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Hiroaki Ueda

Publications and source records attributed to Hiroaki Ueda.

18 recordsLinked to original sources

Exotic Spin Excitation Continuum in a Weakly Coupled Quantum Chainsaw Antiferromagnet

Collective motions in strongly interacting magnets involve many spins and are often described in terms of integer-spin excitations. However, in certain cases, the collective motion can behave as if these integer excitations break apart into smaller, particle-like entities with unusual properties. Such fractionalized excitations in quantum magnets are commonly associated either with topological order in two dimensions or with criticality in one dimension. It remains unclear how these distinct mechanisms are connected across a dimensional crossover. Here we investigate the Ti-based quantum antiferromagnet, $Cs_{8}LiNa_{3}Ti_{12}F_{48}$, in which $Ti^{3+}$ ($3d^{1}$, $S=1/2$) ions interact antiferromagnetically within distorted kagome planes. Our inelastic neutron scattering study on a single crystal reveals a frustrated network of weakly coupled spin-$1/2$ chainsaws, realizing a regime of dimensional frustration in which interchain couplings fail to establish coherent two-dimensional order. The magnetic excitation spectrum exhibits a strong continuum spanning the full measured momentum and energy phase space. In addition, the dynamic spin correlation function displays rod-like scattering in momentum space, indicating a quasi-one-dimensional nature of the magnetic correlations. These results point to fractionalized excitations with intrinsically directional character, demonstrating that signatures of one-dimensional criticality can persist within a two-dimensional lattice. Our findings establish anisotropic fractionalization as a distinct organizing principle for quantum-disordered states.

cond-mat.str-el

Unified Description of Spin-Lattice Coupling and Thermodynamics in the Pyrochlore Heisenberg Antiferromagnet

We study an extended model to describe the spin-lattice coupling, incorporating individual vibrations of bonds and atomic sites alongside distance-dependent exchange interactions. The proposed spin Hamiltonian can be effectively considered as an interpolation between two well-established minimum models, the bond-phonon model and the site-phonon model. The extended model, which treats bond phonons and site phonons on comparable footing, well reproduces successive field-induced phase transitions as well as the thermodynamic properties of a three-up-one-down state in the pyrochlore-lattice Heisenberg antiferromagnet, including negative thermal expansion, an enhanced magnetocaloric effect, and a sharp specific-heat peak. The present approach is broadly applicable to various spin models, providing a framework for identifying the primary phonon modes responsible for spin-lattice coupling and for understanding complex magnetic phase diagrams.

cond-mat.str-el

Miniaturized and robust tunable monochromatic magneto-optical platform for pulsed magnetic fields

Tunable monochromatic magneto-transmission is one of the most established magneto-optical techniques, particularly well suited for pulsed magnetic fields. It employs fixed-wavelength monochromatic light as the probe, while the magnetic field is swept to bring the sample into resonance with the photon energy. The key component of this setup is a tunable laser system, typically consisting of a Ti:sapphire laser coupled with an optical parametric oscillator. However, such laser systems are often bulky, expensive, and inherently unstable, which significantly limits their widespread application in magneto-optical laboratories. In this work, we develop a high-accuracy, cost-effective, and compact tunable monochromatic magneto-transmission system based on a combination of a laser-driven white light source and a mini monochromator, and demonstrate its feasibility and performance in a millisecond-range pulsed magnetic field condition. To verify the accuracy of this new and simplified setup, we performed Faraday rotation measurements on the geometrically frustrated spin system CdCr2O4, as well as magneto-transmission experiments on the Shastry-Sutherland lattice antiferromagnet SrCu2(BO3)2. These results show excellent agreement with previous reports, confirming the reliability and precision of the new setup.

cond-mat.str-el

Superconducting critical temperature and dimensionality tuning of RbV$_3$Sb$_5$ via biaxial strain

Kagome metal AV$_3$Sb$_5$ (A=K, Rb, Cs) has emerged as an intriguing platform for exploring the interplay between superconductivity and other quantum states. Among the three compounds, RbV$_3$Sb$_5$ has a notably lower superconducting critical temperature ($T_c$) at ambient pressure, posing challenges in exploring the superconducting state. For instance, the upper critical field ($H_{c2}$) is small and thus difficult to measure accurately against other control parameters. Hence, enhancing superconductivity would facilitate $H_{c2}$ measurements, providing insights into key superconducting properties such as the dimensionality. In this letter, we report the tuning of the $T_c$ in RbV$_3$Sb$_5$ through the application of biaxial strain. Utilizing a negative thermal expansion material ZrW$_2$O$_8$ as a substrate, we achieve a substantial biaxial strain of $\epsilon=1.50\%$, resulting in a remarkable 75\% enhancement in $T_c$. We investigate the $H_{c2}$ as a function of temperature, revealing a transition from multi-band to single-band superconductivity with increasing tensile strain. Additionally, we study the $H_{c2}$ as a function of field angle, revealing a plausible correlation between the $T_c$ enhancement and the change in dimensionality of the superconductivity under tensile strain. Further analysis quantitatively illustrates a transition towards two-dimensional superconductivity in RbV$_3$Sb$_5$ when subjected to tensile strain. Our work demonstrates that the application of biaxial strain allows for the tuning of both the $T_c$ and superconducting dimensionality in RbV$_3$Sb$_5$.

