arXiv subjects

Holger Mueller

Publications and source records attributed to Holger Mueller.

At least 19 recordsLinked to original sources

arXiv2026

Magic Velocity Selection in Atom Interferometry

Velocity-selective Raman transitions are widely used in atom interferometers to prepare atomic ensembles with narrowly defined momentum distributions. However, differential light shifts between atomic energy levels generate velocity distributions that are correlated with the Raman beam intensity, and therefore with the position of the atoms within the laser beam. We show that these spatially inhomogeneous velocity distributions interact with detuning-dependent systematic effects in a Bragg diffraction-based simultaneous conjugate Ramsey-Bord\'e interferometer. These interactions can induce systematic phase shifts of order 10 milliradians in the interferometer phase. We further identify a "magic" detuning for velocity selection and show that operating at this detuning suppresses the systematic phase shift. Magic velocity selection eliminates systematic errors arising from correlations between atom velocity and position, facilitating high-resolution atom interferometry experiments targeting sub-part-per-billion accuracy.

physics.atom-ph↗

arXiv2026

Serrodyne Matterwave Optics

Bragg diffraction for atom interferometry conventionally requires two laser frequencies whose difference makes the two-photon transition resonant. We show that this frequency difference can instead be generated by serrodyne modulation, allowing Bragg pulses to be driven with a single-frequency laser. The serrodyne modulation is performed using an acousto-optic modulator driven with a phase-modulated RF drive, and generated kilohertz-scale frequency shifts on top of the AOM carrier frequency. While in general serrodyne modulation generates strong unwanted frequency components, we find conditions so that the Bragg diffraction pulses, and atom interferometers constructed from them, are robust to these imperfections, opening the door to the development of ultra compact, single frequency Bragg diffraction based atom interferometers with serrodyne modulation implemented by a position modulated retroreflection mirror.

physics.atom-ph↗

arXiv2026

A fast and accurate method for simulating Bragg atom interferometers

Atom interferometers are used in a variety of applications, from measuring gravity and gravity gradients in the field to performing tests of fundamental physics in the lab. One method of increasing interferometer sensitivity is to produce a larger momentum difference between interferometer arms through the use of large momentum transfer methods, such as Bragg diffraction. However, Bragg diffraction introduces systematic effects in the accumulated interferometer phase that are challenging to characterize. A Bragg atom interferometer is described by the one-dimensional time-dependent Schr\"odinger equation (1D-TDSE). In this paper we show that for the case of Bragg diffraction the 1D-TDSE partial differential equation can be separated into several systems of ordinary differential equations, allowing for the use of adaptive step size Runge-Kutta methods. We compare the convergence of this method to the split-step and Crank-Nicolson methods, and present a method for further computational speed-ups using a lookup table.

physics.atom-ph↗

arXiv2025

Linewidth narrowing and wideband frequency modulation of a DBR laser

We present a scheme to phase-lock a 240 mW, 852 nm distributed Bragg reflector (DBR) laser to a fixed-frequency narrow-linewidth laser with a rapidly tunable frequency offset near 9 GHz. The phase-lock is accomplished by electronic feedback on the beatnote between the two lasers. The frequency offset can be swept 200 MHz in 300 us, limited by the feedback loop bandwidth, allowing for its use in complex cooling and state preparation schemes needed in atomic physics experiments. Additionally, we find that the phase-lock reduces the linewidth of the DBR laser below its natural linewidth of ~400 kHz to ~100 kHz.

physics.atom-ph↗

arXiv2024

Modern approaches to improving phase contrast electron microscopy

Although defocus can be used to generate partial phase contrast in transmission electron microscope images, cryo-electron microscopy (cryo-EM) can be further improved by the development of phase plates which increase contrast by applying a phase shift to the unscattered part of the electron beam. Many approaches have been investigated, including the ponderomotive interaction between light and electrons. We review the recent successes achieved with this method in high-resolution, single-particle cryo-EM. We also review the status of using pulsed or near-field enhanced laser light as alternatives, along with approaches that use scanning transmission electron microscopy (STEM) with a segmented detector rather than a phase plate.

