arXiv subjects

Hoi Chun Po

Publications and source records attributed to Hoi Chun Po.

At least 37 records · Page 2Linked to original sources

arXiv2024

Cascade of strongly correlated quantum states in a partially filled kagome flat band

Coulomb interactions among charge carriers that occupy an electronic flat band have a profound impact on the macroscopic properties of materials. At sufficient strength, these interactions can give rise to captivating phenomena such as quantum criticality, Mott-Hubbard states, and unconventional superconductivity. The appearance of these characteristics sensitively depends on the number of electrons occupying the flat band states. In this work, we present experimental evidence obtained from scanning tunneling microscopy measurements for a cascade of strongly correlated states appearing in the partially occupied kagome flat bands of Co$_{1-x}$Fe$_x$Sn whose filling can be controlled by the Fe-doping level $x$. At elevated temperatures ($T\geq16\,K$), we detect a nematic electronic state across a broad doping range $0.05 100\,$meV) blend the states of two $3d$-orbital derived flat bands and impart a nematic order parameter. This state serves as the parent phase of a strongly correlated phase diagram: At lower temperatures $T<16\,$K, we find spectroscopic evidence for an orbital-selective Mott state enabled by the $3d$-orbital degeneracy of the Co atom. This state can only be detected in samples with ideal Fe doping ($x=0.17$) and descends into pseudogap phases upon electron and hole doping. At $T<8\,$K, the pseudogap phase evolves into another nematic low temperature state. Our observations demonstrate that the electronic ground state of a kagome flat band depends on the complex interplay between strong Coulomb repulsion, $3d$-orbital degeneracy, and flat band filling fraction at different temperatures.

cond-mat.str-el↗

arXiv2024

Constructive Fermionic Matrix Product States for Projected Fermi Sea

Projected wave functions offer a means for incorporating local correlation effects in gapless electronic phases of matter like metals. Although such wave functions can be readily specified formally, it is challenging to compute their associated physical observables. Tensor network approaches offer a modern numerical method for this task. In this work, we develop and demonstrate a constructive tensor-network approach for obtaining physical quantities, like fermion two-point functions and density-density correlation functions, for one-dimensional projected Fermi sea states. We benchmark our method against exact analytical results for spin-1/2 electrons subjected to the Gutzwiller projection, and then present results on spinless fermions with nearest-neighbor repulsion. For a state with two pairs of Fermi points, we reveal a correlation-tuning of the characteristic wave vector of the charge density modulation in the system.

cond-mat.str-el↗

arXiv2024

Coexistence of interacting charge density waves in a layered semiconductor

Coexisting orders are key features of strongly correlated materials and underlie many intriguing phenomena from unconventional superconductivity to topological orders. Here, we report the coexistence of two interacting charge-density-wave (CDW) orders in EuTe4, a layered crystal that has drawn considerable attention owing to its anomalous thermal hysteresis and a semiconducting CDW state despite the absence of perfect FS nesting. By accessing unoccupied conduction bands with time- and angle-resolved photoemission measurements, we find that mono- and bi-layers of Te in the unit cell host different CDWs that are associated with distinct energy gaps. The two gaps display dichotomous evolutions following photoexcitation, where the larger bilayer CDW gap exhibits less renormalization and faster recovery. Surprisingly, the CDW in the Te monolayer displays an additional momentum-dependent gap renormalization that cannot be captured by density-functional theory calculations. This phenomenon is attributed to interlayer interactions between the two CDW orders, which account for the semiconducting nature of the equilibrium state. Our findings not only offer microscopic insights into the correlated ground state of EuTe4 but also provide a general non-equilibrium approach to understand coexisting, layer-dependent orders in a complex system.

cond-mat.str-el↗

arXiv2023

Tunable non-Lifshitz-Kosevich temperature dependence of Shubnikov-de Haas oscillation amplitudes in SmSb

The Lifshitz-Kosevich (LK) theory is the pillar of magnetic quantum oscillations, which have been extensively applied to characterize a wide range of metallic states. In this study, we focus on the Shubnikov-de Haas (SdH) effect observed in SmSb, a rare-earth monopnictide. We observed a significant departure from the expected LK theory near $T_N=2.4$~K: both a peak-like anomaly and an enhancement in the temperature dependence of quantum oscillation amplitude are seen in SmSb. Moreover, we discovered a remarkable sensitivity of the SdH amplitudes to sample purity. By adjusting the sample purity, we were able to tune the temperature dependence of the $α$ band's SdH amplitudes from a peak-like anomalous behavior to an enhancement. Therefore, SdH oscillations from the $α$ band connect the two well-known non-LK behaviours, controllable through varying the sample purity, paving the way for developing further understanding of the mechanism leading to the anomalous quantum oscillations.

