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Hirohiko M. Shimizu

Publications and source records attributed to Hirohiko M. Shimizu.

At least 19 recordsLinked to original sources
arXiv2026

Development and Characterization of Low-Scattering Vanadium Nanoparticle Targets for Short-Range Interaction Searches

We developed high-purity vanadium-based nanoparticle targets for neutron scattering experiments aimed at exploring gravity-like short-range new interactions in the submicron regime. Vanadium and V-Ni nanoparticles were fabricated using top-down and bottom-up methods and quantitatively characterized by SEM-EDS, ICP-AES, NDIR and SAXS. Through the performance tests, an RF thermal plasma method was found to be the best from viewpoints of the reproducibility, dispersion of the radius, and contamination of metallic elements. The oxygen incorporation during fabrication was quantified, and its impact on the effective coherent scattering length was evaluated, leading to a minimum average coherent scattering length of $\mathrm{0.719(23)\,fm}$, comparable to that of natural vanadium. These results demonstrate that vanadium-based nanoparticle targets with controlled composition and nanostructure can be systematically designed and fabricated to suppress nuclear scattering backgrounds, thereby enabling experimentally viable coherent neutron scattering measurements for short-range interaction searches.

physics.ins-det↗
arXiv2026

First Constraint on P-odd/T-odd Cross Section in Polarized Neutron Transmission through Transversely Polarized $^{139}$La

We report the first constraint on time-reversal invariance violating (TRIV) effects in polarized neutron transmission through a transversely polarized $^{139}$La target. We formulate the transmission asymmetry within the density matrix formalism, explicitly incorporating the forward scattering amplitude of $^{139}$La including tensor polarization terms up to third-rank. The formalism is applied to existing transmission data originally obtained to measure the spin-dependent cross section near the $0.75$~eV $p$-wave resonance. Since these data were not optimized for P-odd/T-odd observables, the attainable sensitivity is intrinsically limited; nevertheless, they provide a useful test of the formalism on real experimental data. No statistically significant TRIV signal is observed. By analyzing the global $χ^2$ structure in the parameter space, we obtain an upper limit of $|W_T|<15~\mathrm{eV}$ at the 90\% confidence level. This corresponds to an upper limit on the resonance-averaged TRIV cross section of $|Δσ_{\not{T}\not{P}}|<8.3\times10^2~\mathrm{b}$. These results validate the present theoretical framework and provide guidance for future dedicated TRIV searches in polarized neutron transmission experiments.

nucl-ex↗
arXiv2025

Angular correlations in neutron-gamma reactions

Angular correlations for low-energy neutron induced $γ$ reactions are calculated using nuclear reaction formalism for multi level neutron capture with arbitrary multiplicities of $γ$ transitions. We confirm previous calculations [V. V. Flambaum and O. P. Sushkov, Nucl. Phys.A 435 , 352 (1985)] for dipole transitions obtained with different formalism. The possible applications of n-$γ$ correlations for studies of symmetry violations and electromagnetic transitions are discussed.

nucl-th↗
arXiv2025

Precision measurements of muonium and muonic helium hyperfine structure at J-PARC

At the J-PARC Muon Science Facility (MUSE), the MuSEUM collaboration is now performing new precision measurements of the ground state hyperfine structure (HFS) of both muonium and muonic helium atoms. High-precision measurements of the muonium ground-state HFS are recognized as one of the most sensitive tools for testing bound-state quantum electrodynamics theory to precisely probe the standard model and determine fundamental constants of the positive muon magnetic moment and mass. The same technique can also be employed to measure muonic helium HFS, obtain the negative muon magnetic moment and mass, and test and improve the theory of the three-body atomic system. Measurements at zero magnetic field have already yielded more accurate results than previous experiments for both muonium and muonic helium atoms. High-field measurements are now ready to start collecting data using the world's most intense pulsed muon beam at the MUSE H-line. We aim to improve the precision of previous measurements ten times for muonium and a hundred times or more for muonic helium. We review all the key developments for these new measurements, focusing on the high-field experiment, and report the latest results and prospects.

physics.atom-ph↗
arXiv2024

Polarized cold-neutron reflectometry at JRR-3/MINE2 for the development of ultracold-neutron spin analyzers for a neutron EDM experiment at TRIUMF

