arXiv subjects

Hongbo Wu

Publications and source records attributed to Hongbo Wu.

4 recordsLinked to original sources

arXiv2026

Demonstrating advantages of dynamic quantum circuits on a hybrid superconducting qubit-cavity processor

Dynamic quantum circuits (DQCs) provide a hardware-efficient route to quantum computing by reducing physical-qubit overhead and compressing circuit topology through mid-circuit measurements, qubit reset and reuse, and classical feed-forward control. Here, we demonstrate the advantages of DQCs on a single hybrid superconducting qubit-cavity processor by implementing a hierarchy of algorithms with increasing complexity. This hybrid architecture consists of a high-dimensional cavity qudit serving as the computational register and a dispersively coupled superconducting transmon ancilla that is repeatedly measured, reset, and reused to enable dynamic control. Using this device, we implement a 10-bit Bernstein-Vazirani algorithm with an average success probability of 82%, surpassing state-of-the-art dynamic and static implementations in both scale and performance; an 8-bit quantum phase-estimation protocol with estimation errors below 10-3; and the first dynamic-circuit implementation of Shor's algorithm on a superconducting platform, factoring 15 over all coprime bases with squared statistical overlap values above 99.8%. These results provide concrete benchmarks for future DQC implementations and highlight the versatile advantages of DQCs with the hybrid qubit-qudit architecture, establishing it as a promising route toward scalable, programmable quantum computation.

quant-ph↗

arXiv2025

Exploring Dual-Iron Atomic Catalysts for Efficient Nitrogen Reduction: A Comprehensive Study on Structural and Electronic Optimization

The nitrogen reduction reaction (NRR), as an efficient and green pathway for ammonia synthesis, plays a crucial role in achieving on-demand ammonia production. This study proposes a novel design concept based on dual-iron atomic sites and nitrogen-boron co-doped graphene catalysts, exploring their high efficiency in NRR. By modulating the N and B co-doped ratios, we found that Fe2N3B@G catalyst exhibited significant activity in the adsorption and hydrogenation of N2 molecules, especially with the lowest free energy (0.32 eV) on NRR distal pathway, showing its excellent nitrogen activation capability and NRR performance. The computed electron localization function, crystal orbital Hamiltonian population, electrostatic potential map revealed that the improved NRR kinetics of Fe2N3B@G catalyst derived by N3B co-doping induced optimization of Fe-Fe electronic environment, regulation of Fe-N bond strength, and the continuous electronic support during the N2 breakage and hydrogenation. In particular, machine learning molecular dynamics (MLMD) simulations were employed to verify the high activity of Fe2N3B@G catalyst in NRR, which reveal that Fe2N3B@G effectively regulates the electron density of Fe-N bond, ensuring the smooth generation and desorption of NH3 molecules and avoiding the competition with hydrogen evolution reaction (HER). Furthermore, the determined higher HER overpotential of Fe2N3B@G catalyst can effectively inhibit the HER and enhance the selectivity toward NRR. In addition, Fe2N3B@G catalyst also showed good thermal stability by MD simulations up to 500 K, offering its feasibility in practical applications. This study demonstrates the superior performance of Fe2N3B@G in nitrogen reduction catalysis, and provides theoretical guidance for atomic catalyst design by the co-doping strategy and in-deep electronic environment modulation.

cond-mat.mtrl-sci↗

arXiv2023

Hybrid Nodal-chain Semimetal State in MgCaN2

The distinct over-tilting of band crossings in topological semimetal generates the type-I and typeII classification of Dirac/Weyl and nodal-line fermions, accompanied by the exotic electronic and magnetic transport properties. In this work, we propose a concept of hybrid nodal-chain semimetal, which is identified by the linked type-I and type-II nodal rings in the Brillouin zone. Based on first-principles calculations and swarm-intelligence structure search technique, a new ternary nitride MgCaN2 crystal is proposed as the first candidate to realize a novel 3D hybrid nodal-chain state. Remarkably, a flat band is emergent as a characteristic signature of such a hybrid nodal-chain along certain direction in the momentum space, thereby serving a platform to explore the interplay between topological semimetal state and flat band. Moreover, the underlying protection mechanism of the hybrid nodal-chain is revealed by calculating the mirror Z2 invariant and developing a k.p effective Hamiltonian. Additionally, considerable drumhead-like surface states with unique connection patterns are illustrated to identify the non-trivial band topology, which may be measured by future experiments.

cond-mat.mtrl-sci↗

arXiv2019

Weyl nodal point-line Fermion in ferromagnetic Eu$_5$Bi$_3$

Based on $ab$ $initio$ calculations and low-energy effective $k{\cdot}p$ model, we propose a type of Weyl nodal point-line fermion, composed of 0D Weyl points and 1D Weyl nodal line, in ferromagnetic material Eu$_5$Bi$_3$. In the absence of spin-orbital coupling (SOC), the spin-up bands host a pair of triply degenerate points together with a unique bird-cage like node structure. In the presence of SOC with (001) magnetization, each triplet point splits into a double Weyl point and a single Weyl point accompanied by two nodal rings, forming two sets of Weyl nodal point-line fermions near the Fermi level. The novel properties of Weyl nodal point-line fermion are explored by revealing the unusual Berry curvature field and demonstrating the pinned chiral surface states with exotic Fermi arcs at different planes. Moreover, a large anomalous Hall conductivity of -260 ($\hbar$/$e$)($Ω$cm)$^{-1}$ parallel to [001] direction is predicted. Our work offers a new perspective for exploring novel topological semimetal states with diverse band-crossing dimensions, and provides an ideal material candidate for future experimental realiztion.

cond-mat.mtrl-sci↗