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Hiroaki Kadowaki

Publications and source records attributed to Hiroaki Kadowaki.

At least 19 recordsLinked to original sources

Coherent magnetic excitations in a topological Kondo semimetal

In Kondo insulators the many-body Kondo lattice effect drives the formation of bands containing heavy charge carriers with a hybridization gap, leading to insulating properties. These renormalized bands can host non-trivial topologies driven by strong electron-electron interactions, but probing narrow heavy bands at low temperatures is challenging. We use inelastic neutron scattering (INS) to probe the Kondo lattice CeNiSn, which hosts both semimetallic transport properties and a hybridization gap. The INS response exhibits momentum-dependent magnetic excitations and a spin-gap in the low-temperature Kondo coherent state, which electronic structure calculations corroborate as arising from the renormalized heavy band structure. Dynamical-mean field theory demonstrates that this renormalized band structure corresponds to a topological Kondo insulating state, and hence the INS probes bulk excitations of heavy topological bands. This identification of a Kondo insulator addresses the long-standing mystery of the electronic properties of CeNiSn, and demonstrates the manifestation of a topological many-body coherent state in spectroscopic measurements of strongly correlated narrow band materials.

cond-mat.str-el↗

Spin and quadrupole correlations by three-spin interaction in the frustrated pyrochlore magnet Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$

We have investigated the origin of the magnetic dipole correlations $\langle σ_{\boldsymbol{Q}}^z σ_{\boldsymbol{-Q}}^z \rangle$ characterized by the modulation wave vector $\boldsymbol{k} \sim (\tfrac{1}{2},\tfrac{1}{2},\tfrac{1}{2})$ observed in the frustrated pyrochlore magnet Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$. This magnetic short-range order cannot be accounted for by adding further-neighbor exchange interactions to the nearest-neighbor pseudospin-$\tfrac{1}{2}$ Hamiltonian for quantum pyrochlore magnets. Using classical Monte Carlo simulation and quantum simulation based on thermally pure quantum (TPQ) states we have shown that the spin correlations with $\boldsymbol{k} \sim (\tfrac{1}{2},\tfrac{1}{2},\tfrac{1}{2})$ are induced at low temperatures by a three-spin interaction of a form $σ_{\boldsymbol{r}}^{\pm} σ_{\boldsymbol{r}^{\prime}}^z σ_{\boldsymbol{r}^{\prime \prime}}^z $, which is a correction to the Hamiltonian due to the low crystal-field excitation. Simulations using TPQ states have shown that the spin correlations coexist with electric quadrupole correlations $\langle σ_{\boldsymbol{Q}}^α σ_{\boldsymbol{-Q}}^β \rangle$ ($α, β= x, y$) with $\boldsymbol{k} \sim \boldsymbol{0}$. These results suggest that the putative quantum spin liquid state of Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ is located close to phase boundaries of the spin-ice, quadrupole-ordered, and magnetic-ordered states in the classical approximation, and that the three-spin interaction brings about a quantum disordered ground state with both spin and quadrupole correlations.

cond-mat.str-el↗

Dimensional change of quadrupole orders in pseudospin-$\frac{1}{2}$ pyrochlore magnets under [111] field

We have studied long range orders of electric quadrupole moments described by an effective pseudospin-$\frac{1}{2}$ Hamiltonian representing pyrochlore magnets with non-Kramers ions under [111] magnetic field, in relevance to Tb$_{2}$Ti$_{2}$O$_{7}$. Order parameters and phase transitions of this frustrated system are investigated using classical Monte-Carlo simulations. In zero field, the model undergoes a first-order phase transition from a paramagnetic state to an ordered state with an antiparallel arrangement of pseudospins. This pseudospin order is characterized by the wavevector $\boldsymbol{k}=0$ and is selected by an energetic or an order-by-disorder mechanism from degenerate $\boldsymbol{k}=(h,h,h)$ mean-field orders. Under [111] magnetic field this three-dimensional quadrupole order is transformed to a quasi two-dimensional quadrupole order on each kagomé lattice separated by field-induced ferromagnetic triangular lattices. We discuss implication of the simulation results with respect to experimental data of Tb$_{2}$Ti$_{2}$O$_{7}$.

cond-mat.str-el↗

Universal dynamics of magnetic monopoles in two-dimensional kagomé ice

A magnetic monopole in spin ice is a novel quasiparticle excitation in condensed matter physics, and we found that the ac frequency dependent magnetic susceptibility $χ(ω)$ in the two-dimensional (2D) spin ice (so-called kagomé ice) of Dy$_2$Ti$_2$O$_7$ shows a single scaling form. This behavior can be understood in terms of the dynamical scaling law for 2D Coulomb gas (CG) systems [Phys. Rev. B 90, 144428 (2014)], characterized by the charge correlation length $ξ(\propto1/\sqrt{ω_1})$, where $ω_{1}$ is a characteristic frequency proportional to the peak position of the imaginary part of $χ(ω)$. It is a generic behavior among a wide variety of models such as the vortex dynamics of 2D superconductors, 2D superfluids, classical XY magnets, and dynamics of melting of Wigner crystals.