cond-mat.supr-con

Gapless dispersive continuum in a modulated quantum kagome antiferromagnet

The pursuit of quantum spin liquid (QSL) states in condensed matter physics has drawn attention to kagome antiferromagnets (AFM) where a two-dimensional corner-sharing network of triangles frustrates conventional magnetic orders. While quantum kagome AFMs based on Cu$^{2+}$ (3d$^9$, $s=\frac{1}{2}$) ions have been extensively studied, there is so far little work beyond copper-based systems. Here we present our bulk magnetization, specific heat and neutron scattering studies on single crystals of a new titanium fluoride Cs$_8$RbK$_3$Ti$_{12}$F$_{48}$ where Ti$^{3+}$ (3d$^1$, $s = \frac{1}{2}$) ions form a modulated quantum kagome antiferromagnet that does not order magnetically down to 1.5 K. Our comprehensive map of the dynamic response function $S(Q,\hbar\omega)$ acquired at 1.5 K where the heat capacity is T-linear reveals a dispersive continuum emanating from soft lines that extend along (100). The data indicate fractionalized spinon-like excitations with quasi-one-dimensional dispersion within a quasi-two-dimensional spin system.

cond-mat.str-el

Novel quantum phase of the chromium spinel oxide HgCr$_{\rm 2}$O$_{\rm 4}$ in high magnetic fields

In this study, we have performed the magnetocaloric effect and the specific heat measurements of chromium spinel oxide HgCr$_2$O$_4$, wherein the magnetic Cr$^{3+}$ ions form a highly frustrated pyrochlore lattice with significant spin-lattice coupling. In addition to the known magnetic-field-induced phases, our thermodynamic measurements detect a novel quantum phase just before the saturation of the magnetization, which has not been expected from the classical theories of the pyrochlore lattice antiferromagnet with spin-lattice coupling. Based on recent theoretical model calculation, we discuss the possibility of a spin nematic state appearing for this quantum phase.

cond-mat.str-el

Magnetic ordering with an XY-like anisotropy in the honeycomb lattice iridates ZnIrO$_3$ and MgIrO$_3$ synthesized via a metathesis reaction

We have successfully synthesized the novel antiferromagnets with Ir$^{4+}$ honeycomb lattice ZnIrO$_3$ and MgIrO$_3$ and investigated their magnetic and thermodynamic properties. The two iridates are isomorphic but exhibit qualitatively different magnetic properties. ZnIrO$_3$ shows antiferromagnetic ordering below 46.6 K, whereas MgIrO$_3$ displays weak ferromagnetic behavior below 31.8 K owing to formation of a canted antiferromagnetic ordering. The measurement of magnetic susceptibility with using an oriented powder sample revealed the presence of an XY-like magnetic anisotropy and a tilting magnetic structure which is possibly stabilized by the Kitaev interaction. Moreover, magnetization curves of MgIrO3 and ZnIrO3 up to 60 T show different behaviors, demonstrating that each magnetic ground state is different with each other. We discuss the difference in the ground state between MgIrO$_3$ and ZnIrO$_3$ from the viewpoint a magnetic model consisting of the Kitaev and Dzyaloshinskii-Moriya interactions with the spin frustration effect on the honeycomb lattice.

cond-mat.str-el

Single-particle excitation of core states in epitaxial silicene

Recent studies of core-level X-ray photoelectron spectroscopy (XPS) spectra of silicene on ZrB$_2$(0001) were found to be inconsistent with the density of states (DOS) of a planar-like structure that has been proposed as the ground state by density functional theory (DFT). To resolve the discrepancy, a reexamination of the XPS spectra and direct theoretical access of accurate single-particle excitation energies are desired. By analyzing the XPS data using symmetric Voigt functions, different binding energies and its sequence of Si $2p$ orbitals can be assigned from previously reported ones where asymmetric pseudo-Voigt functions are adopted. Theoretically, we have adopted an approach developed very recently, which follows the sophisticated $Δ$ self-consistent field ($Δ$SCF) methods, to study the single-particle excitation of core states. In the calculations, each single-particle energy and the renormalized core-hole charge density are calculated straightforwardly via two SCF calculations. By comparing the results, the theoretical core-level absolute binding energies including the splitting due to spin-orbit coupling are in good agreement with the observed high-resolution XPS spectra. The good agreement not only resolves the puzzling discrepancy between experiment and theory (DOS) but also advocates the success of DFT in describing many-body interactions of electrons at the surface.

