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Hemant Katiyar

Publications and source records attributed to Hemant Katiyar.

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Experimental Activation of Strong Local Passive States with Quantum Information

Strong local passivity is a property of multipartite quantum systems from which it is impossible to extract energy locally. Surprisingly, if the strong local passive state displays entanglement, it could be possible to locally activate energy density by adding classical communication between different partitions of the system, through so-called "quantum energy teleportation" protocols. Here, we report both the first experimental observation of local activation of energy density on an entangled state and the first realization of a quantum energy teleportation protocol using nuclear magnetic resonance on a bipartite quantum system.

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Fast Simulation of Magnetic Field Gradients for Optimization of Pulse Sequences

We study how to simulate, efficiently, pulse field gradients (PFG) used in nuclear magnetic resonance (NMR). An efficient simulation requires discretization in time and space. We study both discretizations and provide a guideline to choose best discretization values depending on the precision required experimentally. We provide a theoretical study and simulation showing the minimum number of divisions we need in space for simulating, with high precision, a sequence composed of several unitary evolution and PFG. We show that the fast simulation of PFG allow us to optimize sequences composed of PFG, radio-frequency pulses and free evolution, to implement non-unitary evolution (quantum channels). As an evidence of the success of our work, we performed two types of experiments. First, we implement two quantum channels and compare the results with their theoretical predictions. In the second experiment, we used the fast simulation of PFG to optimize and implement a sequence to prepare pseudo pure state with better signal to noise ratio than any known procedure till now.

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Exploration of an augmented set of Leggett-Garg inequalities using a noninvasive continuous-in-time velocity measurement

Macroscopic realism (MR) is the view that a system may possess definite properties at any time independent of past or future measurements, and may be tested experimentally using the Leggett-Garg inequalities (LGIs). In this work we advance the study of LGIs in two ways using experiments carried out on a nuclear magnetic resonance spectrometer. Firstly, we addresses the fact that the LGIs are only necessary conditions for MR but not sufficient ones. We implement a recently-proposed test of necessary and sufficient conditions for MR which consists of a combination of the original four three-time LGIs augmented with a set of twelve two-time LGIs. We explore different regimes in which the two- and three-time LGIs may each be satisfied or violated. Secondly, we implement a recent proposal for a measurement protocol which determines the temporal correlation functions in an approximately non-invasive manner. It employs a measurement of the velocity of a dichotomic variable $Q$, continuous in time, from which a possible sign change of $Q$ may be determined in a single measurement of an ancilla coupled to the velocity. This protocol involves a significantly different set of assumptions to the traditional ideal negative measurement protocol and a comparison with the latter is carried out.

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Gradient-based closed-loop quantum optimal control in a solid-state two-qubit system

Quantum optimal control can play a crucial role to realize a set of universal quantum logic gates with error rates below the threshold required for fault-tolerance. Open-loop quantum optimal control relies on accurate modeling of the quantum system under control, and does not scale efficiently with system size. These problems can be avoided in closed-loop quantum optimal control, which utilizes feedback from the system to improve control fidelity. In this paper, two gradient-based closed-loop quantum optimal control algorithms, the hybrid quantum-classical approach (HQCA) described in [Phys. Rev. Lett. 118, 150503 (2017)] and the finite-difference (FD) method, are experimentally investigated and compared to the open-loop quantum optimal control utilizing the gradient ascent method. We employ a solid-state ensemble of coupled electron-nuclear spins serving as a two-qubit system. Specific single-qubit and two-qubit state preparation gates are optimized using the closed-loop and open-loop methods. The experimental results demonstrate the implemented closed-loop quantum control outperforms the open-loop control in our system. Furthermore, simulations reveal that HQCA is more robust than the FD method to gradient noise which originates from measurement noise in this experimental setting. On the other hand, the FD method is more robust to control field distortions coming from non-ideal hardware

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Enhancing quantum control by bootstrapping a quantum processor of 12 qubits

Accurate and efficient control of quantum systems is one of the central challenges for quantum information processing. Current state-of-the-art experiments rarely go beyond 10 qubits and in most cases demonstrate only limited control. Here we demonstrate control of a 12-qubit system, and show that the system can be employed as a quantum processor to optimize its own control sequence by using measurement-based feedback control (MQFC). The final product is a control sequence for a complex 12-qubit task: preparation of a 12-coherent state. The control sequence is about 10% more accurate than the one generated by the standard (classical) technique, showing that MQFC can correct for unknown imperfections. Apart from demonstrating a high level of control over a relatively large system, our results show that even at the 12-qubit level, a quantum processor can be a useful lab instrument. As an extension of our work, we propose a method for combining the MQFC technique with a twirling protocol, to optimize the control sequence that produces a desired Clifford gate.

