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Hiromitsu Hori

Publications and source records attributed to Hiromitsu Hori.

11 recordsLinked to original sources

Evidence for multimagnon-mediated nuclear spin relaxation in the intertwining double-cain ferrimagnet $Ca_3 Cu_3 (PO_4)_4$

The nuclear spin-lattice relaxation time $T_1$ of $^{31}P$ nuclei in the title compound is measured for the first time and interpreted in terms of a modified spin-wave theory. We establish a novel scenario for one-dimensional ferrimagnetic spin dynamics -- it is three-magnon processes enhanced by exchange scattering, rather than Raman processes, that make the major contribution to $1/T_1$.

cond-mat.str-el

Low-temperature thermodynamics of one-dimensional alternating-spin Heisenberg ferromagnets

Motivated by a novel bimetallic chain compound in which alternating magnetic centers are ferromagnetically coupled, we investigate thermodynamic properties of one-dimensional spin-$(S,s)$ Heisenberg ferromagnets both numerically and analytically. On the one hand, quantum Monte Carlo calculations illuminate the overall thermal behavior. The specific heat may exhibit a double-peaked structure at intermediate temperatures for $S\agt 3s$ in general. On the other hand, a modified spin-wave theory precisely describes the low-temperature properties. Expanding the specific heat and the magnetic susceptibility, we reveal an analogy and a contrast between mixed-spin ferromagnets and ferrimagnets.

cond-mat.stat-mech

Modified spin-wave theory of nuclear magnetic relaxation in one-dimensional quantum ferrimagnets: Three-magnon versus Raman processes

Nuclear spin-lattice relaxation in one-dimensional Heisenberg ferrimagnets is studied by means of a modified spin-wave theory. Calculating beyond the first-order mechanism, where a nuclear spin directly interacts with spin waves through the hyperfine coupling, we demonstrate that the exchange-scattering-enhanced three-magnon nuclear relaxation may generally predominate over the Raman one with increasing temperature and decreasing field. Recent proton spin-lattice relaxation-time (T_1_) measurements on the ferrimagnetic chain compound NiCu(C_7_H_6_N_2_O_6_)(H_2_O)_3_2H_2_O suggest that the major contribution to 1/T_1_ be made by the three-magnon scattering.

cond-mat.str-el

Nuclear Spin-Lattice Relaxation in One-Dimensional Heisenberg Ferrimagnets: Three-Magnon versus Raman Processes

Nuclear spin-lattice relaxation in one-dimensional Heisenberg ferrimagnets is studied by means of a modified spin-wave theory. We consider the second-order process, where a nuclear spin flip induces virtual spin waves which are then scattered thermally via the four-magnon exchange interaction, as well as the first-order process, where a nuclear spin directly interacts with spin waves via the hyperfine interaction. We point out a possibility of the three-magnon relaxation process predominating over the Raman one and suggest model experiments.

cond-mat.stat-mech

Static and Dynamic Properties of Antiferromagnetic Heisenberg Ladders: Fermionic versus Bosonic Approaches

In terms of spinless fermions via the Jordan-Wigner transformation along a snake-like path and spin waves modified so as to restore the sublattice symmetry, we investigate static and dynamic properties of two-leg antiferromagnetic Heisenberg ladders. The specific heat is finely reproduced by the spinless fermions, whereas the magnetic susceptibility is well described by the modified spin waves. The nuclear spin-lattice relaxation rate is discussed in detail with particular emphasis on its novel field dependence.

cond-mat.stat-mech

Nuclear Magnetic Relaxation in the Haldane-Gap Antiferromagnet Ni(C_2_H_8_N_2_)_2_NO_2_(ClO_4_)

A new theory is proposed to interpret nuclear spin-lattice relaxation-time (T_1_) measurements on the spin-1 quasi-one-dimensional Heisenberg antiferromagnet Ni(C_2_H_8_N_2_)_2_NO_2_(ClO_4_) (NENP). While Sagi and Affleck pioneeringly discussed this subject in terms of field-theoretical languages, there is no theoretical attempt yet to explicitly simulate the novel observations of 1/T_1_ reported by Fujiwara et al.. By means of modified spin waves, we solve the minimum of 1/T_1_ as a function of an applied field, pending for the past decade.

cond-mat.stat-mech

Nuclear spin-lattice relaxation in ferrimagnetic clusters and chains: A contrast between zero and one dimensions

Motivated by ferrimagnetic oligonuclear and chain compounds synthesized by Caneschi et al., both of which consist of alternating manganese(II) ions and nitronyl-nitroxide radicals, we calculate the nuclear spin-lattice relaxation rate 1/T_1 employing a recently developed modified spin-wave theory. 1/T_1 as a function of temperature drastically varies with the location of probe nuclei in both clusters and chains, though the relaxation time scale is much larger in zero dimension than in one dimension. 1/T_1 as a function of an applied field in long chains forms a striking contrast to that in finite clusters, diverging with decreasing field like inverse square root at low temperatures and logarithmically at high temperatures.

cond-mat.str-el

Spin-Wave Description of Haldane-gap antiferromagnets

Modifying the conventional antiferromagnetic spin-wave theory which is plagued by the difficulty of the zero-field sublattice magnetizations diverging in one dimension, we describe magnetic properties of Haldane-gap antiferromagnets. The modified spin waves, constituting a grand canonical bosonic ensemble so as to recover the sublattice symmetry, not only depict well the ground-state correlations but also give useful information on the finite-temperature properties.

cond-mat.stat-mech

Quantum and thermal phase transitions in the Bechgaard salts and their analogs

In order to investigate quantum and thermal phase transitions in the Bechgaard salts and their sulfur analogs, we perform finite-temperature Hartree-Fock calculations in one dimension with particular emphasis on the interplay between charge ordering and lattice instability. The coexisting charge- and spin-density-wave state as well as its precursor fluctuations in (TMTSF)2PF6 and the lattice tetramerization in (TMTTF)2ReO4 are well interpreted.

cond-mat.str-el