arXiv subjects

Helmut Ritsch

Publications and source records attributed to Helmut Ritsch.

At least 37 records · Page 2Linked to original sources

arXiv2024

Combining critical and quantum metrology

Critical metrology relies on the precise preparation of a system in its ground state near a quantum phase transition point where quantum correlations get very strong. Typically this increases the quantum Fisher information with respect to changes in system parameters and thus improves the optimally possible measurement precision limited by the Cramér-Rao bound. Hence critical metrology involves encoding information about the unknown parameter in changes of the system's ground state. Conversely, in conventional metrology methods like Ramsey interferometry, the eigenstates of the system remain unchanged, and information about the unknown parameter is encoded in the relative phases that excited system states accumulate during their time evolution. Here we introduce an approach combining these two methodologies into a unified protocol applicable to closed and driven-dissipative systems. We show that the quantum Fisher information in this case exhibits an additional interference term originating from the interplay between eigenstate and relative phase changes. We provide analytical expressions for the quantum and classical Fisher information in such a setup, elucidating as well a straightforward measurement approach that nearly attains the maximum precision permissible under the Cramér-Rao bound. We showcase these results by focusing on the squeezing Hamiltonian, which characterizes the thermodynamic limit of Dicke and Lipkin-Meshkov-Glick Hamiltonians.

quant-ph↗

arXiv2024

Unique Steady-State Squeezing in a Driven Quantum Rabi Model

Squeezing is essential to many quantum technologies and our understanding of quantum physics. Here we develop a theory of steady-state squeezing that can be generated in the closed and open quantum Rabi as well as Dicke model. To this end, we eliminate the spin dynamics which effectively leads to an abstract harmonic oscillator whose eigenstates are squeezed with respect to the physical harmonic oscillator. The generated form of squeezing has the unique property of time-independent uncertainties and squeezed dynamics, a novel type of quantum behavior. Such squeezing might find applications in continuous back-action evading measurements and should already be observable in optomechanical systems and Coulomb crystals.

quant-ph↗

arXiv2023

Scaling law for Kasha's rule in photoexcited molecular aggregates

We study the photophysics of molecular aggregates from a quantum optics perspective, with emphasis on deriving scaling laws for the fast non-radiative relaxation of collective electronic excitations, referred to as Kasha's rule. Aggregates exhibit an energetically broad manifold of collective states with delocalized electronic excitations originating from near field dipole-dipole exchanges between neighboring monomers. Photo-excitation at optical wavelengths, much larger than the monomer-monomer average separation, addresses almost exclusively symmetric collective states, which for an arrangement known as H-aggregate, show an upward hypsochromic shift. The extremely fast subsequent non-radiative relaxation via intramolecular vibrational modes populates lower energy, subradiant states, resulting in an effective inhibition of fluorescence. Our analytical treatment allows for the derivation of an approximate scaling law of this relaxation process, linear in the number of available low energy vibrational modes and directly proportional to the dipole-dipole interaction strength between neighbouring monomers.

quant-ph↗

arXiv2023

A superradiant two-level laser with intrinsic light force generated gain

The implementation of a superradiant laser as an active frequency standard is predicted to provide better short-term stability and robustness to thermal and mechanical fluctuations when compared to standard passive optical clocks. However, despite significant recent progress, the experimental realization of continuous wave superradiant lasing still remains an open challenge as it requires continuous loading, cooling, and pumping of active atoms within an optical resonator. Here we propose a new scenario for creating continuous gain by using optical forces acting on the states of a two-level atom via bichromatic coherent pumping of a cold atomic gas trapped inside a single-mode cavity. Analogous to atomic maser setups, tailored state-dependent forces are used to gather and concentrate excited-state atoms in regions of strong atom-cavity coupling while ground-state atoms are repelled. To facilitate numerical simulations of a sufficiently large atomic ensemble, we rely on a second-order cumulant expansion and describe the atomic motion in a semi-classical point-particle approximation subject to position-dependent light shifts which induce optical gradient forces along the cavity axis. We study minimal conditions on pump laser intensities and detunings required for collective superradiant emission. Balancing Doppler cooling and gain-induced heating we identify a parameter regime of a continuous narrow-band laser operation close to the bare atomic frequency.

quant-ph↗

arXiv2023

Tuning photon-mediated interactions in a multimode cavity: from supersolid to insulating droplets hosting phononic excitations

