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Harry A. Atwater

Publications and source records attributed to Harry A. Atwater.

At least 19 recordsLinked to original sources

Dual-polarized, mid-infrared nonreciprocal absorption

The emission and absorption of thermal radiation are usually coupled via Kirchhoff's law or reciprocity, stated as the equality of spectral directional emissivity and absorptivity. Magneto-optical materials have recently been identified as a promising route to lifting the constraint of reciprocity, with multiple experimental demonstrations using doped InAs. However, these demonstrations have been limited to p-polarized light in the Voigt configuration, whereas thermal radiation from a blackbody is unpolarized. Therefore, to break reciprocity in both polarization channels, we design a nanophotonic, dual-polarized nonreciprocal absorber operating in the mid-infrared spectral range (11-20 $\unicode{x03BC}$m), consisting of an a-Si photonic crystal slab on top of a doped InAs substrate described by an antisymmetric, nonreciprocal dielectric tensor under an applied magnetic field. The photonic crystal slab supports eigenmodes that couple to both s- and p-polarized light, resulting in absorption peaks that frequency shift in opposite directions for forward- and backward-propagating light$\unicode{x2014}$a signature of nonreciprocity in planar, subwavelength systems. We fabricate our design, then measure its room-temperature absorptance using magnetic-field-integrated absorptance spectroscopy, experimentally demonstrating nonreciprocal absorption for both polarizations. Our design is a step toward the complete control of light as heat, which could improve photonic energy conversion, thermal management, and mid-infrared optical isolation and circulation.

physics.optics

An Optically Addressable Transmissive Liquid Crystal Metasurface Spatial Light Modulator

Active wavefront control in high-power laser illumination systems is important for technologies such as additive manufacturing, free-space laser communication, and power transmission. Conventional spatial light modulators (SLMs) and mechanical beam-steering devices are unsuitable for such applications as they rely on metal mirrors and electrical contacts which are damaged under high laser irradiances. Here, we report on the design and realization of an optically addressable metasurface liquid crystal (LC)-based SLM for the modulation of high-power transmitted light. Our device uses a photoactive top contact which is optically addressed with a patterned 435 nm laser, creating a transient electrical contact that selectively switches the underlying LC medium. A TiO$_2$ metasurface, resonant in the 915-985 nm wavelength range, is embedded within a thin (~2 $μ$m) LC layer and enables large optical tunability. We demonstrate 90$^\circ$ linear polarization rotation in reconfigurable patterns across a 5x5 mm$^2$ active area with an overall transmittance of >60%. Additionally, we develop a multiphysics approach to simulate transmittance modulation in our device by modeling the LC interactions with TiO$_2$ nanopillars under an applied electrostatic field. This model exhibits good agreement with measurements and provides improved understanding of how LCs interact with both transmitted light and nanoscale metastructures in active devices. We show that our design and fabrication approach can yield high-efficiency transmissive metasurface SLM devices and lay the groundwork for the design of future LC-based active nanophotonics.

physics.optics

Electro-optic modulation of coherent and incoherent mid-IR radiation in two-dimensional arrays

Light in the mid-infrared (mid-IR) spans wavelengths from 3-8 $μ$m and is important to many applications such as gas sensing and thermal imaging. Due to materials challenges, there is currently a lack of mid-IR reconfigurable optical elements. Here, we present an electrically addressable metasurface for modulation of coherent and incoherent mid-IR radiation in two spatial dimensions. Our device achieves optical modulation due to the field-effect free-carrier depletion in a lightly doped ($10^{19}$ cm$^{-3}$) film of indium-tin-oxide (ITO) coupled to a gap plasmon resonator. By addressing 32 individual elements across the metasurface, we first demonstrate tunable diffraction of coherently reflected mid-IR light. Next, we introduce a scalable perimeter-addressed driving scheme for tunable diffraction in two dimensions. Finally, we demonstrate modulated emissivity with spatially reconfigurable two-dimensional patterns at elevated temperatures. This work advances the development of solid-state reflective beam-steering devices in the mid-IR and manipulation of thermally emitted incoherent radiation.

