arXiv subjects

Himadri S. Dhar

Publications and source records attributed to Himadri S. Dhar.

8 recordsLinked to original sources

arXiv2026

Giant critical response in a driven-dissipative quantum gas

Systems close to a phase transition turn weak perturbations into large responses. At equilibrium, this amplification is closely linked to criticality: fluctuations grow, dynamics slow, and a common soft mode controls the response. Whether this correspondence survives in driven-dissipative quantum systems, sustained by continuous pumping and loss away from thermal equilibrium, remains an open question. Here we show experimentally that it does. In a room-temperature semiconductor photon Bose-Einstein condensate, the critical slowing of spontaneous intensity fluctuations and the amplification of weak pump perturbations are measured independently. Both peak at the same condensate population, $\bar{n}_c = 1250$, where the dimensionless slowing factor and susceptibility reach the same value, $\bar{n}_c/2 = 625$. A single weakly damped collective photon-reservoir mode governs both effects. This fluctuation-response correspondence in a finite open quantum gas establishes critical susceptibility as a measurable dynamical signature of condensation, with peak gain set by system size.

cond-mat.quant-gas↗

arXiv2023

Bose-Einstein Condensation of Light in a Semiconductor Quantum Well Microcavity

When particles with integer spin accumulate at low temperature and high density they undergo Bose-Einstein condensation (BEC). Atoms, solid-state excitons and excitons coupled to light all exhibit BEC, which results in high coherence due to massive occupation of the respective system's ground state. Surprisingly, photons were shown to exhibit BEC much more recently in organic dye-filled optical microcavities, which, owing to the photon's low mass, occurs at room temperature. Here we demonstrate that photons within an inorganic semiconductor microcavity also thermalise and undergo BEC. Although semiconductor lasers are understood to operate out of thermal equilibrium, we identify a region of good thermalisation in our system where we can clearly distinguish laser action from BEC. Based on well-developed technology, semiconductor microcavities are a robust system for exploring the physics and applications of quantum statistical photon condensates. Notably, photon BEC is an alternative to exciton-based BECs, which dissociate under high excitation and often require cryogenic operating conditions. In practical terms, photon BECs offer their critical behaviour at lower thresholds than lasers. Our study shows two further advantages of photon BEC in semiconductor materials: the lack of dark electronic states allows these BECs to be sustained continuously; and semiconductor quantum wells offer strong photon-photon scattering. We measure an unoptimised interaction parameter, $\tilde{g}=0.0023\pm0.0003$, which is large enough to access the rich physics of interactions within BECs, such as superfluid light or vortex formation.

physics.optics↗

arXiv2021

Quest for Vortices in Photon Condensates

We predict that a photon condensate inside a dye-filled microcavity forms long-lived spatial structures that resemble vortices when incoherently excited by a focused pump orbiting around the cavity axis. The finely structured density of the condensates have a discrete rotational symmetry that is controlled by the orbital frequency of the pump spot and is phase-coherent over its full spatial extent despite the absence of any effective photon-photon interactions.

quant-ph↗

arXiv2021

Periodic cavity state revivals from atomic frequency combs

Spin ensembles with a comb-shaped spectrum have shown exciting properties as efficient quantum memories. Here, we present a rigorous theoretical study of such atomic frequency combs in the strong coupling limit of cavity QED, based on a full quantum treatment using tensor-network methods. Our results demonstrate that arbitrary multi-photon states in the cavity are almost perfectly absorbed by the spin ensemble and re-emitted as parity-flipped states at periodic time intervals. Fidelity values near unity are achieved in these revived states by compensating for energy shifts induced by the strong spin-cavity coupling through adjustments of individual coupling values of the teeth in the atomic frequency comb.

quant-ph↗

arXiv2021

Learning the Fuzzy Phases of Small Photonic Condensates

Phase transitions, being the ultimate manifestation of collective behaviour, are typically features of many-particle systems only. Here, we describe the experimental observation of collective behaviour in small photonic condensates made up of only a few photons. Moreover, a wide range of both equilibrium and non-equilibrium regimes, including Bose-Einstein condensation or laser-like emission are identified. However, the small photon number and the presence of large relative fluctuations places major difficulties in identifying different phases and phase transitions. We overcome this limitation by employing unsupervised learning and fuzzy clustering algorithms to systematically construct the fuzzy phase diagram of our small photonic condensate. Our results thus demonstrate the rich and complex phase structure of even small collections of photons, making them an ideal platform to investigate equilibrium and non-equilibrium physics at the few particle level.

cond-mat.quant-gas↗

arXiv2020

Transport and localization of light inside a dye-filled microcavity

The driven-dissipative nature of light-matter interaction inside a multimode, dye-filled microcavity makes it an ideal system to study nonequilibrium phenomena, such as transport. In this work, we investigate how light is efficiently transported inside such a microcavity, mediated by incoherent absorption and emission processes. In particular, we show that there exist two distinct regimes of transport, viz. conductive and localized, arising from the complex interplay between the thermalizing effect of the dye molecules and the nonequilibrium influence of driving and loss. The propagation of light in the conductive regime occurs when several localized cavity modes undergo dynamical phase transitions to a condensed, or lasing, state. Further, we observe that while such transport is robust for weak disorder in the cavity potential, strong disorder can lead to localization of light even under good thermalizing conditions. Importantly, the exhibited transport and localization of light is a manifestation of the nonequilibrium dynamics rather than any coherent interference in the system.

quant-ph↗

arXiv2019

Non-critical slowing down of photonic condensation

We investigate the response of a photonic gas interacting with a reservoir of pumped dye-molecules to quenches in the pump power. In addition to the expected dramatic critical slowing down of the equilibration time around phase transitions we find extremely slow equilibration even far away from phase transitions. This non-critical slowing down can be accounted for quantitatively by fierce competition among cavity modes for access to the molecular environment, and we provide a quantitative explanation for this non-critical slowing down.

quant-ph↗

arXiv2019

Non-stationary Statistics and Formation Jitter in Transient Photon Condensation

While equilibrium phase transitions are well described by a free-energy landscape, there are few tools to describe general features of their non-equilibrium counterparts. On the other hand, near-equilibrium free-energies are easily accessible but their full geometry is only explored in non-equilibrium, e.g. after a quench. In the particular case of a non-stationary system, however, the concepts of an order parameter and free energy become ill-defined, and a comprehensive understanding of non-stationary (transient) phase transitions is still lacking. Here, we probe transient non-equilibrium dynamics of an optically pumped, dye-filled microcavity which exhibits near-equilibrium Bose-Einstein condensation under steady-state conditions. By rapidly exciting a large number of dye molecules, we quench the system to a far-from-equilibrium state and, close to a critical excitation energy, find delayed condensation, interpreted as a transient equivalent of critical slowing down. We introduce the two-time, non-stationary, second-order correlation function as a powerful experimental tool for probing the statistical properties of the transient relaxation dynamics. In addition to number fluctuations near the critical excitation energy, we show that transient phase transitions exhibit a different form of diverging fluctuations, namely timing jitter in the growth of the order parameter. This jitter is seeded by the randomness associated with spontaneous emission, with its effect being amplified near the critical point. The general character of our results are then discussed based on the geometry of effective free-energy landscapes. We thus identify universal features, such as the formation timing jitter, for a larger set of systems undergoing transient phase transitions. Our results carry immediate implications to diverse systems, including micro- and nano-lasers and growth of colloidal nanoparticles.

cond-mat.stat-mech↗