Ultracold atoms trapped in laser-generated optical lattices serve as a versatile platform for quantum simulations. However, as these lattices are infinitely stiff, they do not allow to emulate phonon degrees of freedom. This restriction can be lifted in emerged optical lattices inside multimode cavities. Motivated by recent experimental progress in multimode cavity QED, we propose a scheme to implement and study supersolid and droplet states with phonon-like lattice excitations by coupling a Bose gas to many longitudinal modes of a ring cavity. The interplay between contact collisional and tunable-range cavity-mediated interactions leads to a rich phase diagram, which includes elastic supersolid as well as insulating droplet phases exhibiting roton-type mode softening for a continuous range of momenta across the superradiant phase transition. The non-trivial dynamic response of the system to local density perturbations further proves the existence of phonon-like modes.

cond-mat.quant-gas↗

arXiv2023

Threshold studies for a hot beam superradiant laser including an atomic guiding potential

Recent theoretical predictions hint at an implementation of a superradiant laser based on narrow optical clock transitions by using a filtered thermal beam at high density. Corresponding numerical studies give encouraging results but the required very high densities are sensitive to beam collimation errors and inhomogeneous shifts. Here we present extensive numerical studies of threshold conditions and the predicted output power of such a superradiant laser involving realistic particle numbers and velocities along the cavity axis. Detailed studies target the threshold scaling as a function of temperature as well as the influence of eliminating the hottest part of the atomic distribution via velocity filtering and the benefits of additional atomic beam guiding. Using a cumulant expansion approach allows us to quantify the significance of atom-atom and atom-field correlations in such configurations. We predict necessary conditions to achieve a certain threshold photon number depending on the atomic temperature and density. In particular, we show that the temperature threshold can be significantly increased by using more atoms. Interestingly, a velocity filter removing very fast atoms has only almost negligible influence despite their phase perturbing properties. On the positive side an additional conservative optical guiding towards cavity mode antinodes leads to significantly lower threshold and higher average photon number. Interestingly we see that higher order atom-field and direct atom-atom quantum correlations play only a minor role in the laser dynamics, which is a bit surprising in the superradiant regime.

physics.atom-ph↗

arXiv2023

Nonequilibrium phases of ultracold bosons with cavity-induced dynamic gauge fields

Gauge fields are a central concept in fundamental theories of physics, and responsible for mediating long-range interactions between elementary particles. Recently, it has been proposed that dynamical gauge fields can be naturally engineered by photons in composite, neutral quantum gas--cavity systems using suitable atom-photon interactions. Here we comprehensively investigate nonequilibrium dynamical phases appearing in a two-leg bosonic lattice model with leg-dependent, dynamical complex tunnelings mediated by cavity-assisted two-photon Raman processes. The system constitutes a minimal dynamical flux-lattice model. We study fixed points of the equations of motion and their stability, the resultant dynamical phase diagram, and the corresponding phase transitions and bifurcations. Notably, the phase diagram features a plethora of nonequilibrium dynamical phases including limit-cycle and chaotic phases. In the end, we relate regular periodic dynamics (i.e., limit-cycle phases) of the system to time crystals.

cond-mat.quant-gas↗

arXiv2023

Collectively enhanced Ramsey readout by cavity sub- to superradiant transition

When an inverted ensemble of atoms is tightly packed on the scale of its emission wavelength or when the atoms are collectively strongly coupled to a single cavity mode, their dipoles will align and decay rapidly via a superradiant burst. However, a spread-out dipole phase distribution theory predicts a required minimum threshold of atomic excitation for superradiance to occur. Here we experimentally confirm this predicted threshold for superradiant emission on a narrow optical transition when exciting the atoms transversely and show how to take advantage of the resulting sub- to superradiant transition. A $π/2$-pulse places the atoms in a subradiant state, protected from collective cavity decay, which we exploit during the free evolution period in a corresponding Ramsey pulse sequence. The final excited state population is read out via superradiant emission from the inverted atomic ensemble after a second $π/2$-pulse, and with minimal heating this allows for multiple Ramsey sequences within one experimental cycle. Our scheme is a fundamentally new approach to atomic state readout characterized by its speed, simplicity, and high sensitivity. It demonstrates the potential of sensors using collective effects in cavity-coupled quantum emitters.

quant-ph↗

arXiv2023

Optical Properties of Concentric Nanorings of Quantum Emitters

A ring of sub-wavelength spaced dipole-coupled quantum emitters features extraordinary optical properties when compared to a one-dimensional chain or a random collection of emitters. One finds the emergence of extremely subradiant collective eigenmodes similar to an optical resonator, which feature strong 3D sub-wavelength field confinement. Motivated by structures commonly appearing in natural light harvesting complexes, we extend these studies to stacked concentric multi-ring geometries. We predict that double rings allow to engineer significantly darker and better confined collective excitation states over a broader energy band compared to the single ring case. These potentially enhance weak field absorption and low loss excitation energy transport. For the specific geometry of the three rings appearing in the natural LH2 antenna we show that the coupling between the lower double ring structure and the higher energy blue shifted single ring is very close to a critical value for the actual size of the molecule. This creates collective excitations with significant contributions from all three rings as a vital ingredient for efficient and fast coherent inter-ring transport. Such a geometry thus should prove useful for the design of sub-wavelength weak field antennas.