cond-mat.other↗

Spin correlations of quantum-spin-liquid and quadrupole-ordered states of Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$

Spin correlations of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been investigated by using inelastic neutron scattering on single crystalline samples ($x=-0.007, 0.000,$ and $0.003$), which have the putative quantum-spin-liquid (QSL) or electric-quadrupolar ground states. Spin correlations, which are notably observed in nominally elastic scattering, show short-ranged correlations around $L$ points [$q = (\tfrac{1}{2},\tfrac{1}{2},\tfrac{1}{2})$], tiny antiferromagnetic Bragg scattering at $L$ and $Γ$ points, and pinch-point type structures around $Γ$ points. The short-ranged spin correlations were analyzed using a random phase approximation (RPA) assuming the paramagnetic state and two-spin interactions among Ising spins. These analyses have shown that the RPA scattering intensity well reproduces the experimental data using temperature and $x$ dependent coupling constants of up to 10-th neighbor site pairs. This suggests that no symmetry breaking occurs in the QSL sample, and that a quantum treatment beyond the semi-classical RPA approach is required. Implications of the experimental data and the RPA analyses are discussed.

cond-mat.str-el↗

Field-rotational magnetocaloric effect: A new experimental technique for accurate measurement of the anisotropic magnetic entropy

We developed a new technique for measuring the thermodynamic entropy as a function of the magnetic field angle. This technique enables high-resolution angle-resolved measurements of the entropy in an unprecedentedly short measuring time. When the magnetic field is rotated under adiabatic conditions, the sample temperature changes owing to the field-angle variation of its entropy, which is referred to as the rotational magnetocaloric effect. By investigating this effect along with the specific heat, the field-angle dependence of the entropy can be determined. To demonstrate this technique, we chose the spin-ice compound Dy$_2$Ti$_2$O$_7$ as a benchmark and showed good agreement between the measured and theoretical entropies as a function of the field angle. This development provides a new approach to studying condensed-matter physics, in which multiple degrees of freedom play an important role.

cond-mat.str-el↗

Continuum excitation and pseudospin wave in quantum spin-liquid and quadrupole ordered states of Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$

The ground states of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been studied by inelastic neutron scattering experiments. Three single-crystal samples are investigated; one shows no phase transition ($x=-0.007<x_{\text{c}}\sim -0.0025$), being a putative quantum spin-liquid (QSL), and the other two ($x=0.000, 0.003$) show electric quadrupole ordering (QO) below $T_{\text{c}} \sim 0.5$ K. The QSL sample shows continuum excitation spectra with an energy scale 0.1 meV as well as energy-resolution limited (nominally) elastic scattering. As $x$ is increased, pseudospin wave of the QO state emerges from this continuum excitation, which agrees with that of powder samples and consequently verifies good $x$ control for the present single crystal samples.

cond-mat.str-el↗

Comparative studies of low temperature X-ray diffraction experiments on R2Ir2O7 (R = Nd, Eu, and Pr)

The cubic symmetry of pyrochlore iridium oxides R2Ir2O7 (R = Nd, Eu, and Pr) has been investigated by high resolution X-ray diffraction experiments down to 4 K,in order to clarify the relationship between the metal-insulator transition (MIT) and the small structural phase transition suggested by Raman scattering experiments in these compounds. We have found that a small negative thermal expansion of the order of 10^-3 angstroms appears only in Nd2Ir2O7 below the MIT, T_MIT = 34 K, resulting in the magnetovolume effect of the long-range order of Ir moments. However, any breaking of the cubic symmetry of three iridates has not been observed as appearance of superlattice reflections nor splittings of cubic reflections below T_MIT. These results imply that lowering of the cubic symmetry plays a minor role for the change in the electronic state of these compounds, while a formation of the special arrangement of Ir moments plays a major role for the MIT.

cond-mat.str-el↗

Magnetic structure of the conductive triangular-lattice antiferromagnet PdCrO2

We performed neutron single crystal and synchrotron X-ray powder diffraction experiments in order to investigate the magnetic and crystal structures of the conductive layered triangular-lattice antiferromagnet PdCrO2 with a putative spin chirality, which contributes to an unconventional anomalous Hall effect. We revealed that the ground-state magnetic structure is a commensurate and nearly-coplanar 120-degrees spin structure. The 120-degrees plane in different Cr layers seem to tilt with one another, leading to a small noncoplanarity. Such a small but finite non-coplanar stacking of the 120-degrees planes gives rise to a finite scalar spin chirality, which may be responsible for the unconventional nature of the Hall effect of PdCrO2.

cond-mat.str-el↗

Stabilization of high-Tc phase of BiS2-based superconductor LaO0.5F0.5BiS2 using high-pressure synthesis

High-quality polycrystalline samples of LaO0.5F0.5BiS2 were obtained using high-pressure synthesis technique. The LaO0.5F0.5BiS2 sample prepared by heating at 700 C under 2 GPa showed superconductivity with superconducting transition temperatures (Tc) of Tconset = 11.1 and Tczero = 8.5 K in the electrical resistivity measurements and Tconset = 11.5 and Tcirr = 9.4 K in the magnetic susceptibility measurements, which are obviously higher than those of the LaO0.5F0.5BiS2 polycrystalline samples obtained using conventional solid-state reaction. It was found that the high-Tc phase can be stabilized under high pressure and relatively-low annealing temperature. X-ray diffraction analysis revealed that the high-Tc phase possessed a small ratio of lattice constants of a and c, c/a.