physics.optics

Ultrafast, reconfigurable all-optical beam steering and spatial light modulation

Achieving spatiotemporal control of light at subwavelength and subcycle scales is an important milestone in the development of new photonic materials and technologies. Ultrafast spatiotemporal light modulation currently relies on electronic interband and intraband transitions that yield pronounced refractive index changes but typically suffer from slow, picosecond response times due to carrier relaxation. Here we show that by leveraging resonant light-matter interactions in a high-quality factor metasurface it is possible to use the optical Kerr effect, a weaker, but instantaneous optoelectronic polarization effect, to achieve ultrafast, reconfigurable light modulation with unprecedented spatial and temporal control. By the subwavelength all-optical tuning of the refractive index of the dielectric metasurface unit cells, we experimentally demonstrate pulse-limited beam steering with a 74-fs response time at angles up to $\pm $13° in the near-infrared. The steering originates from the Kerr effect with a background contribution arising from slower two-photon-excited free carrier absorption. Additionally, we observe spatial back-action, linear frequency conversion, and demonstrate arbitrary ultrafast spatial light modulation in two dimensions. Our findings open the possibility of realizing new ultrafast physics in metastructures with applications in signal processing, pulse shaping, and ultrafast imaging.

physics.optics

Optically Actuated Transitions in Multimodal, Bistable Micromechanical Oscillators

We experimentally demonstrate a new class of optomechanical nonlinearities in weakly damped micromechanical resonators, arising from the interplay between the Duffing nonlinearity, intermodal coupling, and thermal fluctuations. Within the bistable regime of a single Duffing mode driven by radiation pressure forces, we observe stochastically generated sidebands, originating from thermal fluctuations around equilibrium trajectories in phase space, and exploit these sidebands to induce probabilistic transitions between bistable states using weak secondary acoustic excitation. Extending this framework to multimodal interactions, we show that nonlinear modes coupling within the same resonator leads to similar transitions due to parametric modulation around the noise-excited sidebands as a result of frequency mixing. Simultaneously, abrupt changes in displacements of modes cause their instantaneous energy exchange rates to span five orders of magnitude. These findings open new avenues for reconfigurable optomechanical networks, nonreciprocal energy transport, and precision sensing based on dynamically tunable mechanical nonlinearities.

physics.optics

Spalled barium titanate single crystal thin films for functional device applications

We report a scalable approach for fabricating single-crystal barium titanate (BTO) thin films through spalling from bulk substrates. Conventional thin film growth techniques often face challenges in achieving high-quality single crystal microstructure over large areas, resulting in reduced performance in functional devices. In contrast, spalling - i.e., performing stress-induced exfoliation of bulk single crystals - enables the separation of single crystal thin films with controllable thicknesses ranging from 100 nm to 15 um and lateral dimensions up to several millimeters. Electro-optic characterization of the spalled films yields a Pockels coefficient of r33 = 55 pm/V in multi-domain regions and 160 pm/V in single-domain regions, leading to projections up to 1980 pm/V for r42 under conditions of unclamped excitation. Our results indicate that spalled BTO single-crystal thin films preserve bulk electro-optic properties and exceed the performance of commercially available thin-film lithium niobate, making them suitable for integration in advanced photonic and optoelectronic devices.

physics.app-ph

Numerical Analysis of Lensless Imaging with Active Metasurfaces and Single-Pixel Detectors

We introduce a conceptual framework for a lensless imaging system which employs an active metasurface as a high-frequency, continuously tunable amplitude and phase modulation aperture, coupled to a discrete single-pixel detector. Using an array factor formalism, we first study fundamental limits in information collection, offering a comparison to existing technologies. We also study the effects of modulation rate and losses on the system acquisition time and signal-to-noise ratio, which place bounds on system performance for set illumination conditions. Considering both an ideal metasurface and the phase and amplitude modulation characteristics of an experimentally realized indium tin oxide-based metasurface operating at 1510 nm, we then simulate image recovery with ~60,000 image points for a 0.2 mm x 0.2 mm active metasurface aperture. We show that aberrations appearing in the simulated images produced by the metasurface can be corrected through post-processing. We further investigate trade-offs between image acquisition time and image quality both through the realization of Hadamard coupling bases and by modifying the k-space width coupling to the detector. Finally, we discuss the technical challenges which remain to be overcome for experimental realization of a lensless single-pixel imaging technology.

