arXiv subjects

Hervé Courtois

Publications and source records attributed to Hervé Courtois.

At least 19 recordsLinked to original sources

arXiv2026

Nanoparticle manipulation with a carbon fiber tip in an electron microscope for $μ$-SQUID magnetometry

We report a carbon-fiber-tip based nanomanipulation system integrated into a scanning electron microscope for individual nanoparticle (NP) manipulation on a surface. Electrochemically etched amorphous carbon fiber tips with excellent mechanical rigidity and sub-100 nm apex radii effectively reduce the van der Waals adhesion and enable reliable positioning of about 100 nm size NPs with about 100 nm precision. This system combines a piezoelectric bimorph for vertical tip motion, a four-quadrant piezo-tube for two-dimensional fine tip control and a two-dimensional piezoelectric walker for coarse lateral translation. Using this setup, we successfully position single Fe$_3$O$_4$ magnetic NPs on micron sized superconducting quantum interference devices for optimal magnetic coupling between them and probe a NP's magnetism.

cond-mat.mes-hall↗

arXiv2024

Heat transport at the nanoscale and ultralow temperatures -- implications for quantum technologies

In this perspective, we discuss thermal imbalance and the associated electron-mediated thermal transport in quantum electronic devices at very low temperatures. We first present the theoretical approaches describing heat transport in nanoscale conductors at low temperatures, in which quantum confinement and interactions play an important role. We then discuss the experimental techniques for generating and measuring heat currents and temperature gradients on the nanoscale. Eventually we review the most important quantum effects on heat transport, and discuss implications for quantum technologies and future directions in the field.

cond-mat.mes-hall↗

arXiv2023

Evidence for chiral supercurrent in quantum Hall Josephson junctions

Hybridizing superconductivity with the quantum Hall (QH) effects has major potential for designing novel circuits capable of inducing and manipulating non-Abelian states for topological quantum computation. However, despite recent experimental progress towards this hybridization, concrete evidence for a chiral QH Josephson junction -- the elemental building block for coherent superconducting-QH circuits -- is still lacking. Its expected signature is an unusual chiral supercurrent flowing in QH edge channels, which oscillates with a specific $2ϕ_0$ magnetic flux periodicity ($ϕ_0=h/2e$ is the superconducting flux quantum, $h$ the Planck constant and $e$ the electron charge). Here, we show that ultra-narrow Josephson junctions defined in encapsulated graphene nanoribbons exhibit such a chiral supercurrent, visible up to 8 teslas, and carried by the spin-degenerate edge channel of the QH plateau of resistance $h/2e^2\simeq 12.9$ k$Ω$. We observe reproducible $2ϕ_0$-periodic oscillation of the supercurrent, which emerges at constant filling factor when the area of the loop formed by the QH edge channel is constant, within a magnetic-length correction that we resolve in the data. Furthermore, by varying the junction geometry, we show that reducing the superconductor/normal interface length is pivotal to obtain a measurable supercurrent on QH plateaus, in agreement with theories predicting dephasing along the superconducting interface. Our findings mark a critical milestone along the path to explore correlated and fractional QH-based superconducting devices that should host non-Abelian Majorana and parafermion zero modes.

cond-mat.mes-hall↗

arXiv2023

Absence of edge reconstruction for quantum Hall edge channels in graphene devices

Electronic edge states in topological insulators have become a major paradigm in physics. The oldest and primary example is that of quantum Hall (QH) edge channels that propagate along the periphery of two-dimensional electron gases (2DEGs) under perpendicular magnetic field. Yet, despite 40 years of intensive studies using a variety of transport and scanning probe techniques, imaging the real-space structure of QH edge channels has proven difficult, mainly due to the buried nature of most 2DEGs in semiconductors. Here, we show that QH edge states in graphene are confined to a few magnetic lengths at the crystal edges by performing scanning tunneling spectroscopy up to the edge of a graphene flake on hexagonal boron nitride. These findings indicate that QH edge states are defined by boundary conditions of vanishing electronic wavefunctions at the crystal edges, resulting in ideal one-dimensional chiral channels, free of electrostatic reconstruction. We further evidence a uniform charge carrier density at the edges, contrasting with conjectures on the existence of non-topological upstream modes. The absence of electrostatic reconstruction of quantum Hall edge states has profound implications for the universality of electron and heat transport experiments in graphene-based systems and other 2D crystalline materials.

