arXiv subjects

Helen M. Chrzanowski

Publications and source records attributed to Helen M. Chrzanowski.

At least 19 recordsLinked to original sources

arXiv2026

Scalable generation of heralded single photons via active feed-forward switching of a fiber delay line

Quasi-deterministic single-photon generation is a key requirement for many photonic quantum technologies. Photon sources based on spontaneous parametric down-conversion (SPDC) are widely used for producing high-quality photons; however, the probabilistic nature of the process limits the generation of synchronized multi-photon states. Here, we demonstrate temporal synchronization of multiple photon-generation events using a free-space-fiber hybrid delay line with feed-forward control, enabling fast and efficient switching and scalable operation. Narrow-band, telecom-wavelength photons compatible for fiber transmission are heralded from a monolithic cavity SPDC source and synchronized across 20 time bins. This yields a sixfold enhancement in synchronized rates and enables multi-photon synchronization, with only a marginal increase of higher-order photon-number contributions.

quant-ph↗

arXiv2026

Pure narrowband photon-pair generation in a monolithic cavity

Photonic quantum technologies require efficient sources of pure single photons. We present a heralded single-photon source based on spontaneous parametric down-conversion in a monolithic cavity optimized for high spectral and spatial purity. The source heralds single photons at a wavelength of 1540 nm and a spectral bandwidth of 168 MHz, with a maximum heralding efficiency of 70% including all transmission and detection losses, while keeping the multi-photon contamination below 3%. The cavity enhancement predominantly generates photons into the central cavity mode, with a theoretical upper bound on the spectral purity of 79.4% arising from nonzero overlap with adjacent cavity modes. Spectral isolation of the central cavity mode with an etalon yields an increased measured spectral purity of (96.2 $\pm$ 2.7)%.

quant-ph↗

arXiv2026

Polymer identification via undetected photons using a low footprint nonlinear interferometer

Plastic pollution has become a critical global challenge, with microplastics pervading ecosystems and entering human food chains. Effectively monitoring this widespread contamination demands rapid, reliable, and portable material identification techniques that often elude conventional Raman and FTIR spectroscopy. Undetected photon spectroscopy within a nonlinear interferometer (NLI) offers a solution, allowing the retrieval of mid-infrared absorption spectra by detecting only near-infrared signal photons using standard silicon-based technology. Here, we demonstrate a highly compact, micro-integrated, thermally-stabilised NLI with a Michelson-like geometry designed for the rapid spectroscopy of plastics. We benchmarked its room-temperature performance, demonstrating a signal-to-noise ratio of 34 with a measurement rate of 100 Hz and a spectral resolution of 6 cm$^{-1}$. We show that we can accurately and rapidly retrieve the characteristic vibrational absorption spectra of common polymers such as polypropylene, polyethene, and polystyrene, without using mid-infrared technology. These results establish our compact module as a promising field-deployable platform for robust, real-time environmental monitoring systems and other mid-infrared spectroscopy applications.

quant-ph↗

arXiv2025

Hong-Ou-Mandel effect with two frequency-entangled photons of vastly different color

In the original formulation of the Hong-Ou-Mandel (HOM) experiment, when two otherwise indistinguishable photons are incident upon the two input ports of a balanced beam splitter, they coalesce, always leaving via the same output port. It is often interpreted that this interference arises due to the indistinguishability of the single photons at the beam splitter; the situation, however, is often more nuanced. Here, we demonstrate an analog of HOM interference between two photons of completely different color. To do so, we utilize a quantum frequency converter based on sum- and difference-frequency generation as an `active' beam splitter -- coupling frequency-entangled red and telecom single photons with an octave-spanning energy difference of 282 THz. We achieve an uncorrected two-photon interference visibility beyond 90%. This work presents the first demonstration of HOM interference between two single photons of distinctly different color, deepening our understanding of what underlies quantum interference. It also suggests a novel approach to interfacing photonic qubits in heterogeneous quantum systems where frequency conversion and quantum interference are unified.

