arXiv subjects

Hiroyuki Nojiri

Publications and source records attributed to Hiroyuki Nojiri.

41 records · Page 3Linked to original sources

arXiv2009

Elementary excitations of S=1/2 one-dimensional antiferromagnet KCuGaF6 in magnetic field and quantum sine-Gordon model

Elementary excitations of the S=1/2 one-dimensional Heisenberg antiferromagnet KCuGaF$_6$ with exchange constant $J/k_B$=103 K were investigated by high-frequency ESR measurements combined with a pulsed high magnetic field. When an external magnetic field H is applied in KCuGaF$_6$, a staggered magnetic field h is induced perpendicular to H owing to the staggered g tensor and the Dzyaloshinsky-Moriya (DM) interaction with an alternating D vector. Consequently, KCuGaF$_6$ in a magnetic field is represented by the quantum sine-Gordon (SG) model. We observed many resonance modes including a soliton resonance, breathers, interbreather transitions and two-breather excitation. Their resonance conditions are beautifully described by the quantum SG field theory with one adjustable parameter $c_ s=h/H$. To investigate the relationship between the Curie term due to the DM interaction and the proportional coefficient $c_s$, magnetic susceptibility measurements were also performed varying the external field direction.

cond-mat.str-el↗

arXiv2008

Anomalous frequency and intensity scaling of collective and local modes in a coupled spin tetrahedron system

We report on the magnetic excitation spectrum of the coupled spin tetrahedral system Cu$_{2}$Te$_{2}$O$_{5}$Cl$_{2}$ using Raman scattering on single crystals. The transition to an ordered state at T$_{N}^{Cl}$=18.2 K evidenced from thermodynamic data leads to the evolution of distinct low-energy magnetic excitations superimposed by a broad maximum. These modes are ascribed to magnons with different degree of localization and a two-magnon continuum. Two of the modes develop a substantial energy shift with decreasing temperature similar to the order parameter of other Neel ordered systems. The other two modes show only a negligible temperature dependence and dissolve above the ordering temperature in a continuum of excitations at finite energies. These observations point to a delicate interplay of magnetic inter- and intra-tetrahedra degrees of freedom and an importance of singlet fluctuations in describing a spin dynamics.

cond-mat.str-el↗

arXiv2007

Thermodynamic Properties and Elementary Excitations in Quantum Sine-Gordon Spin System KCuGaF6

Thermodynamic properties and elementary excitations in $S=1/2$ one-dimensional Heisenberg antiferromagnet KCuGaF$_6$ were investigated by magnetic susceptibility, specific heat and ESR measurements. Due to the Dzyaloshinsky-Moriya interaction with alternating $D$-vectors and/or the staggered $g$-tensor, the staggered magnetic field is induced when subjected to external magnetic field. Specific heat in magnetic field clearly shows the formation of excitation gap, which is attributed to the staggered magnetic field. The specific heat data was analyzed on the basis of the quantum sine-Gordon (SG) model. We observed many ESR modes including one soliton and three breather excitations characteristic of the quantum SG model.

cond-mat.str-el↗

arXiv2005

Observation of field-dependent magnetic parameters in the magnetic molecule {Ni4Mo12}

We investigate the bulk magnetic, electron paramagnetic resonance, and magneto-optical properties of {Ni4Mo12}, a magnetic molecule with antiferromagnetically coupled tetrahedral {Ni4Mo12} in a diamagnetic molybdenum matrix. The low-temperature magnetization exhibits steps at irregular field intervals, a result that cannot be explained using a Heisenberg model even if it is augmented by magnetic anisotropy and biquadratic terms. Allowing the exchange and anisotropy parameters to depend on the magnetic field provides the best fit to our data, suggesting that the molecular structure (and thus the interactions between spins) may be changing with applied magnetic field.

cond-mat.mtrl-sci↗

arXiv2004

Magnetic characterization of the frustrated three-leg ladder compound [(CuCl2tachH)3Cl]Cl2

We report the magnetic features of a new one-dimensional stack of antiferromagnetically coupled equilateral copper(II) triangles. High-field magnetization measurements show that the interaction between the copper triangles is of the same order of magnitude as the intra-triangle exchange although only coupled via hydrogen bonds. The infinite chain turns out to be an interesting example of a frustrated cylindrical three-leg ladder with competing intra- and inter-triangle interactions. We demonstrate that the ground state is a spin singlet which is gaped from the triplet excitation.

cond-mat.mtrl-sci↗