cond-mat.mes-hall↗

arXiv2022

Imaging tunable quantum Hall broken-symmetry orders in graphene

When electrons populate a flat band their kinetic energy becomes negligible, forcing them to organize in exotic many-body states to minimize their Coulomb energy. The zeroth Landau level of graphene under magnetic field is a particularly interesting strongly interacting flat band because inter-electron interactions are predicted to induce a rich variety of broken-symmetry states with distinct topological and lattice-scale orders. Evidence for these stems mostly from indirect transport experiments that suggest that broken-symmetry states are tunable by boosting the Zeeman energy or by dielectric screening of the Coulomb interaction. However, confirming the existence of these ground states requires a direct visualization of their lattice-scale orders. Here, we image three distinct broken-symmetry phases in graphene using scanning tunneling spectroscopy. We explore the phase diagram by tuning the screening of the Coulomb interaction by a low or high dielectric constant environment, and with a magnetic field. In the unscreened case, we unveil a Kekulé bond order, consistent with observations of an insulating state undergoing a magnetic-field driven Kosterlitz-Thouless transition. Under dielectric screening, a sublattice-unpolarized ground state emerges at low magnetic fields, and transits to a charge-density-wave order with partial sublattice polarization at higher magnetic fields. The Kekulé and charge-density-wave orders furthermore coexist with additional, secondary lattice-scale orders that enrich the phase diagram beyond current theory predictions. This screening-induced tunability of broken-symmetry orders may prove valuable to uncover correlated phases of matter in other quantum materials.

cond-mat.mes-hall↗

arXiv2022

Magnetization Reversal Across Multiple Serial Barriers in a Single Fe$_3$O$_4$ Nanoparticle

Depinning of nanoscale magnetic textures, such as domain walls, vortices and skyrmions, is of paramount importance for magnetic storage and information processing. We measure time-resolved magnetic switching statistics of an individual, non-single-domain Fe$_3$O$_4$ nanoparticle using a micrometer-scale superconducting quantum interference device. Surprisingly, a strong narrowing of the waiting-time distributions before reaching the final state is observed as compared to the exponential distribution expected for a single barrier. The magnetization reversal across the nanostructure is thus shown to result from multiple serial barriers in the minimum energy pathway.

cond-mat.mes-hall↗

arXiv2019

Elimination of thermal bistability in superconducting weak links by an inductive shunt

The quantum phase-coherent behavior of superconducting weak links (WL) is often quenched in the finite voltage state, due to the heat dissipation and related thermal hysteresis. The latter can be reduced by improving heat evacuation and/or by lowering the critical current, so that a phase-dynamic regime is obtained, albeit over a narrow bias-current and temperature range. Here we demonstrate that an inductive shunt with well-chosen parameters introduces unexpected nonlinear dynamics that destabilize an otherwise stable fixed point in the dissipative branch. This leads to a nonhysteretic behavior with large voltage oscillations in intrinsically hysteretic WL-based micron-size superconducting quantum interference devices. A dynamic thermal model quantitatively describes our observations and further allows us to elaborate on the optimal shunting conditions.

cond-mat.supr-con↗

arXiv2019

Full electrostatic control of quantum interference in an extended trenched Josephson junction

Hybrid semiconductor/superconductor devices constitute an important platform for a wide range of applications, from quantum computing to topological-state-based architectures. Here, we demonstrate full modulation of the interference pattern in a superconducting interference device with two parallel islands of ballistic InAs quantum wells separated by a trench, by acting independently on two side-gates. This so far unexplored geometry enables us to tune the device with high precision from a SQUID-like to a Fraunhofer-like behavior simply by electrostatic gating, without the need for an additional in-plane magnetic field. These measurements are successfully analyzed within a theoretical model of an extended tunnel Josephson junction, taking into account the focusing factor of the setup. The impact of these results on the design of novel devices is discussed.