quant-ph↗

arXiv2025

Mid-IR hyperspectral imaging with undetected photons

Sensing with undetected photons has become a vibrant, application-driven research domain with a special focus on the mid-infrared (mid-IR) wavelength region. Since the mid-IR contains spectral bands with highly specific and strong molecular absorbance signatures, often referred to as fingerprints, a multitude of different samples and their compositions can be detected and quantified spectroscopically. Enhancing this inherently sample alteration-free spectroscopic method with imaging capabilities leads to a powerful technique for environmental monitoring and biomedical applications that enables automated diagnostics while omitting time-consuming and non-reversible labeling steps. To evade the shortcomings of state-of-the-art instruments for mid-IR hyperspectral microscopy related to cost, complexity, power-consumption, and performance, which are associated with technological challenges for mid-IR cameras and low-noise and broadband mid-IR sources, here, we construct a proof-of-concept nonlinear interferometer in a wide-field imaging arrangement combined with high-resolution spectral acquisition by pixelwise quantum Fourier transform infrared spectroscopy. For the broadband range of 2300-3100 cm$^{-1}$, covering the important CH-stretch band, we perform hyperspectral imaging that simultaneously resolves 3500 spatial modes, each with a spectral resolution of 10 cm$^{-1}$ leveraging in total around 10$^5$ spatio-spectrally entangled photon modes. Our image acquisition uses a commercial, megapixel sCMOS camera, while a medium-power and compact c.w. pump laser is the only necessary light source.

physics.optics↗

arXiv2024

The Influence of Experimental Imperfections on Photonic GHZ State Generation

While the advantages of photonic quantum computing, including direct compatibility with communication, are apparent, several imperfections such as loss and distinguishability presently limit actual implementations. These imperfections are unlikely to be completely eliminated, and it is therefore beneficial to investigate which of these are the most dominant and what is achievable under their presence. In this work, we provide an in-depth investigation of the influence of photon loss, multi-photon terms and photon distinguishability on the generation of photonic 3-partite GHZ states via established fusion protocols. We simulate the generation process for SPDC and solid-state-based single-photon sources using realistic parameters and show that different types of imperfections are dominant with respect to the fidelity and generation success probability. Our results indicate what are the dominant imperfections for the different photon sources and in which parameter regimes we can hope to implement photonic quantum computing in the near future.

quant-ph↗

arXiv2024

Noise analysis of a quasi-phase-matched quantum frequency converter and higher-order counter-propagating SPDC

Quantum frequency conversion (QFC) will be an indispensable ingredient in future quantum technologies. For example, large-scale fibre-based quantum networks will require QFC to interconnect heterogeneous building blocks like emitters, channels, memories and detectors. The performance of existing QFC devices - typically realised in periodically-poled nonlinear crystals - is often severely limited by parasitic noise that arises when the pump wavelength lies between the inter-converted wavelengths. Here we comprehensively investigate the noise spectrum of a QFC device pumped by a CW 1064 nm laser. The converter was realised as a bulk periodically-poled potassium titanyl phosphate (ppKTP) crystal quasi-phase-matched for conversion between 637 nm and 1587 nm, which was also polished and coated to resonantly enhance the pump field by a factor of 50. While Raman scattering dominates the noise background from 1140 nm to 1330 nm, at larger energy shifts (beyond 60 THz), parasitic spontaneous parametric down-conversion (SPDC) is the strongest noise source. Further, the noise spectrum was contaminated by a regular succession of narrow-band peaks, which we attribute to a heretofore unidentified higher-order counter-propagating SPDC processes - with quasi-phase-matching orders up to 44 evident in our measurements. This work provides a comprehensive overview of the limiting noise sources in QFC devices that use quasi-phase-matched crystals and will prove an invaluable resource in guiding their future development.

quant-ph↗

arXiv2023

Quantum light microscopy

Much of our progress in understanding microscale biology has been powered by advances in microscopy. For instance, super-resolution microscopes allow the observation of biological structures at near-atomic-scale resolution, while multi-photon microscopes allow imaging deep into tissue. However, biological structures and dynamics still often remain out of reach of existing microscopes, with further advances in signal-to-noise, resolution and speed needed to access them. In many cases, the performance of microscopes is now limited by quantum effects -- such as noise due to the quantisation of light into photons or, for multi-photon microscopes, the low cross-section of multi-photon scattering. These limitations can be overcome by exploiting features of quantum mechanics such as entanglement. Quantum effects can also provide new ways to enhance the performance of microscopes, such as new super-resolution techniques and new techniques to image at difficult to reach wavelengths. This review provides an overview of these various ways in which quantum techniques can improve microscopy, including recent experimental progress. It seeks to provide a realistic picture of what is possible, and what the constraints and opportunities are.

quant-ph↗

arXiv2023

Low-noise quantum frequency conversion in a monolithic cavity with bulk periodically poled potassium titanyl phosphate