The neutron electric dipole moment (EDM) is a sensitive probe for currently undiscovered sources of charge-parity symmetry violation. As part of the TRIUMF Ultracold Advanced Neutron (TUCAN) collaboration, we are developing spin analyzers for ultracold neutrons (UCNs) to be used for a next-generation experiment to measure the neutron EDM with unprecedented precision. Spin-state analysis of UCNs constitutes an essential part of the neutron EDM measurement sequence. Magnetized iron films used as spin filters of UCNs are crucial experimental components, whose performance directly influences the statistical sensitivity of the measurement. To test such iron film spin filters, we propose the use of polarized cold-neutron reflectometry, in addition to conventional UCN transmission experiments. The new method provides information on iron film samples complementary to the UCN tests and accelerates the development cycles. We developed a collaborative effort to produce iron film spin filters and test them with cold and ultracold neutrons available at JRR-3/MINE2 and J-PARC/MLF BL05. In this article, we review the methods of neutron EDM measurements, discuss the complementarity of this new approach to test UCN spin filters, provide an overview of our related activities, and present the first results of polarized cold-neutron reflectometry recently conducted at the MINE2 beamline.

physics.ins-det↗
arXiv2024

Combination of crystal growth with optical floating zone and evaluation of Nd3+:LaAlO3 crystals with the dynamic nuclear polarization of 139La and 27Al

Producing a polarized lanthanum (La) target with high polarization and long relaxation time is crucial for realizing time-reversal violation experiments using polarized neutron beams. We use a LaAlO3 crystal doped with a small amount of Nd3+ ions for the polarized lanthanum target. Optimizing the amount of Nd3+ ions is considerably important because the achievable polarization and relaxation time strongly depend on this amount. We established a fundamental method to grow single crystals of Nd3+:LaAlO3 using an optical floating zone method that employs halogen lamps and evaluated the crystals with the dynamic nuclear polarization (DNP) method for polarizing nuclear spins. Two crystal samples were grown by ourselves and evaluated with the DNP at 1.3 K and 2.3 T for the first time except for the target materials of protons. The enhancement of NMR signals for 139La and 27Al was successfully observed, and the enhancement factors were eventually 3.5+-0.3 and 13+-3 for the samples with Nd3+ ions of 0.05 and 0.01 mol%, respectively. These enhancement factors correspond to absolute vector polarizations of 0.27+-0.02% (Nd 0.05 mol%) and 1.4+-0.3% (Nd 0.01 mol%). Although the obtained polarizations are still low, they are acceptable as a first step. The combination scheme of the crystal growth and evaluation of the crystals is found to be effectively applicable for optimizing the amount of Nd3+ ions for improving the performance of the polarized target.

physics.ins-det↗
arXiv2024

Demonstration of Near-Epithermal Neutron Reflective Optics

Specular reflection of neutrons on material surfaces has been demonstrated in the energy range of 0.09-0.7 eV. The results suggest that the applicable energy range of reflective neutron optics can be extended to the near-epithermal region by using existing techniques.

physics.ins-det↗
arXiv2023

Development of Neutron Interferometer using Multilayer Mirrors and Measurements of Neutron-Nuclear Scattering Length with Pulsed Neutron Source

This study entailed the successful deployment of a novel neutron interferometer that utilizes multilayer mirrors. The apparatus facilitates a precise evaluation of the wavelength dependence of interference fringes utilizing a pulsed neutron source. Our interferometer achieved an impressive precision of 0.02 rad within a 20-min of recording time. Compared to systems using silicon crystals, the measurement sensitivity was maintained even when using a simplified disturbance suppressor. By segregating beam paths entirely, we achieved successful measurements of neutron-nuclear scattering lengths across various samples. The values measured for Si, Al, and Ti were in agreement with those found in the literature, while V showed a disparity of 45%. This discrepancy may be attributable to impurities encountered in previous investigations. The accuracy of measurements can be enhanced further by mitigating systematic uncertainties that are associated with neutron wavelength, sample impurity, and thickness. This novel neutron interferometer enables us to measure fundamental parameters, such as the neutron-nuclear scattering length of materials, with a precision that surpasses that of conventional interferometers.

