arXiv subjects

Hiroki Hayashi

Publications and source records attributed to Hiroki Hayashi.

7 recordsLinked to original sources

arXiv2026

Violation of local reciprocity in charge-orbital interconversion

We demonstrate a violation of local reciprocity in the interconversion between charge and orbital currents. By investigating orbital torque and orbital pumping in W/Ni bilayers, we show that the charge-orbital interconversion in the bulk of the W layer exhibits opposite signs in the direct and inverse processes -- the direct and inverse orbital Hall effects being positive and negative, respectively. This finding provides direct evidence of local nonreciprocity in the charge-orbital interconversion, in agreement with a theoretical prediction. These results highlight the unique characteristics of charge-orbital coupled transport and offer fundamental insights into the mechanisms underlying orbital-current-driven phenomena.

cond-mat.mes-hall↗

arXiv2025

Identification of orbital pumping from spin pumping and rectification effects

The recently predicted mechanism of orbital pumping enables the generation of pure orbital current from a precessing ferromagnet (FM) without the need for electrical current injection. This orbital current can be efficiently injected into an adjacent nonmagnetic material (NM) without being hampered by electrical conductivity mismatch. However, experimentally identifying this novel effect presents significant challenges due to the substantial background contributions from spin pumping and spin rectification effects (SREs). In this work, we disentangle the effects of orbital pumping from spin pumping in bilayer structures composed of Nb/Ni and Nb/$\mathrm{Fe_{60}Co_{20}B_{20}}$ by observing a sign reversal of the measured voltage. This reversal arises from the competing signs of the spin and orbital Hall effects in the Nb. We establish methods to differentiate the pumping signal from SREs by analyzing the distinct angular dependence of the measured voltage and its spatial dependence relative to the radio frequency excitation source.

cond-mat.mtrl-sci↗

arXiv2023

Observation of orbital pumping

Harnessing spin and orbital angular momentum is a fundamental concept in condensed matter physics, materials science, and quantum-device applications. In particular, the search for new phenomena that generate a flow of spin angular momentum, a spin current, has led to the development of spintronics, advancing the understanding of angular momentum dynamics at the nanoscale. In contrast to this success, the generation and detection of orbital currents, the orbital counterpart of spin currents, remains a significant challenge. Here, we report the observation of orbital pumping, a phenomenon in which magnetization dynamics pumps an orbital current, a flow of orbital angular momentum. The orbital pumping is the orbital counterpart of the spin pumping, which is one of the most versatile and powerful mechanisms for spin-current generation. We show that the orbital pumping in Ni/Ti bilayers injects an orbital current into the Ti layer, which is detected through the inverse orbital Hall effect. Our findings provide a promising approach for generating orbital currents and pave the way for exploring the physics of orbital transport in solids.

cond-mat.mes-hall↗

arXiv2023

Time-domain observation of ballistic orbital-angular-momentum currents with giant relaxation length in tungsten

The emerging field of orbitronics exploits the electron orbital momentum $\textit{L}$. Compared to spin-polarized electrons, $\textit{L}$ may allow magnetic-information transfera with significantly higher density over longer distances in more materials. However, direct experimental observation of $\textit{L}$ currents, their extended propagation lengths and their conversion into charge currents has remained challenging. Here, we optically trigger ultrafast angular-momentum transport in Ni|W|SiO$_2$ thin-film stacks. The resulting terahertz charge-current bursts exhibit a marked delay and width that grow linearly with W thickness. We consistently ascribe these observations to a ballistic $\textit{L}$ current from Ni through W with giant decay length (~80 nm) and low velocity (~0.1 nm/fs). At the W/SiO$_2$ interface, the $\textit{L}$ flow is efficiently converted into a charge current by the inverse orbital Rashba-Edelstein effect, consistent with ab-initio calculations. Our findings establish orbitronic materials with long-distance ballistic $\textit{L}$ transport as possible candidates for future ultrafast devices and an approach to discriminate Hall- and Rashba-Edelstein-like conversion processes.

physics.app-ph↗

arXiv2023

Observation of long-range orbital transport and giant orbital torque

Modern spintronics relies on the generation of spin currents through spin-orbit coupling. The spin-current generation has been believed to be triggered by current-induced orbital dynamics, which governs the angular momentum transfer from the lattice to the electrons in solids. The fundamental role of the orbital response in the angular momentum dynamics suggests the importance of the orbital counterpart of spin currents: orbital currents. However, evidence for its existence has been elusive. Here, we demonstrate the generation of giant orbital currents and uncover fundamental features of the orbital response. We experimentally and theoretically show that orbital currents propagate over longer distances than spin currents by more than an order of magnitude in a ferromagnet and nonmagnets. Furthermore, we find that the orbital current enables electric manipulation of magnetization with efficiencies significantly higher than the spin counterpart. These findings open the door to orbitronics that exploits orbital transport and spin-orbital coupled dynamics in solid-state devices.

cond-mat.mes-hall↗

arXiv2020

Spin-orbit torques originating from bulk and interface in Pt-based structures

We investigated spin-orbit torques in prototypical Pt-based spintronic devices. We found that, in Pt/Ni and Pt/Fe bilayers, the damping-like torque efficiency depends on the thickness of the Pt layer. We also found that the damping-like torque efficiency is almost identical in the Pt/Ni and Pt/Fe bilayers despite the stronger spin memory loss at the Pt/Fe interface. These results suggest that although the dominant source of the damping-like torque is the bulk spin Hall effect in the Pt layer, a sizable damping-like torque is generated by the interface in the Pt/Fe bilayer due to the stronger interfacial spin-orbit coupling. In contrast to the damping-like torque, whose magnitude and sign are almost identical in the Pt/Ni and Pt/Fe bilayers, the field-like torque strongly depends on the choice of the ferromagnetic layer. The sign of the field-like torque originating from the bulk spin Hall effect in the Pt layer is opposite between the Pt/Ni and Pt/Fe bilayers, which can be attributed to the opposite sign of the imaginary part of the spin-mixing conductance. These results demonstrate that the spin-orbit torques are quite sensitive to the electronic structure of the FM layer.

cond-mat.mtrl-sci↗

arXiv2020

Current-induced torque originating from orbital current

The electrical manipulation of magnetization by current-induced spin torques has given access to realize a plethora of ultralow power and fast spintronic devices such as non-volatile magnetic memories, spin-torque nano-oscillators, and neuromorphic computing devices. Recent advances have led to the notion that relativistic spin-orbit coupling is an efficient source for current-induced torques, opening the field of spin-orbitronics. Despite the significant progress, however, the fundamental mechanism of magnetization manipulation, the requirement of spin currents in generating current-induced torques, has remained unchanged. Here, we demonstrate the generation of current-induced torques without the use of spin currents. By measuring the current-induced torque for naturally-oxidized-Cu/ferromagnetic-metal bilayers, we observed an exceptionally high effective spin Hall conductivity at low temperatures despite the absence of strong spin-orbit coupling. Furthermore, we found that the direction of the torque depends on the choice of the ferromagnetic layer, which counters the conventional understanding of the current-induced torque. These unconventional features are best interpreted in terms of an orbital counterpart of the spin torque, an orbital torque, which arises from the orbital Rashba effect and orbital current. These findings will shed light on the underlying physics of current-induced magnetization manipulation, potentially altering the landscape of spin-orbitronics.

cond-mat.mtrl-sci↗