Interfacing the different building blocks of a future large scale quantum network will demand efficient and noiseless frequency conversion of quantum light. Nitrogen-vacancy (NV) centers in diamond are a leading candidate to form the nodes of such a network. However, the performance of a suitable converter remains a bottleneck, with existing demonstrations severely limited by parasitic noise arising at the target telecom wavelength. Here, we demonstrate a new platform for efficient low-noise quantum frequency conversion based on a monolithic bulk ppKTP cavity and show its suitability for the conversion of 637 nm single photons from NV centers in diamond to telecommunication wavelengths. By resonantly enhancing the power of an off-the-shelf pump laser, we achieve an internal conversion efficiency of $(72.3\pm 0.4)\%$ while generating only $(110\pm 4) \mbox{ kHz/nm}$ noise at the target wavelength without the need for any active stabilization. This constitutes a 5-fold improvement in noise over existing state-of-the-art single-step converters at this wavelengths. We verify the almost ideal preservation of non-classical correlations by converting photons from a spontaneous parametric down-conversion source and moreover show the preservation of time-energy entanglement via Franson interferometry.

quant-ph↗

arXiv2021

Mid-IR spectroscopy with NIR grating spectrometers

Mid-infrared (mid-IR) spectroscopy is a crucial workhorse for a plethora of analytical applications and is suitable for diverse materials, including gases, polymers or biological tissue. However, this technologically significant wavelength regime between 2.5-10$μ$m suffers from technical limitations primarily related to the large noise in mid-IR detectors and the complexity and cost of bright, broadband mid-IR light sources. Here, using highly non-degenerate, broadband photon pairs from bright spontaneous parametric down-conversion (SPDC) in a nonlinear interferometer, we circumvent these limitations and realise spectroscopy in the mid-IR using only a visible (VIS) solid-state laser and an off-the-shelf, commercial near-infrared (NIR) grating spectrometer. With this proof-of-concept implementation, covering a broad range from 3.2$μ$m to 4.4$μ$m, we access short integration times down to 1s and signal-to-noise ratios above 200 at a spectral resolution from 12cm$^{-1}$ down to 1.5cm$^{-1}$ for longer integration times. Through the analysis of polymer samples and the ambient CO$_2$ in our laboratory, we highlight the potential of this measurement technique for real-world applications.

physics.optics↗

arXiv2021

Mid-Infrared Microscopy via Position Correlations of Undetected Photons

Quantum imaging with undetected photons (QIUP) has recently emerged as a new powerful imaging tool. Exploiting the spatial entanglement of photon pairs, it allows decoupling of the sensing and detection wavelengths, facilitating imaging in otherwise challenging spectral regions with mature silicon-based detection technology. All existing implementations of QIUP have so far utilised the momentum correlations within the biphoton state. Here, for the first time, we implement and examine theoretically and numerically the complementary scenario - utilising the tight position correlations formed within photon pair at birth. This image plane arrangement facilitates high resolution imaging with comparative experimental ease, and we experimentally show resolutions below 10 $μ$m at a sensing wavelength of 3.7 $μ$m. Moreover, imaging a slice of mouse heart tissue at the mid-IR to reveal morphological features on the cellular level, we further demonstrate the viability of the technique for the life sciences. These results offer new perspectives on the capabilities of QIUP for label-free wide-field microscopy, enabling new real-world applications in biomedical as well as industrial imaging at inaccessible wavelengths.

quant-ph↗

arXiv2021

Low random duty-cycle errors in periodically-poled KTP revealed by sum-frequency generation

Low-noise quantum frequency conversion in periodically-poled nonlinear crystals has proved challenging when the pump wavelength is shorter than the target wavelength. This is - at least in large part - a consequence of the parasitic spontaneous parametric down-conversion of pump photons, whose efficiency is increased by fabrication errors in the periodic poling. Here we characterise the poling quality of commercial periodically-poled bulk potassium titanyl phosphate (ppKTP) by measuring the sum-frequency generation (SFG) efficiency over a large phase mismatch range from 0 to more than 400$π$. Over the probed range the SFG efficiency behaves nearly ideally and drops to a normalised efficiency of $10^{-6}$. Our results demonstrate that any background pedestal which would be formed by random duty cycle errors in ppKTP is substantially reduced when compared to periodically poled lithium niobate. The standard deviation of the random duty cycle errors can be estimated to be smaller than 2% of the domain length. From this, we expect a noise spectral density which is at least one order of magnitude smaller than that of current state-of-the-art single-step frequency converters.

quant-ph↗

arXiv2020

Frequency-domain optical coherence tomography with undetected mid-infrared photons

Mid-infrared light scatters much less than shorter wavelengths, allowing greatly enhanced penetration depths for optical imaging techniques such as optical coherence tomography (OCT). However, both detection and broadband sources in the mid-IR are technologically challenging. Interfering entangled photons in a nonlinear interferometer enables sensing with undetected photons making mid-IR sources and detectors obsolete. Here we implement mid-infrared frequency-domain OCT based on ultra-broadband entangled photon pairs. We demonstrate 10 $μ$m axial and 20 $μ$m lateral resolution 2D and 3D imaging of strongly scattering ceramic and paint samples. Together with $10^6$ times less noise scaled for the same amount of probe light and also vastly reduced footprint and technical complexity this technique can outperform conventional approaches with classical mid-IR light.