quant-ph↗

arXiv2022

Density-wave ordering in a unitary Fermi gas with photon-mediated interactions

A density wave (DW) is a fundamental type of long-range order in quantum matter tied to self-organization into a crystalline structure. The interplay of DW order with superfluidity can lead to complex scenarios that pose a great challenge to theoretical analysis. In the last decades, tunable quantum Fermi gases have served as model systems for exploring the physics of strongly interacting fermions, including most notably magnetic ordering, pairing and superfluidity, and the crossover from a Bardeen-Cooper-Schrieffer (BCS) superfluid to a Bose-Einstein condensate (BEC). Here, we realize a Fermi gas featuring both strong, tunable contact interactions and photon-mediated, spatially structured long-range interactions in a transversely driven high-finesse optical cavity. Above a critical long-range interaction strength DW order is stabilized in the system, which we identify via its superradiant light scattering properties. We quantitatively measure the variation of the onset of DW order as the contact interaction is varied across the BCS-BEC crossover, in qualitative agreement with a mean-field theory. The atomic DW susceptibility varies over an order of magnitude upon tuning the strength and the sign of the long-range interactions below the self-ordering threshold, demonstrating independent and simultaneous control over the contact and long-range interactions. Therefore, our experimental setup provides a fully tunable and microscopically controllable platform for the experimental study of the interplay of superfluidity and DW order.

cond-mat.quant-gas↗

arXiv2022

Squeezing and overcoming the Heisenberg scaling with spin-orbit coupled quantum gases

We predict that exploiting spin-orbit coupling in a harmonically trapped spinor quantum gas can lead to scaling of the optimal measurement precision beyond the Heisenberg scaling. We show that quadratic scaling with the number of atoms can be facilitated via squeezed center-of-mass excitations of the atomic motion using a 1D spin-orbit coupled fermions or strongly interacting bosons (Tonks-Girardeau gas). Based on predictions derived from analytic calculations of the corresponding quantum Fisher information, we then introduce a protocol which overcomes the Heisenberg scaling (and limit) with help of a tailored excited and entangled many-body state of a non-interacting Bose-Einstein condensate. We identify corresponding optimal measurements and argue that even finite temperature as a source of decoherence is, in principle, rather favorable for the obtainable precision scaling.

quant-ph↗

arXiv2022

Control of Localized Multiple Excitation Dark States in Waveguide QED

Subradiant excited states in finite chains of two-level quantum emitters coupled to a one-dimensional reservoir are a resource for superior photon storage and controlled photon manipulation. Typically, states storing multiple excitations exhibit fermionic correlations and are thus characterized by an anti-symmetric wavefunction, which makes them hard to prepare experimentally. Here we identify a class of quasi-localized dark states with up to half of the qubits excited, which appear for lattice constants that are an integer multiple of the guided-mode wavelength. They allow for a high-fidelity preparation and minimally invasive read out in state-of-the-art setups. In particular, we suggest an experimental implementation using a coplanar wave-guide coupled to superconducting transmon qubits on a chip. As free space and intrinsic losses are minimal, virtually perfect dark states can be achieved even for a low number of qubits, enabling fast preparation and manipulation with high fidelity.

quant-ph↗

arXiv2022

Demonstration and modelling of time-bin entangled photons from a quantum dot in a nanowire

Resonant excitation of the biexciton state in an InAsP quantum dot by a phase-coherent pair of picosecond pulses allows preparing time-bin entangled pairs of photons via the biexciton-exciton cascade. We show that this scheme can be implemented for a dot embedded in an InP nanowire. The underlying physical mechanisms can be represented and quantitatively analyzed by an effective three-level open system master equation. Simulation parameters including decay and intensity dependent dephasing rates are extracted from experimental data, which in turn let us predict the resulting entanglement and optimal operating conditions.