q-bio.QM↗

arXiv2023

Quantum Sensors for High Energy Physics

Strong motivation for investing in quantum sensing arises from the need to investigate phenomena that are very weakly coupled to the matter and fields well described by the Standard Model. These can be related to the problems of dark matter, dark sectors not necessarily related to dark matter (for example sterile neutrinos), dark energy and gravity, fundamental constants, and problems with the Standard Model itself including the Strong CP problem in QCD. Resulting experimental needs typically involve the measurement of very low energy impulses or low power periodic signals that are normally buried under large backgrounds. This report documents the findings of the 2023 Quantum Sensors for High Energy Physics workshop which identified enabling quantum information science technologies that could be utilized in future particle physics experiments, targeting high energy physics science goals.

hep-ex↗

arXiv2022

Offset Lock with 440 GHz Range using Electro-Optic Modulation

Offset locking is a popular method for stabilizing laser frequency, which is crucial to many physics experiments. Wide range offset locks are desirable, as they increase the span of usable frequencies in an experiment. Here, we experimentally realize a wide-range offset lock using a beat-note setup combined with electro-optic phase modulation. By using frequency down-conversion of the beat note and locking to sidebands generated by electro-optic modulation, we achieve an offset range of $\pm$ 220.1 GHz with offset frequency fluctuations under 0.1 Hz, enabling an optical heterodyne offset lock with the largest known range of any such lock. The relative simplicity of our setup provides a compelling method for locking at offsets in the hundreds of GHz range.

physics.optics↗

arXiv2021

Opportunities for DOE National Laboratory-led QuantISED Experiments

A subset of QuantISED Sensor PIs met virtually on May 26, 2020 to discuss a response to a charge by the DOE Office of High Energy Physics. In this document, we summarize the QuantISED sensor community discussion, including a consideration of HEP science enabled by quantum sensors, describing the distinction between Quantum 1.0 and Quantum 2.0, and discussing synergies/complementarity with the new DOE NQI centers and with research supported by other SC offices. Quantum 2.0 advances in sensor technology offer many opportunities and new approaches for HEP experiments. The DOE HEP QuantISED program could support a portfolio of small experiments based on these advances. QuantISED experiments could use sensor technologies that exemplify Quantum 2.0 breakthroughs. They would strive to achieve new HEP science results, while possibly spinning off other domain science applications or serving as pathfinders for future HEP science targets. QuantISED experiments should be led by a DOE laboratory, to take advantage of laboratory technical resources, infrastructure, and expertise in the safe and efficient construction, operation, and review of experiments. The QuantISED PIs emphasized that the quest for HEP science results under the QuantISED program is distinct from the ongoing DOE HEP programs on the energy, intensity, and cosmic frontiers. There is robust evidence for the existence of particles and phenomena beyond the Standard Model, including dark matter, dark energy, quantum gravity, and new physics responsible for neutrino masses, cosmic inflation, and the cosmic preference for matter over antimatter. Where is this physics and how do we find it? The QuantISED program can exploit new capabilities provided by quantum technology to probe these kinds of science questions in new ways and over a broader range of science parameters than can be achieved with conventional techniques.

physics.ins-det↗

arXiv2020

High-Power Near-Concentric Fabry-Perot Cavity for Phase Contrast Electron Microscopy

Transmission electron microscopy (TEM) of vitrified biological macromolecules (cryo-EM) is limited by the weak phase contrast signal that is available from such samples. Using a phase plate would thus substantially improve the signal-to-noise ratio. We have previously demonstrated the use of a high-power Fabry-Perot cavity as a phase plate for TEM. We now report improvements to our laser cavity that allow us to achieve record continuous-wave intensities of over 450 GW/cm$^{2}$, sufficient to produce the optimal 90° phase shift for 300 keV electrons. In addition, we have performed the first cryo-EM reconstruction using a laser phase plate, demonstrating that the stability of this laser phase plate is sufficient for use during standard cryo-EM data collection.