physics.optics

Photon statistics analysis of h-BN quantum emitters with pulsed and continuous-wave excitation

We report on the quantum photon statistics of hexagonal boron nitride (h-BN) quantum emitters by analyzing the Mandel Q parameter. We have measured the Mandel Q parameter for h-BN quantum emitters under various temperatures and pump power excitation conditions. Under pulsed excitation we can achieve a Mandel Q of -0.002 and under continuous-wave (CW) excitation this parameter can reach -0.0025. We investigate the effect of cryogenic temperatures on Mandel Q and conclude that the photon statistics vary weakly with temperature. Through calculation of spontaneous emission from an excited two-level emitter model, we demonstrate good agreement between measured and calculated Mandel Q parameter when accounting for the experimental photon collection efficiency. Finally, we illustrate the usefulness of Mandel Q in quantum applications by the example of random number generation and analyze the effect of Mandel Q on the speed of generating random bits via this method.

quant-ph

Direct Radiation Pressure Measurements for Lightsail Membranes

Ultrathin lightsails propelled by laser radiation pressure to relativistic speeds are currently the most promising route for flyby-based exoplanet exploration. However, there has been a notable lack of experimental characterization of key parameters essential for lightsail propulsion. Therefore, a model platform for optomechanical characterization of lightsail prototypes made from realistic materials is needed. We propose an approach for simultaneous measurement of optical forces and driving powers, which capitalizes on the multiphysics dynamics induced by the driving laser beam. By modelling the lightsail with a 50-nm thick silicon nitride membrane suspended by compliant micromechanical springs, we quantify force from off-resonantly driven displacement and power from heating-induced mechanical mode softening. This approach allows us to calibrate the measured forces to the driving powers by operating the device as a mechanical bolometer. We report radiation pressure forces of 80 fN using a collimated pump beam of 100 W/cm2 and noise-robust common-path interferometry. As lightsails will inevitably experience non-normal forces, we quantify the effects of incidence angle and spot size on the optical force and explain the nonintuitive trend by edge scattering. Our results provide a framework for comprehensive lightsail characterization and laboratory optomechanical manipulation of macroscopic objects by radiation pressure forces.

physics.optics

Third harmonic generation enhancement and wavefront control using a local high-Q metasurface

High quality factor optical nanostructures provide great opportunity to enhance nonlinear optical processes such as third harmonic generation. However, the field enhancement in these high quality factor structures is typically accompanied by optical mode nonlocality. As a result, the enhancement of nonlinear processes comes at the cost of their local control as needed for nonlinear wavefront shaping, imaging and holography. Here we show simultaneous strong enhancement and spatial control over third harmonic generation with a local high-Q metasurface relying on higher-order Mie-resonant modes. Our results demonstrate third harmonic generation at an efficiency of up to $3.25\times10^{-5}$, high quality wavefront shaping as illustrated by a third harmonic metalens, and a flatband, angle independent, third harmonic response up to $\pm11^{\circ}$ incident angle. The demonstrated high level of local control and efficient frequency conversion offer promising prospects for realizing novel nonlinear optical devices.

physics.optics

All-dielectric high-Q dynamically tunable transmissive metasurfaces

Active metasurfaces, which are arrays of actively tunable resonant elements, can dynamically control the wavefront of the scattered light at a subwavelength scale. To date, most active metasurfaces that enable dynamic wavefront shaping operate in reflection. On the other hand, active metasurfaces operating in transmission are of considerable interest as they can readily be integrated with chip-scale light sources, yielding ultra-compact wavefront shaping devices. Here, we report designs for all-dielectric low-loss active metasurfaces which can dynamically manipulate the transmitted light wavefront in the near-infrared wavelength range. Our active metasurfaces feature an array of amorphous silicon (a-Si) pillars on a silica substate, which support resonances with quality factors (Q-factors) as high as 9800, as well as other lower-Q resonances. First, we demonstrate that high-Q resonance dips observed in transmission can be transformed into a transmission resonance peak by positioning a-Si pillar resonators at a prescribed distance from a crystalline Si substrate, defined by a silica spacer layer. Next, we report the design of metasurface geometry with realistic interconnect architectures that enable thermo-optic dynamic beam switching with switching times as low as 7.3 μs. Beam switching is observed for refractive index differences between neighboring metasurface elements as low as 0.0026. Finally, we demonstrate that metasurface structures with both high-Q and lower-Q modes and realistic interconnect architectures can be used for dynamic beam steering.