cond-mat.mtrl-sci

Ultrafast optical excitation of coherent magnons in antiferromagnetic NiO

In experiment and theory, we resolve the mechanism of ultrafast optical magnon excitation in antiferromagnetic NiO. We employ time-resolved optical two-color pump-probe measurements to study the coherent non-thermal spin dynamics. Optical pumping and probing with linearly and circularly polarized light along the optic axis of the NiO crystal scrutinizes the mechanism behind the ultrafast optical magnon excitation. A phenomenological symmetry-based theory links these experimental results to expressions for the optically induced magnetization via the inverse Faraday effect and the inverse Cotton-Mouton effect. We obtain striking agreement between experiment and theory that, furthermore, allows us to extract information about the spin domain distribution. We also find that in NiO the energy transfer into the magnon mode via the inverse Cotton-Mouton effect is about three orders of magnitude more efficient than via the inverse Faraday effect.

cond-mat.other

Spin Jam: a quantum-fluctuation-induced glassy state of a frustrated magnet

Since the discovery of spin glasses in dilute magnetic systems, their study has been largely focused on understanding randomness and defects as the driving mechanism. The same paradigm has also been applied to explain glassy states found in dense frustrated systems. Recently, however, it has been theoretically suggested that different mechanisms, such as quantum fluctuations and topological features, may induce glassy states in defect-free spin systems, far from the conventional dilute limit. Here we report experimental evidence for the existence of a glassy state, that we call a spin jam, in the vicinity of the clean limit of a frustrated magnet, which is insensitive to a low concentration of defects. We have studied the effect of impurities on SrCr9pGa12-9pO19 (SCGO(p)), a highly frustrated magnet, in which the magnetic Cr3+ (s=3/2) ions form a quasi-two-dimensional triangular system of bi-pyramids. Our experimental data shows that as the nonmagnetic Ga3+ impurity concentration is changed, there are two distinct phases of glassiness: a distinct exotic glassy state, which we call a "spin jam", for high magnetic concentration region (p>0.8) and a cluster spin glass for lower magnetic concentration, (p<0.8). This observation indicates that a spin jam is a unique vantage point from which the class of glassy states in dense frustrated magnets can be understood.

cond-mat.str-el

Structural anomalies and short-range magnetic correlations in the orbitally degenerated system Sr$_2$VO$_4$

We report on the electronic ground state of a layered perovskite vanadium oxide Sr$_2$VO$_4$ studied by the combined use of synchrotron radiation x-ray diffraction (SR-XRD) and muon spin rotation/relaxation ($μ$SR) techniques, where $μ$SR measurements were extended down to 30 mK. We found an intermediate orthorhombic phase between $T_{\rm c2} \sim$~130 K and $T_{\rm c1} \sim$~100 K, whereas a tetragonal phase appears for $T > T_{\rm c2}$ and $T < T_{\rm c1}$. The absence of long-range magnetic order was confirmed by $μ$SR at the reentrant tetragonal phase below $T_{\rm c1}$, where the relative enhancement in the $c$-axis length versus that of the $a$-axis length was observed. However, no clear indication of the lowering of the tetragonal lattice symmetry with superlattice modulation, which is expected in the orbital order state with superstructure of $d_{yz}$ and $d_{zx}$ orbitals, was observed by SR-XRD below $T_{\rm c1}$. Instead, it was inferred from $μ$SR that a magnetic state developed below $T_{\rm c0} \sim$~10 K, which was characterized by the highly inhomogeneous and fluctuating local magnetic fields down to 30 mK. We argue that the anomalous magnetic ground state below $T_{\rm c0}$ originates from the coexistence of ferromagnetic and antiferromagnetic correlations.

cond-mat.str-el

Optical detection of magnetic orders in HgCr$_2$O$_4$ frustrated spin magnet under pulsed high magnetic fields

A magneto-optical survey was conducted for HgCr$_2$O$_4$ powder samples under pulsed high magnetic fields of up to 55 T. Intensity changes in magnetic fields observed for the exciton-magnon-phonon optical transition spectra coincide well with those of magnetization, lattice distortion from X-ray diffraction, and electron-magnetic resonances. The last-ordered phase was detected prior to the fully polarized magnetic phase, similarly to the other chromium spinel oxide, ZnCr$_2$O$_4$ and CdCr$_2$O$_4$.

cond-mat.mtrl-sci

Anomalous Itinerant-Electron Metamagnetic Transition in the Layered Sr1-xCaxCo2P2 System