quant-ph↗

arXiv2022

Cooperative subwavelength molecular quantum emitter arrays

Dipole-coupled subwavelength quantum emitter arrays respond cooperatively to external light fields as they may host collective delocalized excitations (a form of excitons) with super- or subradiant character. Deeply subwavelength separations typically occur in molecular ensembles, where in addition to photon-electron interactions, electron-vibron couplings and vibrational relaxation processes play an important role. We provide analytical and numerical results on the modification of super- and subradiance in molecular rings of dipoles including excitations of the vibrational degrees of freedom. While vibrations are typically considered detrimental to coherent dynamics, we show that molecular dimers or rings can be operated as platforms for the preparation of long-lived dark superposition states aided by vibrational relaxation. In closed ring configurations, we extend previous predictions for the generation of coherent light from ideal quantum emitters to molecular emitters, quantifying the role of vibronic coupling onto the output intensity and coherence.

quant-ph↗

arXiv2022

Open Quantum-System Simulation of Faraday's Induction Law via Dynamical Instabilities

We propose a novel type of a Bose-Hubbard ladder model based on an open quantum-gas--cavity-QED setup to study the physics of dynamical gauge potentials. Atomic tunneling along opposite directions in the two legs of the ladder is mediated by photon scattering from transverse pump lasers to two distinct cavity modes. The resulting interplay between cavity photon dissipation and the optomechanical atomic back-action then induces an average-density-dependent dynamical gauge field. The dissipation-stabilized steady-state atomic motion along the legs of the ladder leads either to a pure chiral current, screening the induced dynamical magnetic field as in the Meissner effect, or generates simultaneously chiral and particle currents. For sufficiently strong pump the system enters into a dynamically unstable regime exhibiting limit-cycle and period-doubled oscillations. Intriguingly, an electromotive force is induced in this dynamical regime as expected from an interpretation based on Faraday's law of induction for the time-dependent synthetic magnetic flux.

cond-mat.quant-gas↗

arXiv2022

Cavity Sub- and Superradiance Enhanced Ramsey Spectroscopy

Ramsey spectroscopy in large, dense ensembles of ultra-cold atoms trapped in optical lattices suffers from dipole-dipole interaction induced shifts and collective superradiance limiting its precision and accuracy. We propose a novel geometry implementing fast signal readout with minimal heating for large atom numbers at lower densities via an optical cavity operated in the weak single atom but strong collective coupling regime. The key idea is controlled collective transverse $π/2$-excitation of the atoms to prepare a macroscopic collective spin protected from cavity superradiance. This requires that the two halves of the atomic ensemble are coupled to the cavity mode with opposite phase, which is naturally realized for a homogeneously filled volume covering odd and even sites of the cavity mode along the cavity axis. The origin of the superior precision can be traced back to destructive interference among sub-ensembles in the complex nonlinear collective atom field dynamics. In the same configuration we find surprising regular self-pulsing of the cavity output for suitable continuous illumination. Our simulations for large atom numbers employing a cumulant expansion are qualitatively confirmed by a full quantum treatment of smaller ensembles.

cond-mat.quant-gas↗

arXiv2021

QuantumCumulants.jl: A Julia framework for generalized mean-field equations in open quantum systems

A full quantum mechanical treatment of open quantum systems via a Master equation is often limited by the size of the underlying Hilbert space. As an alternative, the dynamics can also be formulated in terms of systems of coupled differential equations for operators in the Heisenberg picture. This typically leads to an infinite hierarchy of equations for products of operators. A well-established approach to truncate this infinite set at the level of expectation values is to neglect quantum correlations of high order. This is systematically realized with a so-called cumulant expansion, which decomposes expectation values of operator products into products of a given lower order, leading to a closed set of equations. Here we present an open-source framework that fully automizes this approach: first, the equations of motion of operators up to a desired order are derived symbolically using predefined canonical commutation relations. Next, the resulting equations for the expectation values are expanded employing the cumulant expansion approach, where moments up to a chosen order specified by the user are included. Finally, a numerical solution can be directly obtained from the symbolic equations. After reviewing the theory we present the framework and showcase its usefulness in a few example problems.

quant-ph↗

arXiv2021

Superradiant lasing in inhomogeneously broadened ensembles with spatially varying coupling

Theoretical studies of superradiant lasing on optical clock transitions predict a superb frequency accuracy and precision closely tied to the bare atomic linewidth. Such a superradiant laser is also robust against cavity fluctuations when the spectral width of the lasing mode is much larger than that of the atomic medium. Recent predictions suggest that this unique feature persists even for a hot and thus strongly broadened ensemble, provided the effective atom number is large enough. Here we use a second-order cumulant expansion approach to study the power, linewidth and lineshifts of such a superradiant laser as a function of the inhomogeneous width of the ensemble including variations of the spatial atom-field coupling within the resonator. We present conditions on the atom numbers, the pump and coupling strengths required to reach the buildup of collective atomic coherence as well as scaling and limitations for the achievable laser linewidth.

quant-ph↗