cond-mat.mes-hall↗

arXiv2018

Non-Linear Thermovoltage in a Single-Electron Transistor

We perform direct thermovoltage measurements in a single-electron transistor, using on-chip local thermometers, both in the linear and non-linear regimes. Using a model which accounts for co-tunneling, we find excellent agreement with the experimental data with no free parameters even when the temperature difference is larger than the average temperature (far-from-linear regime). This allows us to confirm the sensitivity of the thermovoltage on co-tunneling and to find that in the non-linear regime the temperature of the metallic island is a crucial parameter. Surprisingly, the metallic island tends to overheat even at zero net charge current, resulting in a reduction of the thermovoltage.

cond-mat.mes-hall↗

arXiv2018

Josephson Coupling in the Dissipative State of a Thermally Hysteretic $μ$-SQUID

Micron-sized superconducting interference devices ($μ$-SQUIDs) based on constrictions optimized for minimizing thermal runaway are shown to exhibit voltage oscillations with applied magnetic flux despite their hysteretic behavior. We explain this remarkable feature by a significant supercurrent contribution surviving deep into the resistive state, due to efficient heat evacuation. A resistively shunted junction model, complemented by a thermal balance determining the amplitude of the critical current, describes well all experimental observations, including the flux modulation of the (dynamic) retrapping current and voltage by introducing a single dimensionless parameter. Thus hysteretic $μ$-SQUIDs can be operated in the voltage read-out mode with a faster response. The quantitative modeling of this regime incorporating both heating and phase dynamics paves the way for further optimization of $μ$-SQUIDs for nano-magnetism.

cond-mat.supr-con↗

arXiv2018

Mesoscopic electron transport and atomic gases, a review of Frank W. J. Hekking's scientific work

Frank W. J. Hekking performed his PhD work on "Aspects of Electron Transport in Semiconductor Nanostructures" at the TU Delft in 1992. He then worked as a postdoc at the University of Karlsruhe, the University of Minnesota, the Cavendish Laboratory at the University of Cambridge, and the Ruhr University at Bochum. In 1999 he joined the LPMMC (Laboratoire de Physique et Mod\' elisation des Milieux Condens\' es) in Grenoble and was appointed Professor at the Universit\' e Joseph Fourier and afterwards Universit\' e Grenoble Alpes. Frank Hekking was nominated as a member of the Institut Universitaire de France, for the periods 2002-2007 and 2012-2017. This review provides an overview of his scientific contributions to several fields of mesoscopic electron transport and superconductivity as well as atomic gases, and is organized along sections describing the different themes.

physics.hist-ph↗

arXiv2016

Interplay Between Electron Over-Heating and ac Josephson Effect

We study the response of high-critical current proximity Josephson junctions to a microwave excitation. Electron over-heating in such devices is known to create hysteretic dc voltage-current characteristics. Here we demonstrate that it also strongly influences the ac response. The interplay of electron over-heating and ac Josephson dynamics is revealed by the evolution of the Shapiro steps with the microwave drive amplitude. Extending the resistively shunted Josephson junction model by including a thermal balance for the electronic bath coupled to phonons, a strong electron over-heating is obtained.

cond-mat.mes-hall↗

arXiv2014

Sub-Gap Structure in the Conductance of a Three-Terminal Josephson Junction

Three-terminal superconductor (S) - normal metal (N) - superconductor (S) Josephson junctions are investigated. In a geometry where a T-shape normal metal is connected to three superconducting reservoirs, new sub-gap structures appear in the differential resistance for specific combinations of the superconductor chemical potentials. Those correspond to a correlated motion of Cooper pairs within the device that persist well above the Thouless energy and is consistent with the prediction of quartets formed by two entangled Cooper pairs. A simplified nonequilibrium Keldysh Green's function calculation is presented that supports this interpretation.

cond-mat.mes-hall↗

arXiv2014

Electronic coolers based on superconducting tunnel junctions: fundamentals and applications