We report magnetic properties of the layered itinerant system, Sr$_{1-x}$Ca$_x$Co$_2$P$_2$ in the magnetic field up to 70 T. As for the exchange-enhanced Pauli paramagnetic metal SrCo$_2$P$_2$, the magnetization curve shows two characteristic anomalies. The low-field anomaly is small without obvious hysteresis, and the high-field one is a typical behavior of the itinerant-electron metamagnetic transition (IEMT). Such a successive transition in the magnetization curve cannot be explained by the conventional phenomenological theory for IEMT due to the Landau expansion of the free energy, but by the extended Landau expansion theory with distinguishable two energy states. In the systematical study of Sr$_{1-x}$Ca$_x$Co$_2$P$_2$, furthermore, the metamagnetic transition field decreases and goes to zero as $x$ increases up to 0.5, indicating that the ferromagnetic quantum critical point (QCP) exists at $x \sim 0.5$.

cond-mat.str-el

A novel magnetic phase prior to a saturation moment in frustrated spinel oxides in ultra-high magnetic fields

We have investigated the magnetic-field induced phases of a typical three-dimensional frustrated magnet, CdCr$_2$O$_4$, in magnetic fields of up to 120 T that is generated by the single-turn coil techniques. We focused on magnetic phase transitions in proximity of a saturated magnetization moment. We utilized both the electromagnetic induction method using magnetic pick-up coils and magneto-optical spectroscopies of the $d$-$d$ transitions and the exciton-magnon-phonon transitions to study the magnetic properties subjected to ultra-high magnetic fields. Anomalies were observed in magneto-optical absorption intensity as well as differential magnetization prior to a fully polarized magnetic phase (a vacuum state in the magnon picture), revealing a novel magnetic phase associated with changes in both crystal and magnetic structures accompanied by the first order phase transition. Magnetic superfluid state such as an umbrella-like magnetic structure or a spin nematic state, is proposed as a candidate for the novel magnetic phase, which is found universal in the series of chromium spinel oxides, $A$Cr$_2$O$_4$ ($A$ = Zn, Cd, Hg).

cond-mat.str-el

Magnetic phases of a highly frustrated magnet, ZnCr2O4, up to an ultra-high magnetic field of 600 T

The Faraday rotation and magneto-optical absorption spectral measurements were conducted to reveal the full-magnetization process and map out a magnetic phase diagram of a typical geometrical frustrated magnet, ZnCr2O4, by using the electromagnetic flux compression method in ultra-magnetic fields up to 600 T. A fully polarized ferromagnetic phase is observed in which the absorption spectra associated with an exciton-magnon-phonon transition disappears. Furthermore, prior to the fully polarized ferromagnetic phase above 410 T, we found a novel magnetic phase above 350 T followed by a canted 3:1 phase.

cond-mat.str-el

Novel Magnetic Phases Revealed by Ultra-High Magnetic Field in the Frustrated Magnet ZnCr2O4

The Faraday rotation technique is used to map out the finite-temperature phase diagram of the prototypical frustrated magnet ZnCr2O4, in magnetic fields of up to 190 T generated by the single-turn coil method. We find evidence for a number of magnetic phase transitions, which are well-described by the theory based on spin-lattice coupling. In addition to the 1/2 plateau and a 3:1 canted phase, a 2:1:1 canted phase is found for the first time in chromium spinel oxides, which has been predicted by a theory of Penc et al. to realize in a small spin-lattice coupling limit. Both the new 2:1:1 and the 3:1 phase are regarded as the supersolid phases according to a magnetic analogy of Matsuda and Tsuneto, and Liu and Fisher.

cond-mat.str-el

Spin Oscillations in Antiferromagnetic NiO Triggered by Circularly Polarized Light

Coherent spin oscillations were non-thermally induced by circularly polarized pulses in fully compensated antiferromagnetic NiO. This effect is attributed to an entirely new mechanism of the action, on the spins, of the effective magnetic field generated by an inverse Faraday effect. The novelty of this mechanism is that spin oscillations are driven by the time derivative of the effective magnetic field acting even on "pure" antiferromagnets with zero net magnetic moment in the ground state. The measured frequencies (1.07 THz and 140 GHz) of the spin oscillations correspond to the out-of-plane and in-plane modes of antiferromagnetic magnons.

cond-mat.str-el

Half-magnetization plateaux in Cr spinels

Magnetization plateaux, visible as anomalies in magnetic susceptibility at low temperatures, are one of the hallmarks of frustrated magnetism. An extremely robust half-magnetization plateau is observed in the spinel oxides CdCr2O4 and HgCr2O4, where it is accompanied by a substantial lattice distortion. We give an overview of the present state experiment for CdCr2O4 and HgCr2O4, and show how such a half-magnetization plateau arises quite naturally in a simple model of these systems, once coupling to the lattice is taken into account.

cond-mat.str-el