physics.optics↗

arXiv2020

Microscopy with undetected photons in the mid-infrared

Owing to its capacity for unique (bio)-chemical specificity, microscopy withmid-IR illumination holds tremendous promise for a wide range of biomedical and industrial applications. The primary limitation, however, remains detection; with current mid-IR detection technology often marrying inferior technical capabilities with prohibitive costs. This has lead to approaches that shift detection towavelengths into the visible regime, where vastly superior silicon-based cameratechnology is available. Here, we experimentally show how nonlinear interferometry with entangled light can provide a powerful tool for mid-IR microscopy, while only requiring near-infrared detection with a standard CMOS camera. In this proof-of-principle implementation, we demonstrate intensity imaging overa broad wavelength range covering 3.4-4.3um and demonstrate a spatial resolution of 35um for images containing 650 resolved elements. Moreover, we demonstrate our technique is fit for purpose, acquiring microscopic images of biological tissue samples in the mid-IR. These results open a new perspective for potential relevance of quantum imaging techniques in the life sciences.

physics.optics↗

arXiv2020

Quantum-enhanced stimulated emission microscopy

Nonlinear optical microscopy techniques have emerged as a set of successful tools for biological imaging. Stimulated emission microscopy belongs to a small subset of pump-probe techniques which can image non-fluorescent samples without requiring fluorescent labelling. However, its sensitivity has been shown to be ultimately limited by the quantum fluctuations in the probe beam. We propose and experimentally implement sub-shot-noise limited stimulated emission microscopy by preparing the probe pulse in an intensity-squeezed state. This technique paves the way for imaging delicate biological samples that have no detectable fluorescence with sensitivity beyond standard quantum fluctuations.

quant-ph↗

arXiv2020

Interfering distinguishable photons

One of the central principles of quantum mechanics is that if there are multiple paths that lead to the same event, and there is no way to distinguish between them, interference occurs. It is usually assumed that distinguishing information in the preparation, evolution or measurement of a system is sufficient to destroy interference. For example, determining which slit a particle takes in Young's double slit experiment or using distinguishable photons in the two-photon Hong-Ou-Mandel effect allow discrimination of the paths leading to detection events, so in both cases interference vanishes. Remarkably for more than three independent quantum particles, distinguishability of the prepared states is not a sufficient condition for multiparticle interference to disappear. Here we experimentally demonstrate this for four photons prepared in pairwise distinguishable states, thus fundamentally challenging intuition of multiparticle interference.

quant-ph↗

arXiv2019

Ultra-broadband SPDC for spectrally far separated photon pairs

Generating photon pairs via spontaneous parametric down-conversion (SPDC) in nonlinear crystals is important for a wide range of quantum optics experiments with spectral properties such as their bandwidths often being a crucial concern. Here, we show the generic existence of particular phase-matching conditions in quasi-phase matched KTP, MgO:LN and SLT crystals that lead to ultra-broadband, widely non-degenerate photon pairs. It is based on the existence of group-velocity matched, far apart wavelength pairs and for 2 mm long crystals results in SPDC bandwidths between 15 and 25 THz (FWHM) for photon pairs with the idler photon in the technologically relevant mid-IR range 3-5 μm and the signal photon in the NIR below 1100 nm. We experimentally demonstrate this type of broadband phase-matching in ppKTP crystals for photon pairs centered at 800 nm and 3800 nm and measure a bandwidth of 15 THz. This novel method of generating broadband photon-pairs will be highly beneficial for SPDC-based imaging, spectroscopy, refractometry and OCT with undetected mid-IR photons.

quant-ph↗

arXiv2018

Entanglement properties of a measurement-based entanglement distillation experiment

Measures of entanglement can be employed for the analysis of numerous quantum information protocols. Due to computational convenience, logarithmic negativity is often the choice in the case of continuous variable systems. In this work, we analyse a continuous variable measurement-based entanglement distillation experiment using a collection of entanglement measures. This includes: logarithmic negativity, entanglement of formation, distillable entanglement, relative entropy of entanglement, and squashed entanglement. By considering the distilled entanglement as a function of the success probability of the distillation protocol, we show that the logarithmic negativity surpasses the bound on deterministic entanglement distribution at a relatively large probability of success. This is in contrast to the other measures which would only be able to do so at much lower probabilities, hence demonstrating that logarithmic negativity alone is inadequate for assessing the performance of the distillation protocol. In addition to this result, we also observed an increase in the distillable entanglement by making use of upper and lower bounds to estimate this quantity. We thus demonstrate the utility of these theoretical tools in an experimental setting.

quant-ph↗