Thermo-electric transport at the nano-scale is a rapidly developing topic, in particular in superconductor-based hybrid devices. In this review paper, we first discuss the fundamental principles of electronic cooling in mesoscopic superconducting hybrid structures, the related limitations and applications. We review recent work performed in Grenoble on the effects of Andreev reflection, photonic heat transport, phonon cooling, as well as on an innovative fabrication technique for powerful coolers.

cond-mat.supr-con↗

arXiv2014

Long-ranged magnetic proximity effects in noble metal-doped cobalt probed with spin- dependent tunnelling

We inserted non-magnetic layers of Au and Cu into sputtered AlOx-based magnetic tunnel junctions and Meservey-Tedrow junctions in order to study their effect on tunnelling magnetoresistance (TMR) and spin polarization (TSP). When either Au or Cu are inserted into a Co/AlOx interface, we find that TMR and TSP remain finite and measurable for thicknesses up to several nanometres. High-resolution transmission electron microscopy shows that the Cu and Au interface layers are fully continuous when their thickness exceeds ~3 nm, implying that spin-polarized carriers penetrate the interface noble metal to dis- tances exceeding this value. A power law model based on exchange scattering is found to fit the data better than a phenomenological exponential decay. The discrepancy between these length scales and the much shorter ones reported from x-ray magnetic circular dichroism studies of magnetic proximitization is ascribed to the fact that our tunnelling transport measurements selectively probe s-like electrons close to the Fermi level. When a 0.1 nm thick Cu or Au layer is inserted within the Co, we find that the suppression of TMR and TSP is restored on a length scale of <=1 nm, indicating that this is a sufficient quantity of Co to form a fully spin-polarized band structure at the interface with the tunnel barrier.

cond-mat.supr-con↗

arXiv2014

Superconducting cascade electron refrigerator

The design and operation of an electronic cooler based on a combination of superconducting tunnel junctions is described. The cascade extraction of hot-quasiparticles, which stems from the energy gaps of two different superconductors, allows for a normal metal to be cooled down to about 100 mK starting from a bath temperature of 0.5 K. We discuss the practical implementation, potential performance and limitations of such a device.

cond-mat.supr-con↗

arXiv2014

Existence of an Independent Phonon Bath in a Quantum Device

At low temperatures, the thermal wavelength of acoustic phonons in a metallic thin film on a substrate can widely exceed the film thickness. It is thus generally believed that a mesoscopic device operating at low temperature does not carry an individual phonon population. In this work, we provide direct experimental evidence for the thermal decoupling of phonons in a mesoscopic quantum device from its substrate phonon heat bath at a sub-Kelvin temperature. A simple heat balance model assuming an independent phonon bath following the usual electron-phonon and Kapitza coupling laws can account for all experimental observations.

cond-mat.mes-hall↗

arXiv2013

Modulating charge density and inelastic optical response in graphene by atmospheric pressure localized intercalation through wrinkles

The intercalation of an oxide barrier between graphene and its metallic substrate for chem- ical vapor deposition is a contamination-free alternative to the transfer of graphene to dielectric supports, usually needed for the realization of electronic devices. Low-cost pro- cesses, especially at atmospheric pressure, are desirable but whether they are achievable remains an open question. Combining complementary microscopic analysis, providing structural, electronic, vibrational, and chemical information, we demonstrate the spontaneous reactive intercalation of 1.5 nm-thick oxide ribbons between graphene and an iridium substrate, at atmospheric pressure and room temperature. We discover that oxygen-containing molecules needed for forming the ribbons are supplied through the graphene wrinkles, which act as tunnels for the efficient diffusion of molecules entering their free end. The intercalated oxide ribbons are found to modify the graphene-support interaction, leading to the formation of quasi-free-standing high quality graphene whose charge density is modulated in few 10-100 nm-wide ribbons by a few 10^12 cm-2, where the inelastic optical response is changed, due to a softening of vibrational modes - red-shifts of Raman G and 2D bands by 6 and 10 cm-1, respectively.

cond-mat.mtrl-sci↗