arXiv subjects

Heon-Jung Kim

Publications and source records attributed to Heon-Jung Kim.

At least 19 recordsLinked to original sources

arXiv2019

Magnetic field-induced type-II Weylsemimetallic state in geometrically frustrated Shastry-Sutherland lattice GdB4

Weyl semimetal is a topologically non-trivial phase of matter with pairs of Weyl nodes in the k-space, which act as monopole and anti-monopole pairs of Berry curvature. Two hallmarks of the Weyl metallic state are the topological surface state called the Fermi arc and the chiral anomaly. It is known that the chiral anomaly yields anomalous magneto-transport phenomena. In this study, we report the emergence of the type-II Weyl semimetallic state in the geometrically frustrated non-collinear antiferromagnetic Shastry-Sutherland lattice (SSL) GdB4 crystal. When we apply magnetic fields perpendicular to the noncollinear moments in SSL plane, Weyl nodes are created above and below the Fermi energy along the M-A line (tau-band) because the spin tilting breaks the time-reversal symmetry and lifts band degeneracy while preserving C4z or C2z symmetry. The unique electronic structure of GdB4 under magnetic fields applied perpendicular to the SSL gives rise to a non-trivial Berry phase, detected in de Haas-van Alphen experiments and chiral-anomaly-induced negative magnetoresistance. The emergence of the magnetic field-induced Weyl state in SSL presents a new guiding principle to develop novel types of Weyl semimetals in frustrated spin systems.

cond-mat.mtrl-sci↗

arXiv2018

Observation of the possible chiral edge mode in Bi1-xSbx

After the classification of topological states of matter has been clarified for non-interacting electron systems, the theoretical connection between gapless boundary modes and nontrivial bulk topological structures, and their evolutions as a function of dimensions are now well understood. However, such dimensional hierarchy has not been well established experimentally although some indirect evidences were reported, for example, such as the half-quantized Hall conductance via quantum Hall effect and extrapolation in the quantum-oscillation measurement. In this paper, we report the appearance of the possible chiral edge mode from the surface state of topological insulators under magnetic fields, confirming the dimensional hierarchy in three dimensional topological insulators. Applying laser pulses to the surface state of Bi1-xSbx, we find that the sign of voltage relaxation in one edge becomes opposite to that in the other edge only when magnetic fields are applied to the topological insulating phase. We show that this sign difference originates from the chirality of edge states, based on coupled time-dependent Poisson and Boltzmann equations.

cond-mat.str-el↗

arXiv2016

Two-parameter scaling theory of the longitudinal magnetoconductivity in a Weyl metal phase: Chiral anomaly, weak disorder, and finite temperature

It is at the heart of modern condensed matter physics to investigate the role of a topological structure in anomalous transport phenomena. In particular, chiral anomaly turns out to be the underlying mechanism for the negative longitudinal magnetoresistivity in a Weyl metal phase. Existence of a dissipationless current channel causes enhancement of electric currents along the direction of a pair of Weyl points or applied magnetic fields ($B$). However, temperature ($T$) dependence of the negative longitudinal magnetoresistivity has not been understood yet in the presence of disorder scattering since it is not clear at all how to introduce effects of disorder scattering into the "topological-in-origin" transport coefficient at finite temperatures. The calculation based on the Kubo formula of the current-current correlation function is simply not known for this anomalous transport coefficient. Combining the renormalization group analysis with the Boltzmann transport theory to encode the chiral anomaly, we reveal how disorder scattering renormalizes the distance between a pair of Weyl points and such a renormalization effect modifies the topological-in-origin transport coefficient at finite temperatures. As a result, we find breakdown of $B/T$ scaling, given by $B/T^{1 + η}$ with $0 < η< 1$. This breakdown may be regarded to be a fingerprint of the interplay between disorder scattering and topological structure in a Weyl metal phase.

cond-mat.dis-nn↗

arXiv2015

Interplay between disorder and inversion symmetry: Extreme enhancement of the mobility near the Weyl point in BiTeI

We show experimental and theoretical evidence that BiTeI hosts a novel disordered metallic state named diffusive helical Fermi liquid (DHFL), characterized by a pair of concentric spin-chiral Fermi surfaces with negligible inter-valley scattering. Key experimental observations are extreme disparity of the mobility between inner and outer helical Fermi surfaces near the Weyl point and existence of the so called universal scaling behavior for the Hall resistivity. Although the extreme enhancement of the inner-Fermi-surface mobility near the Weyl point is quantitatively explained within the self-consistent Born approximation, the existence of universal scaling in the Hall resistivity shows its breakdown, implying necessity of mass renormalization in the inner Fermi-surface beyond the independent electron picture.

