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Harley Suchiang

Publications and source records attributed to Harley Suchiang.

3 recordsLinked to original sources

Incoherent dark excitons extend Floquet-like physics across time and momentum

Floquet phenomena - where a coherent, time-periodic drive hybridizes the conduction band with energy-replicated copies of the valence band - have been demonstrated with intense optical fields and, more recently, other bosonic excitations. However, within mean-field approximations and the current understanding of Floquet phenomena, these effects survive only for the coherence time of the drive, limiting practical use and current demonstrations to the sub-picosecond regime. Here, consistent with recent theoretical predictions beyond the mean-field picture, using time- and angle-resolved photoemission spectroscopy in WSe$_2$/MoS$_2$ heterostructures, we show that incoherent, dense populations of dark interlayer excitons hybridize the conduction band with energy-replicated copies of the valence band, mimicking Floquet-like phenomena - now persisting for nearly a nanosecond. With increasing interlayer exciton density, the valence band and its replica evolve from an inverted-parabolic to a Mexican-hat dispersion, a signature of the predicted non-zero static coupling that hybridizes the bands and scales linearly with the exciton density. By tuning twist angle, we further show that dark excitons with net momentum create replicas that hybridize with bands offset not just in energy but also in momentum, providing another powerful degree of freedom beyond conventional Floquet engineering. These results establish a robust, long-lived route to engineering electronic states, beyond a coherent, zero-momentum drive.

cond-mat.mes-hall↗

Quasiparticle phono-conversion: filming carriers coalescing into excitons

Condensed matter physics is replete with phenomena involving high-energy free particles coalescing into low-energy bound few-particle states. While the cooling of the individual particles is well understood, the crucial step by which cold free carriers form a bound state remains elusive, involving complex energy and momentum relaxation pathways. Here, by combining ultrafast time- and momentum-resolved photoemission spectroscopy on a monolayer WSe$_2$ with the first-principles excitonic-Bloch equations, we resolve the conversion of initially free electrons and holes at the bandedges into bound excitons. With unprecedented energy resolution, we observe the transient \textit{coexistence} of free-carrier and excitonic bands, accompanied by a transfer of spectral weight between the two. We establish the phononic origin of exciton formation and ascribe this coexistence to a sequential relaxation cascade toward the lowest-energy excitonic states, wherein intermediate states remain weakly populated. The efficiency of this process is controlled by valley multiplicity, large-momentum phonon emission and spin-flip processes. By elucidating how bound states emerge from their elementary constituents, our results point to strategies for engineering exciton formation, with direct implications for optical materials and devices that operate with excitons or free carriers.

cond-mat.mtrl-sci↗

Momentum domain polarization probing of forward and inverse spin Hall effect of leaky modes in plasmonic crystals

Simultaneous manifestation of both forward and inverse photonic Spin Hall effect in geometrically tailored anisotropic waveguided plasmonic crystal system is observed through the excitation of the leaky hybridized quasiguided modes. The quasiguided modes of the plasmonic crystal manifested in the far-field momentum (Fourier) domain as circular ring-like intensity distributions, and the different spin orbit interaction (SOI) effects revealed their exclusive signature as polarization-dependent azimuthal intensity lobes on top of it. Using a darkfield Fourier domain polarization Mueller matrix platform, we have observed input spin (circular polarization)- dependent trajectory of the leaky quasiguided modes in the momentum domain (forward spin Hall effect) and its reciprocal effect as the wave vector-controlled spin selection of quasiguided modes (inverse spin Hall effect). These effects are separately manifested in characteristic Mueller matrix elements enabling their interpretation as geometrical circular anisotropy effects. Resonance-enabled enhancement and control of these effects are also demonstrated by exploiting the spectral Fano-type resonance. The far-field manifestation of spin-directional excitation of leaky quasiguided modes, their unique interpretation through momentum domain Mueller matrix, regulation and control of the SOI effects in plasmonic-photonic crystal systems, opens up exciting avenues in spin-orbit photonic research.

physics.optics↗