physics.ins-det↗

arXiv2020

Symmetric Bloch oscillations of matter waves

Cold atoms in an optical lattice provide an ideal platform for studying Bloch oscillations. Here, we extend Bloch oscillations to two superposed optical lattices that are accelerated away from one another, and for the first time show that these symmetric Bloch oscillations can split, reflect and recombine matter waves coherently. Using the momentum parity-symmetry of the Hamiltonian, we map out the energy band structure of the process and show that superpositions of momentum states are created by adiabatically following the ground state of the Hamiltonian. The relative phase and velocity of the two lattices completely determines the trajectories of different branches of the matter wave. Experimentally, we demonstrate symmetric Bloch oscillations using cold Cesium atoms where we form interferometers with up to $240\hbar k$ momentum splitting, one of the largest coherent momentum splittings achieved to date. This work has applications in macroscopic tests of quantum mechanics, measurements of fundamental constants, and searches for new physics.

physics.atom-ph↗

arXiv2020

Observation of the relativistic reversal of the ponderomotive potential

The secular dynamics of a non-relativistic charged particle in an electromagnetic wave can be described by the ponderomotive potential. Although ponderomotive electron-laser interactions at relativistic velocities are important for emerging technologies from laser-based particle accelerators to laser-enhanced electron microscopy, the effects of special relativity on the interaction have only been studied theoretically. Here, we use a transmission electron microscope to measure the position-dependent phase shift imparted to a relativistic electron wave function when it traverses a standing laser wave. The kinetic energy of the electrons is varied between $80\,\mathrm{keV}$ and $300\,\mathrm{keV}$, and the laser standing wave has a continuous-wave intensity of $175\,\mathrm{GW/cm}^2$. In contrast to the non-relativistic case, we demonstrate that the phase shift depends on both the electron velocity and the wave polarization, confirming the predictions of a quasiclassical theory of the interaction. Remarkably, if the electron's speed is greater than $1/\sqrt{2}$ of the speed of light, the phase shift at the electric field nodes of the wave can exceed that at the antinodes. In this case there exists a polarization such that the phase shifts at the nodes and antinodes are equal, and the electron does not experience Kapitza-Dirac diffraction. Our results thus provide new capabilities for coherent electron beam manipulation.

physics.optics↗

arXiv2018

Quantum Sensing for High Energy Physics

Report of the first workshop to identify approaches and techniques in the domain of quantum sensing that can be utilized by future High Energy Physics applications to further the scientific goals of High Energy Physics.

hep-ex↗

arXiv2017

Laser frequency stabilization by combining modulation transfer and frequency modulation spectroscopy

We present a hybrid laser frequency stabilization method combining modulation transfer spectroscopy (MTS) and frequency modulation spectroscopy (FMS) for the cesium D2 transition. In a typical pump-probe setup, the error signal is a combination of the DC-coupled MTS error signal and the AC-coupled FMS error signal. This combines the long-term stability of the former with the high signal-to-noise ratio of the latter. In addition, we enhance the long-term frequency stability with laser intensity stabilization. By measuring the frequency difference between two independent hybrid spectroscopies, we investigate the short-term and long-term stability. We find a long-term stability of 7.8 kHz characterized by a standard deviation of the beating frequency drift over the course of 10 hours, and a short-term stability of 1.9 kHz characterized by an Allan deviation of that at 2 seconds of integration time.

physics.atom-ph↗

arXiv2015

Quantum Test of the Equivalence Principle and Space-Time aboard the International Space Station