cond-mat.mtrl-sci↗

arXiv2023

Stacked tree construction for free-fermion projected entangled pair states

The tensor network representation of a state in higher dimensions, say a projected entangled-pair state (PEPS), is typically obtained indirectly through variational optimization or imaginary-time Hamiltonian evolution. Here, we propose a divide-and-conquer approach to directly construct a PEPS representation for free-fermion states admitting descriptions in terms of filling exponentially localized Wannier functions. Our approach relies on first obtaining a tree tensor network description of the state in local subregions. Next, a stacking procedure is used to combine the local trees into a PEPS. Lastly, the local tensors are compressed to obtain a more efficient description. We demonstrate our construction for states in one and two dimensions, including the ground state of an obstructed atomic insulator on the square lattice.

cond-mat.str-el↗

arXiv2023

Visualizing the Localized Electrons of a Kagome Flat Band

Destructive interference between electron wavefunctions on the two-dimensional (2D) kagome lattice induces an electronic flat band, which could host a variety of interesting many-body quantum states. Key to realize these proposals is to demonstrate the real space localization of kagome flat band electrons. In particular, the extent to which the often more complex lattice structure and orbital composition of realistic materials counteract the localizing effect of destructive interference, described by the 2D kagome lattice model, is hitherto unknown. We used scanning tunneling microscopy (STM) to visualize the non-trivial Wannier states of a kagome flat band at the surface of CoSn, a kagome metal. We find that the local density of states associated with the flat bands of CoSn is localized at the center of the kagome lattice, consistent with theoretical expectations for their corresponding Wannier states. Our results show that these states exhibit an extremely small localization length of two to three angstroms concomitant with a strongly renormalized quasiparticle velocity, which is comparable to that of moiré superlattices. Hence, interaction effects in the flat bands of CoSn could be much more significant than previously thought. Our findings provide fundamental insight into the electronic properties of kagome metals and are a key step for future research on emergent many-body states in transition metal based kagome materials.

cond-mat.mes-hall↗

arXiv2023

Topogivity: A Machine-Learned Chemical Rule for Discovering Topological Materials

Topological materials present unconventional electronic properties that make them attractive for both basic science and next-generation technological applications. The majority of currently known topological materials have been discovered using methods that involve symmetry-based analysis of the quantum wavefunction. Here we use machine learning to develop a simple-to-use heuristic chemical rule that diagnoses with a high accuracy whether a material is topological using only its chemical formula. This heuristic rule is based on a notion that we term topogivity, a machine-learned numerical value for each element that loosely captures its tendency to form topological materials. We next implement a high-throughput procedure for discovering topological materials based on the heuristic topogivity-rule prediction followed by ab initio validation. This way, we discover new topological materials that are not diagnosable using symmetry indicators, including several that may be promising for experimental observation.

cond-mat.mtrl-sci↗

arXiv2022

Non-Abelian nonsymmorphic chiral symmetries

The Hofstadter model exemplifies a large class of physical systems characterized by particles hopping on a lattice immersed in a gauge field. Recent advancements on various synthetic platforms have enabled highly-controllable simulations of such systems with tailored gauge fields featuring complex spatial textures. These synthetic gauge fields could introduce synthetic symmetries that do not appear in electronic materials. Here, in an SU(2) non-Abelian Hofstadter model, we theoretically show the emergence of multiple nonsymmorphic chiral symmetries, which combine an internal unitary anti-symmetry with fractional spatial translation. Depending on the values of the gauge fields, the nonsymmorphic chiral symmetries can exhibit non-Abelian algebra and protect Kramer quartet states in the bulk band structure, creating general four-fold degeneracy at all momenta. These nonsymmorphic chiral symmetries protect double Dirac semimetals at zero energy, which become gapped into quantum confined insulating phases upon introducing a boundary. Moreover, the parity of the system size can determine whether the resulting insulating phase is trivial or topological. Our work indicates a pathway for creating topology via synthetic symmetries emergent from synthetic gauge fields.

cond-mat.mes-hall↗

arXiv2022

Zipper Entanglement Renormalization for Free Fermions

Entanglement renormalization refers to a sequence of real-space coarse-graining transformations in which short-range entanglement on successively longer length scales are distilled out. In this work, we introduce a state-based approach, "zipper entanglement renormalization" (ZER), for free-fermion systems. The name derives from a unitary we construct at every renormalization step, dubbed the zipper, which unzips the state into an approximate tensor product between a short-range entangled state and a renormalized one carrying the longer-range entanglement. By successively performing ZER on the renormalized states, we obtain a unitary transformation of the input state into a state that is approximately factorized over the emergent renormalization spacetime. As a demonstration, we apply ZER to one-dimensional models and show that it efficiently disentangles the ground states of the Su-Schrieffer-Heeger model, a scale-invariant critical state, as well as a more general gapless state with two sets of Fermi points.