physics.ins-det↗
arXiv2022

The Precision nEDM Measurement with UltraCold Neutrons at TRIUMF

The TRIUMF Ultra-Cold Advanced Neutron (TUCAN) collaboration aims at a precision neutron electric dipole moment (nEDM) measurement with an uncertainty of $10^{-27}\,e\cdot\mathrm{cm}$, which is an order-of-magnitude better than the current nEDM upper limit and enables us to test Supersymmetry. To achieve this precision, we are developing a new high-intensity ultracold neutron (UCN) source using super-thermal UCN production in superfluid helium (He-II) and a nEDM spectrometer. The current development status of them is reported in this article.

physics.ins-det↗
arXiv2022

A Novel Nuclear Emulsion Detector for Measurement of Quantum States of Ultracold Neutrons in the Earth's Gravitational Field

Hypothetical short-range interactions could be detected by measuring the wavefunctions of ultracold neutrons (UCNs) on a mirror bounded by the Earth's gravitational field. The Searches require detectors with higher spatial resolution. We are developing a UCN detector for the with a high spatial resolution, which consists of a Si substrate, a thin converter layer including $^{10}$B$_{4}$C, and a layer of fine-grained nuclear emulsion. Its resolution was estimated to be less than 100 nm by fitting tracks of either $^{7}$Li nuclei or $α$-particles, which were created when neutrons interacted with the $^{10}$B$_{4}$C layer. For actual measurements of the spatial distributions, the following two improvements were made: The first was to establish a method to align microscopic images with high accuracy within a wide region of 65 mm $\times$ 0.2 mm. We created reference marks of 1 $μ$m and 5 $μ$m diameter with an interval of 50 $μ$m and 500 $μ$m, respectively, on the Si substrate by electron beam lithography and realized a position accuracy of less than 30 nm. The second was to build a holder that could maintain the atmospheric pressure around the nuclear emulsion to utilize it under vacuum during exposure to UCNs. The intrinsic resolution of the improved detector was estimated by evaluating the blur of a transmission image of a gadolinium grating taken by cold neutrons as better than 0.56 $\pm$ 0.08 $μ$m, which included the grating accuracy. A test exposure to UCNs was conducted to obtain the spatial distribution of UCNs in the Earth's gravitational field. Although the test was successful, a blurring of 6.9 $μ$m was found in the measurements, compared with a theoretical curve. We identified the blurring caused by the refraction of UCNs due to the roughness of the upstream surface of the substrate. Polishing of the surface makes the resolution less than 100 nm.

physics.ins-det↗
arXiv2020

Neutron spin dynamics in polarized targets

We present neutron elastic scattering amplitude for arbitrary polarized target in irreducible spherical tensor representation. The general approach for the description of neutron spin dynamics for the propagation trough the medium with an arbitrary polarization is discussed in a relation to the search for time reversal invariance violation in neutron scattering.

nucl-th↗
arXiv2019

Measurement of the total neutron scattering cross section ratios of noble gases of natural isotopic composition using a pulsed neutron beam

Precision measurements of slow neutron cross sections with atoms have several scientific applications. In particular the n-$^{4}$He s-wave scattering length is important to know both for helping to constrain the nuclear three-body interaction and for the proper interpretation of several ongoing slow neutron experiments searching for other types of neutron-atom interactions. We present new measurements of the ratios of the neutron differential scattering cross sections for natural isotopic-abundance mixtures of the noble gases He, Ar, Kr, and Xe to natural isotopic abundance Ne. These measurements were performed using a recently developed neutron scattering apparatus for gas samples located on a pulsed slow neutron beamline which was designed to search for possible exotic neutron-atom interactions and employs both neutron time of flight information and a position-sensitive neutron detector for scattering event reconstruction. We found agreement with the literature values of scattering cross sections inferred from Ar/Ne, Kr/Ne and Xe/Ne differential cross section ratios over the $q$ range of $1 - 7$ nm$^{-1}$. However for the case of He/Ne we find that the cross section inferred differs by 11.3% (7.6 $σ$) from previously-reported values inferred from neutron phase shift measurements, but is in reasonable agreement with values from other measurements. The very large discrepancy in the He/Ne ratio calls for a new precision measurement of the n-$^{4}$He scattering length using neutron interferometry.