physics.app-ph

Detecting, distinguishing, and spatiotemporally tracking photogenerated charge and heat at the nanoscale

Since dissipative processes are ubiquitous in semiconductors, characterizing how electronic and thermal energy transduce and transport at the nanoscale is vital for understanding and leveraging their fundamental properties. For example, in low-dimensional transition metal dichalcogenides (TMDCs), excess heat generation upon photoexcitation is difficult to avoid since even with modest injected exciton densities, exciton-exciton annihilation still occurs. Both heat and photoexcited electronic species imprint transient changes in the optical response of a semiconductor, yet the unique signatures of each are difficult to disentangle in typical spectra due to overlapping resonances. In response, we employ stroboscopic optical scattering microscopy (stroboSCAT) to simultaneously map both heat and exciton populations in few-layer \ch{MoS2} on relevant nanometer and picosecond length- and time scales and with 100-mK temperature sensitivity. We discern excitonic contributions to the signal from heat by combining observations close to and far from exciton resonances, characterizing photoinduced dynamics for each. Our approach is general and can be applied to any electronic material, including thermoelectrics, where heat and electronic observables spatially interplay, and lays the groundwork for direct and quantitative discernment of different types of coexisting energy without recourse to complex models or underlying assumptions.

cond-mat.mtrl-sci

Quasiparticle and Optical Properties of Carrier-Doped Monolayer MoTe$_2$ from First Principles

The intrinsic weak and highly non-local dielectric screening of two-dimensional materials is well known to lead to high sensitivity of their optoelectronic properties to environment. Less studied theoretically is the role of free carriers on those properties. Here, we use ab initio GW and Bethe-Salpeter equation calculations, with a rigorous treatment of dynamical screening and local-field effects, to study the doping-dependence of the quasiparticle and optical properties of a monolayer transition metal dichalcogenide, 2H MoTe$_2$. We predict a quasiparticle band gap renormalization of several hundreds meV for experimentally-achievable carrier densities, and a similarly sizable decrease in the exciton binding energy. This results in an almost constant excitation energy for the lowest-energy exciton resonance with increasing doping density. Using a newly-developed and generally-applicable quasi-2D plasmon-pole model and a self-consistent solution of the Bethe-Salpeter equation, we reveal the importance of accurately capturing both dynamical and local-field effects to understand detailed photoluminescence measurements.

cond-mat.mtrl-sci

Kerker Transform: Expanding Fields in a Discrete Basis of Directional Harmonics

We present a linear coordinate transform to expand the solution of scattering and emission problems into a basis of forward and backward directional vector harmonics. The transform provides intuitive algebraic and geometric interpretations of systems with directional scattering/emission across a broad range of wavelength-to-size ratios. The Kerker, generalized Kerker, and transverse Kerker effect as well as other forms of highly directional scattering/emission are easily understood through open and closed loop contours in the complex plane. Furthermore, the theoretical maximum directivity of any scattering/emissive system is easily defined. The transformed far field harmonics have coordinates that are polar-angle invariant, interference between forward and backward harmonics weakly interact, and interference of same type harmonics alters directivity. Examples of highly directional scattering are presented including a Kerker scattering magnetic sphere, a directional scattering photonic nanojet, both under plane wave illumination, as well as generalized backward Kerker and transverse Kerker emission from sub-wavelength spheres that are near-field coupled to emitters. Solutions of scattering/emission under the Kerker transform are contrasted to the traditional Mie expansion for comparison.