cond-mat.str-el↗

arXiv2014

Anomalous transport phenomena in Weyl metal beyond the Drude model for Landau's Fermi liquids

Landau's Fermi-liquid theory is the standard model for metals, characterized by the existence of electron quasiparticles near a Fermi surface as long as Landau's interaction parameters lie below critical values for instabilities. Recently, this fundamental paradigm has been challenged by physics of strong spin-orbit coupling although the concept of electron quasiparticles remains valid near the Fermi surface, where the Landau's Fermi-liquid theory fails to describe electromagnetic properties of this novel metallic state, referred to as Weyl metal. A novel ingredient is that such a Fermi surface encloses a Weyl point with definite chirality, referred to as a chiral Fermi surface, which can arise from breaking of either time reversal or inversion symmetry in systems with strong spin-orbit coupling, responsible for both Berry curvature and chiral anomaly. As a result, electromagnetic properties of the Weyl metallic state are described not by conventional Maxwell equations but by axion electrodynamics, where Maxwell equations are modified with a topological-in-origin spatially modulated $θ(\bm{r}) \bm{E} \cdot \bm{B}$ term. This novel metallic state has been realized recently in Bi$_{1-x}$Sb$_{x}$ around $x \sim 3%$ under magnetic fields, where the Dirac spectrum appears around the critical point between the normal semiconducting ($x < 3%$) and topological semiconducting phases ($x > 3%$) and the time reversal symmetry breaking perturbation causes the Dirac point to split into a pair of Weyl points along the direction of the applied magnetic field for such a strong spin-orbit coupled system. In this review article, we discuss how the topological structure of both the Berry curvature and chiral anomaly (axion electrodynamics) gives rise to anomalous transport phenomena in Bi$_{1-x}$Sb$_{x}$ around $x \sim 3%$ under magnetic fields, modifying the Drude model of Landau's Fermi liquids.

cond-mat.mes-hall↗

arXiv2014

Boltzmann-equation approach to anomalous transport in a Weyl metal

Weyl metal is regarded as a platform toward interacting topological states of matter, where its topological structure gives rise to anomalous transport phenomena, referred to as chiral magnetic effect and "negative" magneto-resistivity, the origin of which is chiral anomaly. Recently, the negative magneto-resistivity has been observed with the signature of weak anti-localization at $x = 3 \sim 4 ~ \%$ in Bi$_{1-x}$Sb$_{x}$, where magnetic field is applied in parallel with electric field. Based on the Boltzmann-equation approach, we find the negative magneto-resistivity in the presence of weak anti-localization. An essential ingredient is to introduce the topological structure of chiral anomaly into the Boltzmann-equation approach, resorting to semi-classical equations of motion with Berry curvature.

cond-mat.str-el↗

arXiv2013

Dirac vs. Weyl in topological insulators: Adler-Bell-Jackiw anomaly in transport phenomena

Dirac metals (gapless semi-conductors) are believed to turn into Weyl metals when perturbations, which break either time reversal symmetry or inversion symmetry, are employed. However, no experimental evidence has been reported for the existence of Weyl fermions in three dimensions. Applying magnetic fields near the topological phase transition from a topological insulator to a band insulator in Bi1-xSbx, we observe not only the weak anti-localization phenomenon in magnetoconductivity near zero magnetic fields (B < 0.4 T) but also its upturn above 0.4 T only for E // B. This incompatible coexistence between weak anti-localization and negative magnetoresistivity is attributed to the Adler-Bell-Jackiw anomaly (topological E B term) in the presence of weak anti-localization corrections.

cond-mat.str-el↗

arXiv2013

Topological phase transitions driven by magnetic phase transitions in FexBi2Te3 (0 < x < 0.1) single crystals

We propose a phase diagram for FexBi2Te3 (0 < x < 0.1) single crystals, which belong to a class of magnetically bulk-doped topological insulators. The evolution of magnetic correlations from ferromagnetic- to antiferromagnetic- gives rise to topological phase transitions, where the paramagnetic topological insulator of Bi2Te3 turns into a band insulator with ferromagnetic-cluster glassy behaviours around x ~ 0.025, and it further evolves to a topological insulator with valence-bond glassy behaviours, which spans over the region between x ~ 0.03 up to x ~ 0.1. This phase diagram is verified by measuring magnetization, magnetotransport, and angle-resolved photoemission spectra with theoretical discussions.

