagnetic 3D nano-architectures with full control over the degree of magnetic frustration. By employing micro-Hall sensing, we have determined the magnetic stray field generated by our free-form structures in an externally applied magnetic field and we have performed micromagnetic and macro-spin simulations to deduce the spatial magnetization profiles in the structures and analyze their switching behavior. Furthermore we show that the magnetic 3D elements can be combined with other 3D elements of different chemical composition and intrinsic material properties.

cond-mat.mes-hall

Post-growth purification of Co nanostructures prepared by focused electron beam induced deposition

In the majority of cases nanostructures prepared by focused electron beam induced deposition (FEBID) employing an organometallic precursor contain predominantly carbon-based ligand dissociation products. This is unfortunate with regard to using this high-resolution direct-write approach for the preparation of nanostructures for various fields, such as mesoscopic physics, micromagnetism, electronic correlations, spin-dependent transport and numerous applications. Here we present an in-situ cleaning approach to obtain pure Co-FEBID nanostructures. The purification procedure lies in the exposure of heated samples to a H$_2$ atmosphere in conjunction with the irradiation by low-energy electrons. The key finding is that the combination of annealing at $300^\circ$C, H$_2$ exposure and electron irradiation leads to compact, carbon- and oxygen free Co layers down to a thickness of about 20\,nm starting from as-deposited Co-FEBID structures. In addition to this, in temperature-dependent electrical resistance measurements on post-processed samples we find a typical metallic behavior. In low-temperature magneto-resistance and Hall effect measurements we observe ferromagnetic behavior.

cond-mat.mes-hall

Tunable magnetism on the lateral mesoscale by post-processing of Co/Pt heterostructures

Controlling magnetic properties on the nm-scale is essential for basic research in micro-magnetism and spin-dependent transport, as well as for various applications such as magnetic recording, imaging and sensing. This has been accomplished to a very high degree by means of layered heterostructures in the vertical dimension. Here we present a complementary approach that allows for a controlled tuning of the magnetic properties of Co/Pt heterostructures on the lateral mesoscale. By means of in-situ post-processing of Pt- and Co-based nano-stripes prepared by focused electron beam induced deposition (FEBID) we are able to locally tune their coercive field and remanent magnetization. Whereas single Co-FEBID nano-stripes show no hysteresis, we find hard-magnetic behavior for post-processed Co/Pt nano-stripes with coercive fields up to 850 Oe. We attribute the observed effects to the locally controlled formation of the CoPt L1$_{0}$ phase, whose presence has been revealed by transmission electron microscopy.

cond-mat.mes-hall

Dielectric sensing by charging energy modulation in a nano-granular metal

Several sensing concepts using nanostructures prepared by focused electron beam induced deposition have been developed over the last years. Following work on highly miniaturized Hall sensors for magnetic sensing with soft magnetic Co, strain and force sensing based on nano-granular platinum-carbon structures (Pt(C)) was introduced. Very recently the capability of nano-granular Pt(C) structures to detect the presence of adsorbate water layers by conductance modulations was demonstrated. For magnetic and strain sensing the underlying physical mechanisms of the sensing effect have been analyzed in detail and are now quite well understood. This is not the case for the adsorbate layer induced conductance modulation effect. Here we provide a theoretical framework that allows for a semi-quantitative understanding of the observed water-sensing effect. We show how the near-interface renormalization of the Coulomb charging energy in the nano-granular metal caused by the dielectric screening of the polarizable adsorbate layer leads to a conductance modulation. The model can account for the conductance modulation observed in the water adsorbate experiments and can also be applied to understand similar effects caused by near-interface dielectric anomalies of ferroelectric thin films on top of nano-granular Pt(C). Our findings provide a pathway towards optimized nano-granular layer structures suitable for a wide range of dielectric or local potential sensing applications.

cond-mat.mes-hall