quant-ph↗

arXiv2022

Magnetically brightened dark electron-phonon bound states in a van der Waals antiferromagnet

In van der Waals (vdW) materials, strong coupling between different degrees of freedom can hybridize elementary excitations into bound states with mixed character. Correctly identifying the nature and composition of these bound states is key to understanding their ground state properties and excitation spectra. Here, we use ultrafast spectroscopy to reveal bound states of d-orbitals and phonons in 2D vdW antiferromagnet NiPS3. These bound states manifest themselves through equally spaced phonon replicas in frequency domain. These states are optically dark above the Néel temperature and become accessible with magnetic order. By launching this phonon and spectrally tracking its amplitude, we establish the electronic origin of bound states as localized d-d excitations. Our data directly yield electron-phonon coupling strength which exceeds the highest known value in 2D systems. These results demonstrate NiPS3 as a platform to study strong interactions between spins, orbitals and lattice, and open pathways to coherent control of 2D magnets.

cond-mat.mtrl-sci↗

arXiv2021

Location and topology of the fundamental gap in photonic crystals

The fundamental, or first, band gap is of unmatched importance in the study of photonic crystals. Here, we address precisely where this gap can be opened in the band structure of three-dimensional photonic crystals. Although strongly constrained by symmetry, this problem cannot be addressed directly with conventional band-symmetry analysis due to the existence of a photonic polarization vortex at zero frequency. We develop an approach for overcoming the associated symmetry singularity by incorporating fictitious, auxiliary longitudinal modes. Our strategy also enables us to extend recent developments in symmetry-based topological analysis to the fundamental gap of three-dimensional photonic crystals. Exploiting this, we systematically study the topology of the minimal fundamental gaps. This reveals the existence of topological gap-obstructions that push the fundamental gap higher than what a conventional analysis would suggest. Our work demonstrates that topology can play a crucial role in the opening of the fundamental photonic gap and informs future theoretical and experimental searches for conventional and topological band gaps in three-dimensional photonic crystals.

physics.optics↗

arXiv2021

Signature of Many-Body Localization of Phonons in Strongly Disordered Superlattices

Many-body localization (MBL) has attracted significant attention due to its immunity to thermalization, role in logarithmic entanglement entropy growth, and opportunities to reach exotic quantum orders. However, experimental realization of MBL in solid-state systems has remained challenging. Here we report evidence of a possible phonon MBL phase in disordered GaAs/AlAs superlattices. Through grazing-incidence inelastic X-ray scattering, we observe a strong deviation of the phonon population from equilibrium in samples doped with ErAs nanodots at low temperature, signaling a departure from thermalization. This behavior occurs within finite phonon energy and wavevector windows, suggesting a localization-thermalization crossover. We support our observation by proposing a theoretical model for the effective phonon Hamiltonian in disordered superlattices, and showing that it can be mapped exactly to a disordered 1D Bose-Hubbard model with a known MBL phase. Our work provides momentum-resolved experimental evidence of phonon localization, extending the scope of MBL to disordered solid-state systems.

cond-mat.mtrl-sci↗

arXiv2021

Inherited topological superconductivity in two-dimensional Dirac semimetals

Under what conditions does a superconductor inherit topologically protected nodes from its parent normal state? In the context of Weyl semimetals with broken time-reversal symmetry, the pairing order parameter is classified by monopole harmonics and necessarily nodal [Li and Haldane, Phys. Rev. Lett., 120, 067003 (2018)]. Here, we show that a similar conclusion could also apply to 2D Dirac semimetals, although the conditions for the existence of nodes are more complex, depending on the pairing matrix structure in the valley and sublattice space. We analytically and numerically analyze the Bogoliubov-de-Gennes quasi-particle spectra for Dirac systems based on the monolayer as well as twisted bilayer graphene. We find that in the cases of intra-valley intra-sublattice pairing, and inter-valley inter-sublattice pairing, the point nodes in the BdG spectrum (which are inherited from the Dirac cone in the normal state) are protected by a 1D winding number. The nodal structure of the superconductivity is confirmed using tight-binding models of monolayer and twisted bilayer graphene. Notably, the BdG spectrum is nodal even with a momentum-independent "bare" pairing, which, however, acquires momentum-dependence and point nodes upon projection to the Bloch states on the topologically nontrivial Fermi surface, similar in spirit to the Li--Haldane monopole superconductor and the Fu--Kane proximity-induced superconductor on the surface of a topological insulator.

