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Hiromu Okamoto

Publications and source records attributed to Hiromu Okamoto.

2 recordsLinked to original sources

Signatures of field-induced multi-color kagome spin liquids in the dipole-octupole pyrochlore $\mathrm{Ce_2Hf_2O_7}$

We report low-temperature magnetization and magnetostriction measurements on the dipole-octupole pyrochlore $\mathrm{Ce_2Hf_2O_7}$, revealing an unconventional field response for $\mathbf B\parallel[111]$. The magnetization shows no kagome-ice plateau; instead it evolves continuously and exhibits two rapid changes in slope near 0.35~T and 1.2~T, accompanied by magnetostriction features at the same field scales. Classical Monte Carlo simulations, exact diagonalization, and ground-state analysis of the Hamiltonian show that a representative QSI-compatible parameter set captures the data. For this parameter set, the lower-field anomaly marks a closely spaced transition sequence from a two-color kagome spin liquid (KSL) through a narrow three-color KSL into a mixed two-/three-color KSL, while the upper-field anomaly marks the transition from the mixed KSL into a nearly polarized state. These results identify $\mathrm{Ce_2Hf_2O_7}$, and dipole-octupole pyrochlore magnets more broadly, as promising platforms for exotic KSLs beyond conventional spin ice.

cond-mat.str-el

Anomalies in the thermal conductivity of honeycomb antiferromagnet MnPS$_{3}$

Intrinsic two-dimensional magnets serve as a good platform to explore collective, charge-neutral and low-energy excitations. Distinguishing the crucial role of them in experimental aspect remains a challenge for decades. Here, we study the thermal transport in honeycomb antiferromagnet MnPS$_{3}$ with $T_N$=78 K down to very low temperatures (<0.01$T_N$). At high temperatures (>0.1$T_N$), the field dependence of the thermal Hall conductivity exhibits a linear phonon Hall effect and a peak associated with the spin-flop transition due to a strong spin-lattice coupling, well reproducing the previous report (Phys. Rev. B 110, 165147 (2024)). Notably, below 2 K, we find that the field dependence of the thermal Hall conductivity exhibits sign reversals within the spin-flop phase, at which the field dependence of the longitudinal thermal conductivity also shows multiple valleys. We suggest that these anomalies are caused by the redistribution of Berry curvature in magnon bands, demonstrating the superior performance of the thermal Hall measurements to detect the Berry curvature distributions in magnetic insulators.

cond-mat.mtrl-sci