cond-mat.str-el↗

arXiv2011

Interplay between the Kondo effect and randomness: Griffiths phase in MxTiSe2 (M = Co, Ni, and Fe) single crystals

We investigate the interplay between the Kondo effect and randomness in MxTiSe2 (M = Co, Ni, and Fe) single crystals. Although the typical low-T upturn of resistivity implies the Kondo effect around the single-ion Kondo temperature \overline{T}_{K}, positive magnetoresistance linearly proportional to the magnetic field and the power-law scaling of magnetization suggest the forbidden coexistence between Kondo effect and time reversal symmetry breaking. This puzzling result is resolved by the Griffiths scenario - disorder-induced distribution of the Kondo temperature produces an effective Kondo temperature (\overline{T}_{K}) much lower than \overline{T}_{K}, allowing unscreened local moments above \overline{T}_{K} and resulting in non-Fermi liquid properties in MxTiSe2 below the percolation threshold (x<xc).

cond-mat.str-el↗

arXiv2011

Sondheimer Oscillation as a Fingerprint of Surface Dirac Fermions

Topological states of matter challenge the paradigm of symmetry breaking, characterized by gapless boundary modes and protected by the topological property of the ground state. Recently, angle-resolved photoemission spectroscopy (ARPES) has revealed that semiconductors of Bi$_{2}$Se$_{3}$ and Bi$_{2}$Te$_{3}$ belong to such a class of materials. Here, we present undisputable evidence for the existence of gapless surface Dirac fermions from transport in Bi$_{2}$Te$_{3}$. We observe Sondheimer oscillation in magnetoresistance (MR). This oscillation originates from the quantization of motion due to the confinement of electrons within the surface layer. Based on Sondheimer's transport theory, we determine the thickness of the surface state from the oscillation data. In addition, we uncover the topological nature of the surface state, fitting consistently both the non-oscillatory part of MR and the Hall resistance. The side-jump contribution turns out to dominate around 1 T in Hall resistance while the Berry-curvature effect dominates in 3 T $\sim$ 4 T.

cond-mat.str-el↗

arXiv2005

Comparison of $H_{c2}(T,θ)$ in Mg$_{1-x}$Al$_x$B$_2$ single crystals with the dirty-limit two-gap theory

We studied the temperature and the angular dependences of the upper critical field ($H_{c2}(T,θ$)) of Mg$_{1-x}$Al$_x$B$_2$ single crystals ($x = 0.12$ and 0.21) and compared with the dirty-limit two-gap theory. We found that $H_{c2}(T,θ)$'s were well described in a unified way by this theory. The obtained values of the parameters indicated that as the Al concentration was increased, anisotropic impurity scattering increased, making the $σ$ bands less anisotropic. Accordingly, the temperature dependence of the anisotropy ratio of $H_{c2}$ ($γ_H$) systematically decreased, and for $x=0.21$, $γ_H$ was nearly constant. Our results imply that Mg$_{1-x}$Al$_x$B$_2$ single crystals are in dirty-limit and that two-gap nature survives until $x = 0.21$.

cond-mat.supr-con↗

arXiv2005

Observation of the spontaneous vortex phase in the weakly ferromagnetic superconductor ErNi$_{2}$B$_{2}$C: A penetration depth study

The coexistence of weak ferromagnetism and superconductivity in ErNi$_{2}$B$% _{2}$C suggests the possibility of a spontaneous vortex phase (SVP) in which vortices appear in the absence of an external field. We report evidence for the long-sought SVP from the in-plane magnetic penetration depth $Δλ(T)$ of high-quality single crystals of ErNi$_{2}$B$_{2}$C. In addition to expected features at the Néel temperature $T_{N}$ = 6.0 K and weak ferromagnetic onset at $T_{WFM}=2.3 $K, $Δλ(T)$ rises to a maximum at $T_{m}=0.45$ K before dropping sharply down to $\sim $0.1 K. We assign the 0.45 K-maximum to the proliferation and freezing of spontaneous vortices. A model proposed by Koshelev and Vinokur explains the increasing $Δλ(T)$ as a consequence of increasing vortex density, and its subsequent decrease below $T_{m}$ as defect pinning suppresses vortex hopping.

cond-mat.supr-con↗

arXiv2004

Reversible magnetization measurement of the anisotropy of the London penetration depth in MgB2 single crystals