nucl-ex↗
arXiv2018

A Search for Possible Long Range Spin Dependent Interactions of the Neutron From Exotic Vector Boson Exchange

We present a search for possible spin dependent interactions of the neutron with matter through exchange of spin 1 bosons with axial vector couplings as envisioned in possible extensions of the Standard Model. This was sought using a slow neutron polarimeter that passed transversely polarized slow neutrons by unpolarized slabs of material arranged so that this interaction would tilt the plane of polarization and develop a component along the neutron momentum. The result for the rotation angle, $ϕ'_{V_5} = [2.8\pm\,4.6(stat.)\pm\,4.0(sys.)]\times 10^{-5}~\mbox{rad/m}$ is consistent with zero. This result improves the upper bounds on the neutron-matter coupling $g_{A}^{2}$ from such an interaction by about three orders of magnitude for force ranges in the mm-$μ$m regime.

nucl-ex↗
arXiv2018

Observation of Pendellösung Fringes by Using Pulsed Neutrons

Pendellösung interference fringes of a single silicon crystal were observed by using pulsed cold neutrons. The nuclear scattering length of silicon was obtained as (4.159\pm0.003(stat.)\pm0.028(syst.)) fm using the observed Pendellösung fringes. This indicates the applicability of pulsed neutron beam to observe the Pendellösung fringes by using the time-of-flight analysis.

nucl-ex↗
arXiv2018

The general relativistic effects to the magnetic moment in the Earth's gravity

The magnetic moment of free fermions in the Earth's gravitational field has been studied on the basis of the general relativity. Adopting the Schwarzschild metric for the background spacetime, the dipole coupling between the magnetic moment and the magnetic field has been found to be dependent of the gravity in the calculation up to the post-Newtonian order $O(1/c^2)$. The gravity-dependence can be formulated by employing the effective value of the magnetic moment as a gravity-dependent quantity $μ_{\rm m}^{\rm eff}= (1+3ϕ/c^2) \,\,μ_{\rm m} $ commonly for the cases of minimal coupling, non-minimal coupling and their mixture. The gravitationally induced anomaly is found to be canceled in the experimental values of the anomalous magnetic moment measured in the Penning trap and storage ring methods.

hep-ph↗
arXiv2018

A Search for deviations from the inverse square law of gravity at nm range using a pulsed neutron beam

We describe an experimental search for deviations from the inverse square law of gravity at the nanometer length scale using neutron scattering from noble gases on a pulsed slow neutron beamline. By measuring the neutron momentum transfer ($q$) dependence of the differential cross section for xenon and helium and comparing to their well-known analytical forms, we place an upper bound on the strength of a new interaction as a function of interaction length $λ$ which improves upon previous results in the region $λ< 0.1\,$nm, and remains competitive in the larger $λ$ region. A pseudoexperimental simulation developed for this experiment and its role in the data analysis described. We conclude with plans for improving sensitivity in the larger $λ$ region.

nucl-ex↗
arXiv2018

Fundamental physics activities with pulsed neutron at J-PARC(BL05)

"Neutron Optics and Physics (NOP/ BL05)" at MLF in J-PARC is a beamline for studies of fundamental physics. The beamline is divided into three branches so that different experiments can be performed in parallel. These beam branches are being used to develop a variety of new projects. We are developing an experimental project to measure the neutron lifetime with total uncertainty of 1 s (0.1%). The neutron lifetime is an important parameter in elementary particle and astrophysics. Thus far, the neutron lifetime has been measured by several groups; however, different values are obtained from different measurement methods. This experiment is using a method with different sources of systematic uncertainty than measurements conducted to date. We are also developing a source of pulsed ultra-cold neutrons (UCNs) produced from a Doppler shifter are available at the unpolarized beam branch. We are developing a time focusing device for UCNs, a so called "rebuncher", which can increase UCN density from a pulsed UCN source. At the low divergence beam branch, an experiment to search an unknown intermediate force with nanometer range is performed by measuring the angular dependence of neutron scattering by noble gases. Finally the beamline is also used for the research and development of optical elements and detectors. For example, a position sensitive neutron detector that uses emulsion to achieve sub-micrometer resolution is currently under development. We have succeeded in detecting cold and ultra-cold neutrons using the emulsion detector.

physics.ins-det↗