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Experimentally superposing two pure states with partial prior knowledge

Superposition, arguably the most fundamental property of quantum mechanics, lies at the heart of quantum information science. However, how to create the superposition of any two unknown pure states remains as a daunting challenge. Recently, it is proved that such a quantum protocol does not exist if the two input states are completely unknown, whereas a probabilistic protocol is still available with some prior knowledge about the input states [M. Oszmaniec \emph{et al.}, Phys. Rev. Lett. 116, 110403 (2016)]. The knowledge is that both of the two input states have nonzero overlaps with some given referential state. In this work, we experimentally realize the probabilistic protocol of superposing two pure states in a three-qubit nuclear magnetic resonance system. We demonstrate the feasibility of the protocol by preparing a families of input states, and the average fidelity between the prepared state and expected superposition state is over 99%. Moreover, we experimentally illustrate the limitation of the protocol that it is likely to fail or yields very low fidelity, if the nonzero overlaps are approaching zero. Our experimental implementation can be extended to more complex situations and other quantum systems.

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Experimental violation of the Leggett-Garg inequality in a 3-level system

The Leggett-Garg (LG) test of macroscopic realism involves a series of dichotomic non-invasive measurements that are used to calculate a function which has a fixed upper bound for a macrorealistic system and a larger upper bound for a quantum system. The quantum upper bound depends on both the details of the measurement and the dimension of the system. Here we present an LG experiment on a three-level quantum system, which produces a larger theoretical quantum upper bound than that of a two-level quantum system. The experiment is carried out in nuclear magnetic resonance (NMR) and consists of the LG test as well as a test of the ideal assumptions associated with the experiment, such as measurement non-invasiveness. The non-invasive measurements are performed via the modified ideal negative result measurement scheme on a three-level system. Once these assumptions are tested, the violation becomes small, despite the fact that the LG value itself is large. Our results showcase the advantages of using the modified measurement scheme that can reach the higher LG values, as they give more room for hypothetical malicious errors in a real experiment

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Ancilla assisted measurements on quantum ensembles: General protocols and applications in NMR quantum information processing

Quantum ensembles form easily accessible architectures for studying various phenomena in quantum physics, quantum information science, and spectroscopy. Here we review some recent protocols for measurements in quantum ensembles by utilizing ancillary systems. We also illustrate these protocols experimentally via nuclear magnetic resonance techniques. In particular, we shall review noninvasive measurements, extracting expectation values of various operators, characterizations of quantum states, and quantum processes, and finally quantum noise engineering.

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NMR investigation of contextuality in a quantum harmonic oscillator via pseudospin mapping

Physical potentials are routinely approximated to harmonic potentials so as to analytically solve the system dynamics. Often it is important to know when a quantum harmonic oscillator (QHO) behaves quantum mechanically and when classically. Recently Su et. al. [Phys. Rev. A {\bf 85}, 052126 (2012)] have theoretically shown that QHO exhibits quantum contextuality (QC) for a certain set of pseudospin observables. In this work, we encode the four eigenstates of a QHO onto four Zeeman product states of a pair of spin-1/2 nuclei. Using the techniques of NMR quantum information processing, we then demonstrate the violation of a state-dependent inequality arising from the noncontextual hidden variable model, under specific experimental arrangements. We also experimentally demonstrate the violation of a state-independent inequality by thermal equilibrium states of nuclear spins, thereby assessing their quantumness.

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NMR quantum information processing

Quantum computing exploits fundamentally new models of computation based on quantum mechanical properties instead of classical physics, and it is believed that quantum computers are able to dramatically improve computational power for particular tasks. At present, nuclear magnetic resonance (NMR) has been one of the most successful platforms amongst all current implementations. It has demonstrated universal controls on the largest number of qubits, and many advanced techniques developed in NMR have been adopted to other quantum systems successfully. In this review, we show how NMR quantum processors can satisfy the general requirements of a quantum computer, and describe advanced techniques developed towards this target. Additionally, we review some recent NMR quantum processor experiments. These experiments include benchmarking protocols, quantum error correction, demonstrations of algorithms exploiting quantum properties, exploring the foundations of quantum mechanics, and quantum simulations. Finally we summarize the concepts and comment on future prospects.

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Freezing a Quantum Magnet by Repeated Quantum Interference: An Experimental Realization

We experimentally demonstrate the phenomenon of dynamical many-body freezing in a periodically driven Ising chain. Theoretically [Phys. Rev. B 82, 172402 (2010)], for certain values of the drive parameters all fundamental degrees of freedom contributing to the response dynamics freeze for all time and for arbitrary initial states. Also, since the condition of freezing involves only the drive parameters and not on the quantization of the momentum (i.e., the system-size), our simulation with a small (3-spin) chain captures all salient features of the freezing phenomenon predicted for the infinite chain. Using optimal control techniques, we realize high-fidelity cosine modulated drive, and observe non-monotonic freezing of magnetization at specific frequencies of modulation. Time-evolution of the excitations in momentum space has been tracked directly through magnetization measurements.

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Estimating Franck-Condon factors using an NMR quantum processor

Interaction of molecules with light may lead to electronic transitions and simultaneous vibrational excitations. Franck-Condon factors (FCFs) play an important role in quantifying the intensities of such vibronic transitions occurring during molecular photo-excitations. In this article, we describe a general method for estimating FCFs using a quantum information processor. The method involves the application of a translation operator followed by the measurement of certain projections. We also illustrate the method by experimentally estimating FCFs with the help of a three-qubit NMR quantum information processor. We describe two methods for the measurement of projections - (i) using diagonal tomography and (ii) using Moussa protocol. The experimental results agree fairly well with the theory.

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Monogamy of quantum correlations reveals frustration in a quantum Ising spin system: Experimental demonstration

We report a nuclear magnetic resonance experiment, which simulates the quantum transverse Ising spin system in a triangular configuration and further show that the monogamy of quantum correlations can be used to distinguish between the frustrated and non-frustrated regimes in the ground state of this system. Adiabatic state preparation methods are used to prepare the ground states of the spin system. We employ two different multipartite quantum correlation measures to analyze the experimental ground state of the system in both the frustrated and non-frustrated regimes. In particular, we use multipartite quantum correlation measures generated by monogamy considerations of negativity, a bipartite entanglement measure, and that of quantum discord, an information-theoretic quantum correlation measure. As expected from theoretical predictions, the experimental data confirm that the non-frustrated regime shows higher multipartite quantum correlations compared to the frustrated one.

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Inversion of moments to retrieve joint probabilities in quantum sequential measurements

A sequence of moments encode the corresponding probability distribution. Probing if quantum joint probability distribution can be retrieved from the associated set of moments -- realized in the sequential measurement of a dichotomic observable at different time intervals -- reveals a negative answer i.e., the joint probabilities of sequential measurements do not agree with the ones obtained by inverting the moments. This is indeed a reflection of the non-existence of a bonafide grand joint probability distribution, consistent with all the physical marginal probability distributions. Here we explicitly demonstrate that given the set of moments, it is not possible to retrieve the three-time quantum joint probability distribution resulting from quantum sequential measurement of a single qubit dichotomic observable at three different times. Experimental results using a nuclear magnetic resonance (NMR) system are reported here to corroborate these theoretical observations viz., the incompatibility of the three-time joint probabilties with those extracted from the moment sequence.

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Violation of Entropic Leggett-Garg Inequality in Nuclear Spins

We report an experimental study of recently formulated entropic Leggett-Garg inequality (ELGI) by Usha Devi et al. (arXiv: 1208.4491v2 (2012)). This inequality places a bound on the statistical measurement outcomes of dynamical observables describing a macrorealistic system. Such a bound is not necessarily obeyed by quantum systems, and therefore provides an important way to distinguish quantumness from classical behavior. Here we study ELGI using a two-qubit nuclear magnetic resonance system. To perform the noninvasive measurements required for the ELGI study, we prepare the system qubit in a maximally mixed state as well as use the `ideal negative result measurement' procedure with the help of an ancilla qubit. The experimental results show a clear violation of ELGI by over four standard deviations. These results agree with the predictions of quantum theory. The violation of ELGI is attributed to the fact that certain joint probabilities are not legitimate in the quantum scenario, in the sense they do not reproduce all the marginal probabilities. Using a three-qubit system, we experimentally demonstrate that three-time joint probabilities do not reproduce certain two-time marginal probabilities.

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Evolution of Quantum Discord and its Stability in Two-Qubit NMR Systems

We investigate evolution of quantum correlations in ensembles of two-qubit nuclear spin systems via nuclear magnetic resonance techniques. We use discord as a measure of quantum correlations and the Werner state as an explicit example. We first introduce different ways of measuring discord and geometric discord in two-qubit systems and then describe the following experimental studies: (a) We quantitatively measure discord for Werner-like states prepared using an entangling pulse sequence. An initial thermal state with zero discord is gradually and periodically transformed into a mixed state with maximum discord. The experimental and simulated behavior of rise and fall of discord agree fairly well. (b) We examine the efficiency of dynamical decoupling sequences in preserving quantum correlations. In our experimental setup, the dynamical decoupling sequences preserved the traceless parts of the density matrices at high fidelity. But they could not maintain the purity of the quantum states and so were unable to keep the discord from decaying. (c) We observe the evolution of discord for a singlet-triplet mixed state during a radio-frequency spin-lock. A simple relaxation model describes the evolution of discord, and the accompanying evolution of fidelity of the long-lived singlet state, reasonably well.

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