We have studied the anisotropy of the London penetration depth, which was obtained from reversible magnetization measurements with the magnetic field both parallel and perpendicular to the c-axis. The anisotropy of the London penetration depth has a smaller magnitude than the anisotropy of the upper critical field and increases with temperature while that of the upper critical field decreases as reported earlier. This behavior is in sharp contrast with the behaviors of superconductors with one superconducting energy gap. The temperature dependence of the anisotropies of the London penetration depth and of the upper critical field can be well explained within the theory of two-gap superconductivity in MgB2.

cond-mat.supr-con↗

arXiv2004

Reversible magnetization of MgB2 single crystals with a two-gap nature

We present reversible magnetization measurements on MgB2 single crystals in magnetic fields up to 2.5 T applied parallel to the crystal's c-axis. This magnetization is analyzed in terms of the Hao-Clem model, and various superconducting parameters, such as the critical fields [Hc(0) and Hc2(0)], the characteristic lengths [xi(0) and lambda(0)], and the Ginzburg-Landau parameter, kappa, are derived. The temperature dependence of the magnetic penetration depth, lambda(T), obtained from the Hao-Clem analysis could not be explained by theories assuming a single gap. Our data are well described by using a two-gap model.

cond-mat.supr-con↗

arXiv2002

Effects of unreacted Mg impurities on the transport properties of MgB2

We synthesized polycrystalline MgB2 from a stoichiometric mixture of Mg and the 11 B isotope under different conditions. All the samples showed bulk superconductivity with Tc = 38~39 K. The samples containing the least amount of unreacted Mg showed the highest Tc and the sharpest transition width (Delta_Tc). A residual resistivity ratio (RRR) of ~ 5.8, and a magnetoresistance (MR), at 40 K, of 12% were obtained for these samples. Moreover, there was no upturn of resistivity in a low temperature region at 10 Tesla. The samples containing appreciable amounts of unreacted Mg showed quite different behaviors; the values of Delta_Tc, RRR, and MR were much larger. An upturn appeared in resistivity of the samples below about 50 K at 10 T and is thought to be due to the unreacted Mg.

cond-mat.supr-con↗

arXiv2002

Strongly correlated s-wave pairing in the n-type infinite-layer cuprate

Quasiparticle tunneling spectra of the electron-doped (n-type) infinite-layer cuprate Sr_{0.9}La_{0.1}CuO_2 reveal characteristics that counter a number of common phenomena in the hole-doped (p-type) cuprates. The optimally doped Sr_{0.9}La_{0.1}CuO_2 with T_c = 43 K exhibits a momentum-independent superconducting gap Δ= 13.0 +- 1.0 meV that substantially exceeds the BCS value, and the spectral characteristics indicate insignificant quasiparticle damping by spin fluctuations and the absence of pseudogap. The response to quantum impurities in the Cu-sites also differs fundamentally from that of the p-type cuprates with d_{x^2-y^2}-wave pairing symmetry.

cond-mat.supr-con↗

arXiv2001

Spectroscopic Evidence for Anisotropic S-Wave Pairing Symmetry in MgB2

Scanning tunneling spectroscopy of superconducting MgB$_2$ ($T_c = 39$ K) were studied on high-density pellets and c-axis oriented films. The sample surfaces were chemically etched to remove surface carbonates and hydroxides, and the data were compared with calculated spectra for all symmetry-allowed pairing channels. The pairing potential ($Δ_k$) is best described by an anisotropic s-wave pairing model, with $Δ_k = Δ_{xy} \sin ^2 θ_k + Δ_z \cos ^2 θ_k$, where $θ_k$ is the angle relative to the crystalline c-axis, $Δ_z \sim 8.0$ meV, and $Δ_{xy} \sim 5.0$ meV.

cond-mat.supr-con↗

arXiv2001

X-ray Photoemission Study of the Infinite-Layer Cuprate Superconductor Sr0.9La0.1CuO2

The electron-doped infinite-layer superconductor Sr0.9La0.1CuO2 is studied with x-ray photoemission spectroscopy (XPS). A nonaqueous chemical etchant is shown to effectively remove contaminants and to yield surfaces from which signals intrinsic to the superconductor dominate. These data are compared to measurements from hole-doped La1.85Sr0.15CuO4, from undoped La2CuO4, and from electron-doped Nd1.85Ce0.15CuO4-d. The Cu 2p core level is consistent with a lower value of the O 2p to Cu 3d charge transfer energy D than in hole-doped cuprates. A clear Fermi edge is observed in the valence band region.

cond-mat.supr-con↗