cond-mat.supr-con↗

arXiv2021

Symmetric Jordan-Wigner transformation in higher dimensions

The Jordan-Wigner transformation is traditionally applied to one dimensional systems, but recent works have generalized the transformation to fermionic lattice systems in higher dimensions while keeping locality manifest. These developments could aid the theoretical or even experimental studies of strongly correlated electronic problems through their bosonic counterparts. In this work, we develop a scheme for higher-dimensional Jordan-Wigner transformation which keeps all relevant symmetries manifest on the bosonic side. Our approach connects the discussion of exact lattice bosonization to the familiar notions of fractionalized partons like spinons and chargeons, and works for spin-$1/2$ fermions -- like the physical electrons -- on four-coordinated lattices. The construction is applied to fermions defined on the square, kagome and diamond lattices, and we provide explicit expressions for the bosonized versions of well-known models of strongly correlated electrons, like the Hubbard and $t$-$J$ models.

cond-mat.str-el↗

arXiv2021

Fractional Corner Charge of Sodium Chloride

Recent developments in higher-order topological phases have elucidated on the relationship between nontrivial multipole moments in the bulk and the emergence of fractionally quantized charges at the boundary. Here, we put on the table a proposal of the three-dimensional octupole insulator with fractionally quantized corner charges $\pm e/8$: sodium chloride, commonly known as table salt. The fractional quantization of the corner charge is unaffected by the quantum fluctuation of the electric charge per ion, as we demonstrate explicitly with ab initio calculations. We further show that the electrostatic signature of the fractional charge is well-preserved even when the ideal crystal is sprinkled with defects, and provide a systematic analysis on how the corner charge contribution could be isolated from the electric-field corrections originating from realistic surface relaxation. Our results suggest that the observation of corner charges from quantized multipole moments in solids might be around the corner.

cond-mat.mtrl-sci↗

arXiv2021

Topological Invariants of a Filling-Enforced Quantum Band Insulator

Traditional ionic/covalent compound insulators arise from a commensuration between electron count and system volume. On the other hand, conventional topological insulators, outside of quantum hall effect systems, do not typically display such a commensuration. Tnstead, they can undergo a phase transition to a trivial insulator that preserves the electron filling. Nevertheless, in some crystalline insulators, termed filling-enforced quantum band insulators (feQBIs), electron filling can dictate nontrivial topology in the insulating ground state. Currently, little is known about the relation between feQBIs and conventional topological invariants. In this work, we study such relations for a particularly interesting example of a half-filling feQBI that is realized in space group 106 with spinless electrons. We prove that any 4-band feQBI in space group 106 with filling 2 must have a nontrivial topological invariant, namely the $\mathbb{Z}_2$ glide invariant, and thus must have a quantized magnetoelectric polarizability $θ=π$. We thus have found a three-dimensional example where electron filling and band topology are tied. Such a locking raises intriguing questions about the generality of the band-inversion paradigm in describing the transition between trivial and topological phases.

cond-mat.mes-hall↗

arXiv2021

Higher-dimensional Jordan-Wigner Transformation and Auxiliary Majorana Fermions

We discuss a scheme for performing Jordan-Wigner transformation for various lattice fermion systems in two and three dimensions which keeps internal and spatial symmetries manifest. The correspondence between fermionic and bosonic operators is established with the help of auxiliary Majorana fermions. The current construction is applicable to general lattices with even coordination number and an arbitrary number of fermion flavors. The approach is demonstrated on the single-orbital square, triangular and cubic lattices for spin-1/2 fermions. We also discuss the relation to some quantum spin liquid models.

cond-mat.str-el↗

arXiv2021

Unconventional hysteretic transition in a charge density wave

Hysteresis underlies a large number of phase transitions in solids, giving rise to exotic metastable states that are otherwise inaccessible. Here, we report an unconventional hysteretic transition in a quasi-2D material, EuTe4. By combining transport, photoemission, diffraction, and x-ray absorption measurements, we observed that the hysteresis loop has a temperature width of more than 400 K, setting a record among crystalline solids. The transition has an origin distinct from known mechanisms, lying entirely within the incommensurate charge-density-wave (CDW) phase of EuTe4 with no change in the CDW modulation periodicity. We interpret the hysteresis as an unusual switching of the relative CDW phases in different layers, a phenomenon unique to quasi-2D compounds that is not present in either purely 2D or strongly-coupled 3D systems. Our findings challenge the established theories on metastable states in density wave systems, pushing the boundary of understanding hysteretic transitions in a broken-symmetry state.

cond-mat.mtrl-sci↗