physics.optics

Rydberg Excitons and Trions in Monolayer MoTe$_2$

Monolayer transition metal dichalcogenide (TMDC) semiconductors exhibit strong excitonic optical resonances which serve as a microscopic, non-invasive probe into their fundamental properties. Like the hydrogen atom, such excitons can exhibit an entire Rydberg series of resonances. Excitons have been extensively studied in most TMDCs (MoS$_2$, MoSe$_2$, WS$_2$ and WSe$_2$), but detailed exploration of excitonic phenomena has been lacking in the important TMDC material molybdenum ditelluride (MoTe$_2$). Here, we report an experimental investigation of excitonic luminescence properties of monolayer MoTe$_2$ to understand the excitonic Rydberg series, up to 3s. We report significant modification of emission energies with temperature (4K to 300K), quantifying the exciton-phonon coupling. Furthermore, we observe a strongly gate-tunable exciton-trion interplay for all the Rydberg states governed mainly by free-carrier screening, Pauli blocking, and band-gap renormalization in agreement with the results of first-principles GW plus Bethe-Salpeter equation approach calculations. Our results help bring monolayer MoTe$_2$ closer to its potential applications in near-infrared optoelectronics and photonic devices.

cond-mat.mes-hall

Dynamically Stable Radiation Pressure Propulsion of Flexible Lightsails for Interstellar Exploration

Lightsail spacecraft, propelled to relativistic velocities via photon pressure using high power density laser radiation, offer a potentially new route to space exploration within and beyond the solar system, extending to interstellar distances. Such missions will require meter-scale lightsails of submicron thickness, posing substantial challenges for materials science and engineering. We analyze the structural and photonic design of flexible lightsails, developing a mesh-based multiphysics simulator based on linear elastic theory, treating the lightsail as a flexible membrane rather than a rigid body. We find that flexible lightsail membranes can be spin stabilized to prevent shape collapse during acceleration, and that certain lightsail shapes and designs offer beam-riding stability despite the deformations caused by photon pressure and thermal expansion. Excitingly, nanophotonic lightsails based on planar silicon nitride membranes patterned with suitably designed optical metagratings exhibit both mechanically and dynamically stable propulsion along the pump laser axis. These advances suggest that laser-driven acceleration of membrane-like lightsails to the relativistic speeds needed to access interstellar distances is conceptually feasible, and that fabrication of such lightsails may be within the reach of modern microfabrication technology.

physics.app-ph

High quality factor metasurfaces for two-dimensional wavefront manipulation

The strong interaction of light with micro- and nanostructures plays a critical role in optical sensing, nonlinear optics, active optical devices, and quantum optics. However, for wavefront shaping, the required local control over light at a subwavelength scale limits this interaction, typically leading to low-quality-factor optical devices. Here, we demonstrate an avenue towards high-quality-factor wavefront shaping in two spatial dimensions based on all-dielectric Huygens metasurfaces by leveraging higher-order Mie resonances. We design and experimentally realize transmissive band stop filters, beam deflectors and radial lenses with measured quality factors in the range of 202-1475 at near-infrared wavelengths. The excited optical mode and resulting wavefront control are both local, allowing versatile operation with finite apertures and oblique illumination. Our results represent an improvement in quality factor by nearly two orders of magnitude over previous localized mode designs, and provide a design approach for a new class of compact optical devices.

physics.optics

Excitonic beam steering in an active van der Waals metasurface

Two-dimensional transition metal dichalcogenides (2D TMDCs) are promising candidates for ultra-thin active nanophotonic elements due to the strong tunable excitonic resonances that dominate their optical response. Here we demonstrate dynamic beam steering by an active van der Waals metasurface that leverages large complex refractive index tunability near excitonic resonances in monolayer molybdenum diselenide (MoSe2). Through varying the radiative and nonradiative rates of the excitons, we can dynamically control both the reflection amplitude and phase profiles, resulting in an excitonic phased array metasurface. Our experiments show reflected light steering to angles between -30° to 30° at three different resonant wavelengths corresponding to the A exciton, B exciton, and trion. This active van der Waals metasurface relies solely on the excitonic resonances of the monolayer MoSe2 material rather than geometric resonances of patterned nanostructures, suggesting the potential to harness the tunability of excitonic resonances for wavefront shaping in emerging photonic applications.

physics.optics