We describe the Quantum Test of the Equivalence principle and Space Time (QTEST), a concept for an atom interferometry mission on the International Space Station (ISS). The primary science objective of the mission is a test of Einstein's equivalence principle with two rubidium isotope gases at a precision of better than 10$^{-15}$. Distinct from the classical tests is the use of quantum wave packets and their expected large spatial separation in the QTEST experiment. This dual species atom interferometer experiment will also be sensitive to time-dependent equivalence principle violations that would be signatures for ultralight dark-matter particles. In addition, QTEST will be able to perform photon recoil measurements to better than 10$^{-11}$ precision. This improves upon terrestrial experiments by a factor of 100, enabling an accurate test of the standard model of particle physics and contributing to mass measurement, in the proposed new international system of units (SI), with significantly improved precision. The predicted high measurement precision of QTEST comes from the microgravity environment on ISS, offering extended free fall times in a well-controlled environment. Suppression of systematic errors by use of symmetric interferometer configurations and rejection of common-mode errors drives the QTEST design. It uses Bragg interferometry with a single laser beam at the "magic" wavelength, where the two isotopes have the same polarizability, for mitigating sensitivities to vibrations and laser noise, imaging detection for correcting cloud initial conditions and maintaining contrast, modulation of the atomic hyperfine states for reduced sensitivity to magnetic field gradients, two source regions for simultaneous time reversal measurements and redundancy, and modulation of the gravity vector using a rotating platform to reduce otherwise difficult systematics to below 10$^{-16}$.

physics.atom-ph↗

arXiv2014

Antimatter interferometry for gravity measurements

We describe a light-pulse atom interferometer that is suitable for any species of atom and even for electrons and protons as well as their antiparticles, in particular for testing the Einstein equivalence principle with antihydrogen. The design obviates the need for resonant lasers through far-off resonant Bragg beam splitters and makes efficient use of scarce atoms by magnetic confinement and atom recycling. We expect to reach an initial accuracy of better than 1% for the acceleration of free fall of antihydrogen, which can be improved to the part-per million level.

physics.atom-ph↗

arXiv2013

Quantum mechanics, matter waves, and moving clocks

This paper is divided into three parts. In the first (section 1), we demonstrate that all of quantum mechanics can be derived from the fundamental property that the propagation of a matter wave packet is described by the same gravitational and kinematic time dilation that applies to a clock. We will do so in several steps, first deriving the Schroedinger equation for a nonrelativistic particle without spin in a weak gravitational potential, and eventually the Dirac equation in curved space-time describing the propagation of a relativistic particle with spin in strong gravity. In the second part (sections 2-4), we present interesting consequences of the above quantum mechanics: that it is possible to use wave packets as a reference for a clock, to test general relativity, and to realize a mass standard based on a proposed redefinition of the international system of units, wherein the Planck constant would be assigned a fixed value. The clock achieved an absolute accuracy of 4 parts per billion (ppb). The experiment yields the fine structure constant $α= 7.297\,352\,589(15) \times 10^{-3}$ with 2.0 ppb accuracy. We present improvements that have reduced the leading systematic error about 8-fold and improved the statistical uncertainty to 0.33 ppb in 6 hours of integration time, referred to $α$. In the third part (sections 5-7), we present possible future experiments with atom interferometry: A gravitational Aharonov-Bohm experiment and its application as a measurement of Newton's gravitational constant, antimatter interferometry, interferometry with charged particles, and interferometry in space. We will give a review of previously published material when appropriate, but will focus on new aspects that haven't been published before.

quant-ph↗

arXiv2013

Equivalence Principle and Bound Kinetic Energy

We consider the role of the internal kinetic energy of bound systems of matter in tests of the Einstein equivalence principle. Using the gravitational sector of the standard model extension, we show that stringent limits on equivalence principle violations in antimatter can be indirectly obtained from tests using bound systems of normal matter. We estimate the bound kinetic energy of nucleons in a range of light atomic species using Green's function Monte Carlo calculations, and for heavier species using a Woods-Saxon model. We survey the sensitivities of existing and planned experimental tests of the equivalence principle, and report new constraints at the level of between a few parts in $10^{6}$ and parts in $10^{8}$ on violations of the equivalence principle for matter and antimatter.

gr-qc↗

arXiv2013

Terrestrial vs. spaceborne, quantum vs. classical tests of the equivalence principle

The equivalence principle can be tested by precision experiments based on classical and quantum systems, on the ground as well as in space. In many models, these tests are mostly equivalent in their ability to constrain physics beyond the Standard Model. We mention differences that nevertheless exist between spaceborne and quantum mechanical tests and their conventional competitors.

gr-qc↗