cond-mat.supr-con↗

Correlation between crystal structure and superconductivity in LaO0.5F0.5BiS2

Correlation between crystal structure and superconducting properties of the BiS2-based superconductor LaO0.5F0.5BiS2 was investigated. We have prepared LaO0.5F0.5BiS2 polycrystalline samples with various lattice constants. It was found that the annealing the sample under high pressure generated uniaxial strain along the c axis. Further, the highly-strained sample showed higher superconducting properties. We concluded that the uniaxial strain along the c axis was positively linked with the enhancement of superconductivity in the LaO1-xFxBiS2 system.

cond-mat.supr-con↗

AC Susceptibility of the Dipolar Spin Ice Dy2Ti2O7: Experiments and Monte Carlo Simulations

Experimental data of the frequency-dependent ac susceptibility for the dipolar spin ice Dy2Ti2O7 has been analyzed by Monte Carlo simulations on the basis of the single-spin-flip Metropolis algorithm. We have directly evaluated the ac susceptibility by applying an ac magnetic field. We found that the simulated behaviors reproduces the experimental behavior of the ac susceptibility in the temperature range from 0.6 to 1.0 K, where dilute magnetic monopoles diffusively move. The conversion factor from simulation time to real time, i.e., the rate of hopping of monopoles to nearest-neighbor sites, strongly depends on temperature.

cond-mat.str-el↗

A Scaling Theory for ac Magnetic Response in Kagome Ice

A theory for frequency-dependent magnetic susceptibility χ(ω) is developed for thermally activated magnetic monopoles in kagome ice. By mapping this system to a two-dimensional (2D) Coulomb gas and then to a sine-Gordon model, we have shown that the susceptibility has a scaling form χ(ω)/χ(0)={\cal F}(ω/ω_1), where the characteristic ω_1 is related to a charge correlation length between diffusively moving monopoles, and to the sine-Gordon principal breather. The dynamical scaling is universal among superfluid and superconducting films, and 2D XY magnets above Kosterlitz-Thouless transitions.

cond-mat.str-el↗

Bulk superconductivity in Bi4O4S3 revealed by specific heat measurement

Specific heat experiments on a well-characterized polycrystalline sample of the BiS2 based superconductor Bi4O4S3 revealed that it shows a crear specific heat anomaly at about Tc = 4.4 K, consistent with Tc from the resistivity and dc susceptibility. This observation indicates the superconductivity of Bi4O4S3 to be bulk in nature.

cond-mat.supr-con↗

Evolution of two-step structural phase transition in Fe1+dTe detected by low-temperature x-ray diffraction

The low-temperature crystal structure of Fe1.13Te, which exhibits an anomalous two-step magnetic transition, was clarified by the systematic x-ray diffraction measurements. It was found that two-step structural phase transition, tetragonal-orthorhombic-monoclinic, occurred correspondingly to the two-step magnetic transition. The detailed analysis of the profile at 5 K indicated the coexistence of the minor orthorhombic area inside the major monoclinic lattice, which could explain the lower-shift (suppression) of the antiferromagnetic transition temperature in Fe1.13Te and suggest a possibility of superconductivity at the domain boundary.

cond-mat.supr-con↗

Quantum spin fluctuations in the spin liquid state of Tb2Ti2O7

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally fluctuating paramagnetic state to a spin-liquid ground-state with quantum spin fluctuations. Energy spectra change from quasielastic scattering to a continuum with a double-peak structure at energies of 0 and 0.8 K in the spin-liquid state. Specific heat shows an anomaly at the crossover temperature.

cond-mat.dis-nn↗

Absence of anomalous negative lattice-expansion for polycrystalline sample of Tb2Ti2O7

High resolution X-ray powder-diffraction experiments on a well-characterized polycrystalline sample of the spin liquid Tb2Ti2O7 reveal that it shows normal positive thermal-expansion above 4 K, which does not agree with the intriguing anomalous negative thermal-expansion due to a magneto-elastic coupling reported for a single crystal sample below 20 K. We also performed a Rietveld profile refinement of a powder-diffraction pattern taken at a room temperature, and confirmed that it is consistent with the fully ordered cubic pyrochlore structure.

cond-mat.str-el↗

Observation of Magnetic Monopoles in Spin Ice

Excitations from a strongly frustrated system, the kagome ice state of the spin ice Dy2Ti2O7 under magnetic fields along a [111] direction, have been studied. They are theoretically proposed to be regarded as magnetic monopoles. Neutron scattering measurements of spin correlations show that close to the critical point the monopoles are fluctuating between high- and low-density states, supporting that the magnetic Coulomb force acts between them. Specific heat measurements show that monopole-pair creation obeys an Arrhenius law, indicating that the density of monopoles can be controlled by temperature and magnetic field.

cond-mat.dis-nn↗