Henrique G. Rosa | Searcharxiv

arXiv2025

1T'-MoTe$_2$ as an integrated saturable absorber for photonic machine learning

We investigate the saturable absorption behavior of a 1T'-MoTe$_2$ monolayer integrated with a silicon nitride waveguide for applications in photonic neural networks. Using experimental transmission measurements and theoretical modeling, we characterize the nonlinear response of the material. Our model, incorporating quasi-Fermi level separation and carrier dynamics, successfully explains these behaviors and predicts the material's absorption dependence on the carrier density. Furthermore, we demonstrate a coupling efficiency of up to 20% between the 1T'-MoTe$_2$ monolayer and the silicon nitride waveguide, with saturation achievable at input powers as low as a few uW. These results suggest that 1T'-MoTe$_2$ is a promising candidate for implementing nonlinear functions in integrated photonic neural networks.

physics.optics↗

arXiv2019

Characterization of the second- and third-harmonic optical susceptibilities of atomically thin tungsten diselenide

We report the first detailed characterization of the sheet third-harmonic optical susceptibility, $χ_{s}^{(3)}$, of tungsten diselenide (WSe$_{2}$). With a home-built confocal microscope setup developed to study harmonics generation, we map the second- and third-harmonic intensities as a function of position in the sample, pump power and polarization angle, for single and few layers flakes of WSe$_{2}$. We register a value of $|χ_{s}^{(3)}| \approx$ 0.91 $\times$ 10$^{-28}$ m$^{3}$ V$^{-2}$ at a fundamental excitation frequency of $\hbarω$ = 0.8 eV, which is comparable in magnitude to the third-harmonic susceptibility of other group-VI transition metal dichalcogenides. The simultaneously recorded second-harmonic susceptibility is found to be $|χ_{s}^{(2)}| \approx$ 0.70 $\times$ 10$^{-19}$ m$^{2}$ V$^{-1}$ in very good agreement on the order of magnitude with recent reports for WSe$_{2}$, which asserts the robustness of our values for $|χ_{s}^{